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    Catalysts and method for the production of amines
    2.
    发明授权
    Catalysts and method for the production of amines 有权
    用于生产胺的催化剂和方法

    公开(公告)号：US07183438B2

    公开(公告)日：2007-02-27

    申请号：US10507602

    申请日：2003-03-07

    申请人： Till Gerlach ,  Frank Funke ,  Johann-Peter Melder ,  Stefan Iselborn ,  Martin Rudloff ,  Michael Hüllmann

    发明人： Till Gerlach ,  Frank Funke ,  Johann-Peter Melder ,  Stefan Iselborn ,  Martin Rudloff ,  Michael Hüllmann

    IPC分类号： C07C209/16 ,  C07C209/18 ,  C07C209/29 ,  B01J23/40 ,  B01J23/42

    CPC分类号： C07C213/02 ,  B01J23/70 ,  B01J23/755 ,  B01J37/03 ,  B01J37/06 ,  C07C209/16 ,  C07C209/26 ,  C07D295/023 ,  C07C211/03 ,  C07C217/08

    摘要： Disclosed are catalysts, the catalytically active mass of which contains 22 to 40 percent by weight of oxygen-containing compounds of zirconium, calculated as ZrO2, 1 to 30 percent by weight of oxygen-containing compounds of copper, calculated as CuO, 15 to 50 percent by weight of oxygen-containing compounds of nickel, calculated as NiO, the molar ratio between nickel and copper being greater than 1, 15 to 50 percent by weight of oxygen-containing compounds of cobalt, calculated as CoO, and less than 1 percent by weight of an alkali metal, calculated as alkali metal oxide, prior to being treated with hydrogen. Also disclosed is a method for the production of amines by reacting primary and secondary alcohols, aldehydes, or ketones with hydrogen and nitrogen compounds selected from the group ammonia, primary and secondary amines, in the presence of said catalysts at an elevated temperature and an elevated pressure.

    摘要翻译： 公开了催化剂，其催化活性物质含有22至40重量％的以ZrO 2计算的含氧化合物的锆，1至30重量％的含氧化合物的铜 ，以CuO计，15至50重量％的含氧化合物的镍，以NiO计算，镍和铜之间的摩尔比大于15重量％，含氧化合物的化合物为15至50重量％ 作为CoO，并且在用氢处理之前少于1重量％的碱金属（以碱金属氧化物计）。 还公开了一种通过使伯醇和仲醇，醛或酮与选自氨，伯胺和仲胺的氢和氮化合物在所述催化剂存在下在升高的温度和升高的温度下生产胺的方法 压力。

    METHOD FOR ISOMERIZING OLEFINS
    4.
    发明申请
    METHOD FOR ISOMERIZING OLEFINS 审中-公开
    异烯烃方法

    公开(公告)号：US20100286458A1

    公开(公告)日：2010-11-11

    申请号：US12738034

    申请日：2008-10-15

    申请人： Stefan Iselborn ,  Thomas Heidemann

    发明人： Stefan Iselborn ,  Thomas Heidemann

    IPC分类号： C07C5/03 ,  C07C5/25

    CPC分类号： C07C11/06 ,  C07C5/2512 ,  C07C6/04 ,  C07C2521/04 ,  C07C2523/85 ,  C07C2523/885 ,  C07C2523/888 ,  C07C11/08

    摘要： The present invention relates to a process for isomerizing olefins in olefin-comprising hydrocarbon mixtures having from 4 to 20 carbon atoms at temperatures of from 20 to 200° C. and pressures of from 1 to 200 bar in the liquid phase in the presence of a heterogeneous catalyst, wherein a catalyst comprising from 1 to 20% by weight of nickel in oxidic form and from 1 to 20% by weight of at least one element of group VIB on an aluminum oxide support is used.

    摘要翻译： 本发明涉及一种使含烯烃的烃混合物中的烯烃异构化的方法，该烃混合物在20〜200℃的温度和1〜200巴的压力下，在液相中，在 使用非均相催化剂，其中使用包含1至20重量％的氧化物形式的镍和1至20重量％的至少一种氧化铝载体上VIB族元素的催化剂。

    REACTOR FOR PERFORMING A THREE-PHASE REACTION OF A FLUID AND A GASEOUS PHASE ON A PACKED BED CATALYST
    8.
    发明申请
    REACTOR FOR PERFORMING A THREE-PHASE REACTION OF A FLUID AND A GASEOUS PHASE ON A PACKED BED CATALYST 有权
    用于在包装床催化剂上进行流体和气相的三相反应的反应器

    公开(公告)号：US20100185032A1

    公开(公告)日：2010-07-22

    申请号：US12665533

    申请日：2008-06-20

    申请人： Stefan Iselborn ,  Andreas Daiss ,  Reiner Geier ,  Marcus Bechtel ,  Michael Wille ,  Benjamin Hepfer

    发明人： Stefan Iselborn ,  Andreas Daiss ,  Reiner Geier ,  Marcus Bechtel ,  Michael Wille ,  Benjamin Hepfer

    IPC分类号： C07C5/03 ,  B01F3/04 ,  B01J8/02

    CPC分类号： B01J8/008 ,  B01J8/025 ,  B01J8/0278 ,  B01J8/0453 ,  B01J8/0492 ,  B01J2208/00548 ,  C07C7/167 ,  C10G2400/20 ,  C07C11/08

    摘要： A reactor (R) for carrying out a three-phase reaction of a liquid phase (1) and a gaseous phase (2) over a fixed catalyst bed (F), with the fixed catalyst bed (F) being arranged horizontally in the reactor (R) and the liquid phase (1) and the gaseous phase (2) being passed through the reactor (R) in cocurrent from the top downward via a mixing and distribution device (MD) over the fixed catalyst bed (F), wherein the mixing and distribution device (MD) comprises a trough distributor (TD) for the liquid phase (1) having trough-shaped channels (C) and outlet tubes (O) in the trough-shaped channels (C) for the liquid phase (1) and a distributor plate (P) which is arranged with a spacing below the trough distributor (TD) and in which vertical nozzles (N) having one or more openings (P1) for entry of the gaseous phase (2) and one or more openings (P2), which are arranged below the openings (P1) for entry of the gaseous phase, for entry of the liquid phase (1) into the nozzles (N) are installed, with the number and size of the openings (P2) for entry of the liquid phase (1) being designed so that, at a predetermined liquid feed rate, the surface of the liquid on the distributor plate (P) is established below the openings (P1) for entry of the gaseous phase (2) and above the openings (P2) for entry of the liquid phase (1), is proposed.

    摘要翻译： 用于在固定的催化剂床（F）上进行液相（1）和气相（2）的三相反应的反应器（R），其中固定的催化剂床（F）在反应器中水平布置 （R）和液相（1）和气相（2）通过混合和分配装置（MD）从顶部向下并流通过反应器（R），其中固定催化剂床（F），其中 混合和分配装置（MD）包括用于液相（1）的槽分配器（TD），其具有用于液相的槽形通道（C）中的槽形通道（C）和出口管（O） 1）和分配器板（P），其布置在槽分配器（TD）下方的间隔处，并且其中具有用于进入气相（2）的一个或多个开口（P1）的垂直喷嘴（N）和一个或 布置在用于进入气相的开口（P1）下方的用于将液相（1）进入喷嘴（N）的更多的开口（P2）被安装 其中液相（1）进入的开口（P2）的数量和尺寸被设计成使得以预定的液体进给速率将分配器板（P）上的液体的表面建立在 提出了用于进入液相（2）的气相（2）和用于进入液相（1）的开口（P2）上方的开口（P1）。