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公开(公告)号：US5371312A
公开(公告)日：1994-12-06
申请号：US42430
申请日：1993-04-05
IPC分类号： B01J29/40 , B01J31/02 , B01J31/12 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/27 , C07C5/41 , C07C6/12 , C10G45/64 , C07C5/52
CPC分类号： C10G45/64 , B01J29/40 , B01J31/123 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/2708 , C07C5/41 , C07C6/123 , C07C6/126 , B01J2229/12 , B01J2229/26 , B01J2229/32 , B01J2229/36 , B01J2229/42 , C07C2529/06 , C07C2529/064 , Y02P20/52
摘要： A process for shape selective hydrocarbon conversion involves contacting a hydrocarbon feedstream under conversion conditions with a catalytic molecular sieve which has been modified by treatment with an amino silane polymer while molecular sieve acid sites are protected. When the process is toluene disproportionation, a toluene feedstream may also contain a second silicon source which is a high pxylene selectivating agent. The invention also includes the modification method and the shape selective catalyst which results from the modification.
摘要翻译： 用于形状选择性烃转化的方法包括在转化条件下使烃进料流与催化分子筛接触，催化分子筛在分子筛酸性位点受到保护时已用氨基硅烷聚合物进行改性。 当该方法是甲苯歧化反应时，甲苯进料流还可以含有第二硅源，其是高的吡咯啉选择性试剂。 本发明还包括由改性产生的改性方法和形状选择性催化剂。
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公开(公告)号：US5552357A
公开(公告)日：1996-09-03
申请号：US294801
申请日：1994-08-25
IPC分类号： B01J29/40 , B01J31/02 , B01J31/12 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/27 , C07C5/41 , C07C6/12 , C10G45/64 , B01J29/06
CPC分类号： C10G45/64 , B01J29/40 , B01J31/123 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/2708 , C07C5/41 , C07C6/123 , C07C6/126 , B01J2229/12 , B01J2229/26 , B01J2229/32 , B01J2229/36 , B01J2229/42 , C07C2529/06 , C07C2529/064 , Y02P20/52
摘要： A process for shape selective hydrocarbon conversion involves contacting a hydrocarbon feedstream under conversion conditions with a catalytic molecular sieve which has been modified by treatment with an amino silane polymer while molecular sieve acid sites are protected. When the process is toluene disproportionation, a toluene feedstream may also contain a second silicon source which is a high p-xylene selectivating agent. The invention also includes the modification method and the shape selective catalyst which results from the modification.
摘要翻译： 用于形状选择性烃转化的方法包括在转化条件下使烃进料流与催化分子筛接触，催化分子筛在分子筛酸性位点受到保护时已用氨基硅烷聚合物进行改性。 当该方法是甲苯歧化反应时，甲苯进料流还可含有作为高对二甲苯选择性试剂的第二硅源。 本发明还包括由改性产生的改性方法和形状选择性催化剂。
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公开(公告)号：US5610112A
公开(公告)日：1997-03-11
申请号：US264287
申请日：1994-06-23
CPC分类号： C07C6/123 , B01J29/40 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/2708 , B01J2229/12 , B01J2229/26 , B01J2229/32 , B01J2229/36 , B01J2229/42 , C07C2529/42
摘要： A process for shape selective hydrocarbon conversion involves contacting a hydrocarbon feedsteam under conversion conditions with a modified catalytic molecular sieve which has been modified by being pre-selectivated with a first silicon source, then steamed. The feedstream may also contain a second silicon source which is a high efficiency para-xylene selectivating agent. The method for modifying the molecular sieve is also described.
