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    ELECTROSPINNING TO FABRICATE BATTERY ELECTRODES
    2.
    发明申请
    ELECTROSPINNING TO FABRICATE BATTERY ELECTRODES 审中-公开
    电解电池电极

    公开(公告)号：US20100330419A1

    公开(公告)日：2010-12-30

    申请号：US12787132

    申请日：2010-05-25

    申请人： Yi Cui ,  Song Han ,  Ghyrn E. Loveness ,  Mark C. Platshon

    发明人： Yi Cui ,  Song Han ,  Ghyrn E. Loveness ,  Mark C. Platshon

    IPC分类号： H01M4/02 ,  B05D5/12 ,  H01M4/82

    CPC分类号： H01M4/625 ,  D01D5/0084 ,  D01F1/10 ,  H01M4/04 ,  H01M4/131 ,  H01M4/587 ,  H01M10/052 ,  Y10T29/49115

    摘要： Provided are electrode assemblies that contain electrochemically active materials for use in batteries, such as lithium ion batteries. Provided also are methods for fabricating these assemblies. In certain embodiments, fabrication involves one or more electrospinning operations such as, for example, electrospinning to deposit a layer of fibers on a conductive substrate. These fibers may include one or more electrochemically active materials. In the same or other embodiments, these or similar fibers can serve as templates for depositing one or more electrochemically active materials. Some examples of active materials include silicon, tin, and/or germanium. Also provided are electrode fibers that include cores containing a first active material and shells or optionally second shells (surrounding inner shells) containing a second active material. The second active material is electrochemically opposite to the first active material. One or more shells can function as a separator and/or as an electrolyte.

    摘要翻译： 提供了包含用于电池中的电化学活性材料的电极组件，例如锂离子电池。 还提供了用于制造这些组件的方法。 在某些实施例中，制造涉及一种或多种静电纺丝操作，例如静电纺丝以在导电基底上沉积纤维层。 这些纤维可以包括一种或多种电化学活性材料。 在相同或其它实施方案中，这些或类似的纤维可以用作沉积一种或多种电化学活性材料的模板。 活性材料的一些实例包括硅，锡和/或锗。 还提供了包括含有第一活性材料的芯和包含第二活性材料的壳或任选的第二壳（围绕内壳）的芯的电极纤维。 第二活性材料在电化学上与第一活性材料相反。 一个或多个壳可用作分离器和/或电解质。

    Preloading lithium ion cell components with lithium
    3.
    发明授权
    Preloading lithium ion cell components with lithium 有权
    用锂预加载锂离子电池组件

    公开(公告)号：US08846251B2

    公开(公告)日：2014-09-30

    申请号：US12944593

    申请日：2010-11-11

    申请人： Yi Cui ,  Song Han ,  Mark C. Platshon

    发明人： Yi Cui ,  Song Han ,  Mark C. Platshon

    IPC分类号： H01M4/13 ,  H01M4/58

    CPC分类号： H01M4/366 ,  H01M4/0421 ,  H01M4/0438 ,  H01M4/134 ,  H01M4/1395 ,  H01M4/38 ,  H01M4/386 ,  H01M4/387 ,  H01M4/70 ,  H01M4/75 ,  H01M10/0525 ,  H01M10/0585 ,  H01M10/0587 ,  H01M2004/021 ,  H01M2004/025 ,  H01M2220/30 ,  Y10T29/49115

    摘要： Provided are novel negative electrodes for use in lithium ion cells. The negative electrodes include one or more high capacity active materials, such as silicon, tin, and germanium, and a lithium containing material prior to the first cycle of the cell. In other words, the cells are fabricated with some, but not all, lithium present on the negative electrode. This additional lithium may be used to mitigate lithium losses, for example, due to Solid Electrolyte Interphase (SEI) layer formation, to maintain the negative electrode in a partially charged state at the end of the cell discharge cycle, and other reasons. In certain embodiments, a negative electrode includes between about 5% and 25% of lithium based on a theoretical capacity of the negative active material. In the same or other embodiments, a total amount of lithium available in the cell exceeds the theoretical capacity of the negative electrode active material.

    摘要翻译： 提供用于锂离子电池的新型负极。 负极包括一种或多种高容量活性物质，例如硅，锡和锗，以及在电池的第一循环之前的含锂材料。 换句话说，电池制造有一些而不是全部锂存在于负电极上。 这种额外的锂可以用于减轻锂损失，例如，由于固体电解质相（SEI）层形成，以在电池放电循环结束时将负极维持在部分充电状态，以及其它原因。 在某些实施方案中，基于负极活性材料的理论容量，负极包括约5％至25％的锂。 在相同或其它实施方案中，电池中可用的锂的总量超过负极活性材料的理论容量。

    Open structures in substrates for electrodes
    4.
    发明授权
    Open structures in substrates for electrodes 有权
    用于电极的基板中的开放结构

