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公开(公告)号：US20180001277A1
公开(公告)日：2018-01-04
申请号：US15610305
申请日：2017-05-31
Applicant: UOP LLC
Inventor： Chunqing Liu , Nicole K. Karns
CPC classification number: B01D71/64 , B01D53/228 , B01D67/0079 , B01D67/0093 , B01D69/06 , B01D69/08 , B01D69/12 , B01D71/022 , B01D71/82 , C07C7/144
Abstract: A high performance facilitated transport membrane comprising a metal cation exchanged/chelated carboxylic acid functional group containing functional polyimide, a method of making this a membrane, and the use of this membrane for olefin/paraffin separations, particularly for propylene/propane and ethylene/ethane separations. The facilitated transport membrane has either an asymmetric integrally skinned membrane structure or a thin film composite membrane structure, wherein the top selective layer of the membrane comprises a metal cation exchanged/chelated carboxylic acid functional group containing functional polyimide.
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42.发明申请公开(公告)号：US20170354918A1
公开(公告)日：2017-12-14
申请号：US15598168
申请日：2017-05-17
Applicant: UOP LLC
Inventor： Chunqing Liu , Carl W. Liskey , Howie Q. Tran , Nicole K. Karns
CPC classification number: B01D53/228 , B01D67/0088 , B01D69/10 , B01D69/12 , B01D69/148 , B01D71/08 , B01D71/68 , B01D2256/24 , B01D2325/36 , C07C7/144
Abstract: This invention provides a new facilitated transport membrane comprising a relatively hydrophilic, very small pore, nanoporous support membrane, a hydrophilic polymer inside the very small nanopores on the skin layer surface of the support membrane, a thin, nonporous, hydrophilic polymer layer coated on the surface of the support membrane, and metal salts incorporated in the hydrophilic polymer layer coated on the surface of the support membrane and the hydrophilic polymer inside the very small nanopores, a method of making this membrane, and the use of this membrane for olefin/paraffin separations, particularly for C3=/C3 and C2=/C2 separations.
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公开(公告)号：US09662616B2
公开(公告)日：2017-05-30
申请号：US14669457
申请日：2015-03-26
Applicant: UOP LLC
Inventor： Chunqing Liu
IPC: B01D53/22 , B01D71/68 , B01D69/12 , B01D61/36 , B01D69/02 , B01D71/80 , B01D67/00 , B01D69/06 , B01D69/08
CPC classification number: B01D69/125 , B01D53/228 , B01D61/362 , B01D67/009 , B01D69/02 , B01D69/06 , B01D69/08 , B01D71/68 , B01D71/80 , B01D2256/16 , B01D2256/18 , B01D2256/245 , B01D2257/102 , B01D2257/108 , B01D2257/504 , B01D2257/702 , B01D2257/708 , B01D2323/30 , B01D2325/20 , Y02C10/10
Abstract: The present invention provides high flux aromatic alkyl-substituted polyethersulfone membranes and methods for making and using these membranes for gas separations. The membranes may be fabricated into any known membrane configuration including a flat sheet or a hollow fiber. The present invention also provides high selectivity UV cross-linked aromatic alkyl-substituted polyethersulfone membranes and methods for making and using these membranes for gas separations.
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公开(公告)号：US09637586B2
公开(公告)日：2017-05-02
申请号：US14620780
申请日：2015-02-12
Applicant: UOP LLC
Inventor： Chunqing Liu , Howie Q. Tran , Travis C. Bowen
CPC classification number: C08G59/02 , B01D53/228 , B01D63/023 , B01D2053/224 , C08G59/5033
Abstract: The present invention provided a high temperature resistant epoxy resins for producing hollow fiber membrane modules for high temperature gas separation applications such as for natural gas upgrading and hydrogen purifications. This invention also relates to a hollow fiber membrane module comprising a bundle of multiple high performance hollow fiber membranes and a tube sheet formed by a high temperature resistant cured epoxy resin that is used to fix and bound said bundle of multiple high performance hollow fiber membranes. The invention also provides a process for separating at least one gas from a mixture of gases using the hollow fiber membrane modules comprising a bundle of multiple high performance hollow fiber membranes and a tube sheet formed by a high temperature resistant cured epoxy resin that is used to fix and bound said bundle of multiple high performance hollow fiber membranes.
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45.发明授权公开(公告)号：US09567436B2
公开(公告)日：2017-02-14
申请号：US14574319
申请日：2014-12-17
Applicant: UOP LLC
Inventor： Chunqing Liu
CPC classification number: C08G73/1067 , B01D53/228 , B01D69/08 , B01D69/088 , B01D71/64 , B01D71/76 , B01D2053/224 , C08G73/1032 , C08G73/1039 , C08G73/1042 , C08L77/00 , C08L79/08 , Y02C10/10 , Y02C20/20
Abstract: This invention relates to aromatic block copolyimide polymers comprising both hydroxyl functional groups and carboxylic acid functional groups, their membranes and methods for making and using these polymers and membranes. The aromatic block copolyimide polymer described in the present invention comprises both hydroxyl functional groups and carboxylic acid functional groups. The gas transport properties particularly the selectivities of the aromatic block copolyimide comprising both hydroxyl functional groups and carboxylic acid functional groups were significantly improved compared to those of the aromatic random copolyimide comprising both hydroxyl functional groups and carboxylic acid functional groups.
