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1.发明授权Ceramic coatings for insulating modular fuel cell cassettes in a solid-oxide fuel cell stack 有权用于在固体氧化物燃料电池堆中绝缘模块化燃料电池盒的陶瓷涂层公开(公告)号：US07422819B2
公开(公告)日：2008-09-09
申请号：US11158369
申请日：2005-06-22
申请人： Gary F. Reisdorf , Joseph M. Keller , Karl J. Haltiner, Jr. , Subhasish Mukerjee , Kenneth Scott Weil , John S. Hardy
发明人： Gary F. Reisdorf , Joseph M. Keller , Karl J. Haltiner, Jr. , Subhasish Mukerjee , Kenneth Scott Weil , John S. Hardy
IPC分类号： H01M2/08
CPC分类号： H01M8/0282 , H01M8/0286 , H01M2008/1293
摘要： In assembling an SOFC fuel cell stack from a plurality of cassettes, the mounting plate of one cassette is attached to, and insulated from, the separator plate of the next-adjacent cassette by a peripheral dielectric seal consisting of a ceramic coating and a metal braze. Materials suitable for the ceramic coating include yttrium stabilized zirconia (YSZ), zirconia toughened alumina, magnesium silicates such as the mineral forsterite, magnesium aluminates, magnesium aluminosilicates and lanthanum zirconate. The ceramic coating may be applied to the cassette's outer surface in known fashion as by physical vapor deposition, chemical vapor deposition, sputtering, and various methods of plasma spray. An underlayer of alumina may also be used to provide a redundant layer of electrical insulation.
摘要翻译： 在从多个盒组装SOFC燃料电池堆时，一个盒的安装板通过由陶瓷涂层和金属钎焊组成的外围电介质密封件附接到下一相邻盒的隔板并与之隔绝 。 适用于陶瓷涂层的材料包括钇稳定氧化锆（YSZ），氧化锆增韧氧化铝，硅酸镁如矿物镁橄榄石，铝酸镁，硅铝酸镁和锆酸镧。 陶瓷涂层可以通过物理气相沉积，化学气相沉积，溅射和各种等离子体喷涂方法以已知的方式施加到盒的外表面。 也可以使用氧化铝的底层来提供冗余的电绝缘层。
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2.发明授权Method and apparatus for forming electrode interconnect contacts for a solid-oxide fuel cell stack 有权用于形成固体氧化物燃料电池堆的电极互连触点的方法和装置公开(公告)号：US07781123B2
公开(公告)日：2010-08-24
申请号：US11145647
申请日：2005-06-06
申请人： Joseph M. Keller , Karl J. Haltiner, Jr. , Subhasish Mukerjee , Diane M. England , Gary F. Reisdorf , Steven L. Cooper , Willem Vilders, III
发明人： Joseph M. Keller , Karl J. Haltiner, Jr. , Subhasish Mukerjee , Diane M. England , Gary F. Reisdorf , Steven L. Cooper , Willem Vilders, III
CPC分类号： H01M8/0245 , H01M4/8621 , H01M4/8885 , H01M8/0232 , H01M8/0236 , H01M8/0297 , H01M8/1213 , H01M8/1246 , H01M8/2425 , H01M8/2457 , Y02E60/525 , Y02P70/56
摘要： An electrical interconnect for a solid-oxide fuel cell stack assembly, including a novel sintering paste and an improved manufacturing process for an anode and cathode electrical contacts is disclosed. On the anode side, the paste contains a metallic oxide such as NiO, and an amount of sacrificial pore-forming particles, such as carbon particles or polymer spheres, which are vaporized during sintering of the paste, resulting in a very porous connection having good electrical conductivity and good adhesion. A preferred level of pore-former in the paste is about 40 volume percent. On the cathode side, the paste contains a noble metal such as for example, gold, platinum, palladium or rhodium, and an amount of the sacrificial pore-forming particles. The paste may be applied to the surfaces in a grid pattern or, because the resulting contact is porous after sintering, it may be applied as a continuous layer.
