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    Process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons
    3.
    发明授权
    Process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons 有权
    从乙醇生产乙烯的方法，结合烃的催化转化

    公开(公告)号：US08273930B2

    公开(公告)日：2012-09-25

    申请号：US12373585

    申请日：2007-07-12

    Applicant: Zhiguo Wu ,  Wenhua Xie ,  Chaogang Xie ,  Qiang Liu ,  Xuhong Mu ,  Jiushun Zhang ,  Yibin Luo ,  Xingtian Shu ,  Chenghan Yan

    Inventor： Zhiguo Wu ,  Wenhua Xie ,  Chaogang Xie ,  Qiang Liu ,  Xuhong Mu ,  Jiushun Zhang ,  Yibin Luo ,  Xingtian Shu ,  Chenghan Yan

    IPC: C07C1/24

    CPC classification number: C10G57/00 ,  C07C1/24 ,  C07C2529/08 ,  C10G11/05 ,  C10G2300/1033 ,  C10G2300/104 ,  C10G2300/1044 ,  C10G2300/1055 ,  C10G2300/107 ,  C10G2300/1074 ,  C10G2300/1077 ,  C10G2300/4018 ,  C10G2400/20 ,  Y02P20/52 ,  Y02P20/584 ,  C07C11/04

    Abstract: A process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons: an ethanol feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, and a coked catalyst and an target product of ethylene are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, a spent catalyst and an oil vapor are obtained after separating the reaction stream, and the oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with ethanol feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of ethanol, thus ensuring the continuous catalytic conversion of ethanol and generating enormous economic benefits. For the catalytic conversion of the ethanol, the content of ethylene is 95 vol % or more in the gas product; and the conversion of ethylene is not less than 99%. For the catalytic conversion of the hydrocarbons, the yield for the light olefins increases slightly by at least 2 mol %.

    Abstract translation: 将乙烯的催化转化合成乙醇的方法：将乙醇原料与含Y-沸石的催化剂接触，得到产物流，分离出反应物流后得到结焦催化剂和乙烯目标产物; 将烃原料与含Y-沸石的催化剂接触，得到产物流，分离反应流后得到废催化剂和油蒸气，并进一步分离出油蒸汽，得到产物如气体，汽油和 类似; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和 冷却后的另一部分返回与乙醇原料接触。 这个过程不仅合理利用了烃转化的过量热能，而且解决了乙醇转化的供热问题，从而保证了乙醇的连续催化转化，产生了巨大的经济效益。 对于乙醇的催化转化，气体产物中乙烯的含量为95体积％以上; 乙烯的转化率不低于99％。 对于烃的催化转化，轻质烯烃的产率略微增加至少2摩尔％。

    FLUIDIZED CATALYTIC PROCESS FOR PRODUCTION OF DIMETHYL ETHER FROM METHANOL
    4.
    发明申请
    FLUIDIZED CATALYTIC PROCESS FOR PRODUCTION OF DIMETHYL ETHER FROM METHANOL 有权
    用于从甲醇生产二甲醚的流化催化方法

    公开(公告)号：US20100076227A1

    公开(公告)日：2010-03-25

    申请号：US12594006

    申请日：2008-03-27

    Applicant: Zheng Li ,  Qiang Fu ,  Chaogang Xie ,  Minggang Li ,  Anguo Mao ,  Lisheng Li ,  Genquan Zhu ,  Fengmei Zhang ,  Yinbin Luo

    Inventor： Zheng Li ,  Qiang Fu ,  Chaogang Xie ,  Minggang Li ,  Anguo Mao ,  Lisheng Li ,  Genquan Zhu ,  Fengmei Zhang ,  Yinbin Luo

    IPC: C07C41/09

    CPC classification number: B01J29/90 ,  B01J29/005 ,  B01J29/088 ,  B01J29/46 ,  B01J29/85 ,  B01J2229/42 ,  C07C41/09 ,  Y02P20/584 ,  Y02P20/588 ,  C07C43/043

    Abstract: The present invention provides a fluidized catalytic process for production of dimethyl ether from methanol, wherein said process is carried out in a reactor in which the catalyst is in a fluidized state. Said process comprises the following steps of (1) feeding the methanol feedstock via two or more locations selected from the bottom, lower part, middle part and upper part of the reactor, contacting with the catalyst for preparation of dimethyl ether by methanol dehydration, carrying out the reaction of preparing dimethyl ether by methanol dehydration to obtain the reaction stream, separating said reaction stream to obtain a coked catalyst and a crude product primarily containing the target product, i.e. dimethyl ether; (2) totally or partially feeding the coked catalyst obtained in step (1) into a regenerator in a continuous or batch manner for regeneration via coke-burning, the regenerated catalyst being directly recycled to step (1) after being totally or partially cooled.