Abstract translation: 本发明涉及包含羟基官能团和羧酸官能团的芳族嵌段共聚酰亚胺聚合物，它们的膜以及制备和使用这些聚合物和膜的方法。 本发明中描述的芳族嵌段共聚酰亚胺聚合物包括羟基官能团和羧酸官能团。 与包含羟基官能团和羧酸官能团的芳族无规共聚酰亚胺相比，特别是包含羟基官能团和羧酸官能团的芳族嵌段共聚酰亚胺的选择性显着提高。
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Patent Agency Ranking
46.发明申请公开(公告)号：US20160177035A1
公开(公告)日：2016-06-23
申请号：US14574319
申请日：2014-12-17
Applicant: UOP LLC
Inventor： Chunqing Liu
CPC classification number: C08G73/1067 , B01D53/228 , B01D69/08 , B01D69/088 , B01D71/64 , B01D71/76 , B01D2053/224 , C08G73/1032 , C08G73/1039 , C08G73/1042 , C08L77/00 , C08L79/08 , Y02C10/10 , Y02C20/20
Abstract: This invention relates to aromatic block copolyimide polymers comprising both hydroxyl functional groups and carboxylic acid functional groups, their membranes and methods for making and using these polymers and membranes. The aromatic block copolyimide polymer described in the present invention comprises both hydroxyl functional groups and carboxylic acid functional groups. The gas transport properties particularly the selectivities of the aromatic block copolyimide comprising both hydroxyl functional groups and carboxylic acid functional groups were significantly improved compared to those of the aromatic random copolyimide comprising both hydroxyl functional groups and carboxylic acid functional groups.
Abstract translation: 本发明涉及包含羟基官能团和羧酸官能团的芳族嵌段共聚酰亚胺聚合物，它们的膜以及制备和使用这些聚合物和膜的方法。 本发明中描述的芳族嵌段共聚酰亚胺聚合物包括羟基官能团和羧酸官能团。 与包含羟基官能团和羧酸官能团的芳族无规共聚酰亚胺相比，特别是包含羟基官能团和羧酸官能团的芳族嵌段共聚酰亚胺的选择性显着提高。
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公开(公告)号：US20160089627A1
公开(公告)日：2016-03-31
申请号：US14496754
申请日：2014-09-25
Applicant: UOP LLC
Inventor： Chunqing Liu , Howie Q. Tran
CPC classification number: B01D53/228 , B01D67/0006 , B01D69/02 , B01D71/64 , B01D2325/20 , Y02C10/10 , Y02C20/20
Abstract: The polyimide blend membrane in the present invention was prepared by blending a first aromatic polyimide with high permeability and a second aromatic polyimide with high selectivity for gas separation. The polyimide blend membrane in the present invention showed improved permeability compared to membranes made from the second aromatic polyimide and improved selectivity compared to membranes made from the first aromatic polyimide.
Abstract translation: 本发明中的聚酰亚胺共混膜是通过高选择性地混合具有高磁导率的第一芳族聚酰亚胺和第二芳族聚酰亚胺来制备的。 与由第一芳族聚酰亚胺制成的膜相比，本发明的聚酰亚胺共混膜显示出比由第二芳族聚酰亚胺制成的膜提高的渗透性，并提高了选择性。
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48.发明授权Nanoporous macrocycle-containing cross-linked polymeric membranes for separations 有权纳米多孔大分子交联聚合物膜用于分离公开(公告)号：US09238194B2
公开(公告)日：2016-01-19
申请号：US14231716
申请日：2014-03-31
Applicant: UOP LLC
Inventor： Chunqing Liu , Howie Q. Tran , Nicole K. Karns , Travis C. Bowen
CPC classification number: B01D53/228 , B01D69/125 , B01D71/54 , B01D71/58 , B01D2053/221 , B01D2256/24 , B01D2256/245 , B01D2257/504 , B01D2257/702 , B01D2257/7027 , B01D2323/30 , B01D2325/20 , C08G18/42 , C08G18/48 , C08G18/6484 , C08J9/286 , C08J9/365 , C08J2201/026 , C08J2201/0502 , C08J2375/04 , C10L3/101 , Y02C10/10 , Y02P20/152 , C08G18/10 , C08G18/64
Abstract: The present invention involves a type of nanoporous macrocycle-containing cross-linked polymeric membrane, a method of making the membrane, and the use of such a novel membrane system for natural gas liquids (NGL) recovery, fuel gas conditioning, natural gas pre-treatment, sulfur removal from fluidized catalytic cracking (FCC) and other naphtha streams, as well as aromatic separations such as aromatic/paraffin separation and xylene separation. The nanoporous macrocycle-containing cross-linked polymeric membrane is prepared from a diisocyanate-terminated polyether or a diisocyanate-terminated polyester, that is crosslinked with a nanoporous macrocycle comprising hydroxyl functional groups such as α-, β-, and γ-cyclodextrins.
