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    Process for processing sulfur-containing heavy oil
    1.
    发明授权
    Process for processing sulfur-containing heavy oil 失效
    含硫重油加工工艺

    公开(公告)号：US4298460A

    公开(公告)日：1981-11-03

    申请号：US133082

    申请日：1980-03-24

    Applicant: Kuniaki Fujimori ,  Teruo Suzuka ,  Yukio Inoue ,  Shirou Aizawa

    Inventor： Kuniaki Fujimori ,  Teruo Suzuka ,  Yukio Inoue ,  Shirou Aizawa

    IPC: B01J23/745 ,  B01J23/94 ,  C01B3/22 ,  C10G11/02 ,  C10G11/18

    CPC classification number: B01J23/745 ,  B01J23/94 ,  C10G11/02 ,  C10G11/18

    Abstract: A process for processing a sulfur-containing heavy oil, which comprises:in a first zone, catalytically cracking a sulfur-containing heavy oil in the presence of fluidized catalyst particles containing about 30 to 60 wt % Fe to thereby convert the heavy oil to a light oil, deposit sulfur-containing coke on the catalyst particles, and partially fixing the decomposed sulfur compounds with the reduced iron contained in the catalyst particles as iron sulfide;in a second zone, contacting the catalyst from the first zone with an oxygen containing gas in an amount less than that theoretically required to thereby partially combust the coke on the catalyst, reduce the iron in the catalyst, and fix the sulfur compounds contained in the coke as iron sulfide; andin a third zone, contacting the reduced catalyst from the second zone with steam in a fluidized manner to produce hydrogen and hydrogen sulfide and to convert the reduced iron and iron sulfide in the catalyst to iron oxides, with the iron oxide-containing catalyst obtained in the third zone being recirculated into the second zone to be reduced and a part of the reduced-state catalyst obtained in the second zone being recirculated into the first zone.

    Abstract translation: 一种处理含硫重油的方法，其包括：在第一区域中，在含有约30至60重量％Fe的流化催化剂颗粒存在下，将含硫重油催化裂化，从而将重油转化为 轻油，在催化剂颗粒上沉积含硫焦炭，并用硫化铁将催化剂颗粒中所含的还原铁部分固定在分解的硫化合物上; 在第二区域中，将来自第一区域的催化剂与含氧气体接触的量小于理论上所需的量，从而部分燃烧催化剂上的焦炭，减少催化剂中的铁，并固定在 焦炭为硫化铁; 并且在第三区域中，使来自第二区域的还原催化剂以蒸气以流化方式接触以产生氢气和硫化氢，并将催化剂中还原的铁和硫化铁转化为氧化铁，得到含氧化铁的催化剂 在第三区域中被再循环到第二区域以被还原，并且在第二区域中获得的部分还原态催化剂被再循环到第一区域中。

    Process for simultaneously cracking heavy hydrocarbons into light oils and producing hydrogen
    3.
    发明授权
    Process for simultaneously cracking heavy hydrocarbons into light oils and producing hydrogen 失效
    将重质烃同时裂解成轻油并生产氢的方法

    公开(公告)号：US4421635A

    公开(公告)日：1983-12-20

    申请号：US348542

    申请日：1982-02-12

    Applicant: Tadashi Murakami ,  Teruo Suzuka ,  Yukio Inoue ,  Shirou Aizawa

    Inventor： Tadashi Murakami ,  Teruo Suzuka ,  Yukio Inoue ,  Shirou Aizawa

    IPC: C10G11/04 ,  B01J23/00 ,  B01J23/74 ,  B01J23/94 ,  C01B3/10 ,  C01B3/38 ,  C10G11/00 ,  C10G11/14 ,  C10G11/18 ,  C10G47/04

    CPC classification number: C10G11/18 ,  B01J23/94 ,  C10G11/14 ,  Y02E60/36 ,  Y02P30/446

    Abstract: A process for simultaneously cracking a heavy hydrocarbons to form light oil and producing hydrogen is described, which comprises (1) a first step wherein steam and heavy hydrocarbons are simultaneously contacted with a catalyst in a reduced state, containing iron in the form of iron oxide, to produce hydrogen, cracked gases and cracked light oils, to convert the reduced-state catalyst into an oxidized-state catalyst, and to deposit coke on the catalyst, (2) a second step wherein the oxidized-state catalyst with coke deposited thereon is contacted with an oxygen-containing gas to partially combust the coke on the catalyst, to convert the oxidized-state catalyst into a reduced-state catalyst, and to fix a sulfur compound contained in the coke as iron sulfide with a part of the reduced-state catalyst; and (3) a third step wherein catalyst obtained from the second step, the major portion of the catalyst being recycled between the first step and second step, is contacted with an oxygen-containing gas at a temperature of from 600.degree. to 1,000.degree. C. to effect roasting and gasification of iron sulfide in the catalyst.