    Abstract translation: 本发明提供了一种用于从甲醇生产二甲醚的流化催化方法，其中所述方法在催化剂处于流化状态的反应器中进行。 所述方法包括以下步骤：（1）经由选自反应器的底部，底部，中部和上部的两个或多个位置进料甲醇原料，与甲醇脱水制备二甲醚的催化剂接触，携带 通过甲醇脱水制备二甲醚以获得反应流的反应，分离所述反应流，得到主要含有目标产物（即二甲醚）的焦化催化剂和粗产物; （2）将在步骤（1）中获得的焦化催化剂全部或部分地以连续或间歇方式进料到再生器中，以通过焦炭燃烧再生，再生催化剂在全部或部分冷却后直接再循环到步骤（1）。

    Integrated process for hydrogenation and catalytic cracking of hydrocarbon oil
    5.
    发明授权
    Integrated process for hydrogenation and catalytic cracking of hydrocarbon oil 有权
    碳氢化合物氢化和催化裂解的综合工艺

    公开(公告)号：US09309467B2

    公开(公告)日：2016-04-12

    申请号：US12809516

    申请日：2008-12-19

    Applicant: Yongcan Gao ,  Chaogang Xie ,  Chuanfeng Niu ,  Jiushun Zhang ,  Lishun Dai ,  Hong Nie ,  Dadong Li ,  Jun Long ,  Jianguo Ma ,  Yan Cui

    Inventor： Yongcan Gao ,  Chaogang Xie ,  Chuanfeng Niu ,  Jiushun Zhang ,  Lishun Dai ,  Hong Nie ,  Dadong Li ,  Jun Long ,  Jianguo Ma ,  Yan Cui

    IPC: C10G11/18 ,  C10G51/06 ,  C10G69/04

    CPC classification number: C10G11/18 ,  C10G11/182 ,  C10G51/06 ,  C10G69/04 ,  C10G2300/1037 ,  C10G2300/107 ,  C10G2300/1077 ,  C10G2300/301 ,  C10G2300/4006 ,  C10G2300/4012 ,  C10G2300/70 ,  C10G2300/807 ,  C10G2400/02 ,  C10G2400/04 ,  C10G2400/28

    Abstract: Disclosed is a combination process for improved hydrotreating and catalytic cracking of hydrocarbon oils, including: contacting residual oil, catalytic cracking cycle oil, and optional distillate oil with a hydrotreating catalyst under hydrotreating conditions in the presence of hydrogen followed by separation of the reaction products to obtain gas, hydrogenated naphtha, hydrogenated diesel oil, and hydrogenated tail oil; contacting the hydrogenated tail oil and optional normal catalytic cracking feedstock oil with a cracking catalyst under catalytic cracking conditions followed by separation of the reaction products to obtain dry gas, hydrogenated naphtha, liquefied petroleum gas, catalytic cracked gasoline, catalytic cracked diesel oil, and catalytic cracking cycle oil; wherein the hydrogenated tail oil and/or normal catalytic cracking feedstock oil are separated into at least two fractions, the light and the heavy fractions or normal catalytic cracking heavy feedstock oil and normal catalytic cracking light feedstock oil, prior to contacting the hydrogenated tail oil and/or normal catalytic cracking feedstock oil with the cracking catalyst. The process according to the present invention is especially suitable for conversion of hydrocarbon oils to produce more products of gasoline or diesel oil.

    Abstract translation: 公开了用于改进烃油的加氢处理和催化裂化的组合方法，包括：在加氢处理条件下在氢气存在下，用加氢处理催化剂将残油，催化裂化循环油和任选的馏出油接触，然后将反应产物分离 获得气体，氢化石脑油，氢化柴油和氢化尾油; 在催化裂化条件下使氢化尾油和任选的常规催化裂化原料油与裂化催化剂接触，然后分离反应产物，得到干燥气体，氢化石脑油，液化石油气，催化裂化汽油，催化裂化柴油和催化剂 开裂循环油; 其中所述氢化尾油和/或常规催化裂化原料油在将氢化尾油与氢化尾油接触之前分离成至少两个馏分，轻馏分或重馏分或正常催化裂化重原料油和常规催化裂化轻原料油， /或正常催化裂化原料油与裂化催化剂。 根据本发明的方法特别适用于烃油的转化以产生更多的汽油或柴油的产物。

    Fluidized catalytic process for production of dimethyl ether from methanol
    6.
    发明授权
    Fluidized catalytic process for production of dimethyl ether from methanol 有权
    用于从甲醇生产二甲醚的流化催化方法

