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公开(公告)号：US5017357A
公开(公告)日：1991-05-21
申请号：US494711
申请日：1990-03-16
CPC分类号： B01J23/8906 , B01D53/864
摘要： In a process for preparing a reduced material comprising (a) alumina and/or magnesium aluminate as support material, (b) platinum metal and (c) an iron component, the improvement comprises: (1) treating the reduced composition of matter with an acidic liquid; (2) heating the acid-treated material, and (3) treating the material obtained in step (2) with a reduced gas. The prepared material is used as a catalyst for converting CO and O.sub.2 to CO.sub.2.
摘要翻译： 在制备还原材料的方法中，包括（a）作为载体材料的氧化铝和/或铝酸镁，（b）铂金属和（c）铁组分，改进包括：（1）用 酸性液体 （2）加热酸处理材料，（3）用还原气处理步骤（2）中得到的材料。 所制备的材料用作将CO和O 2转化为CO 2的催化剂。
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公开(公告)号：US4943550A
公开(公告)日：1990-07-24
申请号：US366946
申请日：1989-06-14
CPC分类号： B01D53/864 , B01J23/8906
摘要： In a process for preparing a reduced material comprising (a) alumina and/or magnesium aluminate as support material, (b) platinum metal and (c) an iron component, the improvement comprises: (1) treating the reduced composition of matter with an acidic liquid; (2) heating the acid-treated material, and (3) treating the material obtained in step (2) with a reducing gas. The prepared material is used as a catalyst for converting CO and O.sub.2 to CO.sub.2.
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公开(公告)号：US5157204A
公开(公告)日：1992-10-20
申请号：US715943
申请日：1991-06-14
申请人： Scott H. Brown , John H. Kolts
发明人： Scott H. Brown , John H. Kolts
IPC分类号： C07C7/148
CPC分类号： C07C7/148
摘要： A process for removing carbon monoxide and free oxygen from hydrocarbon-containing fluids comprises contacting the fluid feed with at least one of several supported platinum-containing catalyst compositions so as to convert carbon monoxide and free oxygen to carbon dioxide, essentially without oxidizing the hydrocarbon(s).
摘要翻译： 从含烃流体中除去一氧化碳和游离氧的方法包括使流体进料与几种负载的含铂催化剂组合物中的至少一种接触，以将一氧化碳和游离氧转化为二氧化碳，基本上不氧化烃（ s）。
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公开(公告)号：US07868217B2
公开(公告)日：2011-01-11
申请号：US11940115
申请日：2007-11-14
IPC分类号： C07C2/52
CPC分类号： B01J29/90 , B01J27/13 , B01J27/32 , B01J29/62 , B01J38/14 , C07C2/76 , C07C5/31 , C10G35/085 , C10G45/70 , C10G2300/1044 , C10G2400/30 , Y02P20/584 , Y10S585/904 , Y10S585/906 , C07C15/02
摘要： A method of extending the life of an aromatization catalyst comprising identifying a rapid deactivation threshold (RDT) of the catalyst, and oxidizing the catalyst prior to reaching the RDT. A method of aromatizing a hydrocarbon comprising identifying a rapid deactivation threshold (RDT) for an aromatization catalyst, and operating an aromatization reactor comprising the catalyst to extend the Time on Stream of the reactor prior to reaching the RDT. A method of characterizing an aromatization catalyst comprising identifying a rapid deactivation threshold (RDT) of the catalyst. A method of extending the life of an aromatization catalyst comprising predicting a rapid deactivation threshold (RDT) for an aromatization reactor by employing the catalyst in a reactor system under an accelerated fouling condition to identify a test rapid deactivation threshold (t-RDT), predicting the RDT for the aromatization reactor based upon the t-RDT, and oxidizing the catalyst prior to the predicted RDT to extend the Time on Stream of the aromatization catalyst.
