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    Catalyst Regeneration Process
    52.
    发明申请
    Catalyst Regeneration Process 有权
    催化剂再生过程

    公开(公告)号：US20100298117A1

    公开(公告)日：2010-11-25

    申请号：US12738057

    申请日：2008-11-04

    Applicant: Doron Levin ,  James Harding Beech, JR. ,  Selma SheungNam Kwok ,  Julia Elizabeth Steinheider

    Inventor： Doron Levin ,  James Harding Beech, JR. ,  Selma SheungNam Kwok ,  Julia Elizabeth Steinheider

    IPC: B01J38/70

    CPC classification number: B01J29/90 ,  B01J29/06 ,  B01J29/7034 ,  B01J29/74 ,  B01J29/78 ,  B01J38/20 ,  B01J2229/42

    Abstract: This disclosure relates to a process for regenerating a catalyst composition, wherein the catalyst composition comprising a molecular sieve and at least 10 wt. % coke having a C/H ratio in the range of 0.26 to 5, the process comprising (a) contacting the catalyst composition with a first oxidative medium having oxygen and water at first conditions sufficient to form a first regenerated catalyst composition having at least 50 wt. % less coke than the catalyst composition; and then (b) contacting at least a portion of the first regenerated catalyst composition with a second oxidative medium having oxygen, and optionally water, at second conditions sufficient to form a second regenerated catalyst composition having at least 50 wt % less coke than the first regenerated catalyst composition, wherein the catalyst composition in step (a) and the first regenerated catalyst in step (b) have contacted total amount of water in the range of 1 to 50 weight water per weight of the second regenerated catalyst composition.

    Abstract translation: 本公开涉及一种再生催化剂组合物的方法，其中所述催化剂组合物包含分子筛和至少10重量％ ％C / H比在0.26至5范围内的方法，该方法包括（a）在足以形成第一再生催化剂组合物的第一条件下使催化剂组合物与具有氧和水的第一氧化介质接触，所述第一再生催化剂组合物具有至少50 重量 比催化剂组合物少少的焦炭; 然后（b）在足以形成第二再生催化剂组合物的第二条件下使至少一部分第一再生催化剂组合物与具有氧的第二氧化介质和任选的水接触，所述第二再生催化剂组合物的焦炭比第一再生催化剂组合物少至少50重量％ 再生催化剂组合物，其中步骤（a）中的催化剂组合物和步骤（b）中的第一再生催化剂已经接触每重量第二再生催化剂组合物的1至50重量％水的总量。

    Processes for converting oxygenates to olefins using aluminosilicate catalysts
    53.
    发明授权
    Processes for converting oxygenates to olefins using aluminosilicate catalysts 有权
    使用硅铝酸盐催化剂将含氧化合物转化为烯烃的方法

    公开(公告)号：US07829751B2

    公开(公告)日：2010-11-09

    申请号：US11855476

    申请日：2007-09-14

    Applicant: Doron Levin ,  Richard B. Hall

    Inventor： Doron Levin ,  Richard B. Hall

    IPC: C07C1/00

    CPC classification number: C07C1/20 ,  C07C2523/10 ,  C07C2529/85 ,  C07C2529/89 ,  Y02P30/42 ,  C07C11/06 ,  C07C11/04 ,  C07C11/08

    Abstract: The present invention relates to processes for forming mixed alcohols containing methanol and ethanol. The mixed alcohol can then be used as a feedstock for an oxygenate to olefin reaction system for conversion thereof to ethylene, propylene, and the like. In addition, the olefins produced by the oxygenate to olefin reaction can then be used as monomers for a polymerization of olefin-containing polymers and/or oligomers.

