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1.发明授权Hydrocarbon-reforming catalyst and process for producing synthesis gas using the same 有权烃重整催化剂及使用其的合成气的制造方法公开(公告)号：US08178003B2
公开(公告)日：2012-05-15
申请号：US12734053
申请日：2008-10-08
CPC分类号： B01J23/002 , B01J23/825 , B01J23/85 , B01J23/864 , B01J23/866 , B01J23/888 , B01J37/0063 , B01J37/0205 , B01J2523/00 , C01B3/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0283 , C01B2203/1041 , C01B2203/1052 , C01B2203/1058 , C01B2203/1094 , C01B2203/1241 , C01B2203/1247 , Y02P20/142 , Y02P20/52 , B01J2523/22 , B01J2523/23 , B01J2523/32 , B01J2523/845 , B01J2523/847 , B01J2523/69 , B01J2523/67
摘要： A hydrocarbon-reforming catalyst comprising a composite oxide having a composition represented by the following formula (I) in which Co, Ni and M are dispersed in the composite oxide and a process for producing a synthesis gas by using the catalyst are provided. aM.bCo.cNi.dMg.eCa.fO (I) wherein a, b, c, d, e, and f are molar fractions, a+b+c+d+e=1, 0.0001
摘要翻译： 提供了一种烃重整催化剂，其包含具有下式（I）表示的组成的复合氧化物，其中Co，Ni和M分散在复合氧化物中，以及使用该催化剂制备合成气的方法。 其中a，b，c，d，e和f是摩尔分数，a + b + c + d + e = 1，0.0001
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2.发明申请公开(公告)号：US20100207070A1
公开(公告)日：2010-08-19
申请号：US12734053
申请日：2008-10-08
CPC分类号： B01J23/002 , B01J23/825 , B01J23/85 , B01J23/864 , B01J23/866 , B01J23/888 , B01J37/0063 , B01J37/0205 , B01J2523/00 , C01B3/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0283 , C01B2203/1041 , C01B2203/1052 , C01B2203/1058 , C01B2203/1094 , C01B2203/1241 , C01B2203/1247 , Y02P20/142 , Y02P20/52 , B01J2523/22 , B01J2523/23 , B01J2523/32 , B01J2523/845 , B01J2523/847 , B01J2523/69 , B01J2523/67
摘要： The hydrocarbon-reforming catalyst comprising a composite oxide having a composition represented by the following formula (I) in which Co, Ni and M are dispersed in the composite oxide and a process for producing a synthesis gas by using the catalyst are provided. aM.bCo.cNi.dMg.eCa.fO (I) wherein a, b, c, d, e, and f are molar fractions, a+b+c+d+e=1, 0.0001
摘要翻译： 提供了包含具有由下式（I）表示的组成的复合氧化物的烃重整催化剂，其中Co，Ni和M分散在复合氧化物中，以及通过使用催化剂制备合成气的方法。 其中a，b，c，d，e和f是摩尔分数，a + b + c + d + e = 1，0.0001
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3.发明申请公开(公告)号：US20100303712A1
公开(公告)日：2010-12-02
申请号：US12675716
申请日：2007-11-19
CPC分类号： B01J23/63 , B01J23/002 , B01J23/10 , B01J23/83 , B01J37/0201 , B01J37/031 , B01J2523/00 , C01B3/40 , C01B2203/0238 , C01B2203/0261 , C01B2203/0283 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1082 , C01B2203/1211 , C01B2203/1217 , C01B2203/1229 , C01B2203/1241 , C01B2203/1247 , C01B2203/1258 , H01M8/0618 , Y02E60/50 , Y02P20/52 , B01J2523/36 , B01J2523/3712 , B01J2523/48
摘要： The drive of direct-heat-supply type reforming of hydrocarbon at ordinary temperature is necessary in order to realize a self-sustaining, on-site reforming type fuel cell system which does not necessitate the supply of energy from the outside. According to the invention, an oxide, CeO2 or Pr6O11, or a Ce/Zr or Ce/Zr/Y double oxide is used as the oxide containing a rare earth element capable of changing the oxidation number with an active metal and oxygen defects are introduced into the oxide or double oxide by activating the oxide or double oxide with a reducing gas at high temperature. When a reaction gas containing hydrocarbon and oxygen is passed though the catalyst at low temperature, the oxygen defects react with oxygen and thereby return to the original oxide. Since this return reaction is an exothermic reaction, the catalyst itself is heated, which acts as the driving force for advancing the combustion of the hydrocarbon, whereby the catalyst layer is further heated and the reforming is advanced to from hydrogen. Thus, the hydrogen-producing reaction can be driven even at low temperature, particularly ordinary temperature.
