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1.发明申请公开(公告)号：US20120142990A1
公开(公告)日：2012-06-07
申请号：US13320973
申请日：2010-04-29
CPC分类号： B01J29/7042 , B01J29/40 , B01J29/7046 , B01J29/80 , B01J29/90 , B01J35/023 , B01J37/0045 , B01J37/0201 , B01J37/20 , B01J2229/37 , B01J2229/42 , C07C1/20 , Y02P20/584 , Y02P30/42 , C07C11/02
摘要： A process for the preparation of an olefinic product in the presence of an oxygenate conversion catalyst, the catalyst comprising a molecular sieve, wherein the molecular sieves comprises a SAPO-type silicoaluminophosphate, MFI-type aluminosilicate and/or MEL-type aluminosilicate, and a sulphur species at an elemental sulphur loading of at least 0.05 wt % based on total catalyst, the process comprising reacting an oxygenate feedstock under oxygenate conversion conditions to produce an olefinic reaction product. Further a process for the manufacture of an oxygenate conversion catalyst, and an oxygenate conversion catalyst comprising a molecular sieve having n-membered ring channels wherein n is 10 or less, and a sulphur species.
摘要翻译： 一种在含氧化合物转化催化剂存在下制备烯烃产物的方法，所述催化剂包含分子筛，其中分子筛包含SAPO型硅铝磷酸盐，MFI型硅铝酸盐和/或MEL型硅铝酸盐，以及 基于总催化剂，元素硫负载量为至少0.05重量％的硫物质，该方法包括在含氧化合物转化条件下使含氧化合物原料反应以产生烯属反应产物。 还有一种制备含氧化合物转化催化剂的方法，以及含有具有n员为10以下的n员环通道的分子筛和含硫物质的含氧化合物转化催化剂。
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公开(公告)号：US20100261943A1
公开(公告)日：2010-10-14
申请号：US12743273
申请日：2008-11-19
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , B01J29/06 , B01J29/40 , B01J29/70 , C07C2/865 , C07C4/02 , C07C2529/70 , C07C2529/80 , Y02P20/52 , Y02P30/42 , C07C11/06 , C07C11/04 , C07C11/02 , C07C15/08
摘要： Process for the preparation of an olefinic product, which process comprises contacting a reaction mixture comprising an oxygenate feedstock and an olefinic component with an oxygenate conversion catalyst comprising a molecular sieve having one-dimensional 10-membered ring channels, in a flow-through reactor unit defining a flow trajectory for fluids towards a downstream outlet for an olefinic reaction effluent from the flow-through reactor unit, wherein an olefinic co-feed is added at an upstream olefin feed inlet of the flow-through reactor unit, and wherein oxygenate feedstock is admitted to the reactor such that it is added to the reaction mixture at a plurality of locations along the feed trajectory.
摘要翻译： 制备烯烃产物的方法，该方法包括使包含含氧化合物原料和烯烃组分的反应混合物与含有一维10-元环通道的分子筛的含氧化合物转化催化剂在流通反应器单元 为来自流通反应器单元的烯烃反应流出物向下游出口流体流动的流动轨迹，其中在流通反应器单元的上游烯烃进料入口处加入烯烃共进料，其中含氧化合物原料为 进入反应器，使得其在沿着进料轨迹的多个位置处添加到反应混合物中。
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3.发明申请PROCESS FOR THE PREPARATION OF AN OLEFINIC PRODUCT AND AN OXYGENATE CONVERSION CATALYST 审中-公开制备烯烃产物和氧化转化催化剂的方法公开(公告)号：US20110313224A1
公开(公告)日：2011-12-22
申请号：US13140865
申请日：2009-12-21
CPC分类号： B01J29/7484 , B01J29/068 , B01J29/40 , B01J29/7492 , B01J29/80 , B01J2229/18 , B01J2229/36 , B01J2229/42 , C07C1/20 , C07C2529/40 , C07C2529/74 , C10G3/44 , C10G3/49 , C10G2300/1088 , C10G2400/20 , Y02P20/52 , Y02P30/42 , C07C11/04 , C07C11/06
摘要： A process for the preparation of an olefinic product in the presence of a catalyst comprising an aluminosilicate having one-dimensional 10-membered ring channels and a silica-to-alumina-ratio of less than 170, and at least one Group IB metal at a metal loading of between 0.1 and 10 wt % of the aluminosilicate, the process comprising reacting an oxygenate feedstock under oxygenate conversion conditions to produce a reaction, product comprising ethylene and/or propylene. An oxygenate conversion catalyst is also claimed.
