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1.发明授权Use of ECR-1, mazmorite and ECR-18 in the conversion of oxygenates to hydrocarbons 失效使用ECR-1，mazmorite和ECR-18将含氧化合物转化为碳氢化合物
公开(公告)号：US5278345A
公开(公告)日：1994-01-11
申请号：US888668
申请日：1992-05-27
CPC分类号： C07C1/20 , C07C2529/70 , Y02P30/42
摘要： A process for converting an oxygenate feed to light olefins using a microporous zeolite catalysts such as ECR-1, mazmorites, and/or ECR-18 is provided. In a preferred embodiment, the process is conducted at approximately 440.degree. C. (824.degree. F.) to about 460.degree. C. (860.degree. F.) using a methanol:water (approximately 1:4 molar ratio) feed and results in superior production of light olefins.
摘要翻译： 提供了使用微孔沸石催化剂如ECR-1，mazmorite和/或ECR-18将含氧化合物进料转化成轻质烯烃的方法。 在优选的实施方案中，使用甲醇：水（约1:4摩尔比）进料在约440摄氏度（824华氏度）至约460摄氏度（860华氏度）下进行该过程，并得到 优异的轻质烯烃生产。
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公开(公告)号：US07402718B2
公开(公告)日：2008-07-22
申请号：US11805974
申请日：2007-05-25
申请人： Marcel J. G. Janssen , Teng Xu , Cor F. Van Egmond , Keith H. Kuechler , Stephen N. Vaughn , James Harding Beech, Jr.
发明人： Marcel J. G. Janssen , Teng Xu , Cor F. Van Egmond , Keith H. Kuechler , Stephen N. Vaughn , James Harding Beech, Jr.
CPC分类号： C07C1/20 , B01J29/85 , C07C2529/00 , Y02P30/42 , C07C11/02
摘要： The invention relates to a conversion process for making olefin(s) using a molecular sieve catalyst composition. More specifically, the invention is directed to a process for converting a feedstock comprising an oxygenate in the presence of a molecular sieve catalyst composition, wherein the feedstock is free of or substantially free of metal salts.
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3.发明授权Molecular sieve catalyst compositions, their production and use in conversion processes 有权分子筛催化剂组合物，其生产和转化过程中的应用公开(公告)号：US06951830B2
公开(公告)日：2005-10-04
申请号：US10634557
申请日：2003-08-06
申请人： Marcel J. G. Janssen
发明人： Marcel J. G. Janssen
IPC分类号： B01J23/00 , B01J29/06 , B01J29/83 , B01J29/84 , B01J29/85 , B01J35/02 , B01J37/00 , C07C1/20 , C10G3/00
CPC分类号： B01J37/0009 , B01J23/007 , B01J29/06 , B01J29/83 , B01J29/84 , B01J29/85 , B01J35/023 , B01J37/0045 , B01J2208/00672 , C07C1/20 , C07C2529/85 , C10G2400/20 , Y02P30/20 , Y02P30/42 , C07C11/02
摘要： The invention relates to a catalyst composition, a method of making the same and its use in the conversion of a feedstock, preferably an oxygenated feedstock, into one or more olefin(s), preferably ethylene and/or propylene The catalyst composition a molecular sieve, such as a silicoaluminophosphate and/or an aluminophosphate, hydrotalcite, and optionally a rare earth metal component
摘要翻译： 本发明涉及一种催化剂组合物，其制备方法及其在将原料（优选氧化原料）转化为一种或多种烯烃，优选乙烯和/或丙烯中的用途。催化剂组合物分子筛 ，例如硅铝磷酸盐和/或磷酸铝，水滑石和任选的稀土金属组分
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公开(公告)号：US06437208B1
公开(公告)日：2002-08-20
申请号：US09481364
申请日：2000-01-11
申请人： Keith H. Kuechler , Marcel J. G. Janssen , Stephen N. Vaughn , Shun C. Fung , Nicolas P. Coute , Jeffrey Scott Smith , James R. Lattner , Jeffrey L. White , Teng Xu , William L. Kuechler, Sr. , Machteld M. Mertens , Cornelius W. M. Van Oorschot
发明人： Keith H. Kuechler , Marcel J. G. Janssen , Stephen N. Vaughn , Shun C. Fung , Nicolas P. Coute , Jeffrey Scott Smith , James R. Lattner , Jeffrey L. White , Teng Xu , William L. Kuechler, Sr. , Machteld M. Mertens , Cornelius W. M. Van Oorschot
IPC分类号： C07C120
CPC分类号： C10G50/00 , B01J29/85 , B01J29/90 , B01J35/0006 , B01J2229/123 , C10G3/49 , C10G3/57 , C10G3/62 , C10G2300/1022 , C10G2300/1029 , C10G2300/4018 , C10G2300/708 , C10G2400/02 , C10G2400/20 , C10G2400/22 , Y02P30/42
摘要： Disclosed is a method for making olefin product from an oxygenate-containing feedstock. In the method, a silicoaluminophosphate molecular sieve catalyst is contacted with the oxygenate-containing feedstock in a reactor at an average catalyst feedstock exposure index of at least 1.0. The method produces lower coke yield and provides an olefin product which is low in C1-C4 paraffin content. The invention is particularly effective in producing an olefin product having a very low propane content.
