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1.发明授权Catalyst composition including attrition particles and method for making same 有权包含磨耗颗粒的催化剂组合物及其制备方法公开(公告)号：US06509290B1
公开(公告)日：2003-01-21
申请号：US09617714
申请日：2000-07-17
IPC分类号： B01J27182
CPC分类号： B01J29/005 , B01J29/85 , B01J2229/26 , B01J2229/42 , C10G3/45 , C10G3/49 , C10G2300/4081 , C10G2300/708 , C10G2400/20 , Y02P30/20 , Y02P30/42 , Y10S423/30 , Y10S502/514
摘要： Disclosed is a molecular sieve catalyst which contains molecular sieve-containing attrition particles and virgin molecular sieve, the attrition particles having been recycled from a catalyst manufacture process or from a reaction system. The catalyst can be used in a variety of catalytic reaction processes. A desired process is making olefins from an oxygenate feedstock. The recovery and use of the attrition particles in the catalyst is beneficial in minimizing waste, thereby reducing problems relating to both environmental and economic constraints.
摘要翻译： 公开了一种分子筛催化剂，其含有含分子筛的磨损颗粒和原始分子筛，磨损颗粒已经从催化剂制备方法或从反应体系再循环。 催化剂可用于各种催化反应过程。 所需的方法是从含氧化合物原料制备烯烃。 在催化剂中回收和使用磨耗颗粒有利于最小化废物，从而减少与环境和经济限制有关的问题。
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公开(公告)号：US06605749B2
公开(公告)日：2003-08-12
申请号：US10342601
申请日：2003-01-15
IPC分类号： C07C100
CPC分类号： B01J29/005 , B01J29/85 , B01J2229/26 , B01J2229/42 , C10G3/45 , C10G3/49 , C10G2300/4081 , C10G2300/708 , C10G2400/20 , Y02P30/20 , Y02P30/42 , Y10S423/30 , Y10S502/514
摘要： Disclosed is a molecular sieve catalyst which contains molecular sieve-containing attrition particles and virgin molecular sieve, the attrition particles having been recycled from a catalyst manufacture process or from a reaction system. The catalyst can be used in a variety of catalytic reaction processes. A desired process is making olefins from an oxygenate feedstock. The recovery and use of the attrition particles in the catalyst is beneficial in minimizing waste, thereby reducing problems relating to both environmental and economic constraints.
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公开(公告)号：US06541415B2
公开(公告)日：2003-04-01
申请号：US09894158
申请日：2001-06-27
IPC分类号： B01J27182
CPC分类号： B01J29/005 , B01J29/85 , B01J2229/26 , B01J2229/42 , C10G3/45 , C10G3/49 , C10G2300/4081 , C10G2300/708 , C10G2400/20 , Y02P30/20 , Y02P30/42 , Y10S423/30 , Y10S502/514
摘要： Disclosed is a molecular sieve catalyst which contains molecular sieve-containing attrition particles and virgin molecular sieve, the attrition particles having been recycled from a catalyst manufacture process or from a reaction system. The catalyst can be used in a variety of catalytic reaction processes. A desired process is making olefins from an oxygenate feedstock. The recovery and use of the attrition particles in the catalyst is beneficial in minimizing waste, thereby reducing problems relating to both environmental and economic constraints.
