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公开(公告)号：US08912110B2
公开(公告)日：2014-12-16
申请号：US13547351
申请日：2012-07-12
申请人： Manuela Serban , Mark P. Lapinski
发明人： Manuela Serban , Mark P. Lapinski
IPC分类号： B01J31/00 , B01J37/00 , B01J27/138 , B01J27/132 , B01J27/13 , B01J27/125 , B01J23/02 , B01J23/06 , B01J23/10 , B01J23/58 , B01J23/56 , B01J23/42 , B01J23/44 , B01J23/70 , B01J23/72 , B01J23/90 , B01J23/96 , C10G35/04 , C10G35/06 , C08F4/02 , C08F4/60
CPC分类号： B01J37/18 , B01J23/63 , B01J27/10 , B01J27/13 , B01J27/135 , B01J27/138 , B01J35/008 , B01J35/08 , B01J37/0072 , B01J37/0201 , C10G35/06 , C10G69/10 , C10G2300/1044 , C10G2400/02 , C10G2400/04
摘要： One embodiment is a catalyst for catalytic reforming of naphtha. The catalyst can have a noble metal including one or more of platinum, palladium, rhodium, ruthenium, osmium, and iridium, an alkali or alkaline-earth metal, a lanthanide-series metal, and a support. Generally, an average bulk density of the catalyst is about 0.300 to about 1.00 gram per cubic centimeter. The catalyst has a platinum content of less than about 0.375 wt %, a tin content of about 0.1 to about 2 wt %, a potassium content of about 100 to about 600 wppm, and a cerium content of about 0.1 to about 1 wt %. The lanthanide-series metal can be distributed at a concentration of the lanthanide-series metal in a 100 micron surface layer of the catalyst less than two times a concentration of the lanthanide-series metal at a central core of the catalyst.
摘要翻译： 一个实施方案是用于石脑油催化重整的催化剂。 催化剂可以具有包括铂，钯，铑，钌，锇和铱中的一种或多种的贵金属，碱金属或碱土金属，镧系金属和载体。 通常，催化剂的平均体积密度为约0.300至约1.00克/立方厘米。 催化剂的铂含量小于约0.375重量％，锡含量为约0.1至约2重量％，钾含量为约100至约600wppm，铈含量为约0.1至约1重量％。 镧系元素金属可以在催化剂的100微米表面层中以镧系元素金属的浓度分布，其量小于催化剂中心核心处的镧系金属浓度的两倍。
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2.发明授权Counter-current catalyst flow with split feed and two reactor train processing 有权逆流催化剂流动与分流进料和两个反应堆列车加工公开(公告)号：US08882994B2
公开(公告)日：2014-11-11
申请号：US13327164
申请日：2011-12-15
申请人： Mark D. Moser , David A. Wegerer , Kurt M. VandenBussche , Manuela Serban , Mark P. Lapinski , Mary Jo Wier , Gregory J. Gajda
发明人： Mark D. Moser , David A. Wegerer , Kurt M. VandenBussche , Manuela Serban , Mark P. Lapinski , Mary Jo Wier , Gregory J. Gajda
IPC分类号： C10G35/04
CPC分类号： C10G59/02 , C10G59/06 , C10G2400/30
摘要： A process is presented for the increasing the yields of aromatics from reforming a hydrocarbon feedstream. The process includes splitting a naphtha feedstream into a light hydrocarbon stream, and a heavier stream having a relatively rich concentration of naphthenes. The heavy stream is reformed to convert the naphthenes to aromatics and the resulting product stream is further reformed with the light hydrocarbon stream to increase the aromatics yields. The process includes passing a catalyst stream in a counter-current flow relative to the hydrocarbon process stream.
