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公开(公告)号：US08926931B2
公开(公告)日：2015-01-06
申请号：US13566492
申请日：2012-08-03
申请人： Maohong Fan , Morris Argyle , Tiberiu Popa
发明人： Maohong Fan , Morris Argyle , Tiberiu Popa
CPC分类号： C10J3/00 , C10J2300/0906 , C10J2300/093 , C10J2300/0976 , C10J2300/0986 , Y02E20/18
摘要： The present invention generally relates to a catalytic gasification of coal. Catalytic gasification of a Wyodak low-sulfur sub-bituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive sodium carbonate catalyst applied via incipient wetness impregnation. Experiments in an atmospheric pressure fixed-bed laboratory gasifier were performed to evaluate the effects of reaction temperature, feed gas steam content, and Na2CO3 loading on the catalytic gasification of the Wyodak coal. The temperature range investigated (700-900° C.) was selected with consideration of the Na2CO3 melting point (850° C.) to reduce the loss by volatilization of sodium. Sodium was found to be active during both pyrolysis and gasification steps. The catalyst was most cost-effective at addition levels of approximately 3 wt %. The random pore model provided a good fit to the conversion versus time data collected under both the catalytic and the uncatalytic conditions.
摘要翻译： 本发明一般涉及煤的催化气化。 使用廉价的碳酸钠催化剂，通过初始湿度浸渍法研究了怀俄明州粉河流域Wyodak低硫次烟煤的催化气化。 进行大气压固定床实验室气化炉的实验，以评估反应温度，进料气体蒸汽含量和Na2CO3负载对Wyodak煤的催化气化的影响。 考虑到Na 2 CO 3熔点（850℃）来选择所研究的温度范围（700-900℃）以减少钠的挥发损失。 发现在热解和气化步骤期间钠都具有活性。 催化剂在添加量约3重量％时是最具成本效益的。 随机孔模型提供了在催化和非催化条件下收集的转化对时间数据的良好拟合。
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公开(公告)号：US20130032761A1
公开(公告)日：2013-02-07
申请号：US13566492
申请日：2012-08-03
申请人： Maohong Fan , Morris Argyle Provo , Tiberiu Popa
发明人： Maohong Fan , Morris Argyle Provo , Tiberiu Popa
CPC分类号： C10J3/00 , C10J2300/0906 , C10J2300/093 , C10J2300/0976 , C10J2300/0986 , Y02E20/18
摘要： The present invention generally relates to a catalytic gasification of coal. Catalytic gasification of a Wyodak low-sulfur sub-bituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive sodium carbonate catalyst applied via incipient wetness impregnation. Experiments in an atmospheric pressure fixed-bed laboratory gasifier were performed to evaluate the effects of reaction temperature, feed gas steam content, and Na2CO3 loading on the catalytic gasification of the Wyodak coal. The temperature range investigated (700-900° C.) was selected with consideration of the Na2CO3 melting point (850° C.) to reduce the loss by volatilization of sodium. Sodium was found to be active during both pyrolysis and gasification steps. The catalyst was most cost-effective at addition levels of approximately 3 wt %. The random pore model provided a good fit to the conversion versus time data collected under both the catalytic and the uncatalytic conditions.
摘要翻译： 本发明一般涉及煤的催化气化。 使用廉价的碳酸钠催化剂，通过初始湿度浸渍法研究了怀俄明州粉河流域Wyodak低硫次烟煤的催化气化。 进行大气压固定床实验室气化炉的实验，以评估反应温度，进料气体蒸汽含量和Na2CO3负载对Wyodak煤催化气化的影响。 考虑到Na 2 CO 3熔点（850℃）来选择所研究的温度范围（700-900℃）以减少钠的挥发损失。 发现在热解和气化步骤期间钠都具有活性。 催化剂在添加量约3重量％时是最具成本效益的。 随机孔模型提供了在催化和非催化条件下收集的转化对时间数据的良好拟合。
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公开(公告)号：US20120213682A1
公开(公告)日：2012-08-23
申请号：US13276844
申请日：2011-10-19
申请人： Maohong Fan , Morris Argyle , Rodolfo Monterrozo
发明人： Maohong Fan , Morris Argyle , Rodolfo Monterrozo
CPC分类号： B01D53/64 , B01D53/83 , B01D2251/108 , B01D2258/0283 , B01J20/0229 , B01J20/0288 , B01J20/046 , B01J20/20 , B01J20/28057 , B01J20/3204 , B01J20/3236 , F23J2215/60 , F23J2219/30
摘要： The adsorption of vapor phase elemental mercury onto the commercially produced Thief carbon and impregnated Thief carbon with ferric chloride and sodium chloride is disclosed. The results indicate that the impregnation of these sorbents enhanced considerably their capacity and changed the sorption mechanism. Ferric chloride impregnated Thief carbon sorbents presented the highest sorption capacity.