摘要翻译： 延长芳构化催化剂寿命的方法，包括鉴定催化剂的快速失活阈值（RDT），并在达到RDT之前氧化催化剂。 一种芳构化烃的方法，包括鉴定用于芳族化催化剂的快速失活阈值（RDT），以及操作包含催化剂的芳构化反应器以在达到RDT之前延长反应器上的时间。 表征芳构化催化剂的方法包括鉴定催化剂的快速失活阈值（RDT）。 一种延长芳构化催化剂的寿命的方法，包括通过在加速结垢条件下在反应器系统中使用催化剂来预测芳构化反应器的快速失活阈值（RDT），以鉴定测试快速失活阈值（t-RDT），预测 基于t-RDT的芳构化反应器的RDT，以及在预测的RDT之前氧化催化剂以延长芳构化催化剂的时间。
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公开(公告)号：US5698752A
公开(公告)日：1997-12-16
申请号：US685120
申请日：1996-07-23
申请人： Scott H. Brown , James B. Kimble , Stan A. Zisman
发明人： Scott H. Brown , James B. Kimble , Stan A. Zisman
IPC分类号： B01J23/56 , B01J23/58 , B01J23/66 , B01J27/12 , B01J27/13 , B01J27/135 , B01J37/08 , C07B61/00 , C07C5/09 , C07C7/167 , C07C11/02 , C07C11/04 , C07C5/02 , C07C5/03 , C07C5/05 , C07C5/08
CPC分类号： C07C7/167 , B01J23/56 , B01J23/58 , B01J23/66 , B01J27/12 , B01J27/13 , C07C5/09 , C07C2521/04 , C07C2521/06 , C07C2523/04 , C07C2523/44 , C07C2523/50 , C07C2523/58 , C07C2523/66
摘要： A selective hydrogenation of an alkyne in an olefin-containing fluid is provided which comprises contacting the fluid and hydrogen gas with a catalyst in the presence of at least one sulfur compound, under reaction conditions effective to produce at least one alkene wherein the catalyst comprises at least one alkali metal, fluorine and an inorganic support material.
摘要翻译： 提供了含烯烃流体中炔烃的选择性氢化，其包括在有效产生至少一种烯烃的反应条件下，在至少一种硫化合物的存在下使流体和氢气与催化剂接触，其中催化剂包含在 至少一种碱金属，氟和无机载体材料。
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公开(公告)号：US07932425B2
公开(公告)日：2011-04-26
申请号：US11780693
申请日：2007-07-20
申请人： Christopher D. Blessing , Scott H. Brown , Tin-Tack Peter Cheung , David J. Glova , Daniel M. Hasenberg , Dennis L. Holtermann , Gyanesh P. Khare , Daniel B. Knorr, Jr.
发明人： Christopher D. Blessing , Scott H. Brown , Tin-Tack Peter Cheung , David J. Glova , Daniel M. Hasenberg , Dennis L. Holtermann , Gyanesh P. Khare , Daniel B. Knorr, Jr.
CPC分类号： C10G35/095 , C10G2300/4081 , C10G2400/30
摘要： A hydrocarbon aromatization process comprising adding a nitrogenate, an oxygenate, or both to a hydrocarbon stream to produce an enhanced hydrocarbon stream, and contacting the enhanced hydrocarbon stream with an aromatization catalyst, thereby producing an aromatization reactor effluent comprising aromatic hydrocarbons, wherein the catalyst comprises a non-acidic zeolite support, a group VIII metal, and one or more halides. Also disclosed is a hydrocarbon aromatization process comprising monitoring the presence of an oxygenate, a nitrogenate, or both in an aromatization reactor, monitoring at least one process parameter that indicates the activity of the aromatization catalyst, modifying the amount of the oxygenate, the nitrogenate, or both in the aromatization reactor, thereby affecting the parameter.
