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    Thermoplastic silicone elastomers formed from polyester resins
    3.
    发明授权
    Thermoplastic silicone elastomers formed from polyester resins 有权
    由聚酯树脂形成的热塑性硅橡胶

    公开(公告)号：US06417293B1

    公开(公告)日：2002-07-09

    申请号：US09728920

    申请日：2000-12-04

    申请人： Igor Chorvath ,  Craig Steven Gross ,  Kenneth Gerard Gruszynski ,  Michael Kang-Jen Lee ,  Jun Liao ,  Koji Nakanishi ,  Richard Leroy Rabe ,  David Joseph Romenesko

    发明人： Igor Chorvath ,  Craig Steven Gross ,  Kenneth Gerard Gruszynski ,  Michael Kang-Jen Lee ,  Jun Liao ,  Koji Nakanishi ,  Richard Leroy Rabe ,  David Joseph Romenesko

    IPC分类号： C08L6706

    CPC分类号： C08L67/02 ,  C08G77/06 ,  C08G77/12 ,  C08G77/20 ,  C08G77/44 ,  C08K5/0091 ,  C08K5/04 ,  C08K5/16 ,  C08K5/36 ,  C08K5/5419 ,  C08L83/04 ,  C08L83/00 ,  C08L2666/14 ,  C08L2666/28

    摘要： The present invention, therefore, relates to a method for preparing a thermoplastic elastomer, said method comprising: (I) mixing (A) a thermoplastic resin comprising more than 50 percent by volume of a polyester resin other than poly(butylene terephthalate), said thermoplastic resin having a softening point of 23° C. to 300° C., (B) a silicone elastomer comprising (B′) 100 parts by weight of a diorganopolysiloxane gum having a plasticity of at least 30 and having an average of at least 2 alkenyl groups in its molecule and, optionally, (B″) up to 200 parts by weight of a reinforcing filler, the weight ratio of said silicone elastomer (B) to said thermoplastic resin (A) being greater than 35:65 to 85:15, (C) 0.01 to 5 parts by weight of a stabilizer for each 100 parts by weight of said thermoplastic resin and said silicone elastomer, (D) an organohydrido silicon compound which contains an average of at least 2 silicon-bonded hydrogen groups in its molecule and (E) a hydrosilation catalyst, components (D) and (E) being present in an amount sufficient to cure said diorganopolysiloxane (B′); and (II) dynamically curing said diorganopolysiloxane (B′).

    摘要翻译： 因此，本发明涉及一种制备热塑性弹性体的方法，所述方法包括：（I）混合（A）包含超过50体积％的聚（对苯二甲酸丁二醇酯）以外的聚酯树脂的热塑性树脂，所述 软化点为23℃至300℃的热塑性树脂，（B）含有（B'）100重量份塑性为至少30的二有机基聚硅氧烷胶的硅氧烷弹性体，其平均至少为 2个烯基和任选的（B“）至多200重量份的增强填料，所述硅氧烷弹性体（B）与所述热塑性树脂（A）的重量比大于35:65至大于35:65至 85:15，（C）每100重量份所述热塑性树脂和所述硅氧烷弹性体中的稳定剂0.01至5重量份，（D）平均含有至少2个与硅键合的氢的有机氢化硅化合物 （E）硅氢化催化剂，c 组分（D）和（E）以足以固化所述二有机聚硅氧烷（B'）的量存在; 和（II）动态固化所述二有机聚硅氧烷（B'）。

    Thermoplastic silicone elastomers formed from nylon resins
    5.
    发明授权
    Thermoplastic silicone elastomers formed from nylon resins 有权
    由尼龙树脂形成的热塑性硅橡胶

    公开(公告)号：US06362287B1

    公开(公告)日：2002-03-26

    申请号：US09535556

    申请日：2000-03-27

    申请人： Igor Chorvath ,  Michael K. Lee ,  Yongjun Lee ,  Dawei Li ,  Koji Nakanishi ,  Robert Leo Oldinski ,  Richard L. Rabe ,  David Joseph Romenesko ,  Jeffrey Paul Sage