摘要翻译： 公开了将气相元素汞吸附到商业生产的Thief碳上并用氯化铁和氯化钠浸渍的Thief碳。 结果表明，这些吸附剂的浸渍显着提高了其吸附机理，改变了吸附机理。 氯化铁浸渍的硫化碳吸附剂具有最高的吸附能力。
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4.发明授权公开(公告)号：US09474999B2
公开(公告)日：2016-10-25
申请号：US13469890
申请日：2012-05-11
申请人： Maohong Fan
发明人： Maohong Fan
IPC分类号： B01D53/96 , B01D53/02 , B01D53/04 , B01D53/62 , B01J20/34 , B01J20/32 , B01J20/06 , B01J20/28
CPC分类号： B01D53/62 , B01D53/025 , B01D53/96 , B01D2251/80 , B01D2252/20405 , B01D2252/20426 , B01D2252/20484 , B01D2253/1124 , B01D2253/25 , B01D2257/504 , B01D2258/0283 , B01D2259/40083 , B01J20/06 , B01J20/28011 , B01J20/28085 , B01J20/3204 , B01J20/3251 , B01J20/3425 , B01J20/3458 , B01J20/3475 , Y02A50/2342 , Y02C10/04 , Y02C10/08
摘要： The invention generally relates to a bi-directional reactor and supported amine sorbent, and more particularly to a method and system for carbon dioxide sequestration utilizing a bi-directional reactor and monoethenalamine (MEA) on a substrate. The bi-directional reactor is configured to reclaim the sorbent material as the sorbent is immobilized during the sorption phase, but is mobilized during desorption phased. The immobilized sorbent reacts with the desired contaminate to absorb and is transported to another reactor during desorption phase, thereby permitting reclamation of the sorbent.
摘要翻译： 本发明一般涉及一种双向反应器和负载的胺吸附剂，更具体地涉及一种利用双向反应器和单乙胺（MEA）在基材上的二氧化碳螯合的方法和系统。 双向反应器构造成在吸附阶段期间吸附剂被固定回收吸附剂材料，但是在解吸期间被移动。 固定的吸附剂与期望的污染物反应以吸收并在解吸阶段被输送到另一个反应器，从而允许吸附剂的回收。
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5.发明申请公开(公告)号：US20120288429A1
公开(公告)日：2012-11-15
申请号：US13469890
申请日：2012-05-11
申请人： Maohong Fan
发明人： Maohong Fan
CPC分类号： B01D53/62 , B01D53/025 , B01D53/96 , B01D2251/80 , B01D2252/20405 , B01D2252/20426 , B01D2252/20484 , B01D2253/1124 , B01D2253/25 , B01D2257/504 , B01D2258/0283 , B01D2259/40083 , B01J20/06 , B01J20/28011 , B01J20/28085 , B01J20/3204 , B01J20/3251 , B01J20/3425 , B01J20/3458 , B01J20/3475 , Y02A50/2342 , Y02C10/04 , Y02C10/08
摘要： The invention generally relates to a bi-directional reactor and supported amine sorbent, and more particularly to a method and system for carbon dioxide sequestration utilizing a bi-directional reactor and monoethenalamine (MEA) on a substrate. The bi-directional reactor is configured to reclaim the sorbent material as the sorbent is immobilized during the sorption phase, but is mobilized during desorption phased. The immobilized sorbent reacts with the desired contaminate to absorb and is transported to another reactor during desorption phase, thereby permitting reclamation of the sorbent.
摘要翻译： 本发明一般涉及一种双向反应器和负载的胺吸附剂，更具体地涉及一种利用双向反应器和单乙胺（MEA）在基材上的二氧化碳螯合的方法和系统。 双向反应器构造成在吸附阶段期间吸附剂被固定回收吸附剂材料，但是在解吸期间被移动。 固定的吸附剂与期望的污染物反应以吸收并在解吸阶段被输送到另一个反应器，从而允许吸附剂的回收。
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公开(公告)号：US20130142718A1
公开(公告)日：2013-06-06
申请号：US13486222
申请日：2012-06-01
申请人： Maohong Fan , Bo-tao Zhang , Alan Bland
发明人： Maohong Fan , Bo-tao Zhang , Alan Bland
CPC分类号： B01J20/06 , B01D53/62 , B01D2251/306 , B01D2251/606 , B01D2257/504 , B01J20/0229 , B01J20/043 , B01J20/3204 , B01J20/3236 , Y02C10/04
摘要： A sorbent for CO2 wherein K2CO3 is supported on FeOOH.
摘要翻译： 用于CO 2的吸附剂，其中K 2 CO 3负载在FeOOH上。
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公开(公告)号：US20050049433A1
公开(公告)日：2005-03-03
申请号：US10927364
申请日：2004-08-26
申请人： Maohong Fan , Robert Brown
发明人： Maohong Fan , Robert Brown
CPC分类号： C07C51/412 , C07C51/02 , C07C51/42 , C07C53/08 , C07C53/06
摘要： A novel method for recovering carboxylic acid from a waste water stream is described. The method involves first neutralizing the carboxylic acid in the waste water with CaO or Ca(OH)2 to form calcium carboxylate. The resulting calcium carboxylate is then reacted with sulfite or sulfate to regenerate the carboxylic acid. The resulting waste water typically has a carboxylic acid content of at least 25-wt %.