摘要翻译： 形状选择性烃转化的方法包括使转化条件下的烃进料流与改性的催化分子筛接触，所述催化分子筛已经通过用第一硅源预先选择然后被蒸煮而被修饰。 进料流还可以含有作为高效对二甲苯选择剂的第二硅源。 还描述了改性分子筛的方法。
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公开(公告)号：US5349114A
公开(公告)日：1994-09-20
申请号：US42431
申请日：1993-04-05
CPC分类号： C07C6/123 , B01J29/40 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/2708 , B01J2229/12 , B01J2229/26 , B01J2229/32 , B01J2229/36 , B01J2229/42 , C07C2529/42
摘要： A process for shape selective hydrocarbon conversion involves contacting a hydrocarbon feedsteam under conversion conditions with a modified catalytic molecular sieve which has been modified by being pre-selectivated with a first silicon source, then steamed. The feedstream may also contain a second silicon source which is a high efficiency para-xylene selectivating agent. The method for modifying the molecular sieve is also described.
摘要翻译： 形状选择性烃转化的方法包括使转化条件下的烃进料流与改性的催化分子筛接触，所述催化分子筛已经通过用第一硅源预先选择然后被蒸煮而被修饰。 进料流还可以含有作为高效对二甲苯选择剂的第二硅源。 还描述了改性分子筛的方法。
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公开(公告)号：US5481057A
公开(公告)日：1996-01-02
申请号：US217819
申请日：1994-03-25
CPC分类号： C07C2/58 , C10G57/005 , C07C2529/08
摘要： A process for catalytic cracking and C3/C4 olefin alkylation with phosphorus stabilized faujasite catalyst is disclosed. Catalytic cracking produces C3 and C4 olefins, which are alkylated using phosphorus stabilized and water activated cracking catalyst. Spent alkylation catalyst may be discharged into the FCC unit.
摘要翻译： 公开了一种用磷稳定化八面沸石催化剂进行催化裂化和C3 / C4烯烃烷基化的方法。 催化裂化产生C3和C4烯烃，它们使用磷稳定和水活化的裂化催化剂进行烷基化。 废烷基化催化剂可以排放到FCC装置中。
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6.发明授权Isomerization of paraffin hydrocarbons using zeolites with high steam-enhanced acidity 失效使用具有高蒸汽增强酸度的沸石使石蜡烃异构化
公开(公告)号：US4374296A
公开(公告)日：1983-02-15
申请号：US249564
申请日：1981-03-31
申请人： Werner O. Haag , Rudolph M. Lago
发明人： Werner O. Haag , Rudolph M. Lago
IPC分类号： B01J29/40 , B01J29/44 , B01J29/65 , B01J29/70 , B01J29/74 , B01J37/10 , C07C2/54 , C07C4/06 , C07C5/22 , C07C5/27 , C07C5/41 , C07C6/00 , C07C6/12 , C10G11/05 , C10G49/08 , C07C5/13
CPC分类号： B01J29/06 , B01J29/44 , B01J29/7469 , B01J37/10 , C07C2/54 , C07C4/06 , C07C5/222 , C07C5/2724 , C07C5/2791 , C07C5/41 , C07C6/00 , C07C6/123 , C10G11/05 , C10G49/08 , B01J2229/26 , B01J2229/36 , B01J2229/42 , B01J29/65 , B01J29/7046 , C07C2529/40 , C07C2529/65 , C07C2529/70
摘要： A process is provided for effecting hydroisomerization of a C.sub.4 -C.sub.8 paraffin by contacting the same under hydroisomerization conditions with a catalyst comprising a porous crystalline zeolite characterized by a silica/aluminum mole ratio of greater than 12 and a constraint index within the approximate range of 1 to 12, which zeolite has undergone controlled pretreatment by contact with water to enhance the acid activity thereof, expressed as alpha, to greater than about 300. The catalyst also comprises, intimately combined therewith, a minor proportion of a Group VIII metal.
