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    Novel Sulfonic Acid Group-Containing Segmented Block Copolymer and Use Thereof
    6.
    发明申请
    Novel Sulfonic Acid Group-Containing Segmented Block Copolymer and Use Thereof 审中-公开
    新型含磺酸基团的嵌段共聚物及其用途

    公开(公告)号：US20120129076A1

    公开(公告)日：2012-05-24

    申请号：US13388703

    申请日：2010-08-03

    申请人： Shunsuke Ichimura ,  Ryouhei Iwahara ,  Kouta Kitamura ,  Masahiro Yamashita

    发明人： Shunsuke Ichimura ,  Ryouhei Iwahara ,  Kouta Kitamura ,  Masahiro Yamashita

    IPC分类号： H01M8/10

    CPC分类号： H01B1/122 ,  C08G75/23 ,  C08J5/2256 ,  C08J2365/02 ,  C08J2481/06 ,  C08L81/06 ,  H01M8/1025 ,  H01M8/1027 ,  H01M2008/1095

    摘要： Disclosed is a proton exchange membrane for use in fuel cells, which not only has improved proton conductivity and resistance to swelling caused by hot water but also has greater durability when used in a fuel cell, as well as a sulfonic acid group-containing segmented block copolymer constituting the proton exchange membrane, a membrane electrode assembly using the proton exchange membrane, and a fuel cell using the membrane electrode assembly. A sulfonic acid group-containing segmented block copolymer, which is a di- or multi-block copolymer including, within a molecule, at least one kind of hydrophilic segment and at least one kind of hydrophobic segment, a 0.5 g/dL solution thereof dissolved in N-methyl-2-pyrrolidone as a solvent showing a logarithmic viscosity measured at 30° C. in the range of 0.5 to 5.0 dL/g, wherein the copolymer has at least one kind of hydrophobic segment represented by Chemical Formula 1, the segment has a structure bound to a group represented by Chemical Formula 2, and the hydrophilic segment has at least one kind of structure represented by Chemical Formula 3 or Chemical Formula 3-2.

    摘要翻译： 公开了一种用于燃料电池的质子交换膜，其不仅具有改善的质子传导性和耐热水膨胀性，而且当用于燃料电池中时也具有较高的耐久性，以及含有磺酸基的分段嵌段 构成质子交换膜的共聚物，使用质子交换膜的膜电极组件和使用该膜电极组件的燃料电池。 含有磺酸基的分段嵌段共聚物，其为分子内包含至少一种亲水链段和至少一种疏水链段的二嵌段共聚物或多嵌段共聚物，溶解有0.5g / dL的溶液 在作为溶剂的N-甲基-2-吡咯烷酮中，在30℃下测定的对数粘度为0.5〜5.0dL / g，其中共聚物具有至少一种由化学式1表示的疏水链段， 链段具有与化学式2表示的基团结合的结构，亲水性链段具有由化学式3或化学式3-2表示的至少一种结构。

    Electrolyte Membrane-Electrode Assembly, Fuel Cell Using The Same, And Method For Producing Electrolyte Membrane-Electrode Assembly
    7.
    发明申请
    Electrolyte Membrane-Electrode Assembly, Fuel Cell Using The Same, And Method For Producing Electrolyte Membrane-Electrode Assembly 审中-公开
    电解质膜电极组件，使用其的燃料电池，以及用于制造电解质膜 - 电极组件的方法

    公开(公告)号：US20080063917A1

    公开(公告)日：2008-03-13

    申请号：US10566218

    申请日：2004-07-29

    申请人： Masahiro Yamashita ,  Yoshimitsu Sakaguchi ,  Satoshi Takase ,  Kota Kitamura

    发明人： Masahiro Yamashita ,  Yoshimitsu Sakaguchi ,  Satoshi Takase ,  Kota Kitamura

    IPC分类号： H01M8/10 ,  B29C65/02

    CPC分类号： C08J5/2256 ,  C08J2371/12 ,  C08J2381/06 ,  H01M8/1004 ,  H01M8/1025 ,  H01M8/1027 ,  H01M8/1032 ,  Y02P20/582

    摘要： Disclosed is an electrolyte membrane-electrode assembly wherein a hydrocarbon-based solid polymer electrolyte membrane is sandwiched between a pair of electrodes. In this electrolyte membrane-electrode assembly, the glass transition temperature of the electrolyte membrane in a dry state is not less than 160° C. and the maximum moisture content of the electrolyte membrane is 10-120%. By using such a hydrocarbon-based solid polymer electrolyte membrane, there can be obtained an electrolyte membrane-electrode assembly which is excellent in reliability and durability. Also disclosed are a fuel cell using such an electrolyte membrane-electrode assembly and a method for producing such an electrolyte membrane-electrode assembly.