    公开(公告)号：US08637185B2

    公开(公告)日：2014-01-28

    申请号：US12944596

    申请日：2010-11-11

    申请人： Eugene M. Berdichevsky ,  Song Han ,  Yi Cui ,  Rainer J. Fasching ,  Ghyrn E. Loveness ,  William S. DelHagen ,  Mark C. Platshon

    发明人： Eugene M. Berdichevsky ,  Song Han ,  Yi Cui ,  Rainer J. Fasching ,  Ghyrn E. Loveness ,  William S. DelHagen ,  Mark C. Platshon

    IPC分类号： H01M4/38

    CPC分类号： H01M4/134 ,  H01M4/0428 ,  H01M4/1395 ,  H01M4/38 ,  H01M4/661 ,  H01M4/669 ,  H01M4/74 ,  H01M4/742 ,  H01M4/808

    摘要： Provided are conductive substrates having open structures and fractional void volumes of at least about 25% or, more specifically, or at least about 50% for use in lithium ion batteries. Nanostructured active materials are deposited over such substrates to form battery electrodes. The fractional void volume may help to accommodate swelling of some active materials during cycling. In certain embodiments, overall outer dimensions of the electrode remain substantially the same during cycling, while internal open spaces of the conductive substrate provide space for any volumetric changes in the nanostructured active materials. In specific embodiments, a nanoscale layer of silicon is deposited over a metallic mesh to form a negative electrode. In another embodiment, a conductive substrate is a perforated sheet with multiple openings, such that a nanostructured active material is deposited into the openings but not on the external surfaces of the sheet.

    摘要翻译： 提供了具有至少约25％，或更具体地至少约50％的具有开放结构和分数空隙体积的导电基底，用于锂离子电池。 纳米结构的活性材料沉积在这样的衬底上以形成电池电极。 在循环过程中，分数空隙体积有助于适应一些活性物质的溶胀。 在某些实施例中，电极的整个外部尺寸在循环过程中保持基本相同，而导电衬底的内部开放空间为纳米结构活性材料中的任何体积变化提供了空间。 在具体实施方案中，将纳米级的硅层沉积在金属网上以形成负电极。 在另一个实施例中，导电衬底是具有多个开口的穿孔片，使得纳米结构的活性材料沉积到开口中而不是在片的外表面上。

    OPEN STRUCTURES IN SUBSTRATES FOR ELECTRODES
    5.
    发明申请
    OPEN STRUCTURES IN SUBSTRATES FOR ELECTRODES 有权
    电极基板的开放结构

    公开(公告)号：US20110111296A1

    公开(公告)日：2011-05-12

    申请号：US12944596

    申请日：2010-11-11

    申请人： Eugene M. Berdichevsky ,  Song Han ,  Yi Cui ,  Rainer J. Fasching ,  Ghyrn E. Loveness ,  William S. DelHagen ,  Mark C. Platshon

    发明人： Eugene M. Berdichevsky ,  Song Han ,  Yi Cui ,  Rainer J. Fasching ,  Ghyrn E. Loveness ,  William S. DelHagen ,  Mark C. Platshon

    IPC分类号： H01M4/38 ,  H01M4/70 ,  H01M4/66 ,  B05D5/12

    CPC分类号： H01M4/134 ,  H01M4/0428 ,  H01M4/1395 ,  H01M4/38 ,  H01M4/661 ,  H01M4/669 ,  H01M4/74 ,  H01M4/742 ,  H01M4/808

    摘要： Provided are conductive substrates having open structures and fractional void volumes of at least about 25% or, more specifically, or at least about 50% for use in lithium ion batteries. Nanostructured active materials are deposited over such substrates to form battery electrodes. The fractional void volume may help to accommodate swelling of some active materials during cycling. In certain embodiments, overall outer dimensions of the electrode remain substantially the same during cycling, while internal open spaces of the conductive substrate provide space for any volumetric changes in the nanostructured active materials. In specific embodiments, a nanoscale layer of silicon is deposited over a metallic mesh to form a negative electrode. In another embodiment, a conductive substrate is a perforated sheet with multiple openings, such that a nanostructured active material is deposited into the openings but not on the external surfaces of the sheet.

    摘要翻译： 提供了具有至少约25％，或更具体地至少约50％的具有开放结构和分数空隙体积的导电基底，用于锂离子电池。 纳米结构的活性材料沉积在这样的衬底上以形成电池电极。 在循环过程中，分数空隙体积有助于适应一些活性物质的溶胀。 在某些实施例中，电极的整个外部尺寸在循环过程中保持基本相同，而导电衬底的内部开放空间为纳米结构化活性材料中的任何体积变化提供了空间。 在具体实施方案中，将纳米级的硅层沉积在金属网上以形成负电极。 在另一个实施例中，导电衬底是具有多个开口的穿孔片，使得纳米结构的活性材料沉积到开口中而不是在片的外表面上。

    PRELOADING LITHIUM ION CELL COMPONENTS WITH LITHIUM
    9.
    发明申请
    PRELOADING LITHIUM ION CELL COMPONENTS WITH LITHIUM 有权
    推荐锂离子电池组件

