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    Apparatuses and methods for deoxygenating biomass-derived pyrolysis oil
    1.
    发明授权
    Apparatuses and methods for deoxygenating biomass-derived pyrolysis oil 有权
    用于脱氧生物质衍生的热解油的设备和方法

    公开(公告)号：US09222037B2

    公开(公告)日：2015-12-29

    申请号：US13676281

    申请日：2012-11-14

    申请人： UOP LLC

    发明人： Tom N. Kalnes

    IPC分类号： C07C1/20 ,  C10G1/00 ,  C10G49/00 ,  C10G3/00

    CPC分类号： C10G49/00 ,  C10G3/00 ,  C10G3/42 ,  C10G3/50 ,  C10G65/04 ,  C10G2300/4006 ,  Y02P30/20

    摘要： Apparatuses and methods for deoxygenating a biomass-derived pyrolysis oil are provided herein. In one example, the method comprises of dividing a feedstock stream into first and second feedstock portions. The feedstock stream comprises the biomass-derived pyrolysis oil and has a temperature of about 60° C. or less. The first feedstock portion is combined with a heated organic liquid stream to form a first heated diluted pyoil feed stream. The first heated diluted pyoil feed stream is contacted with a first deoxygenating catalyst in the presence of hydrogen to form an intermediate low-oxygen pyoil effluent. The second feedstock portion is combined with the intermediate low-oxygen pyoil effluent to form a second heated diluted pyoil feed stream. The second heated diluted pyoil feed stream is contacted with a second deoxygenating catalyst in the presence of hydrogen to form additional low-oxygen pyoil effluent.

    摘要翻译： 本文提供了用于脱氧生物质衍生的热解油的设备和方法。 在一个实例中，该方法包括将原料流分成第一和第二原料部分。 原料流包含生物质衍生的热解油，其温度为约60℃或更低。 将第一原料部分与加热的有机液体流合并以形成第一加热的稀释的原料流。 在氢的存在下，将第一加热的稀释的原料流与第一脱氧催化剂接触以形成中间体低氧钚流出物。 将第二原料部分与中间体低氧酚流出物混合以形成第二加热的稀释的原料流。 在氢的存在下，将第二加热的稀释的原料流与第二脱氧催化剂接触以形成另外的低氧钚流出物。

    INTEGRATED PROCESS FOR NORMAL PARAFFIN ALKYLATION
    3.
    发明申请
    INTEGRATED PROCESS FOR NORMAL PARAFFIN ALKYLATION 审中-公开
    用于正常PARAFFIN ALKYLATION的集成过程

    公开(公告)号：US20160168053A1

    公开(公告)日：2016-06-16

    申请号：US14567749

    申请日：2014-12-11

    申请人： UOP LLC

    发明人： Tom N. Kalnes ,  Stuart Smith ,  Alakananda Bhattacharyya ,  Mary Wier

    IPC分类号： C07C6/10 ,  C07C2/60 ,  C07C2/62

    CPC分类号： C07C6/10 ,  C07C2/60 ,  C07C2/62 ,  C07C7/04 ,  C07C2521/04 ,  C07C2523/42 ,  C07C2527/054 ,  C07C2527/10 ,  C07C2527/1206 ,  C07C2531/02 ,  C07C2531/025 ,  Y02P20/125 ,  C07C9/12 ,  C07C9/16

    摘要： An integrated alkylation and disproportionation process and apparatus are described. n-C4 and n-C5 are routed to a disproportionation reaction zone for conversion to iso-C4 and C6+ isoparaffin-rich product. The iso-C4 is routed to an alkylation reaction zone and reacted with refinery propylene and butenes to produce alkylate product. The C6+ isoparaffin-rich product and alkylate product are recovered. Unconverted iso-C4 and/or olefins are recycled to the alkylation reaction zone, and unconverted n-C4 and n-C5 are recycled to the disproportionation reaction zone.

