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51.发明授权
公开(公告)号：US4720600A
公开(公告)日：1988-01-19
申请号：US699882
申请日：1985-02-08
摘要： An oligomerization process is provided for upgrading lower olefins to distillate hydrocarbons, especially useful as high quality jet or diesel fuels. The olefinic feedstock is reacted over a shape selective acid zeolite, such as ZSM-5, to oligomerize feedstock olefins and further convert recycled hydrocarbons. Reactor effluent is fractionated to recover a light-middle distillate range product stream and to obtain gasoline and heavy hydrocarbon streams for recycle.
摘要翻译： 提供了一种低聚方法，用于将低级烯烃升级为馏出物烃，特别适用于高质量的喷气或柴油燃料。 烯烃原料在诸如ZSM-5的形状选择性酸性沸石上反应以使原料烯烃低聚并进一步转化回收的烃。 将反应器流出物分馏以回收轻 - 中馏分范围的产物流并获得用于再循环的汽油和重烃流。
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公开(公告)号：US4684756A
公开(公告)日：1987-08-04
申请号：US858620
申请日：1986-05-01
申请人： W. Rodman Derr, Jr. , William E. Garwood , James C. Kuo , Tiberiu M. Leib , Donald M. Nace , Samuel A. Tabak
发明人： W. Rodman Derr, Jr. , William E. Garwood , James C. Kuo , Tiberiu M. Leib , Donald M. Nace , Samuel A. Tabak
CPC分类号： C10L1/06 , C07C1/0485 , C10G2/32 , C10L1/04 , C10G2300/1022
摘要： The waxy liquid phase of an oil suspension of Fischer-Tropsch catalyst containing dissolved wax is separated out and the wax is converted by hydrocracking, dewaxing or by catalytic cracking with a low activity catalyst to provide a highly olefinic product which may be further converted to premium quality gasoline and/or distillate fuel.
摘要翻译： 分离含有溶解蜡的费 - 托催化剂的油悬浮液的蜡状液相，通过加氢裂化，脱蜡或用低活性催化剂进行催化裂化来转化蜡，以提供可进一步转化为优质的高烯烃产物 优质汽油和/或馏出燃料。
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公开(公告)号：US4626415A
公开(公告)日：1986-12-02
申请号：US716317
申请日：1985-03-27
申请人： Samuel A. Tabak
发明人： Samuel A. Tabak
CPC分类号： C07C2/12 , C07C1/0485 , C07C11/02 , C07C2529/40
摘要： Apparatus is disclosed for oligomerizing olefinic Fischer-Tropsch liquids to produce heavier hydrocarbons by converting olefinic feedstock containing oxygenated hydrocarbons over an acidic zeolite catalyst. The improvement comprises an extraction unit for removing oxygenates from the feedstock; means for converting the extracted feedstock in a primary stage distillate mode catalytic reactor system under low severity conditions at high pressure and moderate pressure; means for recovering the oxygenates and light hydrocarbons from the primary stage and a secondary stage reactor system for conversion of oxygenates under high severity conditions at substantially higher temperature than the primary stage, thereby converting oxygenates and light hydrocarbons to heavier hydrocarbons.
摘要翻译： 公开了通过在酸性沸石催化剂上转化含有氧化烃的烯烃原料来使烯属费 - 托液体低聚以产生较重烃的装置。 改进包括用于从原料中除去含氧化合物的提取单元; 用于在低压和中等压力的低苛刻度条件下将提取的原料转化为初级馏分模式催化反应器系统的装置; 用于从初级阶段回收含氧化合物和轻质烃的装置和用于在高苛刻度条件下以比初级阶段高得多的温度转化含氧化合物的二级反应器系统，从而将含氧化合物和轻质烃转化成较重的烃。
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公开(公告)号：US4482772A
公开(公告)日：1984-11-13
申请号：US548377
申请日：1983-11-03
申请人： Samuel A. Tabak
发明人： Samuel A. Tabak
CPC分类号： C10G69/02 , C07C1/20 , C10G3/49 , C10G3/54 , C10G50/00 , C07C2529/40 , C10G2300/301 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2300/802 , C10G2400/02 , C10G2400/04 , C10G2400/20 , C10G2400/30 , Y02P20/125 , Y02P20/52 , Y02P30/20 , Y02P30/42
摘要： An integrated process is provided for converting methanol or the like to heavy hydrocarbon products, especially distillate range hydrocarbons. In a first stage catalytic process oxygenate feedstock is converted to lower olefins. Byproduct aromatics are passed through a second stage oligomerization reactor with olefins. Distillate range hydrocarbons are recovered and hydrotreated to provide an improved fuel product.
摘要翻译： 提供了将甲醇等转化为重质烃产物，特别是馏出物烃类的综合方法。 在第一阶段中，催化过程将含氧化合物原料转化为低级烯烃。 副产物芳烃通过具有烯烃的第二级低聚反应器。 蒸馏馏分烃被回收和加氢处理以提供改进的燃料产物。
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公开(公告)号：US4448672A
公开(公告)日：1984-05-15
申请号：US385159
申请日：1982-06-04
CPC分类号： C10G21/003 , C10G21/12
摘要： A process for the purification of liquefied coal is disclosed, employing a polarity gradient for fractionation. Maltenic and asphaltenic fractions are isolated. Integration of the fractionation process with additional processes such as distillation, partial oxidation, and catalytic hydrotreating is also disclosed.