    发明人： Igor Chorvath ,  Michael K. Lee ,  Yongjun Lee ,  Dawei Li ,  Koji Nakanishi ,  Robert Leo Oldinski ,  Richard L. Rabe ,  David Joseph Romenesko ,  Jeffrey Paul Sage

    IPC分类号： C08G7708

    CPC分类号： C08L83/04 ,  C08G77/12 ,  C08G77/20 ,  C08G77/44 ,  Y10S525/903 ,  C08L2666/14 ,  C08L2666/28

    摘要： A method for preparing a thermoplastic elastomer is disclosed, said method comprising (I) mixing (A) a rheologically stable polyamide resin having a melting point or glass transition temperature of 25° C. to 275° C., (B) a silicone base comprising (B′) 100 parts by weight of a diorganopolysiloxane gum having a plasticity of at least 30 and having an average of at least 2 alkenyl radicals in its molecule and (B″) 5 to 200 parts by weight of a reinforcing filler,  the weight ratio of said silicone base to said polyamide resin being greater than 35:65 to 85:15, (C) 0.1 to 5 parts by weight of a hindered phenol compound for each 100 parts by weight of said polyamide and said silicone base, (D) an organohydrido silicon compound which contains an average of at least 2 silicon-bonded hydrogen groups in its molecule and (E) a hydrosilation catalyst, components (D) and (E) being present in an amount sufficient to cure said diorganopolysiloxane (B′); and (II) dynamically curing said diorganopolysiloxane (B′), wherein at least one property of the thermoplastic elastomer selected from tensile strength or elongation is at least 25% greater than the respective property for a corresponding simple blend wherein said diorganopolysiloxane is not cured and said thermoplastic elastomer has an elongation of at least 25%.

    摘要翻译： 公开了一种制备热塑性弹性体的方法，所述方法包括（I）混合（A）熔点或玻璃化转变温度为25℃至275℃的流变学稳定的聚酰胺树脂，（B）硅氧烷基 包含（B'）100重量份的塑性为至少30的二有机聚硅氧烷胶，其分子中平均具有至少2个烯基，（B“）为5〜200重量份的增强填料， 所述硅氧烷基与所述聚酰胺树脂的重量比大于35:65至85:15，（C）每100重量份所述聚酰胺和所述有机硅基料为0.1至5重量份的受阻酚化合物， （D）在其分子中平均含有至少2个与硅键合的氢基团的有机氢化硅化合物，（E）硅氢化催化剂，组分（D）和（E）以足以固化所述二有机聚硅氧烷的量存在 B'）; 和（II）动态固化所述二有机聚硅氧烷（B'），其中选自拉伸强度或伸长率的热塑性弹性体的至少一种性能比相应的简单混合物的相应性能大至少25％，其中所述二有机聚硅氧烷不固化， 所述热塑性弹性体的伸长率至少为25％。

    Toughened thermoplastic resins
    6.
    发明授权
    Toughened thermoplastic resins 失效
    增韧热塑性树脂

    公开(公告)号：US06281286B1

    公开(公告)日：2001-08-28

    申请号：US09393029

    申请日：1999-09-09

    申请人： Igor Chorvath ,  Gerald Alphonse Gornowicz ,  David Joseph Romenesko ,  Jeffrey Paul Sage

    发明人： Igor Chorvath ,  Gerald Alphonse Gornowicz ,  David Joseph Romenesko ,  Jeffrey Paul Sage

