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公开(公告)号：US09908093B2
公开(公告)日：2018-03-06
申请号：US12420942
申请日：2009-04-09
IPC分类号： B01J19/00 , C01B3/22 , C01B3/32 , C01B3/50 , C01B3/52 , C01B3/56 , C07C1/04 , C07C1/20 , C07C2/84 , C07C9/06 , C07C11/04 , C07C29/152 , C10J3/00
CPC分类号： B01J19/0093 , B01J2219/00835 , B01J2219/00846 , B01J2219/0086 , B01J2219/00873 , B01J2219/00918 , B01J2219/00921 , B01J2219/00984 , C01B3/22 , C01B3/32 , C01B3/501 , C01B3/52 , C01B3/56 , C01B2203/0205 , C01B2203/0266 , C01B2203/0405 , C01B2203/0415 , C01B2203/042 , C01B2203/043 , C01B2203/0465 , C01B2203/0475 , C01B2203/0485 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/0838 , C01B2203/0883 , C01B2203/1217 , C01B2203/84 , C07C1/04 , C07C1/20 , C07C2/84 , C07C9/06 , C07C11/04 , C07C29/152 , C07C2529/85 , C10J3/00 , C10J2300/1662 , C10J2300/1665 , Y02E50/18 , Y02E50/32 , Y02E50/346 , Y02P30/42 , C07C9/04 , C07C11/02 , C07C31/04
摘要： This invention relates to a process for converting a carbonaceous material to a desired product comprising methane, methanol and/or dimethyl ether, the process comprising: gasifying the carbonaceous material at a temperature in excess of about 700° C. to form synthesis gas; and flowing the synthesis gas through two or more reaction zones in a microchannel reactor to convert the synthesis gas to the desired product.
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22.发明授权Process for upgrading a carbonaceous material using microchannel process technology 有权使用微通道工艺技术升级碳质材料的工艺公开(公告)号：US08100996B2
公开(公告)日：2012-01-24
申请号：US12421007
申请日：2009-04-09
申请人： Wayne W. Simmons , Robert Dwayne Litt , Anna Lee Tonkovich , Laura J. Silva , Daniel Francis Ryan , Bruce Stangeland , John Brophy , Jeffrey S. McDaniel
发明人： Wayne W. Simmons , Robert Dwayne Litt , Anna Lee Tonkovich , Laura J. Silva , Daniel Francis Ryan , Bruce Stangeland , John Brophy , Jeffrey S. McDaniel
CPC分类号： C01B3/34 , C01B3/56 , C01B13/0259 , C01B13/0277 , C01B2203/0233 , C01B2203/0238 , C01B2203/043 , C01B2203/0465 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/0495 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/0827 , C01B2203/1241 , C01B2203/148 , C01B2203/84 , C01B2210/0046 , C10J3/00 , C10J3/57 , C10J2300/0916 , C10J2300/092 , C10J2300/1659 , C10K3/02 , Y02E50/32 , Y02E50/346 , Y02P20/145
摘要： This invention relates to a process for converting a carbonaceous material to a desired product comprising one or more hydrocarbons or one or more alcohols, the process comprising: (A) gasifying the carbonaceous material at a temperature in excess of about 700° C. to form synthesis gas; and (B) flowing the synthesis gas in a microchannel reactor in contact with a catalyst to convert the synthesis gas to the desired product.