    Abstract translation: 本发明涉及形成含有甲醇和乙醇的混合醇的方法。 然后可以将混合的醇用作用于将其转化成乙烯，丙烯等的含氧化合物至烯烃反应体系的原料。 此外，由含氧化合物与烯烃反应产生的烯烃然后可以用作含烯烃聚合物和/或低聚物聚合的单体。

    Method of high pressure and high capacity oxygenate conversion with catalyst exposure cycle
    54.
    发明授权
    Method of high pressure and high capacity oxygenate conversion with catalyst exposure cycle 有权
    用催化剂曝光循环的高压和高容量含氧化合物转化方法

    公开(公告)号：US07763765B2

    公开(公告)日：2010-07-27

    申请号：US11698511

    申请日：2007-01-26

    Applicant: Keith H. Kuechler ,  James H. Beech ,  Doron Levin ,  Stephen N. Vaughn ,  Stephen H. Brown

    Inventor： Keith H. Kuechler ,  James H. Beech ,  Doron Levin ,  Stephen N. Vaughn ,  Stephen H. Brown

    IPC: C07C1/00

    CPC classification number: C07C1/20 ,  B01J29/90 ,  B01J38/06 ,  C07C2529/85 ,  C08F10/00 ,  C10G3/49 ,  C10G3/57 ,  C10G3/62 ,  C10G2300/308 ,  C10G2300/4012 ,  C10G2300/4018 ,  C10G2300/802 ,  C10G2300/805 ,  C10G2400/20 ,  Y02P20/584 ,  Y02P30/20 ,  Y02P30/42 ,  C07C11/02 ,  C08F2/00

    Abstract: A gas-solids reaction system is provided for improving product recovery in a multiple reactor reaction system. An oxygenate feedstock, desirably of high concentration in oxygenate, is reacted with a catalyst having a low to modest acidity and a Si/Al2 ratio of from 0.10 to 0.32. The reaction occurs in a reaction zone of a fluidized bed reactor at an oxygenate partial pressure of at least 45 psia and a reactor gas superficial velocity of at least 10 ft/s, conveying catalyst through the reaction zone to a circulation zone. The catalyst undergoes displacement with an inert gas in the circulation zone at a displacement gas superficial velocity of at least 0.03 m/s, after which at least a portion, preferably a large portion is returned to the reaction zone. The catalyst has a residence time in the circulation zone of at least twice that of the residence time of catalyst in the reaction zone. Extraordinary catalyst activity at high olefin selectivity results despite insignificant changes in coke on catalyst and coke yield when compared to lower pressure operations.

    Abstract translation: 提供了一种气体 - 固体反应系统，用于改善多反应器反应体系中的产物回收。 含氧化合物中期望含有高浓度的含氧化合物原料与低至中等酸度和Si / Al 2比为0.10至0.32的催化剂反应。 反应在流化床反应器的反应区中发生，氧化分压至少为45psia，反应器气体表观速度为至少10ft / s，将催化剂通过反应区输送到循环区。 催化剂在循环区中以惰性气体置换，位移气体空速为至少0.03m / s，此后至少一部分，优选大部分返回到反应区。 催化剂在循环区中的停留时间至少是催化剂在反应区中的停留时间的两倍。 尽管与较低压力操作相比，尽管催化剂上的焦炭和焦炭产率都没有显着变化，但是在高烯烃选择性方面具有特殊的催化剂活性。

    Heavy Aromatics Processing Catalyst and Process of Using the Same
    56.
    发明申请
    Heavy Aromatics Processing Catalyst and Process of Using the Same 有权
    重芳烃加工催化剂及其使用方法

    公开(公告)号：US20100093520A1

    公开(公告)日：2010-04-15

    申请号：US12640742

    申请日：2009-12-17

    Applicant: Doron Levin

    Inventor： Doron Levin

    IPC: B01J29/068 ,  B01J29/44

    CPC classification number: C07C6/126 ,  B01J29/44 ,  B01J29/48 ,  B01J29/7469 ,  B01J29/80 ,  B01J35/0006 ,  B01J35/026 ,  B01J37/18 ,  B01J2229/186 ,  B01J2229/42 ,  C07C2529/44 ,  C07C2529/74 ,  Y02P20/52 ,  C07C15/08

