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    Styrene copolymer and process for production thereof
    1.
    发明授权
    Styrene copolymer and process for production thereof 失效
    苯乙烯共聚物及其制备方法

    公开(公告)号：US5391671A

    公开(公告)日：1995-02-21

    申请号：US88523

    申请日：1993-07-09

    申请人： Toshinori Tazaki ,  Masahiko Kuramoto

    发明人： Toshinori Tazaki ,  Masahiko Kuramoto

    IPC分类号： C08F212/04 ,  C08F212/10 ,  C08F212/14

    CPC分类号： C08F212/10 ,  C08F212/04 ,  Y10S526/943

    摘要： A styrene copolymer which comprises a styrene repeating unit (a) represented by the general formula (I): ##STR1## and an acrylonitrile repeating unit (b) represented by the general formula (II-(b)): ##STR2## unsaturated carboxylic acid or its ester repeating unit (c) represented by the general formula (II-(c)): ##STR3## or maleimide or N-substituted maleimide (d) represented by the general formula (II-(d)): ##STR4## (in the formula, symbols are the same as defined in the specification) wherein stereoregularity of the styrene repeating unit (a) chain is a high degree of syndiotactic configuration is disclosed.

    摘要翻译： 包含由通式（I）表示的苯乙烯重复单元（a）：由通式（II-（b））表示的丙烯腈重复单元（b））的苯乙烯共聚物：

    Styrene copolymer and process for production thereof
    2.
    发明授权
    Styrene copolymer and process for production thereof 失效
    苯乙烯共聚物及其制备方法

    公开(公告)号：US5262504A

    公开(公告)日：1993-11-16

    申请号：US598637

    申请日：1990-10-19

    申请人： Toshinori Tazaki ,  Masahiko Kuramoto

    发明人： Toshinori Tazaki ,  Masahiko Kuramoto

    IPC分类号： C08F212/04 ,  C08F212/10 ,  C08F212/08

    CPC分类号： C08F212/10 ,  C08F212/04 ,  Y10S526/943

    摘要： A styrene copolymer which comprises a styrene repeating unit (a) represented by the general formula (I): ##STR1## and an acrylonitrile repeating unit (b) represented by the general formula (II-(b)): ##STR2## an unsaturated carboxylic acid or its ester repeating unit (c) represented by the general formula (II-(c)): ##STR3## or a maleimide or N-substituted maleimide (d) represented by the general formula (II-(d)): ##STR4## (in the formula, symbols are the same as defined in the specification) wherein stereoregularity of the styrene repeating unit (a) chain is a high degree of syndiotactic configuration is disclosed.

    摘要翻译： PCT No.PCT / JP90 / 00371 Sec。 371 1990年10月19日第 102（e）1990年10月19日PCT PCT 1990年3月20日PCT公布。 公开号WO90 / 12039 日本特表1990年10月18日。一种苯乙烯共聚物，其包含由通式（I）表示的苯乙烯重复单元（a）：由通式（II-）表示的丙烯腈重复单元（b） （II-（c））表示的不饱和羧酸或其酯重复单元（c）：（II-（c））： （II-（d））表示的马来酰亚胺或N-取代的马来酰亚胺（d）：（II-（d））（式中，符号与说明书中的定义相同），其中 苯乙烯重复单元（a）链的立构规整性是高程度的间同构型。

    Styrene copolymer and process for production thereof
    3.
    发明授权
    Styrene copolymer and process for production thereof 失效
    苯乙烯共聚物及其制备方法

    公开(公告)号：US5260394A

    公开(公告)日：1993-11-09

    申请号：US582836

    申请日：1990-10-05

    申请人： Toshinori Tazaki ,  Masahiko Kuramoto

    发明人： Toshinori Tazaki ,  Masahiko Kuramoto

    IPC分类号： C08F4/642 ,  C08F210/00 ,  C08F210/02 ,  C08F212/02 ,  C08F212/04 ,  C08F212/08

    CPC分类号： C08F212/04 ,  C08F210/00 ,  C08F212/02 ,  C08F210/02 ,  Y10S526/943

    摘要： A novel styrene copolymer comprising a styrene repeating unit (a) represented by the general formula: ##STR1## (wherein R.sup.1 is a hydrogen atom or a hydrocarbon group having not more than 20 carbon atoms; n is an integer of 1 to 3 and when n is 2 or 3, R.sup.1 s may be the same or different) and olefin repeating unit (b) represented by the general formula: ##STR2## (wherein R.sup.2 is a hydrogen atom or a saturated hydrocarbon group having not more than 20 carbon atoms) or diene repeating unit, which contains 0.1 to 99.9 wt. % of said olefin repeating unit (b) or diene repeating unit (c) wherein intrinsic viscosity measured in 1,2,4-trichlorobenzene at 135.degree. C. is 0.07 to 20 dl/g and the stereoregularity of the styrene repeating unit chain is a high degree of syndiotactic configuration. This styrene copolymer is excellent in heat resistance and chemical resistance, and further it can be injection molded at low temperature, and has good compatibility with other resine and the like.