摘要翻译： 本发明涉及将碳质材料转化成包含一种或多种烃或一种或多种醇的所需产物的方法，该方法包括：（A）在超过约700℃的温度下气化碳质材料，以形成 合成气; 和（B）使合成气在与催化剂接触的微通道反应器中流动以将合成气转化为所需产物。
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23.发明申请PROCESS FOR UPGRADING A CARBONACEOUS MATERIAL USING MICROCHANNEL PROCESS TECHNOLOGY 有权使用微通道工艺技术升级碳材料的方法公开(公告)号：US20090293359A1
公开(公告)日：2009-12-03
申请号：US12421007
申请日：2009-04-09
申请人： Wayne W. Simmons , Robert Dwayne Litt , Anna Lee Tonkovich , Laura J. Silva , Daniel Francis Ryan , Bruce Stangeland , John Brophy , Jeffrey S. McDaniel
发明人： Wayne W. Simmons , Robert Dwayne Litt , Anna Lee Tonkovich , Laura J. Silva , Daniel Francis Ryan , Bruce Stangeland , John Brophy , Jeffrey S. McDaniel
IPC分类号： C10J3/46
CPC分类号： C01B3/34 , C01B3/56 , C01B13/0259 , C01B13/0277 , C01B2203/0233 , C01B2203/0238 , C01B2203/043 , C01B2203/0465 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/0495 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/0827 , C01B2203/1241 , C01B2203/148 , C01B2203/84 , C01B2210/0046 , C10J3/00 , C10J3/57 , C10J2300/0916 , C10J2300/092 , C10J2300/1659 , C10K3/02 , Y02E50/32 , Y02E50/346 , Y02P20/145
摘要： This invention relates to a process for converting a carbonaceous material to a desired product comprising one or more hydrocarbons or one or more alcohols, the process comprising: (A) gasifying the carbonaceous material at a temperature in excess of about 700° C. to form synthesis gas; and (B) flowing the synthesis gas in a microchannel reactor in contact with a catalyst to convert the synthesis gas to the desired product.
摘要翻译： 本发明涉及将碳质材料转化成包含一种或多种烃或一种或多种醇的所需产物的方法，该方法包括：（A）在超过约700℃的温度下气化碳质材料，以形成 合成气; 和（B）使合成气在与催化剂接触的微通道反应器中流动以将合成气转化为所需产物。
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24.发明申请PROCESS FOR CONVERTING A CARBONACEOUS MATERIAL TO METHANE, METHANOL AND/OR DIMETHYL ETHER USING MICROCHANNEL PROCESS TECHNOLOGY 有权使用微通道工艺技术将碳质材料转化成甲醇，甲醇和/或二甲醚的方法公开(公告)号：US20090259076A1
公开(公告)日：2009-10-15
申请号：US12420942
申请日：2009-04-09
CPC分类号： B01J19/0093 , B01J2219/00835 , B01J2219/00846 , B01J2219/0086 , B01J2219/00873 , B01J2219/00918 , B01J2219/00921 , B01J2219/00984 , C01B3/22 , C01B3/32 , C01B3/501 , C01B3/52 , C01B3/56 , C01B2203/0205 , C01B2203/0266 , C01B2203/0405 , C01B2203/0415 , C01B2203/042 , C01B2203/043 , C01B2203/0465 , C01B2203/0475 , C01B2203/0485 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/0838 , C01B2203/0883 , C01B2203/1217 , C01B2203/84 , C07C1/04 , C07C1/20 , C07C2/84 , C07C9/06 , C07C11/04 , C07C29/152 , C07C2529/85 , C10J3/00 , C10J2300/1662 , C10J2300/1665 , Y02E50/18 , Y02E50/32 , Y02E50/346 , Y02P30/42 , C07C9/04 , C07C11/02 , C07C31/04
摘要： This invention relates to a process for converting a carbonaceous material to a desired product comprising methane, methanol and/or dimethyl ether, the process comprising: gasifying the carbonaceous material at a temperature in excess of about 700° C. to form synthesis gas; and flowing the synthesis gas through two or more reaction zones in a microchannel reactor to convert the synthesis gas to the desired product.