Abstract translation: 本发明涉及一种纳米多孔大环交联聚合物膜，一种制备该膜的方法，以及使用这种新型天然气液体（NGL）回收膜系统，燃料气体调节剂，天然气预处理剂， 处理，从流化催化裂化（FCC）和其他石脑油流中除去硫，以及芳族分离，如芳烃/石蜡分离和二甲苯分离。 含有纳米多孔大环的交联聚合物膜由二异氰酸酯封端的聚醚或二异氰酸酯封端的聚酯制备，其与包含羟基官能团如α-，β-环糊精的纳米多孔大环交联。
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49.发明授权Polybenzoxazole membranes from self-cross-linkable aromatic polyimide membranes 有权来自自交联芳香聚酰亚胺膜的聚苯并恶唑膜公开(公告)号：US09211508B2
公开(公告)日：2015-12-15
申请号：US14039570
申请日：2013-09-27
Applicant: UOP LLC
Inventor： Chunqing Liu , Zara Osman , Angela N. Troxell
CPC classification number: B01D71/62 , B01D67/0006 , B01D67/0083 , B01D67/0088 , B01D2323/08 , B01D2323/30
Abstract: A method of making a polybenzoxazole (PBO) membrane from a self-cross-linked aromatic polyimide polymer membrane is provided. These membranes are useful in the separation of gas mixtures and liquid mixtures. The PBO membrane is made by fabricating a self-cross-linkable aromatic polyimide polymer membrane comprising both hydroxyl functional groups and carboxylic acid functional groups; cross-linking the polymer to form a self-cross-linked aromatic polyimide polymer membrane by heating the membrane at 250° to 300° C. under an inert atmosphere; and thermal heating the self-cross-linked aromatic polyimide polymer membrane at a temperature from about 350° to 500° C. under an inert atmosphere to convert the self-cross-linked aromatic polyimide polymer membrane into a PBO membrane. A membrane coating step may be added by coating the selective layer surface of the PBO membrane with a thin layer of high permeability material.
Abstract translation: 提供了一种从自交联的芳族聚酰亚胺聚合物膜制备聚苯并恶唑（PBO）膜的方法。 这些膜可用于气体混合物和液体混合物的分离。 PBO膜通过制造包含羟基官能团和羧酸官能团的自交联芳族聚酰亚胺聚合物膜制成; 交联聚合物以通过在惰性气氛下在250℃至300℃下加热该膜而形成自交联的芳族聚酰亚胺聚合物膜; 并在惰性气氛下，在约350-500℃的温度下自热交联芳族聚酰亚胺聚合物膜，将自交联的芳族聚酰亚胺聚合物膜转化成PBO膜。 可以通过用高渗透性材料的薄层涂布PBO膜的选择性层表面来添加膜涂覆步骤。
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50.发明申请NANOPOROUS MACROCYCLE-CONTAINING CROSS-LINKED POLYMERIC MEMBRANES FOR SEPARATIONS 有权用于分离的含有纳米聚合物的交联聚合物膜公开(公告)号：US20150273389A1
公开(公告)日：2015-10-01
申请号：US14231716
申请日：2014-03-31
Applicant: UOP LLC
Inventor： Chunqing Liu , Howie Q. Tran , Nicole K. Karns , Travis C. Bowen
CPC classification number: B01D53/228 , B01D69/125 , B01D71/54 , B01D71/58 , B01D2053/221 , B01D2256/24 , B01D2256/245 , B01D2257/504 , B01D2257/702 , B01D2257/7027 , B01D2323/30 , B01D2325/20 , C08G18/42 , C08G18/48 , C08G18/6484 , C08J9/286 , C08J9/365 , C08J2201/026 , C08J2201/0502 , C08J2375/04 , C10L3/101 , Y02C10/10 , Y02P20/152 , C08G18/10 , C08G18/64
Abstract: The present invention involves a type of nanoporous macrocycle-containing cross-linked polymeric membrane, a method of making the membrane, and the use of such a novel membrane system for natural gas liquids (NGL) recovery, fuel gas conditioning, natural gas pre-treatment, sulfur removal from fluidized catalytic cracking (FCC) and other naphtha streams, as well as aromatic separations such as aromatic/paraffin separation and xylene separation. The nanoporous macrocycle-containing cross-linked polymeric membrane is prepared from a diisocyanate-terminated polyether or a diisocyanate-terminated polyester, that is crosslinked with a nanoporous macrocycle comprising hydroxyl functional groups such as α-, β-, and γ-cyclodextrins.
Abstract translation: 本发明涉及一种纳米多孔大环交联聚合物膜，一种制备该膜的方法，以及使用这种新型天然气液体（NGL）回收膜系统，燃料气体调节剂，天然气预处理剂， 处理，从流化催化裂化（FCC）和其他石脑油流中除去硫，以及芳族分离，如芳烃/石蜡分离和二甲苯分离。 含有纳米多孔大环的交联聚合物膜由二异氰酸酯封端的聚醚或二异氰酸酯封端的聚酯制备，其与包含羟基官能团如α-，β-环糊精的纳米多孔大环交联。
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