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1.发明授权
公开(公告)号：US4675343A
公开(公告)日：1987-06-23
申请号：US863283
申请日：1986-05-15
IPC分类号： C07C29/15 , B01J23/00 , C07B61/00 , C07C27/00 , C07C29/156 , C07C31/02 , C07C67/00 , C07C27/06
CPC分类号： C07C29/156 , Y02P20/52
摘要： The present invention concerns a process of use of a copper and cobalt-containing catalyst for synthesizing saturated primary aliphatic alcohols. This process comprises a first step consisting in at least one catalyst prereduction by means of a gas mixture containing a reducing compound, a second step wherein the prereduced catalyst is contacted with a mixture of hydrogen and carbon oxides (CO, CO.sub.2) for at least 10 hours, so as to produce a mixture of alcohols; a third step wherein the catalyst obtained in the second step is subjected to a treatment with a gas mixture containing a single reducing gas, during about 1 to 400 hours and a fourth step of synthesizing saturated primary aliphatic alcohols from a mixture containing hydrogen and carbon oxides.Optionally the process also comprises an additional step consisting of subjecting the catalyst, whose activity and/or selectivity has been partially lost, to a new treatment according to the procedure defined for the third step.The process according to the invention is particularly applicable to catalysts containing copper, cobalt and optionally aluminum and/or zinc and/or sodium.
摘要翻译： 本发明涉及使用含铜和钴的催化剂合成饱和伯脂肪醇的方法。 该方法包括通过含有还原化合物的气体混合物进行至少一种催化剂预还原的第一步骤，其中将预还原的催化剂与氢和碳氧化物（CO，CO 2）的混合物接触至少10 小时，以产生醇的混合物; 第三步骤，其中将第二步中得到的催化剂在含有单一还原气体的气体混合物中进行约1-4小时的处理，以及从含有氢和碳氧化物的混合物中合成饱和伯脂肪醇的第四步骤 。 任选地，该方法还包括另外的步骤，该方法包括将其活性和/或选择性已被部分丧失的催化剂按照根据第三步所定义的方法进行新的处理。 根据本发明的方法特别适用于含有铜，钴和任选的铝和/或锌和/或钠的催化剂。
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2.发明授权
公开(公告)号：US4791141A
公开(公告)日：1988-12-13
申请号：US928655
申请日：1986-11-05
IPC分类号： C07C29/15 , B01J21/04 , B01J23/00 , B01J23/72 , B01J23/75 , B01J23/80 , B01J23/89 , B01J37/03 , C07B61/00 , C07C27/00 , C07C29/153 , C07C29/156 , C07C31/02 , C07C67/00 , C07C27/06
CPC分类号： C07C29/156 , B01J23/80 , B01J37/03
摘要： Process for manufacturing primary alcohols by reacting carbon oxides with hydrogen, in the presence of a catalyst containing, as essential elements, copper, zinc and aluminum, in respective atomic ratios of Zn/Al=0.4:1 to 2:1 Co/Al=0.2:1 to 0.75:1; Cu/Al=0.1:1 to 3:1, the proportion by weight of each metal with respect to the total metals weight being: copper: 10-50%; cobalt: 5-25%; aluminum: 5-30%; zinc: 10-70%, the homogeneity of the catalyst being such that the variations of the atomic ratios Al/Co, Cu/Cc, Zn/Co within the catalyst, at the scale of 5 nanometers are lower than 15% with respect to the average value of said ratio. The catalyst may be prepared by complexing or by coprecipitation of the catalyst elements.