摘要翻译： 描述了从废水流中回收羧酸的新方法。 该方法首先用CaO或Ca（OH）2中和废水中的羧酸以形成羧酸钙。 然后将所得羧酸钙与亚硫酸盐或硫酸盐反应以再生羧酸。 所得废水通常具有至少25重量％的羧酸含量。
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8.发明授权Catalytic CO2 desorption on the interface between NaHCO3 and multifunctional nanoporous TiO(OH)2 有权在NaHCO 3和多功能纳米多孔TiO（OH）2之间的界面上的催化二氧化碳解吸附公开(公告)号：US09382127B2
公开(公告)日：2016-07-05
申请号：US13469895
申请日：2012-05-11
申请人： Maohong Fan
发明人： Maohong Fan
IPC分类号： B01D53/48 , C01G23/04 , B01D53/62 , B01D53/96 , B01J20/04 , B01J20/06 , B01J20/28 , B01J20/30 , B01J20/32 , B01J21/06 , B01J27/232
CPC分类号： C01G23/04 , B01D53/62 , B01D53/96 , B01D2251/304 , B01D2255/2065 , B01D2255/20707 , B01D2255/20738 , B01D2255/2092 , B01D2257/504 , B01J20/043 , B01J20/06 , B01J20/28057 , B01J20/28071 , B01J20/28083 , B01J20/3078 , B01J20/3085 , B01J20/3204 , B01J20/3236 , B01J21/063 , B01J27/232 , B01J2220/42 , C01P2002/72 , C01P2002/82 , C01P2002/88 , C01P2004/03 , Y02C10/04 , Y02C10/08 , Y02P20/152
摘要： CO2 capture from flue gas is a costly procedure, usually due to the energy required for regeneration of the capture medium. One potential medium which could reduce such an energy consumption, however, is Na2CO3. It has been well studied as a sorbent, and it is understood that the theoretical energy penalty of use of Na2CO3 for CO2 separation is low, due to the relatively low heat of reaction and low heat capacity of the material. While it offers some advantages over other methods, its primary downfall is the slow reaction with CO2 during adsorption and the slow Na2CO3 regeneration process. An aspect of the invention relates to a catalyst to improve reaction kinetics, and more particularly to a catalyst to improve reaction kinetics for CO2 desorption and CO2 adsorption.
摘要翻译： 烟道气中的二氧化碳捕获是一个昂贵的过程，通常是由于捕获介质再生所需的能量。 然而，可以减少这种能量消耗的一种潜在介质是Na 2 CO 3。 作为吸附剂已经被很好地研究，并且可以理解，由于反应热较少并且材料的热容量低，使用Na 2 CO 3进行CO 2分离的理论能量损失较低。 虽然它比其他方法提供了一些优势，但它的主要垮台是吸附过程中CO2的缓慢反应和缓慢的Na2CO3再生过程。 本发明的一个方面涉及一种改善反应动力学的催化剂，更具体地说涉及一种改善CO 2解吸和CO 2吸附反应动力学的催化剂。
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公开(公告)号：US20130317274A1
公开(公告)日：2013-11-28
申请号：US13901533
申请日：2013-05-23
IPC分类号： A62D3/36
CPC分类号： A62D3/36 , A62D3/33 , A62D2101/08 , A62D2101/24 , A62D2101/43
摘要： A method for removing elements, including heavy metals, from fly ash and from fly ash resulting from removal of SOx/NOx from flue gas using Na2CO3/NaHCO3/trona, is described. An aqueous suspension of the fly ash and/or a solution of the leachate from the fly ash is treated with dissolved ferrous compounds, such as FeSO4.7H2O and/or FeCl2.4H2O, at a chosen initial acidic pH, and the precipitation of the ferrous ions as the solution basifies sequesters the trace elements.
摘要翻译： 描述了使用Na 2 CO 3 / NaHCO 3 /天然碱从烟灰中除去来自飞灰和从烟道气中除去SO x / NO x产生的飞灰的元素（包括重金属）的方法。 在所选择的初始酸性pH下，用溶解的亚铁化合物如FeSO 4·7H 2 O和/或FeCl 2·4H 2 O处理飞灰和/或来自飞灰的渗滤液的溶液的水悬浮液， 作为溶液的亚铁离子可以螯合微量元素。
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公开(公告)号：US20130200009A1
公开(公告)日：2013-08-08
申请号：US13537780
申请日：2012-06-29
申请人： Maohong Fan
发明人： Maohong Fan
CPC分类号： C02F1/72 , C01D1/02 , C02F1/5236 , C02F2101/32 , C02F2305/02
摘要： The present invention is a new, easy method for preparing stable solid Fe6+—Fe3+ agents in a fixed bed reactor by using O3 and FeOOH along with KOH with conversion efficiencies of approximately 27%. In addition, the product has been used to oxidize oil from water and to destroy tetracycline in water
摘要翻译： 本发明是一种用于在固定床反应器中制备稳定的固体Fe6 + -Fe3 +试剂的方法，其中O 3和FeOOH与KOH一起转化效率约为27％。 此外，该产品已经用于从水中氧化油并破坏水中的四环素
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