摘要翻译： 公开了一种用于液化煤净化的方法，采用极性梯度进行分馏。 分离出Maltenic和沥青馏分。 还公开了分馏方法与另外的方法如蒸馏，部分氧化和催化加氢处理的整合。
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公开(公告)号：US4341622A
公开(公告)日：1982-07-27
申请号：US212770
申请日：1980-12-04
申请人： Samuel A. Tabak , Roger A. Morrison
发明人： Samuel A. Tabak , Roger A. Morrison
CPC分类号： C10G45/64 , C10G2400/30
摘要： Benzene, toluene and xylenes are prepared from heavy reformate in substantially the proportion in said reformate of single ring aromatic compounds bearing none, one or two methyl groups by contacting said heavy reformate at 800.degree.-1000.degree. F. with a zeolite of low acid activity.
摘要翻译： 苯，甲苯和二甲苯由重质化合物制成，重量比大约为单环芳族化合物重整油中的一个或两个甲基基团，通过使800-1000°F的重质化合物与低酸活性的沸石接触， 。
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公开(公告)号：US4260841A
公开(公告)日：1981-04-07
申请号：US72819
申请日：1979-09-04
申请人： Robert E. Holland , Samuel A. Tabak
发明人： Robert E. Holland , Samuel A. Tabak
CPC分类号： C07C1/20 , B01J29/40 , C10G3/44 , C10G3/49 , C07C2521/04 , C07C2529/40 , C10G2300/1022 , C10G2300/4081 , C10G2400/02 , C10G2400/28 , C10G2400/30 , Y02P30/20
摘要： Water-soluble oxygenates of Fischer-Tropsch synthesis separated from water and acids are sequentially upgraded by a dehydration catalyst and a special zeolite catalyst to produce gasoline, LPG and light fuel oil.
摘要翻译： 从水和酸分离的费 - 托合成的水溶性含氧化合物通过脱水催化剂和特殊的沸石催化剂依次升级，生产汽油，LPG和轻燃料油。
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公开(公告)号：US4254295A
公开(公告)日：1981-03-03
申请号：US100591
申请日：1979-12-05
申请人： Samuel A. Tabak
发明人： Samuel A. Tabak
CPC分类号： C07C2/12 , C07C2529/70
摘要： A process for the selective oligomerization of linear and branched chain C.sub.2 to C.sub.12 olefins is provided. The process comprises contacting of the said olefin in the liquid phase with ZSM-12 at temperatures of 80.degree. F. to 400.degree. F.
摘要翻译： 提供了一种用于选择性低聚直链和支链C2至C12烯烃的方法。 该方法包括在80°F至400°F的温度下将所述液相烯烃与ZSM-12接触。
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公开(公告)号：US4218573A
公开(公告)日：1980-08-19
申请号：US44824
申请日：1979-06-01
申请人： Samuel A. Tabak , Roger A. Morrison
发明人： Samuel A. Tabak , Roger A. Morrison
CPC分类号： C07C15/08 , B01J29/44 , C07C4/18 , C07C5/2737 , B01J2229/26 , B01J2229/42 , C07C2529/42 , C10G2400/30 , Y02P20/52
摘要： Isomerization of xylenes in admixture with ethyl benzene by contact with a zeolite catalyst such as ZSM-5 is improved by use of zeolite having a substantial alkali metal content at a temperature above about 800.degree. F. At these conditions, conversion of ethylbenzene follows a different reaction path which permits high conversion of ethylbenzene to benzene without loss of xylenes by disproportionation.
摘要翻译： 通过与沸石催化剂如ZSM-5接触，与乙苯混合来二甲苯的异构化通过使用在高于约800°F的温度下具有大量碱金属含量的沸石来改进。在这些条件下，乙苯的转化遵循不同的 反应途径，允许乙苯高效转化成苯，而不损失二甲苯的歧化。
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公开(公告)号：US4188282A
公开(公告)日：1980-02-12
申请号：US914645
申请日：1978-06-12
申请人： Samuel A. Tabak , Roger A. Morrison
发明人： Samuel A. Tabak , Roger A. Morrison
CPC分类号： C07C15/08 , B01J29/44 , C07C4/18 , C07C5/2737 , B01J2229/26 , B01J2229/42 , C07C2529/42 , C10G2400/30 , Y02P20/52
摘要： Benzene, toluene and xylene are prepared from mixtures of single ring alkyl aromatic compounds of eight or more carbon atoms concurrently with isomerization of xylenes by mixing xylenes from which at least one isomer has been separated with a mixture of alkyl benzenes of eight and more carbon atoms, e.g. heavy reformate, and contacting that mixture at 800.degree. to 1000.degree. F. with a zeolite catalyst of reduced activity such as zeolite ZSM-5 having a silica to alumina ratio of at least 200.
摘要翻译： 苯，甲苯和二甲苯由八个或多个碳原子的单环烷基芳族化合物的混合物与二甲苯异构化的混合物制备，通过混合二甲苯，其中至少一种异构体已经与八个或多个碳原子的烷基苯的混合物分离 ，例如 重结晶，并将该混合物在800至1000°F下与活性降低的沸石催化剂接触，例如二氧化硅与氧化铝之比至少为200的沸石ZSM-5。
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