摘要翻译： 在含有作为必需元素的铜，锌和铝的催化剂存在下，碳原子数为1〜4：1〜2：1的Co / Al = 0.2：1〜0.75：1; Cu / Al = 0.1:1〜3:1，各金属重量相对于总金属重量的比例为：铜：10〜50％ 钴：5-25％; 铝：5-30％; 锌：10-70％，催化剂的均匀性使得催化剂中的原子比Al / Co，Cu / Cc，Zn / Co在5纳米尺度上的变化相对于 所述比例的平均值。 催化剂可以通过使催化剂元素络合或共沉淀来制备。
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3.发明授权Process for preparing normally liquid oxygenate and hydrocarbonaceous products from a hydrocarbon feed containing linear- and branched olefins 失效从含有直链和支链烯烃的烃进料制备正常液态含氧化合物和烃类产物的方法
公开(公告)号：US5023389A
公开(公告)日：1991-06-11
申请号：US308489
申请日：1989-02-10
申请人： Pierre Grandvallet , Andras G. T. G. Kortbeek , Johannes P. Van Den Berg , Karl-Heinz Robschlager
发明人： Pierre Grandvallet , Andras G. T. G. Kortbeek , Johannes P. Van Den Berg , Karl-Heinz Robschlager
IPC分类号： B01J29/04 , B01J23/12 , B01J29/24 , B01J29/26 , B01J29/87 , C07B61/00 , C07C1/00 , C07C2/12 , C07C2/58 , C07C5/27 , C07C5/32 , C07C5/393 , C07C5/41 , C07C11/02 , C07C27/00 , C07C29/04 , C07C31/12 , C07C41/00 , C07C41/06 , C07C43/04 , C07C67/00 , C10G50/00 , C10L1/06
摘要： The invention relates to a process for preparing normally liquid hydrocarbon products such as middle distillates and methyl-t-butylether from a hydrocarbon feed containing linear and branched olefins (e.g. propane and butenes in light ends) comprising at least the following steps:i) selectively converting branched olefins in the feed in the presence of a catalyst into a normally liquid hydrocarbonaceous product (e.g. MTBE);ii) separating linear olefins from product obtained in step (i), andiii) catalytically oligomerizing linear olefins obtained from step (ii) into liquid hydrocarbons such as middle distillates.
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公开(公告)号：US5554307A
公开(公告)日：1996-09-10
申请号：US559521
申请日：1995-11-15
IPC分类号： C10G25/00 , C10G67/06 , C10G71/00 , C10M101/02 , C10N30/00 , C10N30/10 , C10N70/00 , C10M125/02
CPC分类号： C10G25/003 , C10G25/00 , C10G67/06
摘要： A process for improving the quality of lubricating base oils, which process comprises contacting a lubricating base oil with dry activated carbon.
摘要翻译： 一种用于提高润滑基础油质量的方法，该方法包括使润滑基础油与干活性炭接触。
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公开(公告)号：US5427703A
公开(公告)日：1995-06-27
申请号：US71428
申请日：1993-06-02
IPC分类号： C10M109/02 , C10M177/00 , C10M133/58 , C10M135/02
CPC分类号： C10M177/00 , C10M109/02
摘要： Process for the preparation of a polar lubricating base oil, including reacting a hydrocarbonaceous product with a polar compound, including at least one heteroatom and which hydrocarbonaceous product has been prepared by contacting hydrocarbons and/or derivatives thereof with an active-hydrogen containing system by a process which includes generating a hydrogen-containing plasma and allowing contact of the hydrocarbons and/or derivatives thereof in liquid form with the plasma-generated system and recovering the hydrocarbonaceous product.
摘要翻译： 用于制备极性润滑基础油的方法，包括使含烃产物与极性化合物反应，所述极性化合物包括至少一个杂原子，并且通过使烃和/或其衍生物与含活性氢的体系通过 该方法包括产生含氢等离子体并允许液体形式的烃和/或其衍生物与等离子体产生的系统接触并回收含烃产物。
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公开(公告)号：US5804058A
公开(公告)日：1998-09-08
申请号：US662596
申请日：1996-06-13
CPC分类号： C10G45/64 , B01J2229/16 , B01J2229/32 , B01J29/40 , B01J29/65
摘要： A process is disclosed for the catalytic dewaxing of a hydrocarbon oil feed comprising waxy molecules, which process comprises: contacting a feed under catalytic dewaxing conditions with a catalyst composition comprising a molecular sieve containing crystallites covalently bound alumina moieties in its framework and having pores with a diameter in the range of from 0.35 to 0.80 nm and recovering a product having a reduced pour point, wherein the molecular sieve has been modified to reduce the mole percentage of alumina by coating the surface of the crystallites with a refractory inorganic oxide which is essentially free of alumina.