摘要翻译： 烃芳构化方法包括将氮化物，含氧化合物或二者加入到烃流中以产生增强的烃流，以及使增强的烃流与芳构化催化剂接触，从而产生包含芳族烃的芳构化反应器流出物，其中催化剂包含 非酸性沸石载体，VIII族金属和一种或多种卤化物。 还公开了一种烃芳构化方法，其包括在芳构化反应器中监测含氧物，氮酸盐或二者的存在，监测指示芳构化催化剂的活性的至少一个工艺参数，改变含氧化合物的量， 或二者在芳构化反应器中，从而影响参数。
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公开(公告)号：US08563794B2
公开(公告)日：2013-10-22
申请号：US13614980
申请日：2012-09-13
IPC分类号： C07C2/52
CPC分类号： B01J29/90 , B01J27/13 , B01J27/32 , B01J29/62 , B01J38/14 , C07C2/76 , C07C5/31 , C10G35/085 , C10G45/70 , C10G2300/1044 , C10G2400/30 , Y02P20/584 , Y10S585/904 , Y10S585/906 , C07C15/02
摘要： A method of extending the life of an aromatization catalyst comprising identifying a rapid deactivation threshold (RDT) of the catalyst, and oxidizing the catalyst prior to reaching the RDT. A method of aromatizing a hydrocarbon comprising identifying a rapid deactivation threshold (RDT) for an aromatization catalyst, and operating an aromatization reactor comprising the catalyst to extend the Time on Stream of the reactor prior to reaching the RDT. A method of extending the life of an aromatization catalyst comprising predicting a rapid deactivation threshold (RDT) for an aromatization reactor by employing the catalyst in a reactor system under an accelerated fouling condition to identify a test rapid deactivation threshold (t-RDT), predicting the RDT for the aromatization reactor based upon the t-RDT, and oxidizing the catalyst prior to the predicted RDT to extend the Time on Stream of the aromatization catalyst.
摘要翻译： 延长芳构化催化剂寿命的方法，包括鉴定催化剂的快速失活阈值（RDT），并在达到RDT之前氧化催化剂。 一种芳构化烃的方法，包括鉴定用于芳族化催化剂的快速失活阈值（RDT），以及操作包含催化剂的芳构化反应器以在达到RDT之前延长反应器上的时间。 一种延长芳构化催化剂的寿命的方法，包括通过在加速结垢条件下在反应器系统中使用催化剂来预测芳构化反应器的快速失活阈值（RDT），以鉴定测试快速失活阈值（t-RDT），预测 基于t-RDT的芳构化反应器的RDT，以及在预测的RDT之前氧化催化剂以延长芳构化催化剂的时间。
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公开(公告)号：US08362310B2
公开(公告)日：2013-01-29
申请号：US13078524
申请日：2011-04-01
申请人： Christopher D. Blessing , Scott H. Brown , Tin-Tack Peter Cheung , David J. Glova , Daniel M. Hasenberg , Dennis L. Holtermann , Gyanesh P. Khare , Daniel B. Knorr, Jr.
发明人： Christopher D. Blessing , Scott H. Brown , Tin-Tack Peter Cheung , David J. Glova , Daniel M. Hasenberg , Dennis L. Holtermann , Gyanesh P. Khare , Daniel B. Knorr, Jr.
CPC分类号： C10G35/095 , C10G2300/4081 , C10G2400/30
摘要： A hydrocarbon aromatization process comprising adding a nitrogenate, an oxygenate, or both to a hydrocarbon stream to produce an enhanced hydrocarbon stream, and contacting the enhanced hydrocarbon stream with an aromatization catalyst, thereby producing an aromatization reactor effluent comprising aromatic hydrocarbons, wherein the catalyst comprises a non-acidic zeolite support, a group VIII metal, and one or more halides. Also disclosed is a hydrocarbon aromatization process comprising monitoring the presence of an oxygenate, a nitrogenate, or both in an aromatization reactor, monitoring at least one process parameter that indicates the activity of the aromatization catalyst, modifying the amount of the oxygenate, the nitrogenate, or both in the aromatization reactor, thereby affecting the parameter.
