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公开(公告)号：US08624055B2
公开(公告)日：2014-01-07
申请号：US12598902
申请日：2008-05-01
申请人： Wayne P. Schammel , Bradley J. Huggins , Matthew A. Kulzick , Philip O. Nubel , Bryan M. Rabatic , Chengxiang Zhou , Victor A. Adamian , William H. Gong , Peter D. Metelski , Jeffrey T. Miller
发明人： Wayne P. Schammel , Bradley J. Huggins , Matthew A. Kulzick , Philip O. Nubel , Bryan M. Rabatic , Chengxiang Zhou , Victor A. Adamian , William H. Gong , Peter D. Metelski , Jeffrey T. Miller
IPC分类号： C07C51/16
CPC分类号： B01J23/6525 , B01J21/06 , B01J21/063 , B01J21/08 , B01J21/18 , B01J23/002 , B01J23/644 , B01J23/6445 , B01J23/686 , B01J35/0053 , B01J35/006 , B01J35/0066 , B01J37/0203 , B01J2523/00 , B01J2523/53 , B01J2523/68 , B01J2523/824 , C07C51/265 , C07C63/26 , B01J2523/19 , B01J2523/54
摘要： Catalytic compositions for conversion of substituted aromatic feed materials to oxidized products comprising aromatic carboxylic acid derivatives of the substituted aromatic feed materials comprise solid particles comprising palladium in combination with at least one of antimony, bismuth and gold, and optionally, an additional metal or metalloid component effective to promote activity or selectivity of the palladium and antimony, bismuth or gold for oxidation to aromatic carboxylic acids. A process for oxidizing substituted aromatic feed materials comprises contacting the feed material with oxygen in the presence of such catalytic compositions in a liquid reaction mixture.
摘要翻译： 用于将取代的芳族原料转化成包含取代的芳族原料的芳族羧酸衍生物的氧化产物的催化组合物包含与锑，铋和金中的至少一种结合的钯的固体颗粒，以及任选的另外的金属或准金属组分 有效地促进钯和锑，铋或金的氧化成芳族羧酸的活性或选择性。 用于氧化取代的芳族原料的方法包括在这种催化组合物存在下，在液体反应混合物中使进料与氧接触。
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公开(公告)号：US20100145094A1
公开(公告)日：2010-06-10
申请号：US12598902
申请日：2008-05-01
申请人： Wayne P. Schammel , Bradley J. Huggins , Matthew A. Kulzick , Philip O. Nubel , Bryan M. Rabatic , Chengxiang Zhou , Victor A. Adamian , William H. Gong , Peter D. Metelski
发明人： Wayne P. Schammel , Bradley J. Huggins , Matthew A. Kulzick , Philip O. Nubel , Bryan M. Rabatic , Chengxiang Zhou , Victor A. Adamian , William H. Gong , Peter D. Metelski
IPC分类号： B01J23/56 , B01J23/44 , B01J23/28 , B01J23/644 , C07C51/255 , C07C63/04 , C07C63/15
CPC分类号： B01J23/6525 , B01J21/06 , B01J21/063 , B01J21/08 , B01J21/18 , B01J23/002 , B01J23/644 , B01J23/6445 , B01J23/686 , B01J35/0053 , B01J35/006 , B01J35/0066 , B01J37/0203 , B01J2523/00 , B01J2523/53 , B01J2523/68 , B01J2523/824 , C07C51/265 , C07C63/26 , B01J2523/19 , B01J2523/54
摘要： Catalytic compositions for conversion of substituted aromatic feed materials to oxidized products comprising aromatic carboxylic acid derivatives of the substituted aromatic feed materials comprise solid particles comprising palladium in combination with at least one of antimony, bismuth and gold, and optionally, an additional metal or metalloid component effective to promote activity or selectivity of the palladium and antimony, bismuth or gold for oxidation to aromatic carboxylic acids. A process for oxidizing substituted aromatic feed materials comprises contacting the feed material with oxygen in the presence of such catalytic compositions in a liquid reaction mixture.