    摘要翻译： 公开了一种电解质膜 - 电极组件，其中烃基固体聚合物电解质膜夹在一对电极之间。 在该电解质膜 - 电极组件中，干燥状态的电解质膜的玻璃化转变温度为160℃以上，电解质膜的最高含水量为10〜120％。 通过使用这种烃基固体高分子电解质膜，可以获得可靠性和耐久性优异的电解质膜 - 电极组件。 还公开了使用这种电解质膜 - 电极组件的燃料电池和这种电解质膜 - 电极组件的制造方法。

    Aromatic hydrocarbon based proton exchange membrane and direct methanol fuel cell using same
    8.
    发明授权
    Aromatic hydrocarbon based proton exchange membrane and direct methanol fuel cell using same 有权
    芳香烃基质子交换膜和直接甲醇燃料电池使用相同

    公开(公告)号：US08216727B2

    公开(公告)日：2012-07-10

    申请号：US11745072

    申请日：2007-05-07

    申请人： Masahiro Yamashita ,  Yoshimitsu Sakaguchi ,  Kota Kitamura

    发明人： Masahiro Yamashita ,  Yoshimitsu Sakaguchi ,  Kota Kitamura

    IPC分类号： H01M8/00

    CPC分类号： H01M8/1025 ,  C08J5/2256 ,  C08J2371/12 ,  H01M8/0289 ,  H01M8/1011 ,  H01M8/1032 ,  H01M2300/0082 ,  Y02E60/523

    摘要： A proton exchange membrane is obtained which can give an excellent power generation characteristic when the membrane is applied to, in particular, a fuel cell wherein high-concentration methanol is used as a fuel. In the aromatic hydrocarbon based proton exchange membrane of the invention, the ion exchange capacity is set into the range of 0.6 to 1.3 meq/g. Moreover, the area swelling rate for a 30% by mass methanol aqueous solution at 40° C. is set into the range of 2 to 30%. Preferably, a sulfonic acid group is bonded to an aromatic ring of the aromatic hydrocarbon based polymer contained in the aromatic hydrocarbon based proton exchange film. Preferably, the aromatic hydrocarbon based polymer is a polyarylene ether based polymer.

    摘要翻译： 获得质子交换膜，当将膜应用于特别是其中使用高浓度甲醇作为燃料的燃料电池时，其可以产生优异的发电特性。 在本发明的芳烃类质子交换膜中，离子交换容量为0.6〜1.3meq / g。 此外，40℃下的30质量％甲醇水溶液的面积溶胀率为2〜30％的范围。 优选地，磺酸基团与芳族烃基质子交换膜中所含的芳香族烃系聚合物的芳香环结合。 优选地，芳族烃基聚合物是聚亚芳基醚基聚合物。

    PROTON-CONDUCTING POLYMER COMPOSITION AND METHOD FOR PREPARATION THEREOF, CATALYST INK CONTAINING SAID PROTON-CONDUCTING POLYMER COMPOSITION AND FUEL CELL INCLUDING SAID CATALYST INK
    9.
    发明申请
    PROTON-CONDUCTING POLYMER COMPOSITION AND METHOD FOR PREPARATION THEREOF, CATALYST INK CONTAINING SAID PROTON-CONDUCTING POLYMER COMPOSITION AND FUEL CELL INCLUDING SAID CATALYST INK 有权
    导电聚合物组合物及其制备方法，含有合成导电聚合物组合物的催化剂和含有催化剂油墨的燃料电池

    公开(公告)号：US20090269643A1

    公开(公告)日：2009-10-29

    申请号：US11718672

    申请日：2005-11-07

    申请人： Masahiro Yamashita ,  Kota Kitamura ,  Yoshimitsu Sakaguchi

    发明人： Masahiro Yamashita ,  Kota Kitamura ,  Yoshimitsu Sakaguchi

    IPC分类号： H01M8/10

    CPC分类号： H01M8/1004 ,  C08G65/40 ,  C08G65/4093 ,  C08L101/12 ,  H01M4/8605 ,  H01M4/8807 ,  H01M4/8828 ,  H01M8/0289 ,  H01M8/1023 ,  Y02P70/56

    摘要： A proton-conducting polymer composition which contains an aromatic hydrocarbon type of proton-conducting polymer in an amount of 1 to 30 mass %, wherein a component of said proton-conducting polymer having a molecular weight in the range of 2,000 to 230,000 in terms of polyethylene glycol accounts for 10 mass % or more of the total amount of said proton-conducting polymer; a method for preparing the proton-conducting polymer composition, a catalyst ink comprising the proton-conducting polymer composition and a fuel cell including the catalyst ink. The above proton-conducting polymer composition can well exploit the performance capability of a catalyst of a fuel cell, especially when it is allowed to be present with the electrode of a fuel cell.

    摘要翻译： 一种质子传导性聚合物组合物，其含有量为1〜30质量％的芳香族烃型质子传导性聚合物，其中，所述质子传导性聚合物的分子量在2000〜230,000范围内的成分为 聚乙二醇占所述质子传导性聚合物总量的10质量％以上; 用于制备质子传导聚合物组合物的方法，包含质子传导性聚合物组合物的催化剂油墨和包含催化剂油墨的燃料电池。 上述质子传导聚合物组合物可以很好地利用燃料电池的催化剂的性能，特别是当允许存在燃料电池的电极时。