摘要翻译： 提出了一种从碳氢化合物原料流重整提高芳族化合物产率的方法。 该方法包括将石脑油进料流分解成轻质烃物流，以及将较稠油的浓度较高的环烷烃。 将重质流重整以将环烷烃转化为芳族化合物，并且所得产物流用轻质烃流进一步重整以提高芳烃产率。 该方法包括使相对于烃工艺物流的逆流流动催化剂流。
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3.发明申请PROCESS AND SYSTEM FOR THE ADDITION OF PROMOTER METAL DURING OPERATION IN A CATALYTIC REFORMING UNIT 审中-公开催化改性装置运行时添加促进剂金属的方法和系统公开(公告)号：US20130256193A1
公开(公告)日：2013-10-03
申请号：US13433617
申请日：2012-03-29
摘要： One exemplary embodiment can be a process for facilitating adding a promoter metal to at least one catalyst particle in situ in a catalytic naphtha reforming unit. The process can include introducing a compound comprising the promoter metal to the catalyst naphtha reforming unit and adding an effective amount of the promoter metal from the compound comprising the promoter metal to the catalyst particle under conditions to effect such addition and improve a conversion of a hydrocarbon feed.
摘要翻译： 一个示例性实施方案可以是促进助催化剂金属在催化石脑油重整单元中原位加入至少一种催化剂颗粒的方法。 该方法可以包括将催化剂石脑油重整单元引入包含助催化剂金属的化合物，并且在实施这种添加的条件下将有效量的助催化剂金属从包含促进剂金属的化合物加入催化剂颗粒中，并改善烃的转化率 饲料。
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4.发明授权Adsorbing polynuclear aromatics from a reforming process at reaction temperatures 有权在反应温度下从重整过程吸附多环芳烃公开(公告)号：US08518240B2
公开(公告)日：2013-08-27
申请号：US12701264
申请日：2010-02-05
申请人： Manuela Serban , Mark P. Lapinski , Mark D. Moser
发明人： Manuela Serban , Mark P. Lapinski , Mark D. Moser
CPC分类号： C10G25/00 , C10G35/04 , C10G2300/1096 , C10G2300/201
摘要： One exemplary embodiment can be a process for removing one or more polynuclear aromatics from at least one reformate stream from a reforming zone. The PNAs may be removed using an adsorption zone. The adsorption zone can include first and second vessels. Generally, the process includes passing the at least a portion of an effluent of the reforming zone through the first vessel containing a first activated carbon. The adsorption zone is operated at a temperature of at least 370° C.
摘要翻译： 一个示例性实施方案可以是从重整区从至少一种重整产物流中除去一种或多种多核芳烃的方法。 可以使用吸附区去除PNA。 吸附区可以包括第一和第二容器。 通常，该方法包括使重整区的流出物的至少一部分通过含有第一活性炭的第一容器。 吸附区在至少370℃的温度下运行
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5.发明申请COUNTER-CURRENT CATALYST FLOW WITH SPLIT FEED AND TWO REACTOR TRAIN PROCESSING 有权具有分离进料的反电流催化剂流和两反应堆火车加工公开(公告)号：US20130158319A1
公开(公告)日：2013-06-20
申请号：US13327164
申请日：2011-12-15
申请人： Mark D. Moser , David A. Wegerer , Kurt M. Vanden Bussche , Manuela Serban , Mark P. Lapinski , Mary Jo Wier , Gregory J. Gajda
发明人： Mark D. Moser , David A. Wegerer , Kurt M. Vanden Bussche , Manuela Serban , Mark P. Lapinski , Mary Jo Wier , Gregory J. Gajda
IPC分类号： C07C7/00
CPC分类号： C10G59/02 , C10G59/06 , C10G2400/30
摘要： A process is presented for the increasing the yields of aromatics from reforming a hydrocarbon feedstream. The process includes splitting a naphtha feedstream into a light hydrocarbon stream, and a heavier stream having a relatively rich concentration of naphthenes. The heavy stream is reformed to convert the naphthenes to aromatics and the resulting product stream is further reformed with the light hydrocarbon stream to increase the aromatics yields. The process includes passing a catalyst stream in a counter-current flow relative to the hydrocarbon process stream.
