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公开(公告)号：US08196387B2
公开(公告)日：2012-06-12
申请号：US12948128
申请日：2010-11-17
申请人： Minish Mahendra Shah , Aqil Jamal , Raymond Francis Dmevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool, III
发明人： Minish Mahendra Shah , Aqil Jamal , Raymond Francis Dmevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool, III
IPC分类号： F02C3/26
CPC分类号： B01D53/75 , B01D53/77 , B01D2256/22 , B01D2257/302 , B01D2257/80 , B01D2259/40 , C01B13/0251 , C01B2210/0046 , C10J3/06 , C10J3/466 , C10J2300/093 , C10J2300/0959 , C10J2300/0973 , C10J2300/1606 , C10J2300/1671 , C10J2300/1675 , C10J2300/1678 , C10J2300/1687 , C10J2300/1838 , C10J2300/1876 , C10J2300/1892 , C10K1/004 , C10K1/024 , C10K3/005 , F01K23/068 , F23J2215/20 , F23J2215/50 , F23L2900/07005 , Y02C10/06 , Y02E20/18 , Y02E20/344
摘要： An apparatus for generating electrical power in which a synthesis gas stream generated in a gasifier is partially oxidized, expanded and thereafter, is combusted in an oxygen transport membrane system of a boiler. The combustion generates heat to raise steam to in turn generate electricity by a generator coupled to a steam turbine. The resultant flue gas can be purified to produce a carbon dioxide product.
摘要翻译： 一种用于产生电力的装置，其中在气化器中产生的合成气流被部分氧化，膨胀，然后在锅炉的氧输送膜系统中燃烧。 燃烧产生热量以升高蒸汽，从而通过耦合到蒸汽轮机的发电机产生电力。 所得烟道气可以被纯化以产生二氧化碳产物。
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公开(公告)号：US20110061361A1
公开(公告)日：2011-03-17
申请号：US12948128
申请日：2010-11-17
申请人： Minish Mahendra SHAH , Aqil Jamal , Raymond Francis Dmevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool, III
发明人： Minish Mahendra SHAH , Aqil Jamal , Raymond Francis Dmevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool, III
IPC分类号： F02G3/00
CPC分类号： B01D53/75 , B01D53/77 , B01D2256/22 , B01D2257/302 , B01D2257/80 , B01D2259/40 , C01B13/0251 , C01B2210/0046 , C10J3/06 , C10J3/466 , C10J2300/093 , C10J2300/0959 , C10J2300/0973 , C10J2300/1606 , C10J2300/1671 , C10J2300/1675 , C10J2300/1678 , C10J2300/1687 , C10J2300/1838 , C10J2300/1876 , C10J2300/1892 , C10K1/004 , C10K1/024 , C10K3/005 , F01K23/068 , F23J2215/20 , F23J2215/50 , F23L2900/07005 , Y02C10/06 , Y02E20/18 , Y02E20/344
摘要： An apparatus for generating electrical power in which a synthesis gas stream generated in a gasifier is partially oxidized, expanded and thereafter, is combusted in an oxygen transport membrane system of a boiler. The combustion generates heat to raise steam to in turn generate electricity by a generator coupled to a steam turbine. The resultant flue gas can be purified to produce a carbon dioxide product.
摘要翻译： 一种用于产生电力的装置，其中在气化器中产生的合成气流被部分氧化，膨胀，然后在锅炉的氧输送膜系统中燃烧。 燃烧产生热量以升高蒸汽，从而通过耦合到蒸汽轮机的发电机产生电力。 所得烟道气可以被纯化以产生二氧化碳产物。
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公开(公告)号：US07856829B2
公开(公告)日：2010-12-28
申请号：US11639459
申请日：2006-12-15
申请人： Minish Mahendra Shah , Aqil Jamal , Raymond Francis Drnevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool, III
发明人： Minish Mahendra Shah , Aqil Jamal , Raymond Francis Drnevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool, III
IPC分类号： F02C6/18
CPC分类号： B01D53/75 , B01D53/77 , B01D2256/22 , B01D2257/302 , B01D2257/80 , B01D2259/40 , C01B13/0251 , C01B2210/0046 , C10J3/06 , C10J3/466 , C10J2300/093 , C10J2300/0959 , C10J2300/0973 , C10J2300/1606 , C10J2300/1671 , C10J2300/1675 , C10J2300/1678 , C10J2300/1687 , C10J2300/1838 , C10J2300/1876 , C10J2300/1892 , C10K1/004 , C10K1/024 , C10K3/005 , F01K23/068 , F23J2215/20 , F23J2215/50 , F23L2900/07005 , Y02C10/06 , Y02E20/18 , Y02E20/344
摘要： A method of generating electrical power in which a synthesis gas stream generated in a gasifier is combusted in an oxygen transport membrane system of a boiler. The combustion generates heat to raise steam to in turn generate electricity by a generator coupled to a steam turbine. The resultant flue gas can be purified to produce a carbon dioxide product.