摘要翻译： 在催化剂存在下制备烯烃产物的方法，该催化剂包含具有一维10-元环通道和二氧化硅 - 氧化铝比小于170的铝硅酸盐，以及至少一种IB族金属 金属负载量为0.1至10重量％的铝硅酸盐，该方法包括在含氧化合物转化条件下使含氧化合物原料反应以产生包含乙烯和/或丙烯的产物。 还要求一种含氧化合物转化催化剂。
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公开(公告)号：US20110288357A1
公开(公告)日：2011-11-24
申请号：US13140885
申请日：2009-12-21
IPC分类号： C07C1/20
摘要： A process for the preparation of an olefinic product, the process comprising reacting an oxygenate feedstock in a reactor in the presence of catalyst comprising an aluminosilicate having one-dimensional 10 membered ring channels, to produce the olefinic product, wherein before reacting the oxygenate feedstock to produce the olefinic product, the acidity of the aluminosilicate has been increased by at least 5% by treating the aluminosilicate with an aqueous solution comprising at least one of a chelating agent and an acid, wherein the increase in acidity is based on the acidity of the aluminosilicate before treatment.
摘要翻译： 一种制备烯烃产物的方法，该方法包括在含有具有一维10元环通道的硅铝酸盐的催化剂存在下在反应器中使含氧化合物原料反应以产生烯烃产物，其中在使含氧化合物原料与 通过用包含螯合剂和酸中的至少一种的水溶液处理铝硅酸盐，硅酸铝的酸度已经增加了至少5％，其中酸度的增加基于酸性 铝硅酸盐处理前。
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5.发明申请公开(公告)号：US20120083640A1
公开(公告)日：2012-04-05
申请号：US13320944
申请日：2010-05-19
CPC分类号： B01J29/80 , B01J29/40 , B01J29/70 , B01J35/023 , B01J37/0036 , B01J37/0045 , B01J37/28 , B01J2229/42 , C07C1/20 , C07C2521/08 , C07C2521/16 , C07C2529/80 , Y02P30/42 , C07C11/02
摘要： The present invention provides a process for the manufacture of a formulated oxygenate conversion catalyst, the process comprising: —treating with a phosphorus containing compound a first molecular sieve comprising aluminosilicate and a second molecular sieve, different from the first molecular sieve, the second molecular sieve having more-dimensional channels; and—combining the first molecular sieve, the second molecular sieve and a matrix material; wherein the catalyst is not treated with a phosphorus containing compound after combination of the molecular sieves with the matrix material. In a further aspect the invention provides a formulated oxygenate conversion catalyst and a process for the preparation of an olefinic product.
摘要翻译： 本发明提供了一种制备配制的含氧化合物转化催化剂的方法，该方法包括：用含磷化合物 - 与第一分子筛不同的第一分子筛和含有硅铝酸盐的第一分子筛和第二分子筛 具有更多维度的渠道; 并组合第一分子筛，第二分子筛和基质材料; 其中在将分子筛与基质材料组合后，不用含磷化合物处理催化剂。 在另一方面，本发明提供配制的含氧化合物转化催化剂和制备烯烃产物的方法。
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6.发明申请CATALYST PARTICLES, PROCESS FOR THE PREPARATION OF AN OLEFINIC PRODUCT, AND PROCESS FOR THE PREPARATION OF AN OXYGENATE CONVERSION CATALYST 审中-公开催化剂颗粒，制备烯烃产品的方法，以及制备氧化转化催化剂的方法公开(公告)号：US20100268009A1
公开(公告)日：2010-10-21
申请号：US12743268
申请日：2008-11-19
CPC分类号： C07C1/20 , B01J29/06 , B01J29/40 , B01J29/70 , C07C2/865 , C07C4/02 , C07C2529/70 , C07C2529/80 , Y02P20/52 , Y02P30/42 , C07C11/06 , C07C11/04 , C07C11/02 , C07C15/08
摘要： Catalyst particles comprising a first molecular sieve having one-dimensional 10-membered ring channels, and a second molecular sieve having more-dimensional channels; a process for the preparation of such catalyst particles; and a process for the preparation of an olefinic product, comprising reacting an oxygenate feedstock in a reaction zone in the presence of catalyst particles of the invention.