摘要翻译： 烃芳构化方法包括将氮化物，含氧化合物或二者加入到烃流中以产生增强的烃流，以及使增强的烃流与芳构化催化剂接触，从而产生包含芳族烃的芳构化反应器流出物，其中催化剂包含 非酸性沸石载体，VIII族金属和一种或多种卤化物。 还公开了一种烃芳构化方法，其包括在芳构化反应器中监测含氧物，氮酸盐或二者的存在，监测指示芳构化催化剂的活性的至少一个工艺参数，改变含氧化合物的量， 或二者在芳构化反应器中，从而影响参数。
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9.发明申请Methods of Isomerizing Xylenes with a Catalyst Reduced in the Presence of Hydrogen and a Base 有权在氢和碱存在下还原催化剂异构化二甲苯的方法公开(公告)号：US20110046428A1
公开(公告)日：2011-02-24
申请号：US12940291
申请日：2010-11-05
IPC分类号： C07C5/27
CPC分类号： C07C5/2724 , C07C5/2708 , C07C5/2754 , C07C7/14841 , C07C2529/40 , C07C2529/44 , C07C2529/70 , Y02P20/52 , Y10S585/906 , C07C15/08
摘要： A xylene isomerization process includes introducing gas comprising hydrogen and a base to a reaction zone in which a catalyst comprising a Group VIII metal and a zeolite support resides. In one embodiment, the base may be formed in situ within the reaction zone from nitrogen and hydrogen that are introduced to the reaction zone. In another embodiment, the base is introduced directly to the reaction zone. The conditions in the reaction zone are effective to reduce the catalyst. A stream comprising C8 aromatics, e.g., xylenes and ethylbenzene may then be fed to the reaction zone containing the reduced catalyst. The reaction zone may be operated at conditions effective to isomerize the xylenes and hydrodealkylate the ethylbenzene. The xylene loss during the isomerization of the xylenes is lowered as a result of using the catalyst reduced in the presence of the gas comprising a base and hydrogen.
摘要翻译： 二甲苯异构化方法包括将包含氢和碱的气体引入到其中包含第VIII族金属和沸石载体的催化剂所在的反应区。 在一个实施方案中，碱可以在反应区内从引入到反应区的氮和氢原位形成。 在另一个实施方案中，将碱直接引入反应区。 反应区中的条件对减少催化剂是有效的。 然后可以将包含C8芳族化合物（例如二甲苯和乙苯）的料流进料至含有还原催化剂的反应区。 反应区可以在有效地异构化二甲苯和加氢脱烷基化乙苯的条件下操作。 二甲苯异构化过程中二甲苯损失降低，因为使用在包含碱和氢的气体存在下还原的催化剂。
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10.发明申请Methods of isomerizing xylenes with a catalyst reduced in the presence of hydrogen and a base 有权在氢和碱的存在下还原催化剂使二甲苯异构化的方法公开(公告)号：US20090163752A1
公开(公告)日：2009-06-25
申请号：US11959872
申请日：2007-12-19
申请人： Scott H. Brown , Tin Tack Cheung
发明人： Scott H. Brown , Tin Tack Cheung
IPC分类号： C07C5/22
CPC分类号： C07C5/2724 , C07C5/2708 , C07C5/2754 , C07C7/14841 , C07C2529/40 , C07C2529/44 , C07C2529/70 , Y02P20/52 , Y10S585/906 , C07C15/08
摘要： A xylene isomerization process includes introducing gas comprising hydrogen and a base to a reaction zone in which a catalyst comprising a Group VIII metal and a zeolite support resides. In one embodiment, the base may be formed in situ within the reaction zone from nitrogen and hydrogen that are introduced to the reaction zone. In another embodiment, the base is introduced directly to the reaction zone. The conditions in the reaction zone are effective to reduce the catalyst. A stream comprising C8 aromatics, e.g., xylenes and ethylbenzene may then be fed to the reaction zone containing the reduced catalyst. The reaction zone may be operated at conditions effective to isomerize the xylenes and hydrodealkylate the ethylbenzene. The xylene loss during the isomerization of the xylenes is lowered as a result of using the catalyst reduced in the presence of the gas comprising a base and hydrogen.
摘要翻译： 二甲苯异构化方法包括将包含氢和碱的气体引入到其中包含第VIII族金属和沸石载体的催化剂所在的反应区。 在一个实施方案中，碱可以在反应区内从引入到反应区的氮和氢原位形成。 在另一个实施方案中，将碱直接引入反应区。 反应区中的条件对减少催化剂是有效的。 然后可以将包含C8芳族化合物（例如二甲苯和乙苯）的料流进料至含有还原催化剂的反应区。 反应区可以在有效地异构化二甲苯和加氢脱烷基化乙苯的条件下操作。 二甲苯异构化过程中二甲苯损失降低，因为使用在包含碱和氢的气体存在下还原的催化剂。
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