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公开(公告)号：US5284984A
公开(公告)日：1994-02-08
申请号：US998807
申请日：1992-12-29
摘要： A method for upgrading an aromatics-containing charge composition boiling in the gasoline boiling range comprises i) contacting the charge composition with a nitrating agent under nitrating conditions to form a product comprising nitrated aromatics; ii) hydrogenating a feed containing the product of i) under conditions sufficient to substantially reduce the nitro group of the nitrated aromatics so as to form a product comprising aromatic amines, water and heavy amines; and iii) removing the water and heavy amines from the product of step ii) to provide a gasoline boiling range product of an octane rating greater than the charge composition.
摘要翻译： 一种用于升级汽油沸程沸腾的含芳烃的电荷组分的方法包括：i）在硝化条件下使电荷组合物与硝化剂接触以形成包含硝化芳族化合物的产物; ii）在足以基本上还原硝化芳族化合物的硝基的条件下氢化含有i）产物的进料，以形成包含芳族胺，水和重胺的产物; 和iii）从步骤ii）的产物中除去水和重胺，以提供辛烷值等于大于电荷组成的汽油沸程产物。
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公开(公告)号：US4857664A
公开(公告)日：1989-08-15
申请号：US265324
申请日：1988-10-27
摘要： Olefin undergoes conversion in the presence of water to a mixture of alcohol and ether which is then subjected to various downstream operations including distillation and decantation to provide an ether-rich product containing little if any water. If desired the ether can be combined in any predetermined ratio with co-produced alcohol to provide alcohol/ether mixtures of desired composition. The foregoing process is especially suitable to the conversion of propylene and propylene-containing streams to diisopropyl ether and mixtures of isopropyl alcohol and diisopropyl ether which are useful, inter alia, as octane improves for gasoline.
摘要翻译： 烯烃在水的存在下经历转化为醇和醚的混合物，然后将其进行各种下游操作，包括蒸馏和倾析，以提供含有少量的含有醚的产物。 如果需要，醚可以以任何预定比例与共同产生的醇组合以提供所需组合物的醇/醚混合物。 上述方法特别适用于将丙烯和含丙烯的物流转化为二异丙基醚以及异丙醇和二异丙醚的混合物，特别是对于汽油而言辛烷值改善。
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73.发明授权Integration of paraffin dehydrogenation with MOGD to minimize compression and gas plant separation 失效石蜡脱氢与MOGD的整合使压缩和气体分离最小化
公开(公告)号：US4749820A
公开(公告)日：1988-06-07
申请号：US650594
申请日：1984-09-14
申请人： James C. Kuo , Samuel A. Tabak
发明人： James C. Kuo , Samuel A. Tabak
摘要： Disclosed is a method and apparatus for producing gasoline and distillate grade products which employs integrating catalytic (or thermal) dehydrogenation of paraffins with MOGD to minimize interstage compression and gas plant separation cost. The process cascades the product from a low temperature propane or butane dehydrogenation zone into a first catalytic reactor zone which operates at low pressure and contains zeolite oligomerization catalysts, where the low molecular weight olefins are reacted to primarily gasoline range materials. These gasoline range materials can then be pressurized to the pressure required for reacting to distillate in a second catalytic reactor zone operating at high pressure and containing zeolite oligomerization catalyst. The first catalytic reactor zone also acts to remove the olefins from the dehydrogenation reactor effluent to allow recycle of the unreacted paraffins.
摘要翻译： 公开了用于生产汽油和馏出物级产物的方法和装置，其采用将链烷烃的催化（或热）脱氢与MOGD整合，以最小化级间压缩和气体分离成本。 该方法将产物从低温丙烷或丁烷脱氢区级联到在低压下操作并含有沸石低聚催化剂的第一催化反应器区，其中低分子量烯烃主要与汽油范围材料反应。 然后可以将这些汽油范围的材料加压至在高压下操作并含有沸石低聚催化剂的第二催化反应器区域中与馏出物反应所需的压力。 第一催化反应器区还用于从脱氢反应器流出物中除去烯烃以允许未反应的链烷烃的再循环。
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公开(公告)号：US4717782A
公开(公告)日：1988-01-05
申请号：US893522
申请日：1986-08-05
CPC分类号： C07C2/12 , C07C2529/46 , Y02P20/52
摘要： A continuous catalytic process for converting ethene-rich olefinic feedstock containing reducing gas to heavier liquid hydrocarbon product, comprising the steps ofcontacting the ethene-rich feedstock at elevated temperature in a catalytic reaction zone with a zeolite catalyst comprising a nickel-ethene oligomerization component and a shape-selective medium pore acid zeolite oligomerization component to convert at least a portion of the lower olefinic components to heavier olefinic hydrocarbons; andfeeding water with the feedstock in sufficient amount to prevent substantial reduction of the nickel component.