摘要翻译： 提供了一种通过在加氢异构化条件下使其与含有多孔结晶沸石的催化剂接触来进行C4-C8链烷烃的加氢异构化的方法，该多孔结晶沸石的特征在于二氧化硅/铝的摩尔比大于12，约束指数在约1范围内 至12，该沸石通过与水接触进行控制预处理，以将其以α表示的酸活性增加至大于约300.催化剂还包括与其紧密结合的少量VIII族金属。
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7.发明授权
公开(公告)号：US5310714A
公开(公告)日：1994-05-10
申请号：US910861
申请日：1992-07-08
IPC分类号： B01D53/02 , B01D53/86 , B01D53/94 , B01J37/02 , C07C5/32 , C07C5/333 , C07C7/13 , B01J29/06 , C01B33/26
CPC分类号： B01D53/9481 , B01D53/02 , B01D53/8668 , B01D53/9418 , B01J37/0246 , C07C5/325 , C07C5/3337 , C07C7/13 , B01D2251/202 , B01D2251/204 , B01D2251/2062 , B01D2251/208 , B01D2251/21 , B01D2255/504 , B01J2229/64
摘要： A method for synthesizing a zeolite bonded to a substrate utilizes a reaction mixture having a H.sub.2 O/YO.sub.2 molar ratio of at least 25 and Y is a tetravalent element, particularly silicon.A structure made according to this method includes a film of interconnected zeolite crystals bonded to a substrate and the structure is characterized by a value r representing the mg of zeolite/cm.sup.2 of substrate surface and a value e representing the coating efficiency as mg of bonded zeolite/mg of YO.sub.2 initially in the synthesis mixture; wherein r is at least 0.5 and e is at least 0.05.Processes are provided for separation, sorption, organic feedstock conversion and NO.sub.x conversion over the structure.
摘要翻译： 合成与底物结合的沸石的方法利用H 2 O / YO 2摩尔比至少为25的反应混合物，Y为四价元素，特别是硅。 根据该方法制造的结构包括结合到基底上的相互连接的沸石晶体的膜，该结构的特征在于表示基底表面的沸石/ cm 2的mg值，代表涂覆效率的值为mg的粘结的沸石 / mg的YO2最初在合成混合物中; 其中r为至少0.5，e为至少0.05。 提供了在结构上进行分离，吸附，有机原料转化和NOx转化的方法。
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公开(公告)号：US4025572A
公开(公告)日：1977-05-24
申请号：US685871
申请日：1976-05-12
申请人： Rudolph M. Lago
发明人： Rudolph M. Lago
CPC分类号： B01J29/40 , B01J35/023 , C07C1/20 , C07C2529/40 , Y02P20/52 , Y10S208/02
摘要： A catalytic process is provided for converting lower monohydric alcohols and their ethers, especially methanol and dimethyl ether, to a hydrocarbon mixture rich in C.sub.2 -C.sub.3 olefins and mononuclear aromatics with high selectivity for para-xylene production by contact, under conversion conditions, with a catalyst bed comprising a major proportion of particle-form inert solid diluent having intermixed therewith a crystalline aluminosilicate zeolite characterized by (1) a crystallite size not greater than 0.5 micron, (2) a particle size less than 2 millimeters in its smallest cross-sectional dimension, (3) a silica to alumina ratio of at least about 12 and (4) a constraint index, as hereinafter defined, within the approximate range of 1 to 12.