摘要翻译： 本发明涉及将碳质材料转化成包含甲烷，甲醇和/或二甲醚的所需产物的方法，该方法包括：在超过约700℃的温度下气化碳质材料以形成合成气; 并使合成气在微通道反应器中流过两个或更多个反应区，以将合成气转化为所需产物。
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25.发明授权Methods for applying microchannels to separate gases using liquid absorbents, especially ionic liquid (IL) absorbents 有权使用液体吸收剂，特别是离子液体（IL）吸收剂应用微通道分离气体的方法公开(公告)号：US08221528B2
公开(公告)日：2012-07-17
申请号：US12184877
申请日：2008-08-01
申请人： Anna Lee Y. Tonkovich , Robert D. Litt , Ravi Arora , Qiu Dongming , Micheal Jay Lamont , Maddalena Fanelli , Wayne W. Simmons , Laura J. Silva , Steven Perry
发明人： Anna Lee Y. Tonkovich , Robert D. Litt , Ravi Arora , Qiu Dongming , Micheal Jay Lamont , Maddalena Fanelli , Wayne W. Simmons , Laura J. Silva , Steven Perry
IPC分类号： B01D53/14
CPC分类号： C01B3/52 , B01D53/1493 , B01D53/18 , B01D2256/10 , B01D2256/24 , B01D2257/102 , B01D2257/104 , B01D2257/304 , B01D2257/306 , B01D2257/406 , B01D2257/702 , B01J2219/00047 , C01B13/0285 , C01B2203/0415 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/86 , C01B2210/0046 , C10G2/32 , C10G2300/1025 , C10G2300/202 , C10G2300/207 , C10G2300/805 , Y02P30/30
摘要： Methods of using microchannel separation systems including absorbents to improve thermal efficiency and reduce parasitic power loss. Energy is typically added to desorb a solute and then energy or heat is removed to absorb a solute using a working solution. The working solution or absorbent may comprise an ionic liquid, or other fluids that demonstrate a difference in affinity between a solute and other gases in a solution.
摘要翻译： 使用包括吸收剂在内的微通道分离系统来提高热效率并降低寄生功率损耗的方法。 通常加入能量以解吸溶质，然后除去能量或热量以使用工作溶液吸收溶质。 工作溶液或吸收剂可以包括离子液体或证明溶质与溶液中的其它气体之间的亲和力差异的其它流体。
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26.发明申请METHODS FOR APPLYING MICROCHANNELS TO SEPARATE GASES USING LIQUID ABSORBENTS, ESPECIALLY IONIC LIQUID (IL) ABSORBENTS 有权使用液体吸收剂，特别是离子液体（IL）吸收剂将微通道应用于分离气体的方法公开(公告)号：US20100024645A1
公开(公告)日：2010-02-04
申请号：US12184877
申请日：2008-08-01
申请人： Anna Lee Y. Tonkovich , Robert D. Litt , Ravi Arora , Qiu Dongming , Micheal Jay Lamont , Maddalena Fanelli , Wayne W. Simmons , Laura J. Silva , Steven Perry
发明人： Anna Lee Y. Tonkovich , Robert D. Litt , Ravi Arora , Qiu Dongming , Micheal Jay Lamont , Maddalena Fanelli , Wayne W. Simmons , Laura J. Silva , Steven Perry
CPC分类号： C01B3/52 , B01D53/1493 , B01D53/18 , B01D2256/10 , B01D2256/24 , B01D2257/102 , B01D2257/104 , B01D2257/304 , B01D2257/306 , B01D2257/406 , B01D2257/702 , B01J2219/00047 , C01B13/0285 , C01B2203/0415 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/86 , C01B2210/0046 , C10G2/32 , C10G2300/1025 , C10G2300/202 , C10G2300/207 , C10G2300/805 , Y02P30/30
摘要： Methods of using microchannel separation systems including absorbents to improve thermal efficiency and reduce parasitic power loss. Energy is typically added to desorb a solute and then energy or heat is removed to absorb a solute using a working solution. The working solution or absorbent may comprise an ionic liquid, or other fluids that demonstrate a difference in affinity between a solute and other gases in a solution.
