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    Combined paraffin isomerization/ring opening process
    11.
    发明授权
    Combined paraffin isomerization/ring opening process 失效
    联合石蜡异构化/开环过程

    公开(公告)号：US5382731A

    公开(公告)日：1995-01-17

    申请号：US95885

    申请日：1993-07-22

    Applicant: Clarence D. Chang ,  Roy D. Bastian ,  Scott Han ,  Jose G. Santiesteban

    Inventor： Clarence D. Chang ,  Roy D. Bastian ,  Scott Han ,  Jose G. Santiesteban

    IPC: C07C5/13 ,  C07C5/22 ,  C07C1/00

    CPC classification number: C07C5/13 ,  C07C5/226 ,  C07C2521/06 ,  Y10S585/94

    Abstract: There is provided a process for ring opening of aromatics or cycloaliphatics, as well as isomerization of aliphatics. The feedstream to this process comprises hydrocarbons having 6 carbon atoms. The process involves the use of a recycle stream containing a source of chlorine, such as carbon tetrachloride, and this process involves the use of at least two reactors connected in series. The first reactor comprises a ring opening catalyst and is operated under conditions which particularly promote ring opening. The catalyst in this first reactor may comprise zirconia modified with tungstate and platinum. A second, downstream reactor is operated under conditions to promote isomerization of aliphatics. The catalyst in the second reactor may comprise alumina, platinum and a chloride component. The catalysts in both the first and second reactors are chlorine resistant.

    Abstract translation: 提供了芳族化合物或环烯烃的开环方法以及脂肪族异构化方法。 该方法的进料流包含具有6个碳原子的烃。 该方法包括使用含有氯源的再循环流，例如四氯化碳，并且该方法涉及使用串联连接的至少两个反应器。 第一反应器包括开环催化剂，并在特别促进开环的条件下操作。 该第一反应器中的催化剂可以包括用钨酸盐和铂改性的氧化锆。 第二个下游反应器在促进脂肪族异构化的条件下运行。 第二反应器中的催化剂可以包括氧化铝，铂和氯化物组分。 第一和第二反应器中的催化剂都是耐氯的。

    Shape selective hydrocarbon conversion over pre-selectivated, activated catalyst
    12.
    发明授权
    Shape selective hydrocarbon conversion over pre-selectivated, activated catalyst 失效
    形状选择性烃转化超过预选择的活化催化剂

    公开(公告)号：US5349113A

    公开(公告)日：1994-09-20

    申请号：US22205

    申请日：1993-02-25

    Applicant: Clarence D. Chang ,  Paul G. Rodewald

    Inventor： Clarence D. Chang ,  Paul G. Rodewald

    IPC: B01J29/40 ,  B01J31/02 ,  C07C6/12 ,  C07C5/52

    CPC classification number: C07C6/123 ,  B01J29/40 ,  B01J2229/12 ,  B01J2229/123 ,  B01J2229/32 ,  B01J2229/42

    Abstract: A process for a shape selective hydrocarbon conversion such as toluene disproportionation involves contacting a reaction stream under conversion conditions with a catalytic molecular sieve which has been pre-selectivated and concurrently activated by contact with a substantially aqueous solution of an organosilicon compound. The invention also includes a method for concurrently preselectivating and activating a catalyst and the shape selectivated, activated catalyst which results from this method.

    Abstract translation: 形成选择性碳氢化合物转化的方法如甲苯歧化过程包括使转化条件下的反应物流与催化分子筛接触，所述催化分子筛已经预选择并通过与基本上有机硅化合物的水溶液接触同时活化。 本发明还包括同时预选择和活化催化剂和由该方法产生的形状选择活化的催化剂的方法。

    Para-selective butylation of phenol over fairly large-pore zeolites
    13.
    发明授权
    Para-selective butylation of phenol over fairly large-pore zeolites 失效
    酚在相当大孔沸石上的对选择性丁基化

    公开(公告)号：US5288927A

    公开(公告)日：1994-02-22

    申请号：US11574

    申请日：1993-02-01

    Applicant: Clarence D. Chang ,  Stuart D. Hellring

    Inventor： Clarence D. Chang ,  Stuart D. Hellring

    IPC: C07C37/14 ,  C07C37/16

    CPC classification number: C07C37/14 ,  C07C37/16

    Abstract: There is provided a process for reacting phenol with butene or butanol over fairly large-pore zeolites to give butylphenol with high para-selectivity. Particular zeolites for use in this reaction include ZSM-12 and zeolite beta. A particular butene or butanol reactant is isobutanol. The product of this reaction may have a high content of the mono-alkylated, tert-butyl product.