    Abstract translation: 描述了同时裂化重质烃以形成轻油并产生氢的方法，其包括（1）第一步骤，其中蒸汽和重质烃同时与还原状态的催化剂接触，所述催化剂含有氧化铁形式的铁 产生氢气，裂化气体和裂解轻油，将还原态催化剂转化为氧化态催化剂，并将焦炭沉积在催化剂上，（2）第二步，其中沉积有焦炭的氧化态催化剂 与含氧气体接触以部分地燃烧催化剂上的焦炭，将氧化态催化剂转化为还原态催化剂，并将包含在焦炭中的硫化合物固定为硫化铁与部分还原剂 状态催化剂 和（3）第三步骤，其中从第二步骤获得的催化剂在第一步骤和第二步骤之间循环的主要部分与含氧气体在600至1000℃的温度下接触 在催化剂中进行硫化铁的焙烧和气化。

    Process for simultaneously cracking heavy hydrocarbons into light oils and producing hydrogen
    4.
    发明授权
    Process for simultaneously cracking heavy hydrocarbons into light oils and producing hydrogen 失效
    将重质烃同时裂解成轻油并生产氢的方法

    公开(公告)号：US4399023A

    公开(公告)日：1983-08-16

    申请号：US348540

    申请日：1982-02-12

    Applicant: Teruo Suzuka ,  Yukio Inoue ,  Shirou Aizawa ,  Yasushi Ishibashi ,  Hidetaka Ohse

    Inventor： Teruo Suzuka ,  Yukio Inoue ,  Shirou Aizawa ,  Yasushi Ishibashi ,  Hidetaka Ohse

    IPC: C01B3/32 ,  B01J23/00 ,  B01J23/745 ,  B01J23/94 ,  C01B3/10 ,  C10G11/00 ,  C10G11/02 ,  C10G11/04 ,  C10G11/14 ,  C10G11/18 ,  C10J3/54

    CPC classification number: C10G11/14 ,  B01J23/94 ,  C10G11/18 ,  Y02E60/36

    Abstract: A process for simultaneously cracking heavy hydrocarbons to form light oil and producing hydrogen is described, which comprises (1) a first step wherein steam and heavy hydrocarbons are simultaneously contacted with a catalyst in a reduced state, containing iron in the form of iron oxide, to produce hydrogen, cracked gases and cracked light oils, to convert the reduced-state catalyst into an oxidized-state catalyst, and to deposit coke on the catalyst, (2) a second step wherein the oxidized-state catalyst with coke deposited thereon is contacted with an oxygen-containing gas to partially combust the coke on the catalyst, to convert the oxidized-state catalyst into a reduced-state catalyst, and to fix a sulfur compound contained in the coke as iron sulfide with a part of the reduced-state catalyst; and (3) a third step wherein catalyst obtained from the first step, the major portion of the catalyst being recycled between the first step and second step, is contacted with an oxygen-containing gas at a temperature of from 600.degree. to 1,000.degree. C. to effect roasting and gasification of iron sulfide in the catalyst.

    Abstract translation: 描述了同时裂化重质烃以形成轻油并产生氢气的方法，其包括（1）第一步骤，其中蒸汽和重质烃同时与还原状态的催化剂接触，所述催化剂含有氧化铁形式的铁， 产生氢气，裂化气体和裂解轻油，将还原态催化剂转化为氧化态催化剂，并将焦炭沉积在催化剂上，（2）第二步，其中沉积有焦炭的氧化态催化剂为 与含氧气体接触以部分地燃烧催化剂上的焦炭，将氧化态催化剂转化为还原态催化剂，并将包含在焦炭中的硫化合物与硫化铁固定在一起， 状态催化剂; 和（3）第三步骤，其中从第一步骤获得的催化剂在第一步骤和第二步骤之间循环的主要部分与含氧气体在600-1000℃的温度下接触 在催化剂中进行硫化铁的焙烧和气化。

    Process for production of methylnaphthalenes
    6.
    发明授权
    Process for production of methylnaphthalenes 失效
    甲基萘生产工艺

    公开(公告)号：US5045178A

    公开(公告)日：1991-09-03

    申请号：US491033

    申请日：1990-03-09

    Applicant: Fumio Maruyama ,  Shirou Aizawa ,  Kazuo Fujiyoshi

    Inventor： Fumio Maruyama ,  Shirou Aizawa ,  Kazuo Fujiyoshi

    IPC: B01J23/42 ,  C07B61/00 ,  C07C5/41 ,  C07C15/24 ,  C10G50/00 ,  C10G65/04 ,  C10G69/08

    CPC classification number: C10G65/043 ,  C10G2400/30

    Abstract: A process for producing methylnaphthalenes is disclosed, comprising subjecting a fraction containing at least 50% by volume of components within the boiling range of 195.degree.-215.degree. C., which is obtained by distilling a raffinate resulting from the recovery of normal paraffins from a hydrodesulfurized kerosene fraction, to reforming reaction and then recovering methylnaphthalenes from the product oil.

    Abstract translation: 公开了一种生产甲基萘的方法，其包括将含至少50体积％组分的馏分在195〜-22℃的沸点范围内进行，该馏分是通过蒸馏由正链烷烃回收得到的萃余液 加氢脱硫煤油馏分，进行重整反应，然后从产物油中回收甲基萘。

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