    Abstract: This disclosure relates to a catalyst system adapted for transalkylation a C9+ aromatic feedstock with a C6-C7 aromatic feedstock, comprising: (a) a first catalyst comprising a first molecular sieve having a Constraint Index in the range of 3-12 and 0.01 to 5 wt. % of at least one source of a first metal element of Groups 6-10; and (b) a second catalyst comprising a second molecular sieve having a Constraint Index less than 3 and 0 to 5 wt. % of at least one source of a second metal element of Groups 6-10, wherein the weight ratio of the first catalyst over the second catalyst is in the range of 5:95 to 75:25 and wherein the first catalyst is located in front of the second catalyst when they are brought into contacting with the C9+ aromatic feedstock and the C6-C7 aromatic feedstock in the present of hydrogen.

    Abstract translation: 本公开涉及一种适于使C 9+芳族原料与C 6 -C 7芳族原料进行烷基转移的催化剂体系，其包含：（a）第一催化剂，其包含第一分子筛，其约束指数为3-12和0.01至5 重量 至少一个第6-10族第一金属元素源的％; 和（b）包含第二分子筛的第二催化剂，所述第二分子筛具有小于3和0-5重量％的约束指数。 至少一种第6-10族第二金属元素源的％，其中第一催化剂与第二催化剂的重量比在5:95至75:25的范围内，其中第一催化剂位于前面 的第二催化剂当它们与C9 +芳族原料和当前氢气中的C6-C7芳族原料接触时。

    Processes For Converting Oxygenates To Olefins Using Aluminosilicate Catalysts
    57.
    发明申请
    Processes For Converting Oxygenates To Olefins Using Aluminosilicate Catalysts 有权
    使用硅铝酸盐催化剂将氧化物转化为烯烃的方法

    公开(公告)号：US20080103345A1

    公开(公告)日：2008-05-01

    申请号：US11855476

    申请日：2007-09-14

    Applicant: Doron Levin ,  Richard B. Hall

    Inventor： Doron Levin ,  Richard B. Hall

    IPC: C07C1/00

    CPC classification number: C07C1/20 ,  C07C2523/10 ,  C07C2529/85 ,  C07C2529/89 ,  Y02P30/42 ,  C07C11/06 ,  C07C11/04 ,  C07C11/08

    Abstract: The present invention relates to processes for forming mixed alcohols containing methanol and ethanol. The mixed alcohol can then be used as a feedstock for an oxygenate to olefin reaction system for conversion thereof to ethylene, propylene, and the like. In addition, the olefins produced by the oxygenate to olefin reaction can then be used as monomers for a polymerization of olefin-containing polymers and/or oligomers.

    Abstract translation: 本发明涉及形成含有甲醇和乙醇的混合醇的方法。 然后可以将混合的醇用作用于将其转化成乙烯，丙烯等的含氧化合物至烯烃反应体系的原料。 此外，由含氧化合物与烯烃反应产生的烯烃然后可以用作含烯烃聚合物和/或低聚物聚合的单体。

    High silica chabazite, its synthesis and its use in the conversion of oxygenates to olefins
    59.
    发明申请
    High silica chabazite, its synthesis and its use in the conversion of oxygenates to olefins 有权
    高二氧化硅菱沸石，其合成及其在含氧化合物转化为烯烃的应用

    公开(公告)号：US20070043251A1

    公开(公告)日：2007-02-22

    申请号：US11590230

    申请日：2006-10-31

    Applicant: Karl Strohmaier ,  Sebastian Reyes ,  Doron Levin

    Inventor： Karl Strohmaier ,  Sebastian Reyes ,  Doron Levin

    IPC: C07C1/00

    CPC classification number: B01J29/7015 ,  C01B39/46 ,  C01B39/48 ,  C07C1/20 ,  Y02P30/42 ,  C07C11/02

    Abstract: A porous crystalline material is described having the chabazite framework type and having a composition involving the molar relationship: X2O3:(n)YO2, wherein X is a trivalent element, such as aluminum, boron, iron, indium, and/or gallium; Y is a tetravalent element such as silicon, tin, titanium and/or germanium; and n is greater than 100 and typically greater than 200, such as about 300 to about 4000, for example from about 400 to about 1200. The material is synthesized in a fluoride medium and exhibits activity and selectivity in the conversion of methanol to lower olefins, especially ethylene and propylene.