摘要翻译： 一种用于将含有还原气体的富含烯烃的烯烃原料转化为较重液体烃产物的连续催化方法，包括以下步骤：使催化反应区中升温的富含乙烯的原料与包含镍 - 乙烯低聚组分的沸石催化剂和 形状选择性中孔酸性沸石低聚组分，将至少一部分较低级烯烃组分转化成较重的烯烃; 并用足够量的原料给予原料以防止镍组分的显着减少。
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75.发明授权Multi-stage system for converting oxygenates to liquid hydrocarbons with aliphatic recycle 失效将含氧化合物转化为具有脂肪族循环的液体烃的多级系统
公开(公告)号：US4689205A
公开(公告)日：1987-08-25
申请号：US824473
申请日：1986-01-31
申请人： Ronald M. Gould , Samuel A. Tabak
发明人： Ronald M. Gould , Samuel A. Tabak
CPC分类号： C07C1/20 , C10G3/49 , C10G3/57 , C10G50/00 , B01J2208/00265 , C07C2529/40 , C10G2300/4081 , C10G2400/02 , C10G2400/04 , C10G2400/20 , Y02P20/582 , Y02P30/20
摘要： An apparatus for converting oxygenated feedstock, such as methanol, dimethyl ether or the like, to liquid hydrocarbons. In the primary catalyst stage the feedstock is contacted with a fluidized zeolite catalyst to produce C.sub.2 -C.sub.4 olefins and C.sub.5.sup.+ hydrocarbons. In a secondary catalytic stage with oligomerization catalyst comprising medium-pore shape selective acidic zeolite at increased pressure converts C.sub.3.sup.+ olefins to gasoline and/or distillate liquids. A portion of the recovered gasoline stream is recycled to the fluidized bed at a point above the bed stratum corresponding to substantially complete oxygenate conversion.
摘要翻译： 将含氧原料如甲醇，二甲醚等转化为液体烃的装置。 在主要催化剂阶段，原料与流化沸石催化剂接触以产生C 2 -C 4烯烃和C 5+烃。 在具有增压压力的中孔形选择性酸性沸石的低聚催化剂的二次催化阶段中，将C3 +烯烃转化成汽油和/或馏出液。 回收的汽油流的一部分在床层上方的点上再循环到流化床，对应于基本上完全的含氧化合物转化。
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76.发明授权Multistage process for converting oxygenates to alkylated liquid hydrocarbons 失效将含氧化合物转化为烷基化液体烃的多步法
公开(公告)号：US4628134A
公开(公告)日：1986-12-09
申请号：US779347
申请日：1985-09-23
申请人： Ronald M. Gould , Samuel A. Tabak
发明人： Ronald M. Gould , Samuel A. Tabak
CPC分类号： C07C1/20 , C10G3/49 , C10G50/00 , C07C2527/1206 , C07C2529/06 , C07C2529/40 , C10G2300/4018 , C10G2300/4081 , C10G2300/805 , C10G2400/02 , C10G2400/04 , C10G2400/20 , Y02P20/582 , Y02P30/20 , Y02P30/42
摘要： Alkylate is produced by catalytically converting oxygenate feedstock, such as methanol, to lower olefins comprising C.sub.2 -C.sub.4 olefins. Ethene is separated for recycle and an isoparaffin is alkylated with C.sub.3 -C.sub.4 olefins.