    公开(公告)号：US20110111304A1

    公开(公告)日：2011-05-12

    申请号：US12944593

    申请日：2010-11-11

    申请人： Yi Cui ,  Song Han ,  Mark C. Platshon

    发明人： Yi Cui ,  Song Han ,  Mark C. Platshon

    IPC分类号： H01M4/38 ,  H01M4/583 ,  H01M4/26

    CPC分类号： H01M4/366 ,  H01M4/0421 ,  H01M4/0438 ,  H01M4/134 ,  H01M4/1395 ,  H01M4/38 ,  H01M4/386 ,  H01M4/387 ,  H01M4/70 ,  H01M4/75 ,  H01M10/0525 ,  H01M10/0585 ,  H01M10/0587 ,  H01M2004/021 ,  H01M2004/025 ,  H01M2220/30 ,  Y10T29/49115

    摘要： Provided are novel negative electrodes for use in lithium ion cells. The negative electrodes include one or more high capacity active materials, such as silicon, tin, and germanium, and a lithium containing material prior to the first cycle of the cell. In other words, the cells are fabricated with some, but not all, lithium present on the negative electrode. This additional lithium may be used to mitigate lithium losses, for example, due to Solid Electrolyte Interphase (SEI) layer formation, to maintain the negative electrode in a partially charged state at the end of the cell discharge cycle, and other reasons. In certain embodiments, a negative electrode includes between about 5% and 25% of lithium based on a theoretical capacity of the negative active material. In the same or other embodiments, a total amount of lithium available in the cell exceeds the theoretical capacity of the negative electrode active material.

    摘要翻译： 提供用于锂离子电池的新型负极。 负极包括一种或多种高容量活性物质，例如硅，锡和锗，以及在电池的第一循环之前的含锂材料。 换句话说，电池制造有一些而不是全部锂存在于负电极上。 这种额外的锂可以用于减轻锂损失，例如，由于固体电解质相（SEI）层形成，以在电池放电循环结束时将负极维持在部分充电状态，以及其它原因。 在某些实施方案中，基于负极活性材料的理论容量，负极包括约5％至25％的锂。 在相同或其它实施方案中，电池中可用的锂的总量超过负极活性材料的理论容量。

    INTERMEDIATE LAYERS FOR ELECTRODE FABRICATION
    10.
    发明申请
    INTERMEDIATE LAYERS FOR ELECTRODE FABRICATION 审中-公开
    电极制造的中间层

    公开(公告)号：US20110111300A1

    公开(公告)日：2011-05-12

    申请号：US12944576

    申请日：2010-11-11

    申请人： William S. DelHagen ,  Rainer J. Fasching ,  Ghyrn E. Loveness ,  Song Han ,  Eugene M. Berdichevsky ,  Constantin I. Stefan ,  Yi Cui ,  Mark C. Platshon

    发明人： William S. DelHagen ,  Rainer J. Fasching ,  Ghyrn E. Loveness ,  Song Han ,  Eugene M. Berdichevsky ,  Constantin I. Stefan ,  Yi Cui ,  Mark C. Platshon

    IPC分类号： H01M4/134 ,  H01M4/13 ,  H01M4/139 ,  B05D5/12

    CPC分类号： H01M10/052 ,  H01M4/13 ,  H01M4/134 ,  H01M4/1395 ,  H01M4/366 ,  H01M4/661

    摘要： Provided are novel electrodes for use in lithium ion batteries. An electrode includes one or more intermediate layers positioned between a substrate and an electrochemically active material. Intermediate layers may be made from chromium, titanium, tantalum, tungsten, nickel, molybdenum, lithium, as well as other materials and their combinations. An intermediate layer may protect the substrate, help to redistribute catalyst during deposition of the electrochemically active material, improve adhesion between the active material and substrate, and other purposes. In certain embodiments, an active material includes one or more high capacity active materials, such as silicon, tin, and germanium. These materials tend to swell during cycling and may loose mechanical and/or electrical connection to the substrate. A flexible intermediate layer may compensate for swelling and provide a robust adhesion interface. Provided also are novel methods of fabricating electrodes containing one or more intermediate layers.

    摘要翻译： 提供用于锂离子电池的新型电极。 电极包括位于基底和电化学活性材料之间的一个或多个中间层。 中间层可以由铬，钛，钽，钨，镍，钼，锂以及其它材料及其组合制成。 中间层可以保护基底，有助于在电化学活性材料的沉积期间重新分布催化剂，改善活性材料和基底之间的粘附性以及其它目的。 在某些实施方案中，活性材料包括一种或多种高容量活性材料，例如硅，锡和锗。 这些材料在循环过程中倾向于膨胀，并可能导致与基底的机械和/或电连接。 柔性中间层可以补偿溶胀并提供牢固的粘合界面。 还提供了制造包含一个或多个中间层的电极的新方法。