摘要翻译： 使用包括吸收剂在内的微通道分离系统来提高热效率并降低寄生功率损耗的方法。 通常加入能量以解吸溶质，然后除去能量或热量以使用工作溶液吸收溶质。 工作溶液或吸收剂可以包括离子液体或证明溶质与溶液中的其它气体之间的亲和力差异的其它流体。
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27.发明申请PROCESS AND APPARATUS FOR CONVERTING NATURAL GAS TO HIGHER MOLECULAR WEIGHT HYDROCARBONS USING MICROCHANNEL PROCESS TECHNOLOGY 有权使用微通道工艺技术将天然气转化为更高分子量烃的工艺和装置公开(公告)号：US20080210596A1
公开(公告)日：2008-09-04
申请号：US12016250
申请日：2008-01-18
CPC分类号： C10G2/341 , B01J19/0093 , B01J23/40 , B01J23/74 , B01J23/75 , B01J23/8896 , B01J23/8913 , B01J35/04 , B01J37/0225 , B01J2219/00788 , B01J2219/0081 , B01J2219/00835 , B01J2219/00867 , B01J2219/00873 , C01B3/382 , C01B3/384 , C01B2203/0233 , C01B2203/0405 , C01B2203/043 , C01B2203/062 , C01B2203/0822 , C01B2203/0827 , C01B2203/1041 , C01B2203/1047 , C01B2203/1058 , C01B2203/107 , C01B2203/1241 , C01B2203/142 , C01B2203/148 , C10G2/334 , C10G2300/1022 , C10G2300/807 , C10G2400/22 , Y02P20/128 , Y02P20/52
摘要： The disclosed invention relates to a process and apparatus for converting natural gas to higher molecular weight hydrocarbons. The process includes steam reforming to form synthesis gas followed by a Fischer-Tropsch reaction to convert the synthesis gas to the high molecular weight hydrocarbons. The reforming and Fischer-Tropsch reactions are conducted in microchannel reactors. The higher molecular weight hydrocarbons may be further treated to form hydrocarbon products such as middle distillate fuels, lubricating oils, and the like. The apparatus includes vessels containing SMR microchannel reactors and Fischer-Tropsch microchannel reactors. A composition comprising a mixture of olefins and paraffins is disclosed.
摘要翻译： 所公开的发明涉及将天然气转化为较高分子量烃的方法和装置。 该方法包括蒸汽重整以形成合成气，然后进行费 - 托反应，将合成气转化为高分子量烃。 重整和费 - 托反应在微通道反应器中进行。 可以进一步处理较高分子量的烃以形成烃产物，例如中间馏分燃料，润滑油等。 该装置包括容纳SMR微通道反应器和费 - 托微通道反应器的容器。 公开了包含烯烃和链烷烃的混合物的组合物。
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公开(公告)号：US09663363B2
公开(公告)日：2017-05-30
申请号：US13429794
申请日：2012-03-26
CPC分类号： C01B3/384 , C01B2203/0233 , C01B2203/061 , C01B2203/0811 , C01B2203/1241 , C01B2203/169 , C10J3/485 , C10J3/506 , C10J3/62 , C10J3/84 , C10J2300/0916 , C10J2300/1223 , C10J2300/1621 , C10J2300/1665 , C10J2300/1853 , C10K1/003 , Y02E50/18 , Y02P20/145 , Y02T50/678
摘要： A multiple stage synthesis gas generation system is disclosed including a high radiant heat flux reactor, a gasifier reactor control system, and a Steam Methane Reformer (SMR) reactor. The SMR reactor is in parallel and cooperates with the high radiant heat flux reactor to produce a high quality syngas mixture for MeOH synthesis. The resultant products from the two reactors may be used for the MeOH synthesis. The SMR provides hydrogen rich syngas to be mixed with the potentially carbon monoxide rich syngas from the high radiant heat flux reactor. The combination of syngas component streams from the two reactors can provide the required hydrogen to carbon monoxide ratio for methanol synthesis. The SMR reactor control system and a gasifier reactor control system interact to produce a high quality syngas mixture for the MeOH synthesis.