    Abstract translation: 提供了在相当大孔沸石上使苯酚与丁烯或丁醇反应以产生具有高对位选择性的丁基苯酚的方法。 用于该反应的特定沸石包括ZSM-12和β沸石。 特殊的丁烯或丁醇反应物是异丁醇。 该反应的产物可以具有高含量的单烷基化叔丁基产物。

    Activation of zeolites
    14.
    发明授权
    Activation of zeolites 失效
    活化沸石

    公开(公告)号：US5271920A

    公开(公告)日：1993-12-21

    申请号：US818722

    申请日：1992-01-07

    Applicant: Clarence D. Chang ,  Nai Y. Chen ,  Cynthis T. Chu ,  Bruce P. Pelrine

    Inventor： Clarence D. Chang ,  Nai Y. Chen ,  Cynthis T. Chu ,  Bruce P. Pelrine

    IPC: B01J20/18 ,  B01J29/40 ,  B01J37/06 ,  C01B33/34

    CPC classification number: B01J37/06 ,  B01J20/186 ,  B01J29/40 ,  Y10S423/22

    Abstract: The invention includes a ZSM-5 composition and the preparation thereof which comprises treating ZSM-5 with solutions of salts of weak acids. The resulting ultrasmall crystal size ZSM-5 component has a sorption capacity for 2,2-dimethylbutane of at least 10 mg/g zeolite and a sorption time for 30% capacity zeolitic sorption at 60.degree. C. and P(2,2-dimethylbutane) of 60 torr, of less than about 4 minutes.

    Abstract translation: 本发明包括ZSM-5组合物及其制备方法，其包括用弱酸盐溶液处理ZSM-5。 所得到的超小晶体尺寸ZSM-5组分对于至少10mg / g沸石的2,2-二甲基丁烷具有吸附能力，在60℃具有30％容量沸石吸附的吸附时间和P（2,2-二甲基丁烷 ）为60托，小于约4分钟。

    Synthesis of crystalline silicoaluminophosphate composition
    17.
    发明授权
    Synthesis of crystalline silicoaluminophosphate composition 失效
    结晶硅铝磷酸盐组合物的合成

    公开(公告)号：US5169614A

    公开(公告)日：1992-12-08

    申请号：US179344

    申请日：1988-04-08

    Applicant: Clarence D. Chang ,  John D. Lutner

    Inventor： Clarence D. Chang ,  John D. Lutner

    IPC: C01B37/04 ,  C01B37/08

    CPC classification number: C01B37/08 ,  C01B37/04

    Abstract: This invention relates to a new crystalline silicoaluminophosphate composition, to a new and useful improvement in synthesizing said crystalline composition and to use of said crystalline composition prepared in accordance herewith as a catalyst component for organic compound, e.g. hydrocarbon compound, conversion.

    Abstract translation: 本发明涉及一种新的结晶硅铝磷酸盐组合物，用于合成所述结晶组合物的新的和有用的改进，以及使用根据本文制备的所述结晶组合物作为有机化合物的催化剂组分。 烃化合物，转化。

    Propylene oligomerization over silica modified zeolites
    19.
    发明授权
    Propylene oligomerization over silica modified zeolites 失效
    二氧化硅改性沸石上的丙烯低聚

    公开(公告)号：US5057640A

    公开(公告)日：1991-10-15

    申请号：US636857

    申请日：1991-01-02

    Applicant: Clarence D. Chang ,  Paul G. Rodewald

    Inventor： Clarence D. Chang ,  Paul G. Rodewald

    IPC: B01J29/06 ,  B01J29/40 ,  C07B61/00 ,  C07C2/12 ,  C07C11/02

    CPC classification number: C07C2/12 ,  B01J29/40 ,  B01J2229/14 ,  B01J2229/32 ,  C07C2529/40 ,  Y02P20/52

    Abstract: There is provided a process for oligomerizing propylene by contacting propylene with silica modified zeolites. The modification of the zeolite with silica results in a product which is enriched in hydrocarbons falling within the boiling range of jet fuel (330.degree.-480.degree. F.) and diesel fuel (480.degree.-650.degree. F.). The zeolite may be ZSM-5, which may be modified by sorbing methylhydrogensilicone into the pores of the zeolite followed by calcination to convert the sorbed methylhydrogensilicone into amorphous silica.

    Abstract translation: 提供了通过使丙烯与二氧化硅改性沸石接触来使丙烯低聚的方法。 用二氧化硅改性沸石产生的一种富含烃类物质落入喷气燃料沸点范围（330°-480°F）和柴油（480°-650°F）的产物。 沸石可以是ZSM-5，其可以通过将甲基氢硅酮吸附到沸石的孔中，然后煅烧以将吸附的甲基氢硅氧烷转化成无定形二氧化硅来进行改性。

    Catalytic conversion
    20.
    发明授权
    Catalytic conversion 失效
    催化转化

    公开(公告)号：US4711970A

    公开(公告)日：1987-12-08

    申请号：US818967

    申请日：1986-01-08

    Applicant: Clarence D. Chang ,  Joseph N. Miale

    Inventor： Clarence D. Chang ,  Joseph N. Miale

    IPC: B01J29/04 ,  B01J29/06 ,  C01B39/02 ,  C07C2/00

    CPC classification number: C01B39/026 ,  B01J29/04 ,  C01B35/1009

    Abstract: A method for increasing the total amount of lattice metal in the framework of a particular porous inorganic crystalline composition, its conversion to hydrogen or hydronium form and use thereof as a catalyst component having enhanced catalytic activity for conversion of paraffins and/or olefins to higher hydrocarbons is provided.

    Abstract translation: 在特定的多孔无机结晶组合物的框架中增加晶格金属的总量的方法，其转化为氢或水合物形式的方法及其作为催化剂组分的用途，其具有用于将链烷烃和/或烯烃转化成高级烃的增强的催化活性 被提供。

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