    公开(公告)号：US08304582B2

    公开(公告)日：2012-11-06

    申请号：US12594006

    申请日：2008-03-27

    Applicant: Zheng Li ,  Qiang Fu ,  Chaogang Xie ,  Minggang Li ,  Anguo Mao ,  Lisheng Li ,  Genquan Zhu ,  Fengmei Zhang ,  Yi bin Luo

    Inventor： Zheng Li ,  Qiang Fu ,  Chaogang Xie ,  Minggang Li ,  Anguo Mao ,  Lisheng Li ,  Genquan Zhu ,  Fengmei Zhang ,  Yi bin Luo

    IPC: C07C41/09 ,  C07C43/04 ,  F27B15/08

    CPC classification number: B01J29/90 ,  B01J29/005 ,  B01J29/088 ,  B01J29/46 ,  B01J29/85 ,  B01J2229/42 ,  C07C41/09 ,  Y02P20/584 ,  Y02P20/588 ,  C07C43/043

    Abstract: The present invention provides a fluidized catalytic process for production of dimethyl ether from methanol, wherein said process is carried out in a reactor in which the catalyst is in a fluidized state. Said process comprises the following steps of (1) feeding the methanol feedstock via two or more locations selected from the bottom, lower part, middle part and upper part of the reactor, contacting with the catalyst for preparation of dimethyl ether by methanol dehydration, carrying out the reaction of preparing dimethyl ether by methanol dehydration to obtain the reaction stream, separating said reaction stream to obtain a coked catalyst and a crude product primarily containing the target product, i.e. dimethyl ether; (2) totally or partially feeding the coked catalyst obtained in step (1) into a regenerator in a continuous or batch manner for regeneration via coke-burning, the regenerated catalyst being directly recycled to step (1) after being totally or partially cooled.

    Abstract translation: 本发明提供了一种用于从甲醇生产二甲醚的流化催化方法，其中所述方法在催化剂处于流化状态的反应器中进行。 所述方法包括以下步骤：（1）经由选自反应器的底部，底部，中部和上部的两个或多个位置进料甲醇原料，与甲醇脱水制备二甲醚的催化剂接触，携带 通过甲醇脱水制备二甲醚以获得反应流的反应，分离所述反应流，得到主要含有目标产物（即二甲醚）的焦化催化剂和粗产物; （2）将在步骤（1）中获得的焦化催化剂全部或部分地以连续或间歇方式进料到再生器中，以通过焦炭燃烧再生，再生催化剂在全部或部分冷却后直接再循环到步骤（1）。

    Catalytic conversion apparatus
    7.
    发明授权
    Catalytic conversion apparatus 有权
    催化转化装置

    公开(公告)号：US08088335B2

    公开(公告)日：2012-01-03

    申请号：US12295523

    申请日：2007-03-30

    Applicant: Jun Long ,  Kejia Xu ,  Shuandi Hou ,  Zhijian Da ,  Chaogang Xie ,  Jiushun Zhang ,  Zhanzhu Zhang

    Inventor： Jun Long ,  Kejia Xu ,  Shuandi Hou ,  Zhijian Da ,  Chaogang Xie ,  Jiushun Zhang ,  Zhanzhu Zhang

    IPC: B01J8/18 ,  F27B15/00

    CPC classification number: C10G11/18 ,  B01J8/0055 ,  B01J8/0065 ,  B01J8/1827 ,  B01J8/26 ,  B01J2219/00038 ,  C10G2300/4093 ,  C10G2400/20 ,  Y02P30/40 ,  Y02P30/446

    Abstract: A conversion apparatus for catalytic cracking a hydrocarbon feed to light hydrocarbon comprises at least one riser reactor, a dense bed reactor, a disengager, and a stripper. A dense bed reactor which is separated from disengage, is employed to enforce further cracking hydrocarbon to light olefins, with low methane yield. Moreover, the spent catalysts discharged from the outlet of the dense bed reactor can be introduced into the stripper via a specific catalyst transporting channel, to maintain catalyst concentration in the dense bed reactor that can be advantageous to deeper cracking of the intermediate products to produce more light olefins, particularly propylene.

    Abstract translation: 用于将烃进料催化裂化成轻质烃的转化装置包括至少一个提升管反应器，致密床反应器，脱分离器和剥离器。 使用与脱离分离的致密床反应器用于进一步将烃裂解成轻质烯烃，甲烷产率低。 此外，从致密床反应器的出口排出的废催化剂可以通过特定的催化剂输送通道引入汽提塔中，以保持致密床反应器中的催化剂浓度，这有利于中间产物的更深裂化以产生更多 轻质烯烃，特别是丙烯。

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