摘要翻译： 提出了一种从碳氢化合物原料流重整提高芳族化合物产率的方法。 该方法包括将石脑油进料流分解成轻质烃物流，以及将较稠油的浓度较高的环烷烃。 将重质流重整以将环烷烃转化为芳族化合物，并且所得产物流用轻质烃流进一步重整以提高芳烃产率。 该方法包括使相对于烃工艺物流的逆流流动催化剂流。
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公开(公告)号：US20130261363A1
公开(公告)日：2013-10-03
申请号：US13547351
申请日：2012-07-12
申请人： Manuela Serban , Mark P. Lapinski
发明人： Manuela Serban , Mark P. Lapinski
IPC分类号： B01J23/63 , C07C5/42 , B01J21/04 , B01J27/135 , B01J27/138 , B01J27/13
CPC分类号： B01J37/18 , B01J23/63 , B01J27/10 , B01J27/13 , B01J27/135 , B01J27/138 , B01J35/008 , B01J35/08 , B01J37/0072 , B01J37/0201 , C10G35/06 , C10G69/10 , C10G2300/1044 , C10G2400/02 , C10G2400/04
摘要： One embodiment is a catalyst for catalytic reforming of naphtha. The catalyst can have a noble metal including one or more of platinum, palladium, rhodium, ruthenium, osmium, and iridium, an alkali or alkaline-earth metal, a lanthanide-series metal, and a support. Generally, an average bulk density of the catalyst is about 0.300 to about 1.00 gram per cubic centimeter. The catalyst has a platinum content of less than about 0.375 wt %, a tin content of about 0.1 to about 2 wt %, a potassium content of about 100 to about 600 wppm, and a cerium content of about 0.1 to about 1 wt %. The lanthanide-series metal can be distributed at a concentration of the lanthanide-series metal in a 100 micron surface layer of the catalyst less than two times a concentration of the lanthanide-series metal at a central core of the catalyst.
摘要翻译： 一个实施方案是用于石脑油催化重整的催化剂。 催化剂可以具有包括铂，钯，铑，钌，锇和铱中的一种或多种的贵金属，碱金属或碱土金属，镧系金属和载体。 通常，催化剂的平均体积密度为约0.300至约1.00克/立方厘米。 催化剂的铂含量小于约0.375重量％，锡含量为约0.1至约2重量％，钾含量为约100至约600wppm，铈含量为约0.1至约1重量％。 镧系元素金属可以在催化剂的100微米表面层中以镧系元素金属的浓度分布，其量小于催化剂中心核心处的镧系金属浓度的两倍。
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7.发明授权Adsorbing polynuclear aromatics from a reforming process using adsorbents containing iron 有权使用含铁吸附剂从重整过程中吸附多核芳烃公开(公告)号：US08262901B2
公开(公告)日：2012-09-11
申请号：US12701187
申请日：2010-02-05
申请人： Manuela Serban , Mark P. Lapinski , Mark D. Moser
发明人： Manuela Serban , Mark P. Lapinski , Mark D. Moser
CPC分类号： C10G25/003 , C10G61/06 , C10G2300/1044 , C10G2300/1096 , C10G2300/301 , C10G2300/305 , C10G2300/4018 , C10G2400/02
摘要： An exemplary embodiment can be a process for removing one or more polynuclear aromatics from at least one reformate stream from a reforming zone. The PNAs may be removed using an adsorption zone. The adsorption zone can include first and second vessels each vessel containing an activated carbon adsorbent. Generally, the process includes passing the at least a portion of an effluent of the reforming zone through the first vessel containing a first activated carbon adsorbent wherein the first activated carbon adsorbent comprises iron.
