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    Processes for the production of fluoropropanes and halopropenes and azeotropic compositions of 2-chloro-3,3,3-trifluoro-1-propene with HF and of 1,1,1,2,2-pentafluoropropane with HF
    6.
    发明授权
    Processes for the production of fluoropropanes and halopropenes and azeotropic compositions of 2-chloro-3,3,3-trifluoro-1-propene with HF and of 1,1,1,2,2-pentafluoropropane with HF 有权
    制备氟丙烷和卤代丙烯的方法和2-氯-3,3,3-三氟-1-丙烯与HF和1,1,1,2,2-五氟丙烷与HF的共沸组合物

    公开(公告)号：US08696926B2

    公开(公告)日：2014-04-15

    申请号：US13688720

    申请日：2012-11-29

    申请人： E I du Pont de Nemours and Company

    发明人： Velliyur Nott Mallikarjuna Rao ,  Allen Capron Sievert

    IPC分类号： C09K5/04 ,  C07C21/18

    CPC分类号： C07C17/21 ,  B01J23/26 ,  B01J23/864 ,  B01J37/26 ,  C07C17/00 ,  C07C17/087 ,  C07C17/20 ,  C07C17/206 ,  C07C17/23 ,  C07C17/25 ,  C07C17/35 ,  C07C19/08 ,  C07C21/18

    摘要： A process is disclosed for making CF3CH2CHF2, CF3CH═CHF and/or CF3CH═CHCl. The process involves reacting at least one starting material selected from the group consisting of halopropanes of the formula CX3CHClCH2X, halopropenes of the formula CX3CCl═CH2 and halopropenes of the formula CX2═CClCH2X, wherein each X is independently F or Cl, with HF in a reaction zone to produce a product mixture comprising HF, HCl, CF3CH2CHF2, CF3CH═CHF and CF3CH═CHCl; and recovering the CF3CH2CHF2, CF3CH═CHF and/or CF3CH═CHCl from the product mixture. Also disclosed is a process for making CF3CF2CH3 and/or CF3CF═CH2. In each of the processes the molar ratio of HF to total amount of starting material fed to the reaction zone is at least stoichiometric. Also disclosed is an azeotropic composition comprising CF3CCl═CH2, and HF. Also disclosed is an azeotropic composition comprising CF3CF2CH3, and HF.

    摘要翻译： 公开了制备CF 3 CH 2 CHF 2，CF 3 CH = CHF和/或CF 3 CH = CHCl的方法。 该方法包括使至少一种选自式CX3CHClCH2X的卤代丙烷，式CX3CCl = CH2的卤代丙烯和式CX2 = CClCH2X的卤代丙烯，其中每个X独立地为F或Cl的起始材料与HF在 反应区以产生包含HF，HCl，CF 3 CH 2 CHF 2，CF 3 CH = CHF和CF 3 CH = CHCl的产物混合物; 并从产物混合物中回收CF 3 CH 2 CHF 2，CF 3 CH = CHF和/或CF 3 CH = CHCl。 还公开了制备CF 3 CF 2 CH 3和/或CF 3 CF = CH 2的方法。 在每个方法中，HF与进料至反应区的原料的总量的摩尔比至少为化学计量。 还公开了包含CF 3 CCl 2 CH 2和HF的共沸组合物。 还公开了包含CF 3 CF 2 CH 3和HF的共沸组合物。

    Process for the epoxidation of hydrocarbons
    10.
    发明授权
    Process for the epoxidation of hydrocarbons 失效
    烃类环氧化方法

    公开(公告)号：US06673949B2

    公开(公告)日：2004-01-06

    申请号：US10214073

    申请日：2002-08-07

    申请人： Ursula Jansen ,  Andreas Wegner

    发明人： Ursula Jansen ,  Andreas Wegner

    IPC分类号： C07D30108

    CPC分类号： C07D301/08 ,  B01J23/686 ,  B01J23/688 ,  B01J23/75 ,  B01J23/755 ,  B01J23/8432 ,  B01J23/864 ,  B01J23/866 ,  B01J23/8878 ,  B01J23/8896 ,  B01J23/89 ,  B01J23/8946 ,  B01J23/8966 ,  B01J23/8973 ,  B01J23/8993 ,  B01J35/1014 ,  B01J35/1019 ,  B01J37/0205

    摘要： The present invention relates to a process for the epoxidation of hydrocarbons. This process comprises reacting at least one hydrocarbon with oxygen or air or nitrous oxide or other gaseous oxidants, in the presence of a mixture comprising at least two elements selected from the group consisting of Sc, Y, Ti, Zr, Hf, V, Nb, Ta, Cr, Mo, W, Re, Fe, Co, Ni, Sn, Pb, Sb, Bi and Se, on a support with a BET surface area of less than 200 m2/g. The present invention also relates to catalysts suitable for the epoxidation of hydrocarbons, wherein the catalyst comprises a mixture comprising at least two metals selected from the group consisting of Sc, Y, Ti, Zr, Hf, V, Nb, Ta, Cr, Mo, W, Re, Fe, Co, Ni, Sn, Pb, Sb, Bi and Se, on a support with a BET surface area of less than 200 m2/g.

    摘要翻译： 本发明涉及烃的环氧化方法。 该方法包括使至少一种烃与氧或空气或一氧化二氮或其它气体氧化剂在包含选自Sc，Y，Ti，Zr，Hf，V，Nb中的至少两种元素的混合物存在下反应 ，Ta，Cr，Mo，W，Re，Fe，Co，Ni，Sn，Pb，Sb，Bi和Se，在BET表面积小于200m 2 / g的载体上。 本发明还涉及适用于烃类环氧化的催化剂，其中催化剂包括选自Sc，Y，Ti，Zr，Hf，V，Nb，Ta，Cr，Mo中的至少两种金属的混合物 ，W，Re，Fe，Co，Ni，Sn，Pb，Sb，Bi和Se在BET表面积小于200m 2 / g的载体上。