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    Catalytic conversion process for producing light olefins with a high yield from petroleum hydrocarbons
    3.
    发明申请
    Catalytic conversion process for producing light olefins with a high yield from petroleum hydrocarbons 有权
    用于从石油烃生产高产率的轻质烯烃的催化转化方法

    公开(公告)号：US20050020867A1

    公开(公告)日：2005-01-27

    申请号：US10878187

    申请日：2004-06-29

    申请人： Chaogang Xie ,  Jun Long ,  Jiushun Zhang ,  Zaiting Li ,  Xieqing Wang

    发明人： Chaogang Xie ,  Jun Long ,  Jiushun Zhang ,  Zaiting Li ,  Xieqing Wang

    IPC分类号： C07C4/06 ,  C10G11/18 ,  C07C4/02

    CPC分类号： C07C4/06 ,  C07C2523/745 ,  C07C2523/755 ,  C07C2523/83 ,  C10G2400/20 ,  Y02P20/52 ,  Y02P20/584 ,  Y02P30/446 ,  C07C11/04 ,  C07C11/06

    摘要： A catalytic conversion process for producing light olefins with a high yield from petroleum hydrocarbons, which comprises the steps of contacting a pre-heated petroleum hydrocarbons feedstock with a catalyst which comprises phosphorus and transition metal modified silica rich zeolite having a structure of pentasil in a riser or a fluidized bed reactor, and converting under the catalytic conversion conditions to produce reaction effluent and a spent catalyst, separating the resulted reaction effluent and spent catalyst, further separating said reaction effluent into liquid products and gaseous products comprising ethylene and propylene; stripping the spent catalyst by steam; regenerating the stripped catalyst by contacting the spent catalyst with oxygen-containing gas and burning off coke; and recycling the regenerated catalyst to reactor for reuse.

    摘要翻译： 一种用于从石油烃生产高产率的轻质烯烃的催化转化方法，其包括以下步骤：使预热的石油烃原料与催化剂接触，所述催化剂包含在提升管中具有pentasil结构的磷和过渡金属改性的富硅沸石 或流化床反应器，并在催化转化条件下转化以产生反应流出物和废催化剂，分离所得反应流出物和废催化剂，进一步将所述反应流出物分离成液体产物和包含乙烯和丙烯的气态产物; 通过蒸汽汽提废催化剂; 通过使废催化剂与含氧气体接触并将焦炭烧掉来再生汽提催化剂; 并将再生的催化剂再循环到反应器中以便再利用。

    Catalytic conversion process for producing light olefins with a high yield petroleum hydrocarbons
    4.
    发明授权
    Catalytic conversion process for producing light olefins with a high yield petroleum hydrocarbons 有权
    用于生产具有高产率石油烃的轻质烯烃的催化转化方法

    公开(公告)号：US07375256B2

    公开(公告)日：2008-05-20

    申请号：US10878187

    申请日：2004-06-29

    申请人： Chaogang Xie ,  Jun Long ,  Jiushun Zhang ,  Zaiting Li ,  Xieqing Wang

    发明人： Chaogang Xie ,  Jun Long ,  Jiushun Zhang ,  Zaiting Li ,  Xieqing Wang

    IPC分类号： C07C4/06

    CPC分类号： C07C4/06 ,  C07C2523/745 ,  C07C2523/755 ,  C07C2523/83 ,  C10G2400/20 ,  Y02P20/52 ,  Y02P20/584 ,  Y02P30/446 ,  C07C11/04 ,  C07C11/06

    摘要： A catalytic conversion process for producing light olefins with a high yield from petroleum hydrocarbons, which comprises the steps of contacting a pre-heated petroleum hydrocarbons feedstock with a catalyst which comprises phosphorus and transition metal modified silica rich zeolite having a structure of pentasil in a riser or a fluidized bed reactor, and converting under the catalytic conversion conditions to produce reaction effluent and a spent catalyst, separating the resulted reaction effluent and spent catalyst, further separating said reaction effluent into liquid products and gaseous products comprising ethylene and propylene; stripping the spent catalyst by steam; regenerating the stripped catalyst by contacting the spent catalyst with oxygen-containing gas and burning off coke; and recycling the regenerated catalyst to reactor for reuse.