摘要翻译： 公开了一种用于固体氧化物燃料电池堆组件的电互连，其包括新颖的烧结膏和用于阳极和阴极电触点的改进的制造工艺。 在阳极侧，糊状物含有NiO等金属氧化物，以及在糊料烧结过程中蒸发的诸如碳颗粒或聚合物球的牺牲性成孔颗粒的量，导致非常多孔的连接具有良好的 导电性好，附着力好。 浆料中成孔剂的优选含量为约40体积％。 在阴极侧，糊状物含有贵金属，例如金，铂，钯或铑，以及一定量的牺牲性成孔颗粒。 糊状物可以以网格图案施加到表面，或者由于所得接触在烧结之后是多孔的，所以可以作为连续层施加。
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公开(公告)号：US07217300B2
公开(公告)日：2007-05-15
申请号：US10607609
申请日：2003-06-27
CPC分类号： H01M8/028 , H01M8/0271 , H01M8/0282 , H01M8/2404 , H01M8/2425 , H01M8/2432 , H01M2008/1293 , H01M2250/20 , Y02E60/525 , Y02T90/32 , Y10T29/4911
摘要： In a solid-oxide fuel cell assembly comprising a plurality of components having electrically-conductive mating surfaces therebetween, the surfaces are sealed by gasket elements that include first and second silver braze alloy layers and a dielectric layer, formed preferably of yttrium-stabilized zirconia (YSZ), disposed between the alloy layers. The alloy is capable of bonding to many ceramics, including YSZ, and is readily brazed to the oxide layer formed on many metals at elevated temperatures. Because the braze alloy is electrically conductive, a dielectric layer must be included to break conductivity in bonding applications where electrical insulation is required. YSZ functions as a reliable insulator and will not crystallize or fracture as do prior art glass insulators. The assembly is useful as an auxiliary power unit in a vehicle.
摘要翻译： 在包括多个在其间具有导电配合表面的部件的固体氧化物燃料电池组件中，这些表面被垫圈元件密封，垫圈元件包括第一和第二银钎焊合金层和介电层，优选由钇稳定的氧化锆 YSZ），设置在合金层之间。 该合金能够与许多陶瓷（包括YSZ）结合，并且易于在高温下钎焊到在许多金属上形成的氧化物层。 由于钎焊合金是导电的，所以必须包括电介质层以破坏需要电绝缘的粘合应用中的导电性。 YSZ作为可靠的绝缘体起作用，不会像现有技术的玻璃绝缘子那样结晶或断裂。 该组件可用作车辆中的辅助动力单元。
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公开(公告)号：US07597986B2
公开(公告)日：2009-10-06
申请号：US11714450
申请日：2007-03-06
CPC分类号： H01M8/028 , H01M8/0271 , H01M8/0282 , H01M8/2404 , H01M8/2425 , H01M8/2432 , H01M2008/1293 , H01M2250/20 , Y02E60/525 , Y02T90/32 , Y10T29/4911
摘要： In a solid-oxide fuel cell assembly comprising a plurality of components having electrically-conductive mating surfaces therebetween, the surfaces are sealed by gasket elements that include first and second silver braze alloy layers and a dielectric layer, formed preferably of yttrium-stabilized zirconia (YSZ), disposed between the alloy layers. The alloy is capable of bonding to many ceramics, including YSZ, and is readily brazed to the oxide layer formed on many metals at elevated temperatures. Because the braze alloy is electrically conductive, a dielectric layer must be included to break conductivity in bonding applications where electrical insulation is required. YSZ functions as a reliable insulator and will not crystallize or fracture as do prior art glass insulators. The assembly is useful as an auxiliary power unit in a vehicle.
摘要翻译： 在包括多个在其间具有导电配合表面的部件的固体氧化物燃料电池组件中，这些表面被垫圈元件密封，垫圈元件包括第一和第二银钎焊合金层和介电层，优选由钇稳定的氧化锆 YSZ），设置在合金层之间。 该合金能够与许多陶瓷（包括YSZ）结合，并且易于在高温下钎焊到在许多金属上形成的氧化物层。 由于钎焊合金是导电的，所以必须包括电介质层以破坏需要电绝缘的粘合应用中的导电性。 YSZ作为可靠的绝缘体起作用，不会像现有技术的玻璃绝缘子那样结晶或断裂。 该组件可用作车辆中的辅助动力单元。
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公开(公告)号：US08168347B2
公开(公告)日：2012-05-01
申请号：US11250678
申请日：2005-10-14
CPC分类号： B23K1/0008 , B23K1/008 , B23K2101/18 , B23K2103/05 , H01M8/0232 , H01M8/0247 , H01M8/0271 , H01M8/0273 , H01M8/0276 , H01M8/0282 , H01M8/0297 , H01M8/2425 , H01M8/247 , H01M2008/1293 , Y02P70/56
摘要： A textured surface is formed on at least one of a fuel cell mounting plate or fuel cell subassembly to define a joint spacing between these two components. In a preferred embodiment, the textured surface comprises a plurality of dimples coined or otherwise formed in the metal mounting plate. The joint spacing improves the manufacturing and assembly process of the fuel cell cassettes through precise application and control of the brazing process which improves the braze joint strength while reducing material cost.
