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    LOW OXYGEN BIOMASS-DERIVED PYROLYSIS OILS AND METHODS FOR PRODUCING THE SAME
    1.
    发明申请
    LOW OXYGEN BIOMASS-DERIVED PYROLYSIS OILS AND METHODS FOR PRODUCING THE SAME 审中-公开
    低氧生物质衍生的热解油及其生产方法

    公开(公告)号：WO2011103054A2

    公开(公告)日：2011-08-25

    申请号：PCT/US2011024722

    申请日：2011-02-14

    Applicant: UOP LLC ,  MARINANGELI RICHARD ,  BRANDVOLD TIMOTHY A ,  KOCAL JOSEPH A

    Inventor： MARINANGELI RICHARD ,  BRANDVOLD TIMOTHY A ,  KOCAL JOSEPH A

    IPC: C10B53/02 ,  B01J23/38 ,  B01J29/04 ,  C10G3/00 ,  F25J1/00

    CPC classification number: C10G3/44 ,  C10G3/45 ,  C10G3/47 ,  C10G3/48 ,  C10G3/49 ,  C10G2400/30 ,  Y02E50/14 ,  Y02P30/20

    Abstract: Low oxygen biomass-derived pyrolysis oils and methods for producing them from carbonaceous biomass feedstock are provided. The carbonaceous biomass feedstock is pyrolyzed in the presence of a catalyst comprising base metal-based catalysts, noble metal- based catalysts, treated zeolitic catalysts, or combinations thereof to produce pyrolysis gases. During pyrolysis, the catalyst catalyzes a deoxygenation reaction whereby at least a portion of the oxygenated hydrocarbons in the pyrolysis gases are converted into hydrocarbons. The oxygen is removed as carbon oxides and water. A condensable portion (the vapors) of the pyrolysis gases is condensed to low oxygen biomass-derived pyrolysis oil.

    Abstract translation: 提供了低氧生物质衍生的热解油及其从碳质生物质原料生产它们的方法。 碳质生物质原料在催化剂存在下热解，该催化剂包含基于贱金属的催化剂，贵金属基催化剂，经处理的沸石催化剂或其组合以产生热解气体。 在热解期间，催化剂催化脱氧反应，由此将热解气体中的至少一部分氧化烃转化成烃。 作为碳氧化物和水除去氧气。 热解气体的可冷凝部分（蒸汽）被冷凝成低氧生物质衍生的裂解油。

    A PROCESS FOR THE DIRECT PRODUCTION OF METHANOL FROM METHANE
    3.
    发明申请
    A PROCESS FOR THE DIRECT PRODUCTION OF METHANOL FROM METHANE 审中-公开
    一种从甲烷直接生产甲醇的方法

    公开(公告)号：WO2007073532A2

    公开(公告)日：2007-06-28

    申请号：PCT/US2006061830

    申请日：2006-12-11

    Applicant: UOP LLC ,  BRANDVOLD TIMOTHY A ,  KOCAL JOSEPH A

    Inventor： BRANDVOLD TIMOTHY A ,  KOCAL JOSEPH A

    CPC classification number: C07C29/48 ,  C07C29/095 ,  C07C29/80 ,  C07C67/035 ,  C07C69/63 ,  C07C31/04

    Abstract: A process for the production of methanol from methane has been developed. The process involves reacting methane with an oxidant such as oxygen or a peroxide in the presence of a catalyst and a solvent in a reaction zone to produce an effluent stream comprising a methanol product. The effluent stream is next separated into a gaseous stream comprising unreacted methane and carbon dioxide and a liquid stream comprising the methanol product and solvent. Next the gaseous stream is further separated to provide a methane stream which is recycled to the reaction zone. Finally, a methanol stream is isolated and a solvent stream is recycled to the reaction zone.

    Abstract translation: 已经开发了从甲烷生产甲醇的方法。 该方法包括使甲烷与氧化剂如氧气或过氧化物在催化剂和溶剂存在下在反应区中反应以产生包含甲醇产物的流出物流。 接着将流出物流分离成包含未反应的甲烷和二氧化碳的气态物流和包含甲醇产物和溶剂的液态物流。 接下来，将气体流进一步分离以提供循环到反应区的甲烷流。 最后，分离甲醇流并将溶剂流循环至反应区。

    PROCESSES FOR CONVERTING LIGNOCELLULOSICS TO REDUCED ACID PYROLYSIS OIL
    4.
    发明申请
    PROCESSES FOR CONVERTING LIGNOCELLULOSICS TO REDUCED ACID PYROLYSIS OIL 审中-公开
    转化木质纤维素以降低酸解热油的过程