    摘要翻译： 描述了一体化的烷基化和歧化过程和装置。 n-C4和n-C5被引导到歧化反应区，以转化为异C4和C6 +富含异构石蜡的产物。 异C4被引导至烷基化反应区，并与炼油丙烯和丁烯反应产生烷基化产物。 回收C6 +异链烷烃富产物和烷基化物产物。 未转化的异C4和/或烯烃被再循环到烷基化反应区，未转化的n-C4和n-C5被再循环到歧化反应区。

    INTEGRATED PROCESS FOR GASOLINE PRODUCTION
    5.
    发明申请
    INTEGRATED PROCESS FOR GASOLINE PRODUCTION 审中-公开
    汽油生产综合工艺

    公开(公告)号：US20160168054A1

    公开(公告)日：2016-06-16

    申请号：US14567804

    申请日：2014-12-11

    申请人： UOP LLC

    发明人： Tom N. Kalnes ,  Stuart Smith ,  Douglas A. Nafis ,  Alakananda Bhattacharyya ,  Bryan K. Glover ,  Susie C. Martins

    IPC分类号： C07C6/10 ,  C07C2/62 ,  C07C2/60

    CPC分类号： B01J31/00 ,  B01J31/0288 ,  B01J31/0298 ,  B01J2231/32 ,  C07C6/10 ,  C10G29/205 ,  C10G2400/02

    摘要： An integrated process for gasoline production is described. The process includes introducing a feed comprising n-C5 hydrocarbons into a disproportionation reaction zone in the presence of a disproportionation catalyst to form a disproportionation mixture comprising iso-C4 and C6+ disproportionation products and unreacted n-C5 hydrocarbons. An iso-C4 hydrocarbon stream and an olefin feed are introduced into an alkylation reaction zone in the presence of an alkylation catalyst to produce an alkylation mixture comprising alkylate and unreacted iso-C4 paraffins. The disproportionation mixture and the alkylation mixture are combined, and the combined mixture is separated into at least a stream comprising the alkylate product, an iso-C4 stream, and an unreacted n-C5 hydrocarbon stream. The iso-C4 stream is recycled to the alkylation reaction zone, and the unreacted n-C5 hydrocarbon stream is recycled to the disproportionation reaction zone. The stream comprising the alkylate product is recovered.

    摘要翻译： 描述了汽油生产的综合过程。 该方法包括在歧化催化剂存在下将包含n-C 5烃的进料引入歧化反应区以形成包含异C4和歧化歧化产物和未反应的n-C 5烃的歧化混合物。 在烷基化催化剂存在下将异C4烃流和烯烃进料引入烷基化反应区，以产生包含烷基化物和未反应的异C4链烷烃的烷基化混合物。 将歧化混合物和烷基化混合物合并，并将合并的混合物分离成至少包含烷基化物产物，异C4流和未反应的n-C 5烃流的物流。 将异C4流再循环至烷基化反应区，将未反应的n-C5烃流循环至歧化反应区。 回收包含烷基化产物的料流。

    SYSTEMS AND METHODS FOR HYDROGEN SELF-SUFFICIENT PRODUCTION OF RENEWABLE HYDROCARBONS
    6.
    发明申请
    SYSTEMS AND METHODS FOR HYDROGEN SELF-SUFFICIENT PRODUCTION OF RENEWABLE HYDROCARBONS 审中-公开
    氢能自由生产可再生烃的系统和方法

    公开(公告)号：US20150344382A1

    公开(公告)日：2015-12-03

    申请号：US14292527

    申请日：2014-05-30

    申请人： UOP LLC

    发明人： Donald A. Eizenga ,  Daniel L. Ellig ,  Tom N. Kalnes

    IPC分类号： C07C1/207

    CPC分类号： C07C1/2078 ,  C01B3/38 ,  C01B2203/0233 ,  C01B2203/0244 ,  C01B2203/0261 ,  C01B2203/065 ,  C01B2203/1258 ,  C01B2203/1264 ,  C01B2203/148 ,  C10G3/48 ,  C10G3/49 ,  C10G3/50 ,  C10G2300/1011 ,  C10G2400/02 ,  C10G2400/04 ,  C10G2400/08 ,  Y02P30/20

    摘要： Methods and systems for hydrogen self-sufficient production of hydrocarbons from a renewable feedstock are provided. An exemplary method includes providing a renewable feedstock; contacting the renewable feedstock and hydrogen from a hydrogen stream with one or more catalysts to generate an effluent comprising n-paraffins and by-product hydrocarbons having 9 or fewer carbon atoms; separating the by-product hydrocarbons from the effluent to generate a hydrocarbon by-product stream; and feeding the hydrocarbon by-product stream to a hydrogen plant to generate the hydrogen stream. In this exemplary embodiment, the by-product hydrocarbons constitute the entire feed and fuel of the hydrogen plant, and wherein no hydrogen is added from an external source.