    Abstract translation: 描述了具有菱沸石骨架类型并且具有摩尔关系的组成的多孔结晶材料：<？in-line-formula description =“In-line Formulas”end =“lead”？> X 2 >○3（n）YO 2，<？in-line-formula description =“In-line Formulas”end =“tail”？>其中X是 三价元素，例如铝，硼，铁，铟和/或镓; Y是四价元素，例如硅，锡，钛和/或锗; 并且n大于100，通常大于200，例如约300至约4000，例如约400至约1200.该物质在氟化物介质中合成，并且在甲醇转化为低级烯烃中表现出活性和选择性 ，特别是乙烯和丙烯。

    Conversion of oxygenates to olefins
    60.
    发明授权
    Conversion of oxygenates to olefins 有权
    含氧化合物转化为烯烃

    公开(公告)号：US07166757B2

    公开(公告)日：2007-01-23

    申请号：US10909014

    申请日：2004-07-30

    Applicant: Shun Chong Fung ,  Doron Levin ,  Jose Santiesteban ,  Nicolas P. Coute

    Inventor： Shun Chong Fung ,  Doron Levin ,  Jose Santiesteban ,  Nicolas P. Coute

    IPC: C07C1/00

    CPC classification number: C07C1/20 ,  B01J23/10 ,  B01J29/85 ,  B01J29/90 ,  B01J38/30 ,  C10G3/42 ,  C10G3/48 ,  C10G3/49 ,  C10G3/57 ,  C10G3/62 ,  C10G2300/708 ,  C10G2400/20 ,  Y02P20/584 ,  Y02P30/20 ,  Y02P30/40 ,  C07C11/02

    Abstract: A process is described for converting an oxygenate-containing feedstock into one or more olefins in which the feedstock is contacted in a reaction zone with a fluidized bed of a particulate catalyst composition comprising a molecular sieve and at least one metal oxide having an uptake of carbon dioxide at 100° C. of at least 0.03 mg/m2 of the metal oxide whereby at least part of the feedstock is converted into a product stream comprising one or more olefins and a carbonaceous material is deposited on the catalyst composition to produce a coked catalyst composition. The coked catalyst composition is separated from the product stream and divided into at least first and second portions. The first portion of the coked catalyst composition is contacted with a regeneration medium in a regeneration zone under conditions to remove at least part of the carbonaceous material from the coked catalyst composition and produce a regenerated catalyst composition, which is subsequently recycled to the reaction zone. The second portion of the coked catalyst composition is also recycled to the reaction zone but without being initially contacted with a regeneration medium.

    Abstract translation: 描述了一种用于将含氧化合物的原料转化成一种或多种烯烃，其中原料在反应区中与包含分子筛和至少一种具有碳吸收性的金属氧化物的颗粒催化剂组合物的流化床接触的烯烃 二氧化碳在100℃下为至少0.03mg / m 2的金属氧化物，由此至少部分原料转化为包含一种或多种烯烃的产物流，并将碳质材料沉积在 用于生产焦化催化剂组合物的催化剂组合物。 将焦炭催化剂组合物与产物流分离并分成至少第一和第二部分。 焦化催化剂组合物的第一部分与再生区中的再生介质接触，在从焦炭催化剂组合物中除去至少一部分碳质材料的条件下，并产生再生催化剂组合物，随后再循环到反应区。 焦炭催化剂组合物的第二部分也被循环到反应区，但不最初与再生介质接触。

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