    公开(公告)号：WO2013019328A3

    公开(公告)日：2013-06-13

    申请号：PCT/US2012043066

    申请日：2012-06-19

    Applicant: UOP LLC ,  KOCAL JOSEPH A ,  BRANDVOLD TIMOTHY A

    Inventor： KOCAL JOSEPH A ,  BRANDVOLD TIMOTHY A

    IPC: C11B1/04 ,  C11B1/10 ,  C11B1/12

    CPC classification number: C10K1/00 ,  B01J23/007 ,  B01J23/02 ,  B01J29/082 ,  C10B49/22 ,  C10B53/02 ,  C10B57/06 ,  C10B57/18 ,  C10C5/00 ,  C10G2300/1014 ,  C10K1/34 ,  C10K3/026 ,  Y02E50/14 ,  Y02P30/20

    Abstract: Processes for producing reduced acid lignocellulosic-derived pyrolysis oil are provided. In a process, lignocellulosic material is fed to a heating zone. A basic solid catalyst is delivered to the heating zone. The lignocellulosic material is pyrolyzed in the presence of the basic solid catalyst in the heating zone to create pyrolysis gases. The oxygen in the pyrolysis gases is catalytically converted to separable species in the heating zone. The pyrolysis gases are removed from the heating zone and are liquefied to form the reduced acid lignocellulosic-derived pyrolysis oil.

    Abstract translation: 提供了生产还原酸木质纤维素衍生的热解油的方法。 在一个过程中，木质纤维素材料被送入加热区。 碱性固体催化剂被输送到加热区。 木质纤维素材料在碱性固体催化剂存在下在加热区中被热解以产生热解气体。 热解气体中的氧在加热区中催化转化成可分离的物质。 将热解气体从加热区中除去并液化以形成还原的酸木质纤维素衍生的热解油。

    A PROCESS FOR THE PRODUCTION OF METHANOL FROM METHANE USING A METAL TRIFLUOROACETATE CATALYST
    6.
    发明申请
    A PROCESS FOR THE PRODUCTION OF METHANOL FROM METHANE USING A METAL TRIFLUOROACETATE CATALYST 审中-公开
    使用金属三氟乙酸盐催化剂从甲烷生产甲醇的方法

    公开(公告)号：WO2007073533A3

    公开(公告)日：2007-11-08

    申请号：PCT/US2006061832

    申请日：2006-12-11

    Applicant: UOP LLC ,  CHEN WENSHENG ,  BRANDVOLD TIMOTHY A ,  BRICKER MAUREEN L ,  KOCAL JOSEPH A ,  WALENGA JOEL T

    Inventor： CHEN WENSHENG ,  BRANDVOLD TIMOTHY A ,  BRICKER MAUREEN L ,  KOCAL JOSEPH A ,  WALENGA JOEL T

    IPC: C07C29/03

    CPC classification number: C07C29/095 ,  C07C67/035 ,  C07C69/63 ,  C07C31/04

    Abstract: A process for converting methane to methanol using a homogeneous catalyst has been developed. The catalyst is a metal compound having an empirical formula of M x X m where M is a metal such as Pd, Cu, Co, and Mn, X is an anion such as acetate, trifluoroacetate, sulfate, propionate, "m" is the oxidation state of M, and "x" is the anion valence of X. Generally the process involves contacting a gas stream containing methane with the homogeneous catalyst and an oxidant such as hydrogen peroxide at oxidation conditions to produce methyl trifluoroacetate. Finally, the methyl trifluoroacetate is hydrolyzed to give a methanol product stream.

    Abstract translation: 已经开发了使用均相催化剂将甲烷转化为甲醇的方法。 催化剂是具有经验式M x SUB x m M的金属化合物，其中M是金属如Pd，Cu，Co和Mn，X是阴离子等 作为乙酸盐，三氟乙酸盐，硫酸盐，丙酸盐，“m”是M的氧化态，“x”是X的阴离子化合价。通常该方法包括使含有甲烷的气流与均相催化剂和氧化剂如氢气 过氧化物在氧化条件下反应生成三氟乙酸甲酯。 最后，将三氟乙酸甲酯水解，得到甲醇产物流。

    METHODS AND CATALYSTS FOR DEOXYGENATING BIOMASS-DERIVED PYROLYSIS OIL
    7.
    发明申请
    METHODS AND CATALYSTS FOR DEOXYGENATING BIOMASS-DERIVED PYROLYSIS OIL 审中-公开
    消除生物质衍生的热解油的方法和催化剂

    公开(公告)号：WO2012166402A2

    公开(公告)日：2012-12-06

    申请号：PCT/US2012038747

    申请日：2012-05-21

    Applicant: UOP LLC ,  TRAYNOR THOMAS ,  BRANDVOLD TIMOTHY A ,  ABRAHAMIAN JENNIFER F

    Inventor： TRAYNOR THOMAS ,  BRANDVOLD TIMOTHY A ,  ABRAHAMIAN JENNIFER F

    IPC: C10G45/08 ,  B01J23/28 ,  B01J23/74 ,  C10G3/00 ,  C10G65/00

    CPC classification number: B01J23/883 ,  C10G3/46 ,  C10G65/04 ,  C10G2300/1011 ,  Y02P30/20