摘要翻译： 烷基化物通过将含氧化合物原料如甲醇催化转化成包含C 2 -C 4烯烃的低级烯烃来制备。 乙烯被分离用于再循环，异链烷烃用C 3 -C 4烯烃烷基化。
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77.发明授权Multistage process for converting oxygenates to liquid hydrocarbons with aliphatic recycle 失效将含氧化合物转化为具有脂肪族循环的液体烃的多阶段过程
公开(公告)号：US4579999A
公开(公告)日：1986-04-01
申请号：US733994
申请日：1985-05-14
申请人： Ronald M. Gould , Samuel A. Tabak
发明人： Ronald M. Gould , Samuel A. Tabak
CPC分类号： C10G50/00 , C07C1/20 , C10G3/49 , B01J2208/00265 , C07C2529/40 , C10G2300/4081 , C10G2400/02 , C10G2400/20 , Y02P20/582 , Y02P20/584 , Y02P30/20
摘要： A process for converting oxygenated feedstock, such as methanol, dimethyl ether or the like, to liquid hydrocarbons.In the primary catalyst stage the feedstock is contacted with zeolite catalyst to produce C.sub.2 -C.sub.4 olefins and C.sub.5.sup.+ hydrocarbons.In a secondary catalytic stage with oligomerization catalyst comprising medium-pore shape selective acidic zeolite at increased pressure converts C.sub.3.sup.+ olefins to gasoline and/or distillate liquids.The improvement is a technique for recovering lower alkene for recycle to the primary catalytic stage.
摘要翻译： 将氧化原料如甲醇，二甲醚等转化成液体烃的方法。 在初级催化剂阶段，原料与沸石催化剂接触以产生C 2 -C 4烯烃和C 5+烃。 在具有增压压力的中孔形选择性酸性沸石的低聚催化剂的二次催化阶段中，将C3 +烯烃转化成汽油和/或馏出液。 该改进是用于回收低级烯烃以再循环到初级催化级的技术。
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公开(公告)号：US4544792A
公开(公告)日：1985-10-01
申请号：US681413
申请日：1984-12-13
申请人： Fritz A. Smith , Samuel A. Tabak
发明人： Fritz A. Smith , Samuel A. Tabak
IPC分类号： C10G57/02 , B01J29/00 , B01J29/06 , C07B61/00 , C07C1/00 , C07C2/00 , C07C2/12 , C07C2/74 , C07C67/00 , C10G3/00 , C10G50/00 , C07C1/20
CPC分类号： C07C2/00 , C07C2/74 , C10G3/49 , C10G3/50 , C10G3/54 , C07C2529/40 , C10G2300/1022 , C10G2300/4006 , C10G2300/4081 , C10G2300/802 , C10G2400/02 , Y02P30/20
摘要： A process for converting olefinic feedstock, such as synthol olefinic liquid product of Fischer-Tropsch synthesis, to distillate hydrocarbons comprising the steps of contacting the feedstock at elevated temperature and pressure with acid zeolite conversion catalyst to oligomerize olefins and convert oxygenated hydrocarbons contained in said light oil at temperatures up to 325.degree. C. and in the presence of H.sub.2, thereby providing an effluent containing heavy distillate range hydrocarbon, light gas and byproduct water.
摘要翻译： 将烯属原料如费 - 托合成的合成烯烃液体产物转化成馏出物烃的方法包括以下步骤：在升高的温度和压力下使酸沸石转化催化剂使原料接触以使烯烃低聚并转化所述光中所含的氧化烃 油在高达325℃的温度和在H 2存在下，从而提供含有重馏分烃，轻质气体和副产物水的流出物。
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公开(公告)号：US4483760A
公开(公告)日：1984-11-20
申请号：US509828
申请日：1983-06-30
申请人： Samuel A. Tabak , Robert E. Holland
发明人： Samuel A. Tabak , Robert E. Holland
CPC分类号： C10G45/64 , C10G65/043
摘要： A process is provided for catalytically dewaxing a middle distillate with a ZSM-5 type catalyst. In this process the olefinic by-product is separated and catalytically converted to additional fuel oil and gasoline of good quality.
摘要翻译： 提供了一种使用ZSM-5型催化剂催化脱蜡中间馏分的方法。 在这个过程中，烯烃副产物被分离并催化转化成额外的燃料油和质量好的汽油。
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公开(公告)号：US4447312A
公开(公告)日：1984-05-08
申请号：US340662
申请日：1982-01-19
CPC分类号： C10G1/002 , C10G2400/04 , F02B3/06 , Y10S585/942
摘要： A process for preparing diesel fuel from coal-derived light fuel oils by alkylating said coal-derived light fuel oils with olefins and hydrotreating said alkylated product.
摘要翻译： 一种通过用烯烃烷基化所述煤源轻燃料油并加氢处理所述烷基化产物从煤衍生的轻质燃料油中制备柴油的方法。
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