    摘要翻译： PCT No.PCT / JP90 / 00342 Sec。 371 1990年10月5日第 102（e）1990年10月5日PCT PCT 1990年3月15日PCT公布。 公开号WO90 / 11305 日期：1990年10月4日。一种包含由以下通式表示的苯乙烯重复单元（a）的新型苯乙烯共聚物：其中R 1为氢原子或碳原子数不超过20的烃基; n为 1至3的整数，当n为2或3时，R 1可以相同或不同）和由以下通式表示的烯烃重复单元（b）：其中R 2为氢原子或饱和烃基， 不超过20个碳原子）或二烯重复单元，其含有0.1至99.9重量％ ％的所述烯烃重复单元（b）或二烯重复单元（c），其中在1,2,4-三氯苯中在135℃下测得的特性粘度为0.07-20dl / g，苯乙烯重复单元链的立构规整度为 高程度的间同构型。 该苯乙烯共聚物的耐热性和耐化学性优异，并且还可以在低温下注塑，并且与其它树脂等具有良好的相容性。

    Styrenic block copolymer and process for producing same
    7.
    发明授权
    Styrenic block copolymer and process for producing same 失效
    苯乙烯嵌段共聚物及其制备方法

    公开(公告)号：US5391626A

    公开(公告)日：1995-02-21

    申请号：US63745

    申请日：1993-05-20

    申请人： Shuji Machida ,  Toshinori Tazaki ,  Noriyuki Tani

    发明人： Shuji Machida ,  Toshinori Tazaki ,  Noriyuki Tani

    IPC分类号： B32B27/06 ,  C08F297/06 ,  C08L25/06 ,  C08L53/00 ,  C08L53/02 ,  C08L101/00 ,  C08F4/76 ,  B32B27/28 ,  B32B27/30 ,  C08F297/00

    CPC分类号： C08F297/06 ,  B32B27/06 ,  C08L25/06 ,  Y10T428/31855

    摘要： There are disclosed a styrenic block copolymer having a reduced viscosity of 0.01 to 20 dl/g (0.05 g/l in 1,2,4-trichlorobenzene at 135.degree. C.) which comprises highly syndiotactic styrenic-polymer segments and 10.sup.-4 to 10 mol % of heteroatom-containing styrenic polymer segments; a resin composition comprising the above styrenic block copolymer and a thermoplastic resin, an inorganic filler or an organic filler; a multi-layer material comprising at least one layer composed of the above styrenic block copolymer or the above resin composition; and a process for producing the above styrenic block copolymer which comprises polymerizing a styrenic monomer in the presence of a specific catalyst and adding a heteroatom-containing styrenic monomer to successively proceed with copolymerization reaction. The above-disclosed styrenic block copolymer and the resin composition exhibit excellent compatibility and adhesivenesss, and the multi-layer material is expected to find a wide range of applications in automobile parts, electrical and electronic parts as well as film, sheet, etc.

    摘要翻译： 公开了一种苯乙烯嵌段共聚物，其具有0.01至20dl / g（在135℃下的1,2,4-三氯苯中为0.05g / l），其包含高度间同立构的苯乙烯 - 聚合物链段，并且10-4至 10mol％的含杂原子的苯乙烯聚合物链段; 包含上述苯乙烯嵌段共聚物和热塑性树脂，无机填料或有机填料的树脂组合物; 包括由上述苯乙烯嵌段共聚物或上述树脂组合物构成的至少一层的多层材料; 以及上述苯乙烯系嵌段共聚物的制造方法，其特征在于，在特定催化剂存在下使苯乙烯类单体聚合，加入含杂原子的苯乙烯类单体，进行共聚反应。 上述公开的苯乙烯嵌段共聚物和树脂组合物表现出优异的相容性和粘合性，多层材料预期在汽车部件，电气和电子部件以及薄膜，片材等方面可以广泛应用。

    Graft copolymer and process for producing the same
    8.
    发明授权
    Graft copolymer and process for producing the same 失效
    接枝共聚物及其制备方法

    公开(公告)号：US5250629A

    公开(公告)日：1993-10-05

    申请号：US802840

    申请日：1991-12-06

    申请人： Noriyuki Tani ,  Shuji Machida ,  Toshinori Tazaki

    发明人： Noriyuki Tani ,  Shuji Machida ,  Toshinori Tazaki

    IPC分类号： B32B27/06 ,  C08F257/02 ,  C08F4/00

    CPC分类号： B32B27/06 ,  C08F257/02 ,  Y10S526/943

    摘要： There is provided a process for producing a styrenic graft copolymer which comprises coplymerizing a styrenic monomer and a styrenic monomer having a hydrocarbon radical with an unsaturated bond in the presence of a catalyst comprising as primary ingredient (A) a transition metal compound and (B) a contact product of an organoaluminum compound and a condensation agent or (C) a compound which produces an ionic complex by reacting with the above-mentioned transition metal compound and subsequently graft polymerizing an ethylenically unsaturated monomer onto the resultant styrenic copolymer.The above-described styrenic graft copolymer is greatly improved in terms of compatibility, adhesivity, coatability and wettability while preserving heat resistance and chemical resistance thereof, and thus effective as a variety of constructional materials and compatibilizing agents. Furthermore, the composition or multi-layer material comprising the above-mentioned styrenic graft copolymer is widely utilized in a variety of application field including film, sheet, especially stampable sheet, container, packaging material, automobile parts, electrical and electronic parts, etc.