    IPC分类号： C08G7708

    CPC分类号： C08L77/00 ,  C08L67/02 ,  C08L69/00 ,  C08L77/02 ,  C08L77/06 ,  C08L83/04 ,  C08L2666/14 ,  C08L83/00

    摘要： A thermoplastic composition having a high impact strength is disclosed, said composition being prepared by (I) mixing (A) a thermoplastic selected from a polyester resin or a polyamide resin, (B) a silicone component comprising (B′) a diorganopolysiloxane gum having a plasticity of at least 30 and having an average of at least 2 alkenyl radicals in its molecule and (B″) a fumed silica filler, (C) an organohydrido silicon compound which contains an average of at least 2 silicon-bonded hydrogen groups in its molecule, and (D) a hydrosilation catalyst, components (C) and (D) being present in an amount sufficient to cure said diorganopolysiloxane; and (II) dynamically curing said diorganopolysiloxane gum. When the above composition is based on preferred poly(butylene terephthalate) resins, molded components thereof exhibit an Izod impact strength of at least 14 ft-lb (747 J/m), this high impact strength also being realized by blending the poly(butylene terephthalate) resin with a polycarbonate resin, the fumed silica then being an optional component.

    摘要翻译： 公开了具有高冲击强度的热塑性组合物，所述组合物通过（I）混合（A）选自聚酯树脂或聚酰胺树脂的热塑性树脂制备，（B）含有（B'）二有机聚硅氧烷胶的硅氧烷组分 至少30的塑性，其分子中平均具有至少2个烯基，和（B“）热解法二氧化硅填料，（C）含有平均至少2个与硅键合的氢基团的有机氢化硅化合物 在其分子中，和（D）硅氢化催化剂，组分（C）和（D）以足以固化所述二有机聚硅氧烷的量存在; 当上述组合物基于优选的聚（对苯二甲酸丁二醇酯）树脂时，其模塑组分表现出至少14ft-lb（747J / m）的艾佐德冲击强度，这种高冲击力 强度也通过将聚（对苯二甲酸丁二醇酯）树脂与聚碳酸酯树脂混合而实现，然后热解法二氧化硅是任选的组分。

    Poly(phenylene ether) resin modified with silicone rubber powder
    8.
    发明授权
    Poly(phenylene ether) resin modified with silicone rubber powder 失效
    用硅橡胶​​粉末改性的聚（苯醚）树脂

    公开(公告)号：US5916952A

    公开(公告)日：1999-06-29

    申请号：US975031

    申请日：1997-11-20

    申请人： David Joseph Romenesko ,  Steven Patrick Mullan

    发明人： David Joseph Romenesko ,  Steven Patrick Mullan

    IPC分类号： C08K3/36 ,  C08K5/5419 ,  C08L71/12 ,  C08L83/04 ,  C08K3/00

    CPC分类号： C08L71/123

    摘要： A free-flowing silicone rubber powder, having an average particle size of 1 to 1000 microns and prepared by mixing a polydiorganosiloxane with a silica filler, is uniformly dispersed in a poly(phenylene ether) resin using conventional equipment, such as a single screw or, preferably, a twin screw extruder. When employed at relatively low concentrations, such as about 0.2 to 3 parts by weight of powder per 100 parts by weight of resin, a significant improvement in the processability is obtained, while modification at higher levels, such as 5 to 20 parts by weight of powder per 100 parts by weight of the resin results in a resin composition having greatly augmented impact resistance.

    摘要翻译： 将平均粒度为1-1000微米并通过将聚二有机硅氧烷与二氧化硅填料混合而制备的自由流动的硅橡胶粉末使用常规设备如单螺杆或均匀分散在聚苯醚树脂中， ，优选双螺杆挤出机。 当以相对低的浓度使用例如每100重量份树脂约0.2-3重量份的粉末时，可获得加工性的显着改善，而在较高水平下进行改性，例如5至20重量份 粉末每100重量份的树脂导致具有极大增强的耐冲击性的树脂组合物。

    Polyolefin composition containing diorganopolysiloxane process aid
    9.
    发明授权
    Polyolefin composition containing diorganopolysiloxane process aid 失效
    含有二有机聚硅氧烷加工助剂的聚烯烃组合物

