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    Selective removal of olefins from hydrocarbon feed streams
    4.
    发明申请
    Selective removal of olefins from hydrocarbon feed streams 有权
    从烃进料流中选择性除去烯烃

    公开(公告)号：US20040156778A1

    公开(公告)日：2004-08-12

    申请号：US10365165

    申请日：2003-02-12

    Applicant: ENGELHARD CORPORATION

    Inventor： Shinn H. Hwang ,  Robert J. Farrauto

    IPC: C01B003/26

    CPC classification number: C01B3/382 ,  C01B2203/0233 ,  C01B2203/0244 ,  C01B2203/0261 ,  C01B2203/0844 ,  C01B2203/1247 ,  C01B2203/1264 ,  C01B2203/142 ,  C01B2203/143 ,  C01B2203/82

    Abstract: Provided is a method of generating a hydrogen-rich reformate from a hydrocarbon feed stream comprising olefins and alkanes (e.g., LPG). An inlet gas stream containing the hydrocarbon feed stream and an oxygen containing gas stream, is preheated to a temperature of from 180 to 300null C. The preheated inlet gas stream is then contacted with a sulfur tolerant partial oxidation catalyst to form a pre-reformed gas stream, which is preferably maintained below about 400null C. The pre-reformed gas stream is then subjected to a reforming process to form the hydrogen-rich reformate.

    Abstract translation: 提供了从包含烯烃和烷烃（例如LPG）的烃进料流产生富氢重整产物的方法。 将含有烃进料流和含氧气流的入口气流预热至180℃至300℃的温度。然后将预热的入口气流与耐硫部分氧化催化剂接触以形成预转化 气流优选保持在约400℃以下。然后将预重整气流进行重整过程以形成富氢重整产物。

    Ruthenium oxidation catalyst
    5.
    发明申请
    Ruthenium oxidation catalyst 审中-公开
    钌氧化催化剂

    公开(公告)号：US20020131925A1

    公开(公告)日：2002-09-19

    申请号：US10100472

    申请日：2002-03-18

    Applicant: ENGELHARD CORPORATION

    Inventor： Lawrence Shore ,  Wolfgang F. Ruettinger ,  Robert J. Farrauto

    IPC: B01J023/60

    CPC classification number: B01J23/63 ,  B01J23/60 ,  B01J35/04 ,  B01J35/1014 ,  B01J37/0215 ,  B01J37/0248 ,  C01B3/16 ,  C01B3/583 ,  C01B2203/044 ,  C01B2203/047 ,  H01M8/0612 ,  H01M8/0618 ,  H01M8/0662 ,  H01M8/0668 ,  H01M2008/1095 ,  Y02P20/52

    Abstract: Provided is a ruthenium-based catalyst having from about 1 to 10 wt. % of a ruthenium component and at least about 0.5 wt. % of zinc oxide. In one embodiment of the catalyst, zinc oxide itself serves as a support on which the ruthenium is dispersed. In another embodiment, the ruthenium component and the zinc oxide are dispersed on a refractory oxide support other than zinc oxide. In a process aspect, the ruthenium-based catalyst can serve as a preferential oxidation catalyst in processes for removing carbon monoxide from an input gas stream containing carbon monoxide, hydrogen and oxygen. The invention also provides articles wherein multi-stage preferential oxidation processes for removal of carbon monoxide from hydrogen streams can be conducted.

    Abstract translation: 提供了一种钌基催化剂，其具有约1-10重量％ ％的钌组分和至少约0.5wt。 ％的氧化锌。 在催化剂的一个实施方案中，氧化锌本身用作其上分散有钌的载体。 在另一个实施方案中，钌组分和氧化锌分散在氧化锌以外的难熔氧化物载体上。 在方法方面，钌基催化剂可用作从含有一氧化碳，氢气和氧气的输入气流中除去一氧化碳的方法中的优先氧化催化剂。 本发明还提供了可以进行用于从氢气流中除去一氧化碳的多级优先氧化方法的制品。

    Process for generating hydrogen-rich gas
    6.
    发明申请
    Process for generating hydrogen-rich gas 有权
    产生富氢气体的方法

    公开(公告)号：US20030021748A1

    公开(公告)日：2003-01-30

    申请号：US10185033

    申请日：2002-08-19

    Applicant: Engelhard Corporation

    Inventor： H. Shinn Hwang ,  Robert J. Farrauto

    IPC: C01B003/26

    CPC classification number: B01J23/40 ,  B01J23/44 ,  B01J23/464 ,  B01J37/0244 ,  C01B3/382 ,  C01B3/40 ,  C01B2203/0244 ,  C01B2203/0283 ,  C01B2203/0844 ,  C01B2203/1017 ,  C01B2203/1023 ,  C01B2203/1029 ,  C01B2203/1041 ,  C01B2203/1047 ,  C01B2203/1052 ,  C01B2203/1064 ,  C01B2203/107 ,  C01B2203/1076 ,  C01B2203/1082 ,  C01B2203/1241 ,  C01B2203/1247 ,  C01B2203/142 ,  C01B2203/82 ,  Y02P20/129 ,  Y02P20/52

    Abstract: A process for catalytically generating a hydrogen-rich gas from a hydrocarbon feed. A stream comprising the hydrocarbon feed, water and air is preheated to a temperature sufficiently high to initiate catalytic partial oxidation of the hydrocarbon feed. The preheated stream is then introduced into an autothermal reactor containing a layered catalyst member at a temperature sufficient to initiate and sustain both catalytic partial oxidation and catalytic steam reforming. At least part of the hydrocarbon feed is catalytically partially oxidized to produce a hydrogen-rich gas comprising hydrogen and carbon oxides and hydrocarbons remaining in the feed are steam reformed to produce further quantities of the hydrogen-rich gas. The layered catalyst member comprises a monolith substrate containing at least one layer of a steam reforming catalyst in contact with at least one layer of a catalytic partial oxidation catalyst. The steam reforming catalyst comprises one or more platinum group metal components and the catalytic partial oxidation catalyst comprises palladium components.

    Abstract translation: 从烃进料催化产生富氢气体的方法。 将包含烃进料，水和空气的料流预热至足够高的温度以引发烃进料的催化部分氧化。 然后将预热的物流引入含有层状催化剂构件的自热反应器中，其温度足以启动和维持催化部分氧化和催化蒸汽重整。 至少部分烃进料被催化部分氧化以产生包含氢和碳氧化物的富氢气体，并且进料中剩余的烃被蒸汽重整以产生更多量的富氢气体。 层状催化剂构件包括含有至少一层与至少一层催化部分氧化催化剂接触的蒸汽重整催化剂层的整料基材。 蒸汽重整催化剂包含一种或多种铂族金属组分，催化部分氧化催化剂包括钯组分。

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