    摘要翻译： 提供了从可再生原料氢气自给自足生产碳氢化合物的方法和系统。 示例性方法包括提供可再生原料; 使来自氢气流的可再生原料和氢与一种或多种催化剂接触以产生包含具有9个或更少碳原子的正链烷烃和副产物烃的流出物; 将副产物烃与流出物分离以产生烃副产物流; 并将烃副产物流进料到氢气装置以产生氢气流。 在该示例性实施方案中，副产物烃构成氢气厂的整个进料和燃料，并且其中不从外部来源加入氢。

    COMBINED NAPHTHA REFINING AND BUTANE UPGRADING PROCESS
    7.
    发明申请
    COMBINED NAPHTHA REFINING AND BUTANE UPGRADING PROCESS 审中-公开
    组合的石墨精制和丁醇升级方法

    公开(公告)号：US20150299593A1

    公开(公告)日：2015-10-22

    申请号：US14257789

    申请日：2014-04-21

    申请人： UOP LLC

    发明人： Tom N. Kalnes ,  Stuart Smith ,  Hayim Abrevaya ,  Mary Wier ,  Alakananda Bhattacharyya

    IPC分类号： C10L1/04

    CPC分类号： C10G69/02 ,  C10G63/00 ,  C10G69/00 ,  C10G69/123

    摘要： A process for refining naphtha and upgrading butanes is described. The process involves separating a hydrotreated heavy naphtha feed into a C7-rich fraction and a C8+-rich fraction in a separation zone and then reacting the C7-rich fraction with C4 paraffins to form to a low aromatic gasoline blendstock. The C8+-rich fraction is sent to a reforming zone to form a reformed product with higher octane and lower RVP than a reformed product derived from heavy naphtha.

    摘要翻译： 描述了精制石脑油和升级丁烷的方法。 该方法包括将加氢处理的重质石脑油进料在分离区中分离成富含C7的级分和富含C8 +的馏分，然后使富含C7的馏分与C4链烷烃反应，形成低芳烃汽油混合原料。 将富含C8 +的级分送入重整区，以形成具有较高辛烷值和较低RVP的重整产物，而不是衍生自重质石脑油的重整产物。

    METHODS OF AND APPARATUSES FOR UPGRADING A HYDROCARBON STREAM INCLUDING A DEOXYGENATED PYROLYSIS PRODUCT
    8.
    发明申请
    METHODS OF AND APPARATUSES FOR UPGRADING A HYDROCARBON STREAM INCLUDING A DEOXYGENATED PYROLYSIS PRODUCT 审中-公开
    用于升级包含脱氧热解产物的烃流的方法和装置

    公开(公告)号：US20140336427A1

    公开(公告)日：2014-11-13

    申请号：US13890343

    申请日：2013-05-09

    申请人： UOP LLC

    发明人： Lance Awender Baird ,  Douglas B. Galloway ,  Tom N. Kalnes

    IPC分类号： C10G1/00

    CPC分类号： C10G21/28 ,  C10G3/40 ,  C10G21/00 ,  C10G2300/1011 ,  Y02P30/20

    摘要： Methods of and apparatuses for upgrading a hydrocarbon stream are provided. In an embodiment, a method of upgrading a hydrocarbon stream includes providing the hydrocarbon stream that includes a deoxygenated pyrolysis product. The hydrocarbon stream also includes a residual oxygen-containing compound content. The residual oxygen-containing compound content of the hydrocarbon stream is reduced to form an upgraded hydrocarbon stream.