    公开(公告)号：US5789473A

    公开(公告)日：1998-08-04

    申请号：US404739

    申请日：1995-01-24

    申请人： Dale Earl Hauenstein ,  David Joseph Romenesko

    发明人： Dale Earl Hauenstein ,  David Joseph Romenesko

    IPC分类号： C08L23/00 ,  C08J3/20 ,  C08L23/02 ,  C08L23/08 ,  C08L83/04 ,  C08L87/00 ,  C08J5/32

    CPC分类号： C08L23/02 ,  C08L23/06 ,  C08L23/0815 ,  C08L2207/066 ,  C08L83/04 ,  Y10T428/31855 ,  Y10T428/31913

    摘要： There is disclosed a polyolefin composition which can be extruded at relatively high rates to provide extrudate having a low surface roughness (sharkskin), said composition comprising (A) 100 parts by weight of a polyolefin resin; and (B) 0.01 to 1 part by weight of a hydroxy-functional diorganopolysiloxane process aid, said diorganopolysiloxane having a number average molecular weight of at least 10,000. In particularly preferred embodiments, a hydroxy-functional diorganopolysiloxane in combination with a low density polyethylene is used as a process aid for linear low density polyethylene.

    摘要翻译： 公开了可以以相对高的速率挤出以提供具有低表面粗糙度（鲨鱼皮）的挤出物的聚烯烃组合物，所述组合物包含（A）100重量份的聚烯烃树脂; 和（B）0.01至1重量份的羟基官能二有机聚硅氧烷加工助剂，所述二有机聚硅氧烷的数均分子量至少为10,000。 在特别优选的实施方案中，将羟基官能二有机聚硅氧烷与低密度聚乙烯组合用作线性低密度聚乙烯的加工助剂。

    Thermoplastic silicone elastomers
    10.
    发明授权
    Thermoplastic silicone elastomers 失效
    热塑性硅橡胶

    公开(公告)号：US6013715A

    公开(公告)日：2000-01-11

    申请号：US34089

    申请日：1998-03-03

    申请人： Gerald Alphonse Gornowicz ,  Kevin Edward Lupton ,  David Joseph Romenesko ,  Kim Struble ,  Hongxi Zhang

    发明人： Gerald Alphonse Gornowicz ,  Kevin Edward Lupton ,  David Joseph Romenesko ,  Kim Struble ,  Hongxi Zhang

    IPC分类号： C08L23/02 ,  C08L23/04 ,  C08L67/02 ,  C08L83/04 ,  C08K3/00

    CPC分类号： C08L23/02 ,  C08L23/04 ,  C08L23/10 ,  C08L67/02 ,  C08L2312/00 ,  C08L83/04

    摘要： There is disclosed a method for preparing a thermoplastic elastomer, said method comprising:(I) mixing(A) a thermoplastic resin selected from the group consisting of a polyolefin and a poly(butylene terephthalate),(B) a diorganopolysiloxane having a plasticity of at least 30 and having an average of at least 2 alkenyl radicals in its molecule,(C) an organohydrido silicon compound which contains an average of at least 2 silicon-bonded hydrogen groups in its molecule,(D) optionally, a reinforcing filler and(E) a hydrozilation catalyst; and(II) dynamically curing said diorganopolysiloxane (B), wherein the amount of said diorganopolysiloxane (B) used is such that at least one property of the thermoplastic elastomer selected from tensile strength or elongation is at least 25% greater than the respective property for a corresponding simple blend wherein said diorganopolysiloxane is not cured.

    摘要翻译： 公开了一种制备热塑性弹性体的方法，所述方法包括：（I）将（A）选自聚烯烃和聚（对苯二甲酸丁二醇酯）的热塑性树脂混合，（B）具有可塑性的二有机聚硅氧烷 至少30，并且在其分子中平均具有至少2个烯基，（C）有机氢化硅化合物，其在其分子中平均含有至少2个与硅键合的氢基团，（D）任选的增强填料和 （E）氢化齐平催化剂; 和（II）动态固化所述二有机聚硅氧烷（B），其中使用的所述二有机基聚硅氧烷（B）的量使得选自拉伸强度或伸长率的热塑性弹性体的至少一种性质比相对于 相应的简单混合物，其中所述二有机聚硅氧烷不固化。