摘要翻译： 一种产生电力的方法，其中在气化器中产生的合成气流在锅炉的氧输送膜系统中燃烧。 燃烧产生热量以升高蒸汽，从而通过耦合到蒸汽轮机的发电机产生电力。 所得烟道气可以被纯化以产生二氧化碳产物。
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公开(公告)号：US20080141672A1
公开(公告)日：2008-06-19
申请号：US11639459
申请日：2006-12-15
申请人： Minish Mahendra Shah , Aqil Jamal , Raymond Francis Dmevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool
发明人： Minish Mahendra Shah , Aqil Jamal , Raymond Francis Dmevich , Bart Antonie van Hassel , Gervase Maxwell Christie , Hisashi Kobayashi , Lawrence E. Bool
CPC分类号： B01D53/75 , B01D53/77 , B01D2256/22 , B01D2257/302 , B01D2257/80 , B01D2259/40 , C01B13/0251 , C01B2210/0046 , C10J3/06 , C10J3/466 , C10J2300/093 , C10J2300/0959 , C10J2300/0973 , C10J2300/1606 , C10J2300/1671 , C10J2300/1675 , C10J2300/1678 , C10J2300/1687 , C10J2300/1838 , C10J2300/1876 , C10J2300/1892 , C10K1/004 , C10K1/024 , C10K3/005 , F01K23/068 , F23J2215/20 , F23J2215/50 , F23L2900/07005 , Y02C10/06 , Y02E20/18 , Y02E20/344
摘要： A method of generating electrical power in which a synthesis gas stream generated in a gasifier is combusted in an oxygen transport membrane system of a boiler. The combustion generates heat to raise steam to in turn generate electricity by a generator coupled to a steam turbine. The resultant flue gas can be purified to produce a carbon dioxide product.
摘要翻译： 一种产生电力的方法，其中在气化器中产生的合成气流在锅炉的氧输送膜系统中燃烧。 燃烧产生热量以升高蒸汽，从而通过耦合到蒸汽轮机的发电机产生电力。 所得烟道气可以被纯化以产生二氧化碳产物。
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公开(公告)号：US08323463B2
公开(公告)日：2012-12-04
申请号：US12968699
申请日：2010-12-15
CPC分类号： B01D71/024 , B01D53/228 , B01D69/12 , B01D2325/021 , B01D2325/10 , C01B13/0255 , C01B2210/0046
摘要： A composite oxygen transport membrane having a dense layer, a porous support layer and an intermediate porous layer located between the dense layer and the porous support layer. Both the dense layer and the intermediate porous layer are formed from an ionic conductive material to conduct oxygen ions and an electrically conductive material to conduct electrons. The porous support layer has a high permeability, high porosity, and a high average pore diameter and the intermediate porous layer has a lower permeability and lower pore diameter than the porous support layer. Catalyst particles selected to promote oxidation of a combustible substance are located in the intermediate porous layer and in the porous support adjacent to the intermediate porous layer. The catalyst particles can be formed by wicking a solution of catalyst precursors through the porous support toward the intermediate porous layer.
摘要翻译： 一种复合氧传输膜，其具有致密层，多孔载体层和位于致密层和多孔载体层之间的中间多孔层。 致密层和中间多孔层都由离子导电材料形成以导电氧离子和导电材料以导电。 多孔支撑层具有高渗透性，高孔隙率和高平均孔径，并且中间多孔层具有比多孔载体层更低的渗透性和更低的孔直径。 被选择用于促进可燃物质的氧化的催化剂颗粒位于中间多孔层和邻近中间多孔层的多孔载体中。 可以通过将催化剂前体的溶液通过多孔载体向中间多孔层芯吸而形成催化剂颗粒。
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公开(公告)号：US07556676B2
公开(公告)日：2009-07-07
申请号：US11507486
申请日：2006-08-22
申请人： Nagendra Nagabhushana , Jonathan Andrew Lane , Gervase Maxwell Christie , Bart Antonie van Hassel
发明人： Nagendra Nagabhushana , Jonathan Andrew Lane , Gervase Maxwell Christie , Bart Antonie van Hassel
IPC分类号： B01D53/22
CPC分类号： H01M4/8621 , B01D53/228 , B01D69/12 , B01D69/141 , B01D71/02 , B01D2257/104 , B01D2323/12 , B01D2325/02 , B01D2325/04 , B01D2325/26 , C01B13/0255 , C04B35/42 , C04B35/486 , C04B35/488 , C04B35/636 , C04B38/00 , C04B2111/00612 , C04B2111/00801 , C04B2235/3213 , C04B2235/3224 , C04B2235/3225 , C04B2235/3227 , C04B2235/3229 , C04B2235/3239 , C04B2235/3243 , C04B2235/3246 , C04B2235/3262 , C04B2235/3275 , C04B2235/422 , C04B2235/5445 , C04B2235/77 , C04B2235/80 , H01M4/8657 , H01M4/9016 , H01M4/9025 , H01M8/1246 , H01M8/1253 , H01M8/126 , H01M2300/0074 , H01M2300/0077 , H01M2300/0094 , Y02E60/525 , Y02P70/56 , C04B35/48 , C04B38/0054 , C04B38/0074
摘要： A composite oxygen ion transport membrane having a dense layer, a porous support layer, an optional intermediate porous layer located between the porous support layer and the dense layer and an optional surface exchange layer, overlying the dense layer. The dense layer has electronic and ionic phases. The ionic phase is composed of scandia doped, yttrium or cerium stabilized zirconia. The electronic phase is composed of a metallic oxide containing lanthanum, strontium, chromium, manganese and vanadium and optionally cerium. The porous support layer is composed of zirconia partially stabilized with yttrium, scandium, aluminum or cerium or mixtures thereof. The intermediate porous layer, if used, contains the same ionic and electronic phases as the dense layer. The surface exchange layer is formed of an electronic phase of a metallic oxide of lanthanum and strontium that also contains either manganese or iron and an ionic phase of scandia doped zirconia stabilized with yttrium or cerium.