摘要翻译： 公开了一种用于包含蜡质分子的烃油进料的催化脱蜡的方法，该方法包括：在催化脱蜡条件下使进料与催化剂组合物接触，所述催化剂组合物包含其框架中含有微晶共价结合的氧化铝部分的分子筛，并具有孔 直径在0.35至0.80nm的范围内并回收具有降低的倾点的产物，其中分子筛已经被改性以通过用基本上没有的耐火无机氧化物涂覆微晶表面来降低氧化铝的摩尔百分比 的氧化铝。
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公开(公告)号：US5470454A
公开(公告)日：1995-11-28
申请号：US71434
申请日：1993-06-02
CPC分类号： C10G15/12 , C10G2400/10
摘要： A process for the preparation of a lubricating base oil, comprising treating a hydrocarbonaceous product with hydrogen, at elevated temperature and pressure and in the presence of a catalyst, which hydrocarbonaceous product has been prepared by contacting hydrocarbons and/or derivatives thereof with an active hydrogen-containing system by a process which comprises generating a hydrogen-containing plasma and allowing contact of the hydrocarbons and/or derivatives thereof in liquid form with the plasma-generated system and recovering the hydrocarbonaceous product.
摘要翻译： 一种用于制备润滑基础油的方法，包括在升高的温度和压力下和在催化剂存在下用氢处理含烃产物，所述烃类产物是通过使烃和/或其衍生物与活性氢接触而制备的 其包括产生含氢等离子体并允许液体形式的烃和/或其衍生物与等离子体产生的系统接触并回收含烃产物的方法。
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公开(公告)号：US07261808B2
公开(公告)日：2007-08-28
申请号：US10492720
申请日：2002-10-16
IPC分类号： C01M175/02 , C10G65/02
CPC分类号： C10M175/0041
摘要： A process to further upgrade a pre-processed used lubricating oil by: (a) contacting the partially upgraded used oil in the presence of hydrogen with a hydrodemetallization catalyst; (b) contacting the effluent of step (a) in the presence of hydrogen with a hydrotreating catalyst; (c) contacting the effluent of step (b) in the presence of hydrogen with a dewaxing catalyst; and (d) contacting the effluent of step (c) in the presence of hydrogen with a hydrotreating catalyst.
摘要翻译： 一种通过以下步骤进一步升级预处理用过的润滑油的方法：（a）在氢气存在下使部分升级的二手油与加氢脱金属催化剂接触; （b）在氢气存在下使步骤（a）的流出物与加氢处理催化剂接触; （c）在氢存在下使步骤（b）的流出物与脱蜡催化剂接触; 和（d）在氢气存在下将步骤（c）的流出物与加氢处理催化剂接触。
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公开(公告)号：US20050006282A1
公开(公告)日：2005-01-13
申请号：US10492720
申请日：2002-10-16
申请人： Pierre Grandvallet , Anthony Hagan , Laurent Huve
发明人： Pierre Grandvallet , Anthony Hagan , Laurent Huve
IPC分类号： C10M175/00 , C10N70/00 , C10M175/02 , C10G65/02
CPC分类号： C10M175/0041
摘要： A process to further upgrade a pre-processed used lubricating oil by: (a) contacting the partially upgraded used oil in the presence of hydrogen with a hydrodemetallization catalyst; (b) contacting the effluent of step (a) in the presence of hydrogen with a hydrotreating catalyst; (c) contacting the effluent of step (b) in the presence of hydrogen with a dewaxing catalyst; and (d) contacting the effluent of step (c) in the presence of hydrogen with a hydrotreating catalyst.
摘要翻译： 一种通过以下步骤进一步升级预处理用过的润滑油的方法：（a）在氢气存在下使部分升级的二手油与加氢脱金属催化剂接触; （b）在氢气存在下使步骤（a）的流出物与加氢处理催化剂接触; （c）在氢存在下使步骤（b）的流出物与脱蜡催化剂接触; 和（d）在氢气存在下将步骤（c）的流出物与加氢处理催化剂接触。
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公开(公告)号：US5951847A
公开(公告)日：1999-09-14
申请号：US741504
申请日：1996-10-31
CPC分类号： C10G45/64
摘要： A process for catalytically dehazing lubricating base oils is disclosed, which comprises contacting the lubricating base oil in the presence of hydrogen with a catalyst comprising naturally occurring and/or synthetic ferrierite which ferrierite has been modified to reduce the mole percentage of alumina and a low acidity refractory oxide binder material which is essentially free of alumina.
摘要翻译： 公开了一种用于催化脱脂润滑基础油的方法，其包括在氢存在下使润滑基础油与包含天然存在和/或合成的镁碱沸石的催化剂接触，所述镁碱沸石已经被修饰以降低氧化铝的摩尔百分数和低酸度 基本上不含氧化铝的难熔氧化物粘合剂材料。
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