    摘要翻译： 一种用于从石油烃生产高产率的轻质烯烃的催化转化方法，其包括以下步骤：使预热的石油烃原料与催化剂接触，所述催化剂包含在提升管中具有pentasil结构的磷和过渡金属改性的富硅沸石 或流化床反应器，并在催化转化条件下转化以产生反应流出物和废催化剂，分离所得反应流出物和废催化剂，进一步将所述反应流出物分离成液体产物和包含乙烯和丙烯的气态产物; 通过蒸汽汽提废催化剂; 通过使废催化剂与含氧气体接触并将焦炭烧掉来再生汽提催化剂; 并将再生的催化剂再循环到反应器中以便再利用。

    Catalytic conversion process for producing isobutane and isoparaffin-enriched gasoline
    7.
    发明授权
    Catalytic conversion process for producing isobutane and isoparaffin-enriched gasoline 有权
    用于生产异丁烷和富含异构烷烃的汽油的催化转化方法

    公开(公告)号：US06495028B1

    公开(公告)日：2002-12-17

    申请号：US09556079

    申请日：2000-04-21

    申请人： Youhao Xu ,  Jiushun Zhang ,  Yinan Yang ,  Jun Long ,  Xieqing Wang ,  Zaiting Li ,  Raichi Zhang

    发明人： Youhao Xu ,  Jiushun Zhang ,  Yinan Yang ,  Jun Long ,  Xieqing Wang ,  Zaiting Li ,  Raichi Zhang

    IPC分类号： C10G5700

    CPC分类号： C10G11/18

    摘要： A process for catalytic conversion of hydrocarbon feedstock to produce isobutane and isoparaffin-enriched gasoline which comprises two different reactions, the preheated feedstock is contacted with hot regenerated catalyst in the lower part of a reactor with the result that catalytic cracking reaction takes place, and the mixture of vapors and the coke deposited catalyst are up-flowed and enter into a suitable reaction environment with the result that isomerization and hydrogen transfer reaction take place. The produced LPG has an isobutane content of about 20 wt % to about 40 wt % and the produced gasoline contains isoparaffin content of about 30 wt % to about 45 wt % and olefin content of less than 30 wt %. RON and MON of the gasoline are 90˜93 and 80˜84 respectively.

    摘要翻译： 催化转化烃原料以生产异丁烷和富含异构烷烃的汽油的方法，其包括两个不同的反应，预热的原料与反应器下部的热再生催化剂接触，结果发生催化裂化反应， 蒸汽和焦炭沉积催化剂的混合物向上流动并进入合适的反应环境，结果发生异构化和氢转移反应。 生产的LPG具有约20重量％至约40重量％的异丁烷含量，并且所生产的汽油含有约30重量％至约45重量％的异链烷烃含量和小于30重量％的烯烃含量。 汽油的RON和MON分别为90〜93和80〜84。

    Titanium-silicalite molecular sieve and the method for its preparation
    8.
    发明授权
    Titanium-silicalite molecular sieve and the method for its preparation 有权
    钛 - 硅沸石分子筛及其制备方法

    公开(公告)号：US06475465B2

    公开(公告)日：2002-11-05

    申请号：US09732100

    申请日：2000-12-06

    申请人： Min Lin ,  Xingtian Shu ,  Xieqing Wang ,  Bin Zhu

    发明人： Min Lin ,  Xingtian Shu ,  Xieqing Wang ,  Bin Zhu

    IPC分类号： C01B3700

    CPC分类号： C01B37/005 ,  Y10S423/22

    摘要： The present invention relates to a titanium-silicalite (TS-1) molecular sieve and the method for preparation of the same, wherein each crystallite of said titanium-silicalite molecular sieve has a hollow cavity with a radial length of 5-300 nm. The benzene adsorption capacity of the molecular sieve determined at 25° C. and P/P0=0.10 for 1 hour is at least 70 mg/g; and the method for preparation of said molecular sieve comprises an acid-treatment and then an organic-base treatment of the synthesized TS-1 molecular sieve, or only an organic-base treatment. The TS-1 molecular sieve of the present invention has a relatively high reactivity and activity stability in the catalytic oxidation.

    摘要翻译： 本发明涉及钛 - 硅沸石（TS-1）分子筛及其制备方法，其中所述钛 - 硅沸石分子筛的每个微晶具有径向长度为5-300nm的中空腔。 在25℃和P / P0 = 0.10下测定1小时的分子筛的苯吸附能力为至少70mg / g; 并且所述分子筛的制备方法包括对所合成的TS-1分子筛进行酸处理，然后进行有机碱处理，或仅进行有机碱处理。 本发明的TS-1分子筛在催化氧化中具有较高的反应活性和活性稳定性。