摘要翻译： 公开了一种从含氧化合物的原料制备烯烃产物的方法。 在该方法中，将硅铝磷酸盐分子筛催化剂在反应器中与含氧化合物的原料接触，平均催化剂原料暴露指数为至少1.0。 该方法产生较低的焦炭产量，并提供C1-C4链烷烃含量低的烯烃产物。 本发明在生产丙烷含量非常低的烯烃产物方面特别有效。
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公开(公告)号：US07375050B2
公开(公告)日：2008-05-20
申请号：US10425587
申请日：2003-04-28
IPC分类号： C01B15/16 , C01B25/26 , B01J27/00 , B01J27/182 , C07C1/00
CPC分类号： B01J29/7015 , B01J29/85 , C01B37/04 , C01B37/08 , C01B39/54 , C10G3/45 , C10G3/49 , C10G3/62 , C10G2400/20 , Y02P30/20 , Y10S423/32
摘要： Disclosed are methods and compositions of synthesis mixtures for the synthesis of aluminophosphates and silicoaluminophosphate molecular sieves, which enable the control and adjustment of the crystal particle size of aluminophosphates and silicoaluminophosphate molecular sieves. The synthesis mixture compositions used have two or more organic templates present at a molar ratio of total template to aluminum of ≦1.25; such a synthesis mixture is susceptible to control of product particle size through variation in the amount of seeds used in the synthesis.
摘要翻译： 公开了用于合成铝磷酸盐和硅铝磷酸盐分子筛的合成混合物的方法和组合物，其能够控制和调节铝磷酸盐和硅铝磷酸盐分子筛的晶体粒径。 所用的合成混合物组合物具有两个或更多个有机模板，其总模板与铝的摩尔比为<= 1.25; 这样的合成混合物易于通过合成中使用的种子的量的变化来控制产物的粒度。
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6.发明授权Molecular sieve catalyst compositions, their production and use in conversion processes 有权分子筛催化剂组合物，其生产和转化过程中的应用公开(公告)号：US07238845B2
公开(公告)日：2007-07-03
申请号：US11185350
申请日：2005-07-20
申请人： Marcel J. G. Janssen
发明人： Marcel J. G. Janssen
IPC分类号： C07C1/20
CPC分类号： B01J37/0009 , B01J23/007 , B01J29/06 , B01J29/83 , B01J29/84 , B01J29/85 , B01J35/023 , B01J37/0045 , B01J2208/00672 , C07C1/20 , C07C2529/85 , C10G2400/20 , Y02P30/20 , Y02P30/42 , C07C11/02
摘要： The invention relates to a catalyst composition, a method of making the same and its use in the conversion of a feedstock, preferably an oxygenated feedstock, into one or more olefin(s), preferably ethylene and/or propylene The catalyst composition a molecular sieve, such as a silicoaluminophosphate and/or an aluminophosphate, hydrotalcite, and optionally a rare earth metal component
摘要翻译： 本发明涉及一种催化剂组合物，其制备方法及其在将原料（优选氧化原料）转化为一种或多种烯烃，优选乙烯和/或丙烯中的用途。催化剂组合物分子筛 ，例如硅铝磷酸盐和/或磷酸铝，水滑石和任选的稀土金属组分
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公开(公告)号：US06979756B2
公开(公告)日：2005-12-27
申请号：US10281645
申请日：2002-10-28
申请人： Shun C. Fung , Marcel J. G. Janssen , Stephen N. Vaughn , Machteld M. Mertens , Albert Edward Schweizer , Cornelius W. M. Van Oorschot , Luc R. M. Martens , Richard B. Hall , Wilfried J. Mortier , Ronald G. Searle , Yi-Gang Xiong
发明人： Shun C. Fung , Marcel J. G. Janssen , Stephen N. Vaughn , Machteld M. Mertens , Albert Edward Schweizer , Cornelius W. M. Van Oorschot , Luc R. M. Martens , Richard B. Hall , Wilfried J. Mortier , Ronald G. Searle , Yi-Gang Xiong
CPC分类号： C01B39/02 , B01J29/04 , B01J29/85 , B01J37/084 , B01J2229/14 , B01J2229/24 , B01J2229/40 , B01J2229/42 , C01B37/00 , C07C1/20 , C07C2529/85 , C07C11/02
摘要： Disclosed is a method of heat treating a molecular sieve. The method comprises providing a template-containing molecular sieve, heating the molecular sieve under conditions effective to remove a portion of the template from the molecular sieve, and cooling the heated molecular sieve to leave an amount of template effective to cover catalytic sites within the molecular sieve. A catalyst composition is also provided which comprises a molecular sieve having a microporous structure and a binder, wherein between 10 and 90 vol % of the microporous structure is occupied by a material, the material comprising a template or a carbonaceous residue of a template, and the catalyst composition exhibits a Davison Index of not greater than 30.