    Abstract: Embodiments of methods and catalysts for deoxygenating a biomass-derived pyrolysis oil are provided. The method comprises the step of contacting the biomass-derived pyrolysis oil with a first deoxygenating catalyst in the presence of hydrogen at first predetermined hydroprocessing conditions to form a first low-oxygen biomass-derived pyrolysis oil effluent. The first deoxygenating catalyst comprises a neutral catalyst support, nickel, cobalt, and molybdenum. The first deoxygenating catalyst comprises nickel in an amount calculated as an oxide of from 0.1 to 1.5 wt. %.

    Abstract translation: 提供了用于脱氧生物质衍生的热解油的方法和催化剂的实施方案。 该方法包括在第一预定加氢处理条件下，在氢存在下使生物质衍生的热解油与第一脱氧催化剂接触的步骤，以形成第一低氧生物质衍生的热解油流出物。 第一脱氧催化剂包括中性催化剂载体，镍，钴和钼。 第一脱氧催化剂包含以0.1至1.5重量％的氧化物计算的量的镍。 ％。

    PROCESSES FOR PRODUCING LOW ACID BIOMASS-DERIVED PYROLYSIS OILS
    8.
    发明申请
    PROCESSES FOR PRODUCING LOW ACID BIOMASS-DERIVED PYROLYSIS OILS 审中-公开
    生产低酸生物质衍生的热解油的过程

    公开(公告)号：WO2012018518A3

    公开(公告)日：2012-07-05

    申请号：PCT/US2011044469

    申请日：2011-07-19

    Applicant: UOP LLC ,  TRAYNOR THOMAS ,  BRANDVOLD TIMOTHY A

    Inventor： TRAYNOR THOMAS ,  BRANDVOLD TIMOTHY A

    IPC: C10G29/22 ,  B01J29/04 ,  B01J29/076 ,  C10G3/00 ,  C10L1/02

    CPC classification number: C10L1/02 ,  Y02P30/20

    Abstract: Processes for producing a low acid biomass-derived pyrolysis oil are provided that include pre-treating a biomass-derived pyrolysis oil to form a treated acid-containing biomass-derived pyrolysis oil. The processes also include esterifying the treated acid-containing biomass-derived pyrolysis oil in the presence of supercritical alcohol and a catalyst composition to form the low-acid biomass-derived pyrolysis oil, the catalyst composition comprising a material selected from the group consisting of an unsupported solid acid catalyst, an unsupported solid base catalyst, and a catalytic metal dispersed on a metal oxide support.

    Abstract translation: 提供了用于生产低酸生物质衍生的热解油的方法，其包括预处理生物质衍生的热解油以形成处理过的含酸生物质衍生的热解油。 所述方法还包括在超临界醇和催化剂组合物存在下酯化经处理的含酸生物质衍生的热解油以形成低酸生物质衍生的热解油，所述催化剂组合物包含选自如下的材料： 未负载的固体酸催化剂，未负载的固体碱催化剂和分散在金属氧化物载体上的催化金属。

    LOW WATER BIOMASS-DERIVED PYROLYSIS OIL AND PROCESSES FOR PREPARING THE SAME
    9.
    发明申请
    LOW WATER BIOMASS-DERIVED PYROLYSIS OIL AND PROCESSES FOR PREPARING THE SAME 审中-公开
    低水生物质衍生的热解油及其制备方法

    公开(公告)号：WO2011087675A3

    公开(公告)日：2011-11-03

    申请号：PCT/US2010060397

    申请日：2010-12-15

    Applicant: UOP LLC ,  BRANDVOLD TIMOTHY A ,  FREY STANLEY J

    Inventor： BRANDVOLD TIMOTHY A ,  FREY STANLEY J

    IPC: C10G7/00 ,  C10G29/00

    CPC classification number: C10L1/02 ,  B01D3/36

    Abstract: Low water-containing biomass-derived pyrolysis oils and processes for preparing them are provided. Water-containing biomass-derived pyrolysis oil is distilled in the presence of an azeotrope-forming liquid to form an azeotrope. The azeotrope is removed at or above the boiling point of the azeotrope and low water biomass-derived pyrolysis oil is obtained.

    Abstract translation: 提供了低含水生物质衍生的热解油及其制备方法。 在形成共沸物质的液体存在下蒸馏含水生物质的热解油，形成共沸物。 在共沸物的沸点以上沸腾除去共沸物，得到低水生物质衍生的热解油。

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