摘要翻译： 为了实现不需要从外部供应能量的自持式现场重整型燃料电池系统，需要在常温下直接进行碳氢化合物的重整的驱动。 根据本发明，使用氧化物CeO 2或Pr 6 O 11或Ce / Zr或Ce / Zr / Y双氧化物作为含有能够用活性金属改变氧化数的稀土元素的氧化物，并引入氧缺陷 通过在高温下还原气体活化氧化物或双氧化物而进入氧化物或双氧化物。 当含有烃和氧的反应气体在低温下通过催化剂时，氧缺陷与氧反应，从而返回到原始氧化物。 由于该返回反应是放热反应，所以催化剂本身被加热，其作为促进烃的燃烧的驱动力，由此催化剂层进一步加热并且重整进行到氢。 因此，即使在低温，特别是常温也可以驱动制氢反应。
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4.发明授权Hydrogen production catalyst, production method of the same and hydrogen production method 有权氢气生产催化剂，生产方法相同，氢气生产方法公开(公告)号：US09073043B2
公开(公告)日：2015-07-07
申请号：US12675716
申请日：2007-11-19
IPC分类号： C01B3/26 , B01J23/63 , B01J23/00 , B01J23/10 , B01J23/83 , C01B3/40 , H01M8/06 , B01J37/02 , B01J37/03
CPC分类号： B01J23/63 , B01J23/002 , B01J23/10 , B01J23/83 , B01J37/0201 , B01J37/031 , B01J2523/00 , C01B3/40 , C01B2203/0238 , C01B2203/0261 , C01B2203/0283 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1082 , C01B2203/1211 , C01B2203/1217 , C01B2203/1229 , C01B2203/1241 , C01B2203/1247 , C01B2203/1258 , H01M8/0618 , Y02E60/50 , Y02P20/52 , B01J2523/36 , B01J2523/3712 , B01J2523/48
摘要： The drive of direct-heat-supply type reforming of hydrocarbon at ordinary temperature is necessary in order to realize a self-sustaining, on-site reforming type fuel cell system which does not necessitate the supply of energy from the outside. According to the invention, an oxide, CeO2 or Pr6O11, or a Ce/Zr or Ce/Zr/Y double oxide is used as the oxide containing a rare earth element capable of changing the oxidation number with an active metal and oxygen defects are introduced into the oxide or double oxide by activating the oxide or double oxide with a reducing gas at high temperature. When a reaction gas containing hydrocarbon and oxygen is passed though the catalyst at low temperature, the oxygen defects react with oxygen and thereby return to the original oxide. Since this return reaction is an exothermic reaction, the catalyst itself is heated, which acts as the driving force for advancing the combustion of the hydrocarbon, whereby the catalyst layer is further heated and the reforming is advanced to from hydrogen. Thus, the hydrogen-producing reaction can be driven even at low temperature, particularly ordinary temperature.
摘要翻译： 为了实现不需要从外部供应能量的自持式现场重整型燃料电池系统，需要在常温下直接进行碳氢化合物的重整的驱动。 根据本发明，使用氧化物CeO 2或Pr 6 O 11或Ce / Zr或Ce / Zr / Y双氧化物作为含有能够用活性金属改变氧化数的稀土元素的氧化物，并引入氧缺陷 通过在高温下还原气体活化氧化物或双氧化物而进入氧化物或双氧化物。 当含有烃和氧的反应气体在低温下通过催化剂时，氧缺陷与氧反应，从而返回到原始氧化物。 由于该返回反应是放热反应，所以催化剂本身被加热，其作为促进烃的燃烧的驱动力，由此催化剂层进一步加热并且重整进行到氢。 因此，即使在低温，特别是常温也可以驱动制氢反应。
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