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    Catalytic conversion with improved catalyst
    5.
    发明授权
    Catalytic conversion with improved catalyst 失效
    催化转化催化剂改进

    公开(公告)号：US5348643A

    公开(公告)日：1994-09-20

    申请号：US090872

    申请日：1993-07-13

    申请人： Robert P. L. Absil ,  Joseph A. Herbst

    发明人： Robert P. L. Absil ,  Joseph A. Herbst

    IPC分类号： B01J27/16 ,  B01J29/40 ,  B01J37/00 ,  C10G11/05 ,  C01G11/05

    CPC分类号： B01J27/16 ,  B01J29/40 ,  B01J37/0045 ,  C10G11/05 ,  B01J2229/42

    摘要： A process is provided for converting feedstock hydrocarbon compounds over a catalyst composition which comprises clay and a zeolite component, at least one of which has been treated with a phosphorus-containing compound, for example, ammonium dihydrogen phosphate or phosphoric acid, and which is spray dried at a low pH, preferably lower than about 3. An embodiment of the present invention comprises an improved catalytic cracking process to produce high octane gasoline and increased lower olefins, especially propylene and butylene.

    摘要翻译： 提供了一种用于在包含粘土和沸石组分的催化剂组合物中转化原料烃化合物的方法，其中至少一种已经用含磷化合物，例如磷酸二氢铵或磷酸二氢铵处理，并且是喷雾 在低pH，优选低于约3℃下干燥。本发明的一个实施方案包括改进的催化裂化方法以产生高辛烷值汽油和增加的低级烯烃，特别是丙烯和丁烯。

    Catalytic cracking process utilizing a zeolite beta catalyst synthesized with a chelating agent
    6.
    发明授权
    Catalytic cracking process utilizing a zeolite beta catalyst synthesized with a chelating agent 失效
    使用与螯合剂合成的沸石β催化剂的催化裂化方法

    公开(公告)号：US5232579A

    公开(公告)日：1993-08-03

    申请号：US715189

    申请日：1991-06-14

    申请人： Robert P. L. Absil ,  Joseph A. Herbst ,  Jocelyn A. Kowalski ,  Mae K. Rubin

    发明人： Robert P. L. Absil ,  Joseph A. Herbst ,  Jocelyn A. Kowalski ,  Mae K. Rubin

    IPC分类号： B01J29/70 ,  B01J29/80 ,  C01B39/48

    CPC分类号： B01J29/7007 ,  B01J29/80 ,  C01B39/48 ,  B01J2229/36 ,  B01J2229/37 ,  B01J2229/38

    摘要： A catalytic cracking process for converting a hydrocarbon fraction, preferably boiling in the range of a heavy gas oil, is disclosed in which the cracking catalyst is a large crystal fully crystalline zeolite Beta having a broad range of silica-to-alumina mole ratios, i.e. 20->1000. The zeolite Beta catalyst is synthesized with a nitrogenous organic chelating agent, such as a tertiary alkanolamine, preferably triethanolamine, in the synthesis mixture along with at least one source of organic directing agent such as tetraethylammonium hydroxide, tetraethylammonium bromide and tetraethylammonium fluoride. The zeolite Beta can be used as a stand alone catalyst or an additive catalyst for hydrocarbon cracking reactions along with another molecular seive type catalyst such as a faujasite catalyst or ZSM-5. The large crystal zeolite Beta can also be treated with a source of phosphorus to enhance the properties of the zeolite.

    摘要翻译： 公开了一种用于转化优选在重质瓦斯油范围内沸腾的烃馏分的催化裂化方法，其中裂化催化剂是具有宽范围二氧化硅与氧化铝摩尔比的大晶体完全结晶沸石β，即 20-> 1000。 沸石β催化剂与合成混合物中的含氮有机螯合剂如叔链烷醇胺，优选三乙醇胺一起，与至少一种有机导向剂如四乙基氢氧化铵，四乙基溴化铵和四乙基氟化铵源一起合成。 β沸石可以用作独立催化剂或用于烃裂化反应的添加剂催化剂以及另一种分子筛型催化剂如八面沸石催化剂或ZSM-5。 也可以用磷源处理大的晶体沸石β以增强沸石的性能。

    Cracking catalyst
    9.
    发明授权
    Cracking catalyst 失效
    开裂催化剂

    公开(公告)号：US4880787A

    公开(公告)日：1989-11-14

    申请号：US140872

    申请日：1988-01-06

    申请人： Robert G. Bundens ,  Joseph A. Herbst

    发明人： Robert G. Bundens ,  Joseph A. Herbst

    IPC分类号： B01J29/08 ,  C10G11/05

    CPC分类号： B01J29/084 ,  C10G11/05 ,  B01J2229/16

    摘要： New catalyst compositions of superior hydrothermal stability, which evidence increased gasoline plus distillate yields, improved coke selectivity and reduced C.sub.4.sup.- gas yields, are based on framework dealuminated faujasitic zeolites having a framework silica to alumina molar ratio of from about 5 to 100. In a preferred embodiment, an "ultrastable Y" composited with a matrix, is subjected to a treatment with a source of aluminum and rare earth compounds followed by hydrothermal treatments to improve the hydrothermal stability and selectivity of the catalyst for catalytic cracking. This is evidenced by higher gasoline plus distillate yields and lower coke and gas production at lower catalyst useage per barrel of feed relative to commercial cracking catalysts currently being used.

    摘要翻译： 具有优异的水热稳定性的新催化剂组合物，其基于具有约5至100的骨架二氧化硅与氧化铝摩尔比的框架脱铝的八面沸石沸石，其证明增加的汽油加馏出物产率，改善的焦炭选择性和降低的C4气体产率。 优选的实施方案中，将与基质复合的“超稳定Y”用铝和稀土化合物源进行处理，接着进行水热处理，以提高催化剂裂化催化剂的水热稳定性和选择性。 相对于目前使用的商业裂化催化剂，每桶原料的催化剂用量较低，这表明汽油加馏油产率较高，焦炭和天然气产量较低。