摘要翻译： 包含具有一维10-元环通道的第一分子筛和具有多维通道的第二分子筛的催化剂颗粒; 一种制备这种催化剂颗粒的方法; 以及制备烯烃产物的方法，包括在本发明的催化剂颗粒存在下在反应区中使含氧化合物原料反应。
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7.发明申请PROCESS FOR CONVERTING AN OXYGENATE INTO AN OLEFIN-CONTAINING PRODUCT, AND REACTOR SYSTEM 审中-公开将氧化剂转化为含有烯烃的产品和反应器系统的方法公开(公告)号：US20100268007A1
公开(公告)日：2010-10-21
申请号：US12743280
申请日：2008-11-19
CPC分类号： C07C1/20 , B01J29/06 , B01J29/40 , B01J29/70 , C07C2/865 , C07C4/02 , C07C2529/70 , C07C2529/80 , Y02P20/52 , Y02P30/42 , C07C11/06 , C07C11/04 , C07C11/02 , C07C15/08
摘要： A process for converting an oxygenate to an olefin-containing product, wherein oxygenate is contacted with an oxygenate conversion catalyst in a reactor system comprising two or more serially arranged riser reactor stages to obtain a riser reactor effluent from each stage, wherein each riser reactor stage comprises a single riser reactor or a plurality of parallel riser reactors, such that at least part of the riser reactor effluent of a preceding riser reactor stage is fed into a subsequent riser reactor stage, and wherein oxygenate is added to a plurality of the riser reactor stages; and a reactor system comprising two or more serially arranged riser reactor stages wherein the first of the two or more serially arranged riser reactor stages has a smaller total cross-sectional area than at least one of the subsequent riser reactor stages.
摘要翻译： 一种将含氧化合物转化为含烯烃的产物的方法，其中含氧化合物在包含两个或更多个连续排列的提升管反应器级的反应器系统中与含氧化合物转化催化剂接触以获得来自每个级的提升管反应器流出物，其中每个提升管反应器阶段 包括单个提升管反应器或多个平行提升管反应器，使得先前提升管反应器阶段的提升管反应器流出物的至少一部分进料到随后的提升管反应器阶段中，并且其中将含氧化合物加入多个提升管反应器 阶段 以及包括两个或更多个串联布置的提升管反应器级的反应器系统，其中两个或更多个串联布置的提升管反应器级中的第一个具有比随后的提升管反应器级中的至少一个更小的总横截面面积。
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8.发明授权公开(公告)号：US09120078B2
公开(公告)日：2015-09-01
申请号：US13141014
申请日：2009-12-21
CPC分类号： B01J29/061 , B01J29/40 , B01J29/70 , B01J29/80 , B01J37/0045 , B01J37/346 , B01J2229/20 , B01J2229/42 , C07C1/20 , C07C2521/16 , C07C2529/70 , C07C2529/80 , C10G3/44 , C10G3/49 , C10G2300/1088 , C10G2400/02 , C10G2400/20 , C10G2400/22 , Y02P30/20 , C07C11/02
摘要： The invention provides a process for the preparation of an olefinic product, the process comprising reacting an oxygenate feedstock in the presence of formulated oxygenate conversion catalyst particles to produce the olefinic product, the formulated catalyst particles comprising a combination of at least a molecular sieve having one-dimensional 10-membered ring channels and a matrix wherein a Group II metal species has been added to the catalyst particles after the combination of said molecular sieve and the matrix. Further a process for the manufacture of formulated oxygenate conversion catalyst particles, comprising combining of at least a molecular sieve having one-dimensional 10-membered ring channels and a matrix to form catalyst particles, and adding a Group II metal species to the catalyst particles after the combination of said molecular sieve and the matrix; and also oxygenate conversion catalyst particles comprising a combination of at least a molecular sieve having one-dimensional 10-membered ring channels, a further molecular sieve having more-dimensional channels, a matrix, and a Group II metal species.