摘要翻译： 具有致密层的复合氧离子传输膜，多孔载体层，位于多孔载体层和致密层之间的任选的中间多孔层和覆盖致密层的任选的表面交换层。 致密层具有电子和离子相。 离子相由掺杂钪，钇或铈稳定的氧化锆组成。 电子相由含有镧，锶，铬，锰和钒的金属氧化物和任选的铈组成。 多孔支撑层由用钇，钪，铝或铈部分稳定的氧化锆或其混合物组成。 如果使用中间多孔层，则包含与致密层相同的离子和电子相。 表面交换层由还含有锰或铁的镧和锶金属氧化物的电子相以及用钇或铈稳定的掺杂氧化钪的离子相形成。
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公开(公告)号：US20080047431A1
公开(公告)日：2008-02-28
申请号：US11507486
申请日：2006-08-22
申请人： Nagendra Nagabhushana , Jonathan Andrew Lane , Gervase Maxwell Christie , Bart Antonie van Hassel
发明人： Nagendra Nagabhushana , Jonathan Andrew Lane , Gervase Maxwell Christie , Bart Antonie van Hassel
IPC分类号： B01D53/22
CPC分类号： H01M4/8621 , B01D53/228 , B01D69/12 , B01D69/141 , B01D71/02 , B01D2257/104 , B01D2323/12 , B01D2325/02 , B01D2325/04 , B01D2325/26 , C01B13/0255 , C04B35/42 , C04B35/486 , C04B35/488 , C04B35/636 , C04B38/00 , C04B2111/00612 , C04B2111/00801 , C04B2235/3213 , C04B2235/3224 , C04B2235/3225 , C04B2235/3227 , C04B2235/3229 , C04B2235/3239 , C04B2235/3243 , C04B2235/3246 , C04B2235/3262 , C04B2235/3275 , C04B2235/422 , C04B2235/5445 , C04B2235/77 , C04B2235/80 , H01M4/8657 , H01M4/9016 , H01M4/9025 , H01M8/1246 , H01M8/1253 , H01M8/126 , H01M2300/0074 , H01M2300/0077 , H01M2300/0094 , Y02E60/525 , Y02P70/56 , C04B35/48 , C04B38/0054 , C04B38/0074
摘要： A composite oxygen ion transport membrane having a dense layer, a porous support layer, an optional intermediate porous layer located between the porous support layer and the dense layer and an optional surface exchange layer, overlying the dense layer. The dense layer has electronic and ionic phases. The ionic phase is composed of scandia doped, yttrium or cerium stabilized zirconia. The electronic phase is composed of a metallic oxide containing lanthanum, strontium, chromium, manganese and vanadium and optionally cerium. The porous support layer is composed of zirconia partially stabilized with yttrium, scandium, aluminum or cerium or mixtures thereof. The intermediate porous layer, if used, contains the same ionic and electronic phases as the dense layer. The surface exchange layer is formed of an electronic phase of a metallic oxide of lanthanum and strontium that also contains either manganese or iron and an ionic phase of scandia doped zirconia stabilized with yttrium or cerium.