摘要翻译： 提供了一种催化方法，用于将低级一元醇及其醚，特别是甲醇和二甲醚转化为富含C 2 -C 3烯烃的烃混合物和单核芳烃，并且在转化条件下通过接触将对二甲苯生产具有高选择性， 催化剂床包含主要比例的颗粒状惰性固体稀释剂，其与其混合结晶硅铝酸盐沸石，其特征在于（1）微晶尺寸不大于0.5微米，（2）颗粒尺寸小于2毫米的最小横截面 尺寸，（3）二氧化硅与氧化铝的比例至少约为12，（4）如下文定义的约1到12的约束指数。
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公开(公告)号：US5316661A
公开(公告)日：1994-05-31
申请号：US47137
申请日：1993-04-16
IPC分类号： B01D53/02 , B01D53/86 , B01D53/94 , B01J29/06 , B01J37/02 , C01B39/00 , C01B39/02 , C01B39/06 , C01B39/36 , C01B39/38 , C01B39/42 , C01B39/44 , C07B61/00 , C07C5/27 , C07C5/32 , C07C5/333 , C07C6/12 , C07C7/13 , C07C11/02 , C07C15/08
CPC分类号： B01D53/9481 , B01D53/02 , B01D53/8668 , B01D53/9418 , B01J37/0246 , C07C5/325 , C07C5/3337 , C07C7/13 , B01D2251/2062 , B01D2255/102 , B01D2255/207 , B01D2255/50 , B01J2229/64
摘要： A method for synthesizing a zeolite bonded to a substrate utilizes a reaction mixture having a H.sub.2 O/YO.sub.2 molar ratio of at least 25 and Y is a tetravalent element, particularly silicon.A structure made according to this method includes a film of interconnected zeolite crystals bonded to a substrate and the structure is characterized by a value r representing the mg of zeolite/cm.sup.2 of substrate surface and a value e representing the coating efficiency as mg of bonded zeolite/mg of YO.sub.2 initially in the synthesis mixture; wherein r is at least 0.5 and e is at least 0.05.Processes are provided for separation, sorption, organic feedstock conversion, light paraffin dehydrogenation and NO.sub.X conversion over the structure.
摘要翻译： 合成与底物结合的沸石的方法利用H 2 O / YO 2摩尔比至少为25的反应混合物，Y为四价元素，特别是硅。 根据该方法制造的结构包括结合到基底上的相互连接的沸石晶体的膜，该结构的特征在于表示基底表面的沸石/ cm 2的mg值，代表涂覆效率的值为mg的粘结的沸石 / mg的YO2最初在合成混合物中; 其中r为至少0.5，e为至少0.05。 提供了在结构上进行分离，吸附，有机原料转化，轻链烷烃脱氢和NOX转化的方法。
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公开(公告)号：US5374410A
公开(公告)日：1994-12-20
申请号：US148943
申请日：1993-11-08
IPC分类号： B01D53/02 , B01D53/86 , B01D53/94 , B01J29/06 , B01J37/02 , C01B39/00 , C01B39/02 , C01B39/06 , C01B39/36 , C01B39/38 , C01B39/42 , C01B39/44 , C07B61/00 , C07C5/27 , C07C5/32 , C07C5/333 , C07C6/12 , C07C7/13 , C07C11/02 , C07C15/08 , B01J8/00
CPC分类号： B01D53/9481 , B01D53/02 , B01D53/8668 , B01D53/9418 , B01J37/0246 , C07C5/325 , C07C5/3337 , C07C7/13 , B01D2251/2062 , B01D2255/102 , B01D2255/207 , B01D2255/50 , B01J2229/64
摘要： A process for converting noxious nitrogen oxides present in gaseous effluent to N.sub.2 comprising reacting the gaseous effluent with an effective amount of reducing agent, e.g., ammonia, in the presence of a catalyst structure comprising a film of interconnected zeolite crystals bonded to a substrate, said catalyst structure being characterized by a value r representing the mg of zeolite/cm.sup.2 of substrate surface and a value e representing the coating efficiency as mg of bonded zeolite/mg of YO.sub.2 initially in the synthesis mixture, wherein r is at least 0.5 and e is at least 0.05.
摘要翻译： 在气态流出物中存在的有害氮氧化物转化为N 2的方法包括使气态流出物与有效量的还原剂（例如氨）在催化剂结构存在下反应，所述催化剂结构包含键合到基底的相互连接的沸石晶体的膜， 催化剂结构的特征在于表示基质表面的沸石/ cm 2的mg值，最初在合成混合物中表示作为结合沸石/ mg的YO的涂层效率的值e，其中r为至少0.5，e为 至少0.05。
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