摘要翻译： 公开了分子筛热处理方法。 该方法包括提供含模板的分子筛，在有效从分子筛除去一部分模板的条件下加热分子筛，并冷却加热的分子筛，留下一定量的模板，以有效地覆盖分子内的催化位点 筛。 还提供了一种催化剂组合物，其包括具有微孔结构和粘合剂的分子筛，其中10至90体积％的微孔结构被材料占据，所述材料包含模板或模板的碳质残余物，以及 催化剂组合物的Davison指数不大于30。
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公开(公告)号：US06812372B2
公开(公告)日：2004-11-02
申请号：US09924016
申请日：2001-08-07
申请人： Marcel J. G. Janssen , An Verberckmoes , Machteld M. Mertens , Antonie Jan Bons , Wilfried J. Mortier
发明人： Marcel J. G. Janssen , An Verberckmoes , Machteld M. Mertens , Antonie Jan Bons , Wilfried J. Mortier
IPC分类号： B01J27182
CPC分类号： C01B39/54 , B01J29/005 , B01J29/85 , B01J37/0009 , C01B37/08 , C07C1/20 , C10G3/49 , C10G2400/20 , Y02P30/20 , Y02P30/42 , C07C11/02
摘要： The present invention relates to a silicoaluminophosphate molecular sieve comprising at least one intergrown phase of molecular sieves having AEI and CHA framework types, wherein said intergrown phase has an AEI/CHA ratio of from about 5/95 to 40/60 as determined by DIFFaX analysis, using the powder X-ray diffraction pattern of a calcined sample of said silicoaluminophosphate molecular sieve. It also relates to methods for its preparation and to its use in the catalytic conversion of methanol to olefins.
摘要翻译： 本发明涉及包含具有AEI和CHA骨架类型的分子筛的至少一个共生相的硅铝磷酸盐分子筛，其中所述共生相具有通过DIFFaX分析测定的约5/95至40/60的AEI / CHA比 ，使用所述硅铝磷酸盐分子筛的煅烧样品的粉末X射线衍射图。 它还涉及其制备方法及其在将甲醇催化转化成烯烃中的用途。
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公开(公告)号：US06797852B2
公开(公告)日：2004-09-28
申请号：US10206574
申请日：2002-07-26
申请人： Marcel J. G. Janssen , Cornelius W. M. Van Oorschot , Shun C. Fung , Luc R. M. Martens , Wilfried J. Mortier , Ronald G. Searle , Machteld M. Mertens , Stephen N. Vaughn
发明人： Marcel J. G. Janssen , Cornelius W. M. Van Oorschot , Shun C. Fung , Luc R. M. Martens , Wilfried J. Mortier , Ronald G. Searle , Machteld M. Mertens , Stephen N. Vaughn
IPC分类号： C07C100
CPC分类号： B01J29/85 , B01J37/08 , B01J2229/24 , B01J2229/40 , B23K1/002 , B23K2101/06 , C07C1/20 , C07C2529/85 , Y02P30/20 , Y10S502/514 , Y10S585/906 , C07C11/02
摘要： This invention is directed to a method of making an olefin product from an oxygenate feedstock and a method of protecting catalytic activity of a silicoaluminophosphate molecular sieve. The methods comprise providing a silicoaluminophosphate molecular sieve having catalytic sites within the molecular sieve; shielding the catalytic sites to protect from loss of catalytic activity; and contacting the protected sieve in its activated state with an oxygenate feedstock under conditions effective to produce an olefin product before undesirable loss of catalytic activity. Undesirable loss in catalytic activity occurs when activated molecular sieve contacting the oxygenate feedstock has a methanol uptake index of at least 0.15.
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公开(公告)号：US06639117B2
公开(公告)日：2003-10-28
申请号：US10161873
申请日：2002-06-04
IPC分类号： C07C2207
CPC分类号： B01J38/02 , B01J29/85 , B01J37/32 , C07C1/20 , Y02P20/52 , Y02P20/584 , Y02P30/42 , C07C11/02
摘要： Disclosed is a method of rejuvenating molecular sieve and molecular sieve catalyst. The method includes freeze drying a molecular sieve having a methanol conversion ratio of less than 1, or a catalyst containing molecular sieve and a binder having a methanol conversion ratio of less than 1. The rejuvenated molecular sieve or catalyst is used to make an olefin product from an oxygenate. The olefin product containing ethylene and propylene can then be used to make polyethylene and polypropylene, respectively.
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