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    Salts Comprising Aryl-Alkyl-Substituted Imidazolium and Triazolium Cations and the Use Thereof
    23.
    发明申请
    Salts Comprising Aryl-Alkyl-Substituted Imidazolium and Triazolium Cations and the Use Thereof 有权

    公开(公告)号：US20110105761A1

    公开(公告)日：2011-05-05

    申请号：US12864750

    申请日：2009-01-30

    申请人： Thomas Strassner ,  Sebastian Ahrens

    发明人： Thomas Strassner ,  Sebastian Ahrens

    IPC分类号： C07D233/56 ,  C07D249/08 ,  C07D233/54 ,  C07F5/02 ,  C07D233/61

    CPC分类号： C07D233/58 ,  B01D15/38 ,  B01J31/0284 ,  B01J31/0298 ,  C07D233/60 ,  C07D249/08

    摘要： The present invention relates to salts comprising novel aryl-alkyl-substituted imidazolium and triazolium cations and arbitrary anions. The invention further relates to methods for the chemical conversion and separation of substances, comprising the salts according to the invention as solvents, solvent additives, or extraction means, and to the use of the salts according to the invention, for example as solvents or solvent additives in chemical reactions, as extracting agents for the separation of substances, or for storing hydrogen. According to the invention, the object is achieved by salts of the general formula (I), where X— is an anion, Y1 and Y2 are CH, or Y1 is CH and Y2 is N, or Y1 is N and Y2 is CH, n is a number from 1 up to an including 18, Q is selected from —CH3, —OH, —ORx, —S03H, —S03Rx, —COOH, —COORx, —CORx, NH2, —NHRx, —N(Rx)2, and —CH(Rx)2, Z is H or Rx, R1, R2, R3, R4 and R5 independently from each other are —H, -halogen, —N02, —NH2, —NHRx, —N(Rx)2, —Rx, —COORx or —ORx, where Rx is an optionally substituted and/or branched C1 to C18-alkyl group, excluding compounds of the general formula (I), where Y1 and Y2 are CH and R1, R2, R3, R4 and R5 are H, excluding compounds of the general formula (I), where Y1 and Y2 are CH, R1=R3=R5=CH3 is true, n=1, 2, 6 and Q=CH3 is true, excluding compounds of the general formula (I), where Y1 is CH and Y2 is N, R1, R2, R3, R4 and R5 are H, n=1 is true, and Q=CH3 is true, and excluding compounds of the general formula (I), where Y1 and Y2 are CH, R1, R2, R4, R5=H is true, R3=ORx is true, and Rx is a hydrocarbon having 3 or 12 carbon atoms.

    Salts comprising aryl-alkyl-substituted imidazolium and triazolium cations and the use thereof
    26.
    发明授权
    Salts comprising aryl-alkyl-substituted imidazolium and triazolium cations and the use thereof 有权

    公开(公告)号：US09260397B2

    公开(公告)日：2016-02-16

    申请号：US12864750

    申请日：2009-01-30

    申请人： Thomas Strassner ,  Sebastian Ahrens

    发明人： Thomas Strassner ,  Sebastian Ahrens

    IPC分类号： C07D233/58 ,  B01J31/02 ,  C07D233/60 ,  C07D249/08 ,  B01D15/38

    CPC分类号： C07D233/58 ,  B01D15/38 ,  B01J31/0284 ,  B01J31/0298 ,  C07D233/60 ,  C07D249/08

    摘要： The present invention relates to salts comprising novel aryl-alkyl-substituted imidazolium and triazolium cations and arbitrary anions. The invention further relates to methods for the chemical conversion and separation of substances, comprising the salts according to the invention as solvents, solvent additives, or extraction means, and to the use of the salts according to the invention, for example as solvents or solvent additives in chemical reactions, as extracting agents for the separation of substances, or for storing hydrogen. According to the invention, the object is achieved by salts of the general formula (I), where X— is an anion, Y1 and Y2 are CH, or Y1 is CH and Y2 is N, or Y1 is N and Y2 is CH, n is a number from 1 up to an including 18, Q is selected from —CH3, —OH, —ORx, —S03H, —S03Rx, —COOH, —COORx, —CORx, NH2, —NHRx, —N(Rx)2, and —CH(Rx)2, Z is H or Rx, R1, R2, R3, R4 and R5 independently from each other are —H, -halogen, —N02, —NH2, —NHRx, —N(Rx)2, —Rx, —COORx or —ORx, where Rx is an optionally substituted and/or branched C1 to C18-alkyl group, excluding compounds of the general formula (I), where Y1 and Y2 are CH and R1, R2, R3, R4 and R5 are H, excluding compounds of the general formula (I), where Y1 and Y2 are CH, R1=R3=R5=CH3 is true, n=1, 2, 6 and Q=CH3 is true, excluding compounds of the general formula (I), where Y1 is CH and Y2 is N, R1, R2, R3, R4 and R5 are H, n=1 is true, and Q=CH3 is true, and excluding compounds of the general formula (I), where Y1 and Y2 are CH, R1, R2, R4, R5=H is true, R3=ORx is true, and Rx is a hydrocarbon having 3 or 12 carbon atoms.

    PROCESS FOR PREPARING BENZENE FROM METHANE
    29.
    发明申请
    PROCESS FOR PREPARING BENZENE FROM METHANE 有权
    从甲烷制备苄苯的方法

    公开(公告)号：US20120165585A1

    公开(公告)日：2012-06-28

    申请号：US13393837

    申请日：2010-08-23

    申请人： Christian Schneider ,  Martin Karches ,  Joana Coelho Tsou ,  Sebastian Ahrens ,  Dieter Stuetzer

    发明人： Christian Schneider ,  Martin Karches ,  Joana Coelho Tsou ,  Sebastian Ahrens ,  Dieter Stuetzer

    IPC分类号： C07C2/76

    CPC分类号： C07C2/76 ,  Y02P20/584 ,  C07C15/02

    摘要： The present invention relates to a process for nonoxidatively dehydroaromatizing a reactant stream comprising C1-C4-aliphatics, comprising the steps of I. feeding reactant stream E into a reaction zone 1, converting reactant stream E under nonoxidative conditions in the presence of a particulate catalyst to a product stream P comprising aromatic hydrocarbons and discharging product stream P from reaction zone 1, II. transferring the catalyst with reduced activity as a result of deposited coke into a reaction zone 2, III. at least partly regenerating the catalyst with supply of a hydrogen-comprising gas stream H in a reaction zone 2, at least some of the coke deposited being converted to methane to form a methane-comprising gas stream M which is fed at least partly to reaction zone 1, IV. discharging the catalyst from reaction zone 2 and V. recycling at least a portion of the discharged catalyst into reaction zone 1, reaction zone 1 and reaction zone 2 being arranged spatially adjacent to one another in the same reactor.

    摘要翻译： 本发明涉及一种使含有C 1 -C 4脂族化合物的反应物流非氧化脱氢芳化的方法，其包括以下步骤：将反应物流E加入到反应区1中，在非氧化条件下在颗粒催化剂存在下转化反应物流E 涉及包含芳烃并从反应区1排出产物流P的产物流P。 由于沉积的焦炭导致反应区2，III的转移，催化剂活性降低。 在反应区2中供应含氢气流H至少部分地再生催化剂，沉积的焦炭中的至少一些转化成甲烷以形成含甲烷的气流M，其至少部分地进料至反应 区1，IV。 将催化剂从反应区2排出，并将至少一部分排出的催化剂再循环到反应区1中，反应区1和反应区2在相同的反应器中彼此空间上相邻布置。