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    AMMONIA DECOMPOSITION CATALYST
    1.
    发明申请
    AMMONIA DECOMPOSITION CATALYST 审中-公开
    氨基酸分解催化剂

    公开(公告)号：US20110306489A1

    公开(公告)日：2011-12-15

    申请号：US13203376

    申请日：2010-02-18

    申请人： Susumu Hikazudani ,  Takuma Mori ,  Chikashi Inazumi ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Hironobu Kumagai

    发明人： Susumu Hikazudani ,  Takuma Mori ,  Chikashi Inazumi ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Hironobu Kumagai

    IPC分类号： B01J21/18

    CPC分类号： C01B3/047 ,  B01J21/18 ,  B01J21/185 ,  B01J23/462 ,  B01J23/745 ,  B01J35/0046 ,  B01J35/0053 ,  B01J37/0201 ,  B01J37/08 ,  B01J37/086 ,  B01J37/18 ,  B82Y30/00 ,  C08G14/06 ,  C08L61/04 ,  Y02E60/364

    摘要： Disclosed is an ammonia decomposition catalyst which is obtained by heat-treating a complex at a temperature of 360° C. to 900° C. in a reducing atmosphere, wherein the complex containing a polymer having a molecular weight of 1,000 to 500,000 represented by the formula [I], a transition metal coordinated with the polymer, and an activated carbon or a carbon nanotube added thereto. In a case of using the carbon nanotube, an alkali metal compound or an alkaline earth metal compound is added to the heat-treated complex. R1 represents H or hydrocarbon having 1 to 10 carbon atoms, R2 and R3 each represent H, halogen, nitro, acyl, ester, carboxyl, formyl, nitrile, sulfone, aryl, or alkyl group having 1 to 15 carbon atoms, X and Y each represent H or OH, Z represents CH or N, R4 and R5 each represent H, OH, ether, amino, aryl, or alkyl group having 1 to 15 carbon atoms, x represents a real number of 1 to 2, y represents a real number of 1 to 3, and n represents a real number of 2 to 120. The amount of the transition metal deposited on the catalyst can be increased without deteriorating the dispersion of the metal, so that the amount of the catalyst required to obtain a desired activity can be reduced.

    摘要翻译： 公开了一种氨还原催化剂，其通过在还原气氛中在360℃至900℃的温度下热处理络合物获得，其中所述络合物含有分子量为1,000至500,000的聚合物，其由 式[I]，与聚合物配位的过渡金属，和加入其中的活性炭或碳纳米管。 在使用碳纳米管的情况下，向热处理复合体中添加碱金属化合物或碱土金属化合物。 R1表示H或碳原子数1〜10的烃，R2和R3各自表示H，卤素，硝基，酰基，酯，羧基，甲酰基，腈，砜，芳基或碳原子数1〜15的烷基，X和Y 各自表示H或OH，Z表示CH或N，R 4和R 5各自表示H，OH，醚，氨基，芳基或具有1至15个碳原子的烷基，x表示1至2的实数，y表示 实数1〜3，n表示2〜120的实数。可以提高沉积在催化剂上的过渡金属的量，而不会使金属的分散性恶化，从而获得所需催化剂的量 可以减少所需的活动。

    Ammonia synthesis process
    4.
    发明授权
    Ammonia synthesis process 失效
    氨合成工艺

    公开(公告)号：US08623313B2

    公开(公告)日：2014-01-07

    申请号：US13143619

    申请日：2009-12-22

    申请人： Norihiko Nakamura ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Chikashi Inazumi

    发明人： Norihiko Nakamura ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Chikashi Inazumi

    IPC分类号： C01C1/04

    CPC分类号： C01B3/042 ,  B01J35/004 ,  C01B3/025 ,  C01B3/061 ,  C01B3/063 ,  C01B3/501 ,  C01B3/56 ,  C01B5/00 ,  C01B13/0207 ,  C01B13/0251 ,  C01B13/0281 ,  C01B2203/042 ,  C01B2203/068 ,  C01B2210/0053 ,  C01C1/0405 ,  Y02E60/364 ,  Y02P20/134 ,  Y02P20/52

    摘要： The invention provides a process for efficient synthesis of ammonia. The process includes a water-splitting step in which water is decomposed to obtain a first source gas comprising hydrogen and oxygen, a first oxygen removal step in which the oxygen contained in the first source gas is at least partially separated and removed by an oxygen separating membrane or hydrogen separating membrane to obtain a second source gas having a lower oxygen concentration than the first source gas, a second oxygen removal step in which the oxygen in the second source gas is reacted with hydrogen to produce water for removal, or is adsorbed onto an adsorption medium for removal, to obtain a third source gas having a lower oxygen concentration than the second source gas, and an ammonia synthesis step in which the hydrogen in the third source gas is reacted with nitrogen to synthesize ammonia.

    摘要翻译： 本发明提供了一种有效合成氨的方法。 该方法包括水分解步骤，其中水被分解以获得包含氢和氧的第一源气体，第一氧除去步骤，其中通过氧分离将至少部分地分离和除去第一源气体中所含的氧 膜或氢分离膜，以获得具有比第一源气体低的氧浓度的第二源气体;第二氧除去步骤，其中第二源气体中的氧与氢反应以产生除去水或吸附到 用于除去的吸附介质，以获得具有比第二源气体低的氧浓度的第三源气体，以及氨合成步骤，其中第三源气体中的氢与氮反应以合成氨。

    Ammonia synthesis process
    6.
    发明授权
    Ammonia synthesis process 有权

    公开(公告)号：US08585996B2

    公开(公告)日：2013-11-19

    申请号：US13143619

    申请日：2009-12-22

    申请人： Norihiko Nakamura ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Chikashi Inazumi

    发明人： Norihiko Nakamura ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Chikashi Inazumi

    IPC分类号： C01C1/04

    摘要： The invention provides a process for efficient synthesis of ammonia. The process includes a water-splitting step in which water is decomposed to obtain a first source gas comprising hydrogen and oxygen, a first oxygen removal step in which the oxygen contained in the first source gas is at least partially separated and removed by an oxygen separating membrane or hydrogen separating membrane to obtain a second source gas having a lower oxygen concentration than the first source gas, a second oxygen removal step in which the oxygen in the second source gas is reacted with hydrogen to produce water for removal, or is adsorbed onto an adsorption medium for removal, to obtain a third source gas having a lower oxygen concentration than the second source gas, and an ammonia synthesis step in which the hydrogen in the third source gas is reacted with nitrogen to synthesize ammonia.