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4.发明授权Molecular sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US07541508B2
公开(公告)日：2009-06-02
申请号：US11640559
申请日：2006-12-18
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： C07C1/00
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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5.发明授权Molecular-sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和在转化过程中的应用公开(公告)号：US07301065B2
公开(公告)日：2007-11-27
申请号：US10893642
申请日：2004-07-16
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： C07C1/20
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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6.发明授权Molecular sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US07160831B2
公开(公告)日：2007-01-09
申请号：US10178374
申请日：2002-06-24
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： B01J29/06
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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7.发明授权Molecular sieve catalyst composition, its making and use in conversion processes 失效分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US06787501B2
公开(公告)日：2004-09-07
申请号：US10178578
申请日：2002-06-24
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： B01J2906
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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公开(公告)号：US06395674B1
公开(公告)日：2002-05-28
申请号：US09399675
申请日：1999-09-21
申请人： Shun C. Fung , Marcel J. G. Janssen , Stephen N. Vaughn , Machteld M. Mertens , Albert E. Schweizer , Luc R. M. Martens , Richard B. Hall , Wilfried J. Mortier , Ronald G. Searle , Yi-Gang Xiong
发明人： Shun C. Fung , Marcel J. G. Janssen , Stephen N. Vaughn , Machteld M. Mertens , Albert E. Schweizer , Luc R. M. Martens , Richard B. Hall , Wilfried J. Mortier , Ronald G. Searle , Yi-Gang Xiong
IPC分类号： B01J27182
CPC分类号： C01B39/02 , B01J29/04 , B01J29/85 , B01J37/084 , B01J2229/14 , B01J2229/24 , B01J2229/40 , B01J2229/42 , C01B37/00 , C07C1/20 , C07C2529/85 , C07C11/02
摘要： Disclosed is a method of heat treating a molecular sieve. The method comprises providing a template-containing molecular sieve, heating the molecular sieve under conditions effective to remove a portion of the template from the molecular sieve, and cooling the heated molecular sieve to leave an amount of template effective to cover catalytic sites within the molecular sieve. A catalyst composition is also provided which comprises a molecular sieve having a microporous structure and a binder, wherein between 10 and 90 vol % of the microporous structure is occupied by a material, the material comprising a template or a carbonaceous residue of a template, and the catalyst composition exhibits a Davison Index of not greater than 30.
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公开(公告)号：US07230151B2
公开(公告)日：2007-06-12
申请号：US10891975
申请日：2004-07-15
IPC分类号： C07C1/20
CPC分类号： C07C1/20 , C07C2529/80 , Y02P30/42 , C07C11/02
摘要： This invention is to a process of making olefin, particularly ethylene and propylene, from an oxygenate feed. The invention uses two or more zeolite catalysts. Examples of zeolite catalysts include a first catalyst containing of ZSM-5, and a second catalyst containing a 10-ring molecular sieve, including but not limited to, ZSM-22, ZSM-23, ZSM35, ZSM-48, and mixtures thereof. The ZSM-5 can be unmodified, phosphorous modified, steam modified having a micropore volume reduced to not less than 50% of that of the unsteamed ZSM-5, or various mixtures thereof.
摘要翻译： 本发明是由含氧化合物进料制备烯烃，特别是乙烯和丙烯的方法。 本发明使用两种或更多种沸石催化剂。 沸石催化剂的实例包括含有ZSM-5的第一催化剂和含有10环分子筛的第二催化剂，包括但不限于ZSM-22，ZSM-23，ZSM35，ZSM-48及其混合物。 ZSM-5可以是未改性的，磷改性的，蒸汽改性的，具有减小到不少于未蒸发的ZSM-5或其各种混合物的50％的微孔体积。
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公开(公告)号：US06797851B2
公开(公告)日：2004-09-28
申请号：US09943610
申请日：2001-08-30
IPC分类号： C07C1207
CPC分类号： C07C1/20 , C07C2529/80 , Y02P30/42 , C07C11/02
摘要： This invention is to a process of making olefin, particularly ethylene and propylene, from an oxygenate feed. The invention uses two or more zeolite catalysts. Examples of zeolite catalysts include a first catalyst containing of ZSM-5, and a second catalyst containing a 10-ring molecular sieve, including but not limited to, ZSM-22, ZSM-23, ZSM35, ZSM-48, and mixtures thereof. The ZSM-5 can be unmodified, phosphorous modified, steam modified having a micropore volume reduced to not less than 50% of that of the unsteamed ZSM-5, or various mixtures thereof.
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