摘要翻译： 在燃料电池安装板或燃料电池子组件中的至少一个上形成纹理表面以限定这两个部件之间的接合间隔。 在优选实施例中，纹理表面包括在金属安装板中形成或以其他方式形成的多个凹坑。 接头间距通过钎焊工艺的精确应用和控制改善了燃料电池盒的制造和组装过程，从而提高了钎焊接头强度，同时降低了材料成本。
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公开(公告)号：US20090220813A1
公开(公告)日：2009-09-03
申请号：US12386120
申请日：2009-04-14
CPC分类号： B23K35/0244 , B23K35/025 , B23K35/30 , C04B37/003 , C04B37/006 , C04B37/023 , C04B37/026 , C04B2237/125 , C04B2237/708 , H01M8/0282 , H01M2008/1293 , Y10T428/12049 , Y10T428/252 , Y10T428/31678
摘要： A minimum joint thickness can be assured by incorporating beads or particles having a diameter corresponding to the joint thickness desired and which are infusible at the brazing temperature. Preferably such particles are formed of high-melting metals, metal oxides, ceramics, or cermets and are mixed into the alloy paste prior to fusing. In a preferred embodiment, the particle-containing paste is mixed with a non-flux carrier to facilitate application to the elements to be brazed. Exemplary application methods may include painting, rolling, screening, or extrusion dispensing. Brazing alloys in accordance with the invention are useful in bonding ceramics to ceramics, ceramics to metals, and metals to metals.
摘要翻译： 可以通过引入具有对应于期望的接合厚度的直径的珠子或颗粒并且在钎焊温度下是不可熔的来确保最小接合厚度。 优选地，这样的颗粒由高熔点金属，金属氧化物，陶瓷或金属陶瓷形成，并且在熔融之前混合到合金糊料中。 在优选的实施方案中，含有颗粒的糊剂与非助焊剂载体混合以便于施用于要钎焊的元件。 示例性的施加方法可以包括涂漆，轧制，筛分或挤出分配。 根据本发明的钎焊合金可用于将陶瓷结合到陶瓷，陶瓷与金属和金属与金属结合。
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公开(公告)号：US07179558B2
公开(公告)日：2007-02-20
申请号：US10892591
申请日：2004-07-15
IPC分类号： H01M8/00
CPC分类号： B23K35/0244 , B23K35/025 , B23K35/30 , C04B37/003 , C04B37/006 , C04B37/023 , C04B37/026 , C04B2237/125 , C04B2237/708 , H01M8/0282 , H01M2008/1293 , Y10T428/12049 , Y10T428/252 , Y10T428/31678
摘要： A minimum joint thickness can be assured by incorporating beads or particles having a diameter corresponding to the joint thickness desired and which are infusible at the brazing temperature. Preferably such particles are formed of high-melting metals, metal oxides, ceramics, or cermets and are mixed into the alloy paste prior to fusing. In a preferred embodiment, the particle-containing paste is mixed with a non-flux carrier to facilitate application to the elements to be brazed. Exemplary application methods may include painting, rolling, screening, or extrusion dispensing. Brazing alloys in accordance with the invention are useful in bonding ceramics to ceramics, ceramics to metals, and metals to metals.
摘要翻译： 可以通过引入具有对应于期望的接合厚度的直径的珠子或颗粒并且在钎焊温度下是不可熔的来确保最小接合厚度。 优选地，这样的颗粒由高熔点金属，金属氧化物，陶瓷或金属陶瓷形成，并且在熔融之前混合到合金糊料中。 在优选的实施方案中，含有颗粒的糊剂与非助焊剂载体混合以便于施用于要钎焊的元件。 示例性的施加方法可以包括涂漆，轧制，筛分或挤出分配。 根据本发明的钎焊合金可用于将陶瓷结合到陶瓷，陶瓷与金属和金属与金属结合。
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公开(公告)号：US5829113A
公开(公告)日：1998-11-03
申请号：US690222
申请日：1996-07-19
CPC分类号： B25B27/0092 , B23P19/047 , Y10T29/49872 , Y10T29/53657
摘要： A rotatable wheeled tool for simultaneously inserting and staking a weatherstrip into a slot, said tool comprising a body having a channel extending longitudinally from a first end to a second end, said channel configured to accommodate a length of weatherstrip through the body having sides extending a distance beyond the second end to form two legs and a rotatable wheel having an inserting edge and a staking edge, and mounted axially between said the legs with both the inserting and staking edges extending beyond the legs.
摘要翻译： 一种可旋转的轮式工具，用于同时将密封条插入并固定在槽中，所述工具包括主体，该主体具有从第一端至第二端纵向延伸的通道，所述通道构造成容纳通过主体的一定长度的密封条， 超过第二端的距离以形成两个腿部，以及具有插入边缘和铆钉边缘的可旋转轮，并且轴向地安装在所述腿之间，两个插入和铆合边缘都延伸超出腿部。
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