    Process for production of ethylene and propylene by catalytic pyrolysis of heavy hydrocarbons
    9.
    发明授权
    Process for production of ethylene and propylene by catalytic pyrolysis of heavy hydrocarbons 有权
    通过重烃催化裂解生产乙烯和丙烯的方法

    公开(公告)号：US06210562B1

    公开(公告)日：2001-04-03

    申请号：US09172651

    申请日：1998-10-15

    申请人： Chaogang Xie ,  Zaiting Li ,  Wenyuan Shi ,  Xieqing Wang

    发明人： Chaogang Xie ,  Zaiting Li ,  Wenyuan Shi ,  Xieqing Wang

    IPC分类号： C10G1102

    CPC分类号： B01J38/06 ,  C10G2400/20

    摘要： A catalytic pyrolysis process for production of ethylene and propylene from heavy hydrocarbons, comprises that heavy hydrocarbons are contacted with a pillared interlayered clay molecular sieve and/or phosphorus and aluminum or magnesium or calcium modified high silica zeolite having a structure of pentasil contained catalysts in a riser or downflow transfer line reactor in the presence of steam and catalytically pyrolysed at a temperature of 650° C. to 750° C. and a pressure of 0.15 to 0.4 MPa for a contact time of 0.2 to 5 seconds, a weight ratio of catalyst to feedstock of 15:1 to 40:1 and a weight ratio of steam to feedstock of 0.3:1 to 1:1. The yields of ethylene and propylene by the present invention are over 18 wt %.

    摘要翻译： 用于从重质烃生产乙烯和丙烯的催化裂解方法包括使重质烃与柱状粘土分子筛和/或具有pentasil结构的磷和铝或镁或钙改性的高二氧化硅沸石与含有催化剂的催化剂接触 立管或下流输送管线反应器，在蒸汽存在下，在650℃至750℃的温度和0.15至0.4MPa的压力下进行催化热解，接触时间为0.2至5秒，催化剂的重量比 至原料为15：1至40：1，蒸汽与原料的重量比为0.3：1至1：1。 本发明的乙烯和丙烯的产率超过18重量％。

    Pentasil-type molecular sieve containing composition and its preparation method
    10.
    发明授权
    Pentasil-type molecular sieve containing composition and its preparation method 有权
    五仙子型分子筛组合物及其制备方法

    公开(公告)号：US6080698A

    公开(公告)日：2000-06-27

    申请号：US154581

    申请日：1998-09-17

    申请人： Fengmei Zhang ,  Xingtian Shu ,  Zhicheng Shi ,  Weidong Wang ,  Fengming Qin ,  Xieqing Wang

    发明人： Fengmei Zhang ,  Xingtian Shu ,  Zhicheng Shi ,  Weidong Wang ,  Fengming Qin ,  Xieqing Wang

    IPC分类号： B01J29/42 ,  B01J29/40 ,  B01J29/48 ,  C01B39/36 ,  C01B39/38 ,  C10G11/05

    CPC分类号： C10G11/05 ,  B01J29/40 ,  B01J2229/36 ,  C10G2400/20

    摘要： A molecular sieve containing composition, which can be applied in catalytic cracking reaction for producing more ethylene and propylene, and its preparation method. The composition contains a pentasil-type molecular sieve having a SiO.sub.2 /Al.sub.2 O.sub.3 molar ratio of 15-60, prepared by activation and modification with phosphorus, alkaline earth metal and transition metal. The composition essentially includes 85.about.98% wt of pentasil-type molecular sieve, 1.about.10% wt of P.sub.2 O.sub.5, 0.3.about.5% wt of alkaline earth oxide, and 0.3.about.5% wt of transition metal oxide. The molecular sieve structure and active centers have high thermal and hydrothermal stability. The salient feature of this composition is that when applied as an active component of cracking catalyst for catalytic pyrolysis process, the yield of ethylene is above 18% and the total yield of ethylene and propylene is more than 40%.

    摘要翻译： 一种含分子筛的组合物及其制备方法，可用于催化裂化反应生产更多的乙烯和丙烯。 该组合物含有通过用磷，碱土金属和过渡金属的活化和改性制备的SiO 2 / Al 2 O 3摩尔比为15-60的pentasil型分子筛。 该组合物基本上包含85％的pentinil型分子筛98％wt，10％wt的P2O5，0.3％的5％wt的碱土金属氧化物和0.3％的5％wt的过渡金属氧化物。 分子筛结构和活性中心具有较高的热和水热稳定性。 该组合物的显着特点是当作为催化裂解工艺的裂化催化剂的活性组分使用时，乙烯的产率高于18％，乙烯和丙烯的总产率大于40％。