摘要翻译： 用于将取代的芳族原料转化成包含取代的芳族原料的芳族羧酸衍生物的氧化产物的催化组合物包含与锑，铋和金中的至少一种结合的钯的固体颗粒，以及任选的另外的金属或准金属组分 有效地促进钯和锑，铋或金的氧化成芳族羧酸的活性或选择性。 用于氧化取代的芳族原料的方法包括在这种催化组合物存在下，在液体反应混合物中使进料与氧接触。
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公开(公告)号：US20090088585A1
公开(公告)日：2009-04-02
申请号：US12298554
申请日：2007-05-04
申请人： Wayne P. Schammel , Victor Adamian , Stephen P. Brugge , William H. Gong , Peter D. Metelski , Philip O. Nubel , Chengxiang Zhou
发明人： Wayne P. Schammel , Victor Adamian , Stephen P. Brugge , William H. Gong , Peter D. Metelski , Philip O. Nubel , Chengxiang Zhou
IPC分类号： C07C51/255 , B01J23/652 , B01J23/16 , B01J23/66 , B01J23/60 , B01J31/04 , C09K3/00
CPC分类号： B01J23/002 , B01J23/6525 , B01J35/1014 , B01J37/0201 , B01J37/0203 , B01J2523/00 , C07C51/265 , C07C63/26 , C07C63/24 , C07C63/38 , B01J2523/43 , B01J2523/55 , B01J2523/68 , B01J2523/824 , B01J2523/53 , B01J2523/67 , B01J2523/847 , B01J2523/49 , B01J2523/23 , B01J2523/3712 , B01J2523/32 , B01J2523/828 , B01J2523/56 , B01J2523/47 , B01J2523/18
摘要： Catalytic compositions for conversion of substituted aromatic feed materials to oxidized products comprising aromatic carboxylic acid derivatives of the substituted aromatic feed materials comprise a combination comprising a palladium component, an antimony component and/or a bismuth component, and one or more Group 4, 5, 6 or 14 metal or metalloid components. A process for oxidizing substituted aromatic feed materials comprises contacting the feed material with oxygen in the presence of such a catalytic composition in a liquid reaction mixture.
摘要翻译： 用于将取代的芳族原料转化为包含取代的芳族原料的芳族羧酸衍生物的氧化产物的催化组合物包括包含钯组分，锑组分和/或铋组分的组合，以及一种或多种组4,5， 6或14个金属或准金属组分。 用于氧化取代的芳族原料的方法包括在液体反应混合物中，在这种催化组合物存在下使进料与氧接触。
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公开(公告)号：US20090069594A1
公开(公告)日：2009-03-12
申请号：US12298586
申请日：2007-05-04
申请人： William H. Gong , Victor Adamian , Stephen P. Brugge , Peter D. Metelski , Philip O. Nubel , Wayne P. Schammel , Chengxiang Zhou
发明人： William H. Gong , Victor Adamian , Stephen P. Brugge , Peter D. Metelski , Philip O. Nubel , Wayne P. Schammel , Chengxiang Zhou
IPC分类号： C07C63/14 , C07C63/00 , B01J23/42 , B01J23/22 , B01J23/26 , B01J23/28 , B01J23/24 , B01J23/652 , B01J23/18
CPC分类号： B01J23/002 , B01J23/6525 , B01J35/1014 , B01J37/0201 , B01J37/0203 , B01J2523/00 , C07C51/265 , C07C63/26 , C07C63/24 , C07C63/38 , B01J2523/43 , B01J2523/55 , B01J2523/68 , B01J2523/824 , B01J2523/53 , B01J2523/67 , B01J2523/847 , B01J2523/49 , B01J2523/23 , B01J2523/3712 , B01J2523/32 , B01J2523/828 , B01J2523/56 , B01J2523/47 , B01J2523/18
摘要： Catalytic compositions for conversion of substituted aromatic feed materials to oxidized products comprising aromatic carboxylic acid derivatives of the substituted aromatic feed materials comprise at least two metal or metalloid elements, at least one of which is palladium, platinum, vanadium or titanium, and at least one of which is a Group 5, 6, 14 or 15 metal or metalloid. A process for oxidizing substituted aromatic feed materials comprises contacting the feed material with oxygen in the presence of such a catalytic composition in a liquid reaction mixture.
摘要翻译： 用于将取代的芳族原料转化成包含取代的芳族原料的芳族羧酸衍生物的氧化产物的催化组合物包含至少两种金属或准金属元素，其中至少一种是钯，铂，钒或钛，以及至少一种 其中第5,6,14或15族是金属或准金属。 用于氧化取代的芳族原料的方法包括在液体反应混合物中，在这种催化组合物存在下使进料与氧接触。
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公开(公告)号：US08163954B2
公开(公告)日：2012-04-24
申请号：US12298554
申请日：2007-05-04
申请人： Wayne P. Schammel , Victor Adamian , Stephen P. Brugge , William H. Gong , Peter D. Metelski , Philip O. Nubel , Chengxiang Zhou
发明人： Wayne P. Schammel , Victor Adamian , Stephen P. Brugge , William H. Gong , Peter D. Metelski , Philip O. Nubel , Chengxiang Zhou
IPC分类号： C07C51/16
CPC分类号： B01J23/002 , B01J23/6525 , B01J35/1014 , B01J37/0201 , B01J37/0203 , B01J2523/00 , C07C51/265 , C07C63/26 , C07C63/24 , C07C63/38 , B01J2523/43 , B01J2523/55 , B01J2523/68 , B01J2523/824 , B01J2523/53 , B01J2523/67 , B01J2523/847 , B01J2523/49 , B01J2523/23 , B01J2523/3712 , B01J2523/32 , B01J2523/828 , B01J2523/56 , B01J2523/47 , B01J2523/18
摘要： Catalytic compositions for conversion of substituted aromatic feed materials to oxidized products comprising aromatic carboxylic acid derivatives of the substituted aromatic feed materials comprise a combination comprising a palladium component, an antimony component and/or a bismuth component, and one or more Group 4, 5, 6 or 14 metal or metalloid components. A process for oxidizing substituted aromatic feed materials comprises contacting the feed material with oxygen in the presence of such a catalytic composition in a liquid reaction mixture.