    摘要翻译： 提供了用于升级烃流的方法和装置。 在一个实施方案中，改进烃流的方法包括提供包含脱氧热解产物的烃流。 烃流还包括残留的含氧化合物含量。 烃流的残余含氧化合物含量减少以形成升级的烃流。

    CATALYTIC PYROLYSIS OF BIOMASS USING A MULTI-STAGE CATALYST REGENERATOR
    9.
    发明申请
    CATALYTIC PYROLYSIS OF BIOMASS USING A MULTI-STAGE CATALYST REGENERATOR 审中-公开
    使用多级催化剂再生器的生物质催化热解

    公开(公告)号：US20140318944A1

    公开(公告)日：2014-10-30

    申请号：US13870884

    申请日：2013-04-25

    申请人： UOP LLC

    发明人： Lance A. Baird ,  Tom N. Kalnes ,  Douglas B. Galloway

    IPC分类号： B01J38/20 ,  C10B57/00

    CPC分类号： B01J38/20 ,  B01J29/90 ,  B01J38/12 ,  C08H8/00 ,  C10B49/22 ,  C10B53/02 ,  C10B57/06 ,  C10G3/57 ,  C10G3/60 ,  C10G3/62 ,  C10G11/182 ,  C10G11/187 ,  C10G2300/1011 ,  C10G2300/70 ,  C10G2400/02 ,  C10G2400/04 ,  C10G2400/06 ,  Y02E50/14 ,  Y02P20/145 ,  Y02P20/584 ,  Y02P30/20

    摘要： Disclosed in one embodiment is a method for the catalytic pyrolysis of a carbonaceous material that includes contacting the carbonaceous material with a plurality of catalyst particles to produce a gas phase product and a solid phase product and separating the gas phase product from the solid phase product and the plurality of catalyst particles. The method further includes partially regenerating the plurality of catalyst particles by exposing the solid phase product and the catalyst particles to a first oxidizing condition to produce an oxidized solid phase and a partially-regenerated catalyst and cooling the partially-regenerated catalyst and a non-oxidized portion of the solid phase product. Still further, the method includes further regenerating the partially-regenerated catalyst by exposing the non-oxidized portion of the solid phase product and the partially-regenerated catalyst to a second oxidizing condition.

    摘要翻译： 在一个实施方案中公开了一种用于碳质材料的催化热解的方法，其包括使碳质材料与多个催化剂颗粒接触以产生气相产物和固相产物，并将气相产物与固相产物分离，以及 多个催化剂颗粒。 该方法还包括通过将固相产物和催化剂颗粒暴露于第一氧化条件以产生氧化固相和部分再生催化剂并冷却部分再生催化剂和未氧化的催化剂颗粒来部分地再生多个催化剂颗粒 部分固相产物。 此外，该方法包括通过将固相产物和部分再生催化剂的未氧化部分暴露于第二氧化条件来进一步再生部分再生的催化剂。

    Integrated process for gasoline production
    10.
    发明授权
    Integrated process for gasoline production 有权

    公开(公告)号：US10369556B2

    公开(公告)日：2019-08-06

    申请号：US14567804

    申请日：2014-12-11

    申请人： UOP LLC

    发明人： Tom N. Kalnes ,  Stuart Smith ,  Douglas A. Nafis ,  Alakananda Bhattacharyya ,  Bryan K. Glover ,  Susie C. Martins

    IPC分类号： C07C6/00 ,  B01J31/00 ,  C07C6/10 ,  C10G29/20 ,  B01J31/02

    摘要： An integrated process for gasoline production is described. The process includes introducing a feed comprising n-C5 hydrocarbons into a disproportionation reaction zone in the presence of a disproportionation catalyst to form a disproportionation mixture comprising iso-C4 and C6+ disproportionation products and unreacted n-C5 hydrocarbons. An iso-C4 hydrocarbon stream and an olefin feed are introduced into an alkylation reaction zone in the presence of an alkylation catalyst to produce an alkylation mixture comprising alkylate and unreacted iso-C4 paraffins. The disproportionation mixture and the alkylation mixture are combined, and the combined mixture is separated into at least a stream comprising the alkylate product, an iso-C4 stream, and an unreacted n-C5 hydrocarbon stream. The iso-C4 stream is recycled to the alkylation reaction zone, and the unreacted n-C5 hydrocarbon stream is recycled to the disproportionation reaction zone. The stream comprising the alkylate product is recovered.