摘要翻译： 具有致密层的复合氧离子传输膜，多孔载体层，位于多孔载体层和致密层之间的任选的中间多孔层和覆盖致密层的任选的表面交换层。 致密层具有电子和离子相。 离子相由掺杂钪，钇或铈稳定的氧化锆组成。 电子相由含有镧，锶，铬，锰和钒的金属氧化物和任选的铈组成。 多孔支撑层由用钇，钪，铝或铈部分稳定的氧化锆或其混合物组成。 如果使用中间多孔层，则包含与致密层相同的离子和电子相。 表面交换层由还含有锰或铁的镧和锶金属氧化物的电子相以及用钇或铈稳定的掺杂氧化钪的离子相形成。
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公开(公告)号：US20110180399A1
公开(公告)日：2011-07-28
申请号：US12968699
申请日：2010-12-15
CPC分类号： B01D71/024 , B01D53/228 , B01D69/12 , B01D2325/021 , B01D2325/10 , C01B13/0255 , C01B2210/0046
摘要： A composite oxygen transport membrane having a dense layer, a porous support layer and an intermediate porous layer located between the dense layer and the porous support layer. Both the dense layer and the intermediate porous layer are formed from an ionic conductive material to conduct oxygen ions and an electrically conductive material to conduct electrons. The porous support layer has a high permeability, high porosity, and a high average pore diameter and the intermediate porous layer has a lower permeability and lower pore diameter than the porous support layer. Catalyst particles selected to promote oxidation of a combustible substance are located in the intermediate porous layer and in the porous support adjacent to the intermediate porous layer. The catalyst particles can be formed by wicking a solution of catalyst precursors through the porous support toward the intermediate porous layer.
摘要翻译： 一种复合氧传输膜，其具有致密层，多孔载体层和位于致密层和多孔载体层之间的中间多孔层。 致密层和中间多孔层都由离子导电材料形成以导电氧离子和导电材料以导电。 多孔支撑层具有高渗透性，高孔隙率和高平均孔径，并且中间多孔层具有比多孔载体层更低的渗透性和更低的孔直径。 被选择用于促进可燃物质的氧化的催化剂颗粒位于中间多孔层和邻近中间多孔层的多孔载体中。 可以通过将催化剂前体的溶液通过多孔载体向中间多孔层芯吸而形成催化剂颗粒。
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公开(公告)号：US09486765B2
公开(公告)日：2016-11-08
申请号：US14508344
申请日：2014-10-07
申请人： Sean M. Kelly , Gervase Maxwell Christie , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
发明人： Sean M. Kelly , Gervase Maxwell Christie , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
IPC分类号： B01J7/00 , B01J8/00 , F22B1/00 , F22B1/16 , B01J8/06 , B01J12/00 , B01J19/24 , C01B3/38 , C01B13/02
CPC分类号： B01J8/009 , B01J8/065 , B01J8/067 , B01J12/007 , B01J19/242 , B01J19/2425 , B01J19/243 , B01J19/2475 , B01J2208/00309 , B01J2208/00938 , B01J2219/00006 , B01J2219/0004 , B01J2219/0006 , B01J2219/00117 , C01B3/382 , C01B3/384 , C01B13/0255 , C01B2203/0233 , C01B2203/0244 , C01B2203/0894 , C01B2203/127 , F22B1/003 , F22B1/16 , Y02P20/129
摘要： The invention relates to a commercially viable modular ceramic oxygen transport membrane reforming reactor configured using repeating assemblies of oxygen transport membrane tubes and catalytic reforming reactors.
摘要翻译： 本发明涉及一种商业上可行的模块化陶瓷氧传输膜重整反应器，其配置为使用氧传输膜管和催化重整反应器的重复组件。
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公开(公告)号：US20150098872A1
公开(公告)日：2015-04-09
申请号：US14508297
申请日：2014-10-07
申请人： Sean M. Kelly , Gervase Maxwell Christie , Lee J. Rosen , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
发明人： Sean M. Kelly , Gervase Maxwell Christie , Lee J. Rosen , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
IPC分类号： B01J8/00
CPC分类号： B01J8/009 , B01J8/065 , B01J8/067 , B01J12/007 , B01J19/242 , B01J19/2425 , B01J19/243 , B01J19/2475 , B01J2208/00309 , B01J2208/00938 , B01J2219/00006 , B01J2219/0004 , B01J2219/0006 , B01J2219/00117 , C01B3/382 , C01B3/384 , C01B13/0255 , C01B2203/0233 , C01B2203/0244 , C01B2203/0894 , C01B2203/127 , F22B1/003 , F22B1/16 , Y02P20/129
摘要： A commercially viable modular ceramic oxygen transport membrane reforming reactor for producing a synthesis gas that improves the thermal coupling of reactively-driven oxygen transport membrane tubes and catalyst reforming tubes required to efficiently and effectively produce synthesis gas.
摘要翻译： 一种用于生产合成气的商业可行的模块化陶瓷氧传输膜重整反应器，其改善了有效且有效地产生合成气所需的反应驱动的氧气输送膜管和催化剂重整管的热偶合。
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