摘要翻译： 示例性实施方案可以是从重整区从至少一种重整产物流中除去一种或多种多核芳烃的方法。 可以使用吸附区去除PNA。 吸附区可以包括第一和第二容器，每个容器含有活性炭吸附剂。 通常，该方法包括使重整区的流出物的至少一部分通过包含第一活性炭吸附剂的第一容器，其中第一活性炭吸附剂包含铁。
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8.发明申请Adsorbing Polynuclear Aromatics From a Reforming Process at Reaction Temperatures 有权在反应温度下从重整过程吸附多核芳烃公开(公告)号：US20110147265A1
公开(公告)日：2011-06-23
申请号：US12701264
申请日：2010-02-05
申请人： Manuela Serban , Mark P. Lapinski , Mark D. Moser
发明人： Manuela Serban , Mark P. Lapinski , Mark D. Moser
CPC分类号： C10G25/00 , C10G35/04 , C10G2300/1096 , C10G2300/201
摘要： One exemplary embodiment can be a process for removing one or more polynuclear aromatics from at least one reformate stream from a reforming zone. The PNAs may be removed using an adsorption zone. The adsorption zone can include first and second vessels. Generally, the process includes passing the at least a portion of an effluent of the reforming zone through the first vessel containing a first activated carbon. The adsorption zone is operated at a temperature of at least 370° C.
摘要翻译： 一个示例性实施方案可以是从重整区从至少一种重整产物流中除去一种或多种多核芳烃的方法。 可以使用吸附区去除PNA。 吸附区可以包括第一和第二容器。 通常，该方法包括使重整区的流出物的至少一部分通过含有第一活性炭的第一容器。 吸附区在至少370℃的温度下运行
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公开(公告)号：US09266091B2
公开(公告)日：2016-02-23
申请号：US13547335
申请日：2012-07-12
IPC分类号： B01J23/58 , C10G35/09 , B01J37/18 , B01J21/04 , B01J23/62 , B01J27/10 , B01J35/08 , B01J37/00 , B01J37/02 , B01J27/13 , B01J27/135 , B01J27/138
CPC分类号： B01J23/58 , B01J21/04 , B01J23/626 , B01J27/10 , B01J27/13 , B01J27/135 , B01J27/138 , B01J35/08 , B01J37/0072 , B01J37/0201 , B01J37/18 , C10G35/09
摘要： One exemplary embodiment can be a catalyst for catalytic reforming of naphtha. The catalyst can have a noble metal including one or more of platinum, palladium, rhodium, ruthenium, osmium, and iridium, at least two alkali metals or at least two alkaline earth metals, or mixtures of alkali metals and alkaline earth metals and a support.
摘要翻译： 一个示例性实施方案可以是用于石脑油的催化重整的催化剂。 催化剂可以具有包括铂，钯，铑，钌，锇和铱中的一种或多种的贵金属，至少两种碱金属或至少两种碱土金属，或碱金属和碱土金属的混合物和载体 。
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公开(公告)号：US20130256194A1
公开(公告)日：2013-10-03
申请号：US13547335
申请日：2012-07-12
CPC分类号： B01J23/58 , B01J21/04 , B01J23/626 , B01J27/10 , B01J27/13 , B01J27/135 , B01J27/138 , B01J35/08 , B01J37/0072 , B01J37/0201 , B01J37/18 , C10G35/09
摘要： One exemplary embodiment can be a catalyst for catalytic reforming of naphtha. The catalyst can have a noble metal including one or more of platinum, palladium, rhodium, ruthenium, osmium, and iridium, at least two alkali metals or at least two alkaline earth metals, or mixtures of alkali metals and alkaline earth metals and a support.
摘要翻译： 一个示例性实施方案可以是用于石脑油的催化重整的催化剂。 催化剂可以具有包括铂，钯，铑，钌，锇和铱中的一种或多种的贵金属，至少两种碱金属或至少两种碱土金属，或碱金属和碱土金属的混合物和载体 。
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