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29.发明授权Various methods and apparatuses for an ultra-high heat flux chemical reactor 有权用于超高热通量化学反应器的各种方法和装置公开(公告)号：US09011560B2
公开(公告)日：2015-04-21
申请号：US13254020
申请日：2010-12-08
申请人： Wayne W. Simmons , Christopher Perkins , Zoran Jovanovic , Courtland M. Hilton , Peter Popp , Bryan J. Schramm , John T. Turner
发明人： Wayne W. Simmons , Christopher Perkins , Zoran Jovanovic , Courtland M. Hilton , Peter Popp , Bryan J. Schramm , John T. Turner
CPC分类号： C07C29/152 , C01B3/24 , C01B3/34 , C01B2203/0216 , C01B2203/0222 , C01B2203/0272 , C01B2203/0485 , C01B2203/0495 , C01B2203/061 , C01B2203/062 , C01B2203/0816 , C01B2203/0822 , C01B2203/0877 , C01B2203/0894 , C01B2203/1241 , C10G2300/1011 , C10G2300/807 , C10G2400/02 , C10J3/485 , C10J3/506 , C10J3/84 , C10J2200/152 , C10J2300/0906 , C10J2300/0909 , C10J2300/0916 , C10J2300/0976 , C10J2300/0989 , C10J2300/1223 , C10J2300/1246 , C10J2300/1269 , C10J2300/1292 , C10J2300/1621 , C10J2300/1665 , C10J2300/1687 , C10J2300/1693 , C10J2300/1884 , C10J2300/1892 , F28D2021/0022 , Y02E50/18 , Y02P20/128 , Y02P20/129 , Y02P20/134 , Y02P20/145 , Y02P30/20 , C07C31/04
摘要： Various processes and apparatus are discussed for an ultra-high heat flux chemical reactor. A thermal receiver and the reactor tubes are aligned to 1) absorb and re-emit radiant energy, 2) highly reflect radiant energy, and 3) any combination of these, to maintain an operational temperature of the enclosed ultra-high heat flux chemical reactor. Particles of biomass are gasified in the presence of a steam carrier gas and methane in a simultaneous steam reformation and steam biomass gasification reaction to produce reaction products that include hydrogen and carbon monoxide gas using the ultra-high heat flux thermal energy radiated from the inner wall and then into the multiple reactor tubes. The multiple reactor tubes and cavity walls of the receiver transfer energy primarily by radiation absorption and re-radiation, rather than by convection or conduction, to the reactants in the chemical reaction to drive the endothermic chemical reaction flowing in the reactor tubes.
摘要翻译： 讨论了超高热通量化学反应器的各种工艺和装置。 热接收器和反应器管对齐为1）吸收并重新发射辐射能，2）高度反射辐射能，3）任何组合，以保持封闭的超高热通量化学反应器的工作温度 。 生物质颗粒在蒸汽载体气体和甲烷的存在下在同时蒸汽重整和蒸汽生物质气化反应中气化，以产生包含氢气和一氧化碳气体的反应产物，使用从内壁辐射的超高热通量热能 然后进入多个反应管。 接收器的多个反应器管和空腔壁主要通过辐射吸收和再辐射而不是通过对流或传导将能量转移到化学反应中的反应物以驱动在反应器管中流动的吸热化学反应。
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公开(公告)号：US08961628B2
公开(公告)日：2015-02-24
申请号：US13531318
申请日：2012-06-22
IPC分类号： B01J7/00
CPC分类号： C07C29/1518 , C10G2300/1014 , C10G2300/1022 , C10G2400/04 , C10G2400/22 , C10J3/485 , C10J2300/0906 , C10J2300/0909 , C10J2300/0916 , C10J2300/092 , C10J2300/0976 , C10J2300/1223 , C10J2300/1665 , C10J2300/1853 , C10K3/02 , C10L9/083 , D21C1/02 , Y02E50/15 , Y02E50/18 , Y02P20/145 , Y02P30/20 , C07C31/04
摘要： An integrated plant that includes a steam explosion process unit and biomass gasifier to generate syngas from biomass. A steam explosion process unit applies a combination of heat, pressure, and moisture to the biomass to make the biomass into a moist fine particle form. The steam explosion process unit applies steam with a high pressure to heat and pressurize any gases and fluids present inside the biomass to internally blow apart the bulk structure of the biomass via a rapid depressurization of the biomass with the increased moisture content. Those produced moist fine particles of biomass are subsequently fed to a feed section of the biomass gasifier, which reacts the biomass particles in a rapid biomass gasification reaction to produce syngas components.
摘要翻译： 一个综合工厂，其中包括蒸汽爆炸处理装置和生物质气化器，以从生物质产生合成气。 蒸汽爆炸处理单元将热量，压力和水分的组合应用于生物质，以使生物质成为潮湿的细颗粒形式。 蒸汽爆炸过程单元应用高压蒸汽来对生物质内存在的任何气体和流体进行加压并对其进行加压，以通过具有增加的水分含量的生物质的快速减压来内部吹散生物质的本体结构。 产生生物质的湿细颗粒的产物随后被送入生物质气化器的进料部分，其使生物质颗粒在快速的生物质气化反应中反应以产生合成气组分。
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