    Ammonia synthesis apparatus and process
    7.
    发明授权
    Ammonia synthesis apparatus and process 有权
    氨合成装置及工艺

    公开(公告)号：US08597583B2

    公开(公告)日：2013-12-03

    申请号：US12705056

    申请日：2010-02-12

    申请人： Haruyuki Nakanishi ,  Norihiko Nakamura ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Sadao Araki ,  Chikashi Inazumi

    发明人： Haruyuki Nakanishi ,  Norihiko Nakamura ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Sadao Araki ,  Chikashi Inazumi

    IPC分类号： C01C1/00 ,  B01J19/00 ,  B01J8/00 ,  C01B21/00 ,  C01C1/04

    CPC分类号： C01C1/0405 ,  B01J7/02 ,  B01J8/009 ,  B01J8/0423 ,  B01J8/0496 ,  B01J2208/00168 ,  C01B3/025 ,  C01B3/061 ,  C01B3/08 ,  C01B13/0251 ,  C01B2210/0046 ,  C01C1/0417 ,  Y02E60/36 ,  Y02P20/52

    摘要： An ammonia synthesis apparatus includes: a first gas channel; a second gas channel disposed outside the first gas channel; a third gas channel disposed outside the second gas channel; an air supply unit that supplies air to the second or third gas channel; a water supply unit that supplies water to the first gas channel; and a heat supply unit that supplies heat to the first gas channel. A metal or a metal oxide that reduces water to produce hydrogen is placed in the first gas channel. An ammonia synthesis catalyst is placed in the second gas channel located downstream of the downstream end portion of the first gas channel. The second and third gas channels are at least partially partitioned by an oxygen permeation membrane, or a nitrogen permeation membrane, so that oxygen is supplied to the third gas channel, and nitrogen is supplied to the second gas channel.

    摘要翻译： 氨合成装置包括：第一气体通道; 设置在第一气体通道外侧的第二气体通道; 设置在所述第二气体通道外侧的第三气体通道; 空气供应单元，其向第二或第三气体通道供应空气; 供水单元，其向第一气体通道供水; 以及向第一气体通道供热的供热单元。 减少水以产生氢的金属或金属氧化物被放置在第一气体通道中。 氨合成催化剂被放置在位于第一气体通道的下游端部下游的第二气体通道中。 第二和第三气体通道至少部分地被氧气渗透膜或氮气渗透膜分隔开，使得向第三气体通道供应氧气，并且向第二气体通道供应氮气。

    AMMONIA SYNTHESIS PROCESS
    9.
    发明申请
    AMMONIA SYNTHESIS PROCESS 失效
    氨基酸合成方法

    公开(公告)号：US20110286907A1

    公开(公告)日：2011-11-24

    申请号：US13143619

    申请日：2009-12-22

    申请人： Norihiko Nakamura ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Chikashi Inazumi

    发明人： Norihiko Nakamura ,  Haruyuki Nakanishi ,  Hidekazu Arikawa ,  Susumu Hikazudani ,  Chikashi Inazumi

    IPC分类号： C01C1/04

    CPC分类号： C01B3/042 ,  B01J35/004 ,  C01B3/025 ,  C01B3/061 ,  C01B3/063 ,  C01B3/501 ,  C01B3/56 ,  C01B5/00 ,  C01B13/0207 ,  C01B13/0251 ,  C01B13/0281 ,  C01B2203/042 ,  C01B2203/068 ,  C01B2210/0053 ,  C01C1/0405 ,  Y02E60/364 ,  Y02P20/134 ,  Y02P20/52

    摘要： The invention provides a process for efficient synthesis of ammonia. The process includes a water-splitting step in which water is decomposed to obtain a first source gas comprising hydrogen and oxygen, a first oxygen removal step in which the oxygen contained in the first source gas is at least partially separated and removed by an oxygen separating membrane or hydrogen separating membrane to obtain a second source gas having a lower oxygen concentration than the first source gas, a second oxygen removal step in which the oxygen in the second source gas is reacted with hydrogen to produce water for removal, or is adsorbed onto an adsorption medium for removal, to obtain a third source gas having a lower oxygen concentration than the second source gas, and an ammonia synthesis step in which the hydrogen in the third source gas is reacted with nitrogen to synthesize ammonia.

    摘要翻译： 本发明提供了一种有效合成氨的方法。 该方法包括水分解步骤，其中水被分解以获得包含氢和氧的第一源气体，第一氧除去步骤，其中通过氧分离将至少部分地分离和除去第一源气体中所含的氧 膜或氢分离膜，以获得具有比第一源气体低的氧浓度的第二源气体;第二氧除去步骤，其中第二源气体中的氧与氢反应以产生除去水或吸附到 用于除去的吸附介质，以获得具有比第二源气体低的氧浓度的第三源气体，以及氨合成步骤，其中第三源气体中的氢与氮反应以合成氨。