摘要翻译： 本发明提供了制备烯烃产物的方法，该方法包括在配制的含氧化合物转化催化剂颗粒的存在下使含氧化合物原料反应以产生烯烃产物，所配制的催化剂颗粒包含至少一种具有一个 其中在所述分子筛和基质的组合之后已将II族金属物质加入到催化剂颗粒中。 进一步制备配制的含氧化合物转化催化剂颗粒的方法，包括至少将具有一维10-元环通道的分子筛与基质结合以形成催化剂颗粒，并在第二组金属物质后加入到催化剂颗粒中 所述分子筛与基质的组合; 以及包含至少具有一维10-元环通道的分子筛的组合的含氧化合物转化催化剂颗粒，具有多维通道的另外的分子筛，基质和II族金属物质。
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公开(公告)号：US08822749B2
公开(公告)日：2014-09-02
申请号：US12743265
申请日：2008-11-19
CPC分类号： C07C1/20 , B01J29/06 , B01J29/40 , B01J29/70 , C07C2/865 , C07C4/02 , C07C2529/70 , C07C2529/80 , Y02P20/52 , Y02P30/42 , C07C11/06 , C07C11/04 , C07C11/02 , C07C15/08
摘要： Process for the preparation of an olefinic product, which process comprises reacting an oxygenate feedstock and an olefinic co-feed in a reactor in the presence of an oxygenate conversion catalyst comprising a molecular sieve having one-dimensional 10-membered ring channels, and a further molecular sieve having more-dimensional channels, wherein the weight ratio between the one-dimensional molecular sieve and the further molecular sieve is in the range of from 1:1 to 100:1, to prepare an olefinic reaction effluent; separating the olefinic reaction effluent into at least a first olefinic fraction and a second olefinic fraction; recycling at least part of the second olefinic fraction; and recovering at least part of the first olefinic fraction as olefinic product.
摘要翻译： 制备烯烃产物的方法，该方法包括在包含具有一维10-元环通道的分子筛的含氧化合物转化催化剂存在下，使反应器中的含氧化合物原料和烯烃共进料反应， 具有多维通道的分子筛，其中一维分子筛与另外的分子筛之间的重量比在1:1至100:1的范围内，以制备烯烃反应流出物; 将烯烃反应流出物分离成至少第一烯烃馏分和第二烯烃馏分; 回收至少部分第二烯属馏分; 并回收至少部分第一烯属馏分作为烯属产物。
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公开(公告)号：US20120108876A1
公开(公告)日：2012-05-03
申请号：US13140933
申请日：2009-12-21
CPC分类号： B01J8/1827 , B01J8/0055 , B01J8/26 , B01J19/02 , B01J2208/00176 , B01J2208/0084 , B01J2219/0004 , B01J2219/0218 , B01J2219/0236 , C07C1/20 , C10G2400/20 , C07C11/02
摘要： A process and a reactor system for the preparation of an olefinic product by reacting an oxygenate feedstock in the presence of an oxygenate conversion catalyst within a reactor system under oxygenate-to-olefin conversion conditions, to obtain the olefinic product, wherein the reactor system has a contact surface coming in contact with oxygenates and wherein at least part of the contact surface is an material of the formula MX wherein: M is a metal and X is C, or M is a metal or Si and X is N.
摘要翻译： 一种用于制备烯烃产物的方法和反应器系统，其通过在含氧化合物 - 烯烃转化条件下的反应器系统内的含氧化合物转化催化剂存在下使含氧化合物原料反应得到烯烃产物，其中反应器体系具有 与氧化物接触的接触表面，并且其中至少部分接触表面是式MX的材料，其中：M是金属，X是C，或M是金属或Si，X是N.
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