摘要翻译： 用于将取代的芳族原料转化为包含取代的芳族原料的芳族羧酸衍生物的氧化产物的催化组合物包括包含钯组分，锑组分和/或铋组分的组合，以及一种或多种组4,5， 6或14个金属或准金属组分。 用于氧化取代的芳族原料的方法包括在液体反应混合物中，在这种催化组合物存在下使进料与氧接触。
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公开(公告)号：US20090118536A1
公开(公告)日：2009-05-07
申请号：US12295303
申请日：2007-05-04
申请人： James M. Tibbitt , William H. Gong , Wayne P. Schammel , Robert P. Hepfer , Victor Adamian , Stephen P. Brugge , Peter D. Metelski , Chengxiang Zhou
发明人： James M. Tibbitt , William H. Gong , Wayne P. Schammel , Robert P. Hepfer , Victor Adamian , Stephen P. Brugge , Peter D. Metelski , Chengxiang Zhou
IPC分类号： C07C51/255
CPC分类号： B01J23/002 , B01J23/6525 , B01J35/1014 , B01J37/0201 , B01J37/0203 , B01J2523/00 , C07C51/265 , C07C63/26 , C07C63/24 , C07C63/38 , B01J2523/43 , B01J2523/55 , B01J2523/68 , B01J2523/824 , B01J2523/53 , B01J2523/67 , B01J2523/847 , B01J2523/49 , B01J2523/23 , B01J2523/3712 , B01J2523/32 , B01J2523/828 , B01J2523/56 , B01J2523/47 , B01J2523/18
摘要： A process is disclosed for producing at least one aromatic carboxylic acid by contacting a liquid reaction mixture comprising an aromatic feedstock and water with oxygen in the presence of a bromine-free metal catalyst composition wherein the metal catalyst composition has activity in the absence of bromine for oxidation of the aromatic feedstock with at least 80% conversion to oxidized aromatic derivatives of the aromatic feedstock and with at least 80% selectivity to the aromatic carboxylic acid. This process operates in water without the use of bromine at temperatures and residence times substantially the same as conventional processes for aromatic carboxylic acid manufacture, as well as with less total burning and with yields to product equivalent or higher than conventional processes.
摘要翻译： 公开了一种通过在无溴金属催化剂组合物存在下使包含芳族原料和水的液体反应混合物与氧气接触来生产至少一种芳族羧酸的方法，其中金属催化剂组合物在不存在溴的情况下具有活性 芳族原料的氧化至少80％转化为芳族原料的氧化芳族衍生物，并且对芳族羧酸具有至少80％的选择性。 该方法在温度和停留时间基本上与用于芳族羧酸制备的常规方法相同的温度和停留时间下在水中不使用溴，以及较少的总燃烧和产率相当于或高于常规方法。
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7.发明授权公开(公告)号：US07378544B2
公开(公告)日：2008-05-27
申请号：US10980718
申请日：2004-11-03
IPC分类号： C07C51/255 , B01J31/02 , B01J31/26
CPC分类号： B01J27/135 , B01J27/128 , C07C51/265 , C07C63/38 , C07C63/26 , C07C63/24 , C07C63/307
摘要： The present invention relates to the liquid phase oxidation of aromatic hydrocarbons in the presence of at least one heavy metal oxidation catalyst and bromine, which is activated by at least one of anthracene or another polycyclic aromatic compound to produce aromatic carboxylic acids.
摘要翻译： 本发明涉及在至少一种重金属氧化催化剂和溴的存在下芳族烃的液相氧化，其由至少一种蒽或其它多环芳族化合物活化以产生芳族羧酸。
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公开(公告)号：US5012030A
公开(公告)日：1991-04-30
申请号：US418855
申请日：1989-10-10
申请人： Kelley R. Lane , Wayne P. Schammel
发明人： Kelley R. Lane , Wayne P. Schammel
CPC分类号： C07C2/22 , C08F10/08 , C07C2527/126 , C07C2531/02
摘要： Viscous, liquid polybutenes of at least 50 wt. % vinylidene content are disclosed together with a procedure for preparing the compounds using an aluminum chloride-organic nitro compound catalyst.
摘要翻译： 至少50重量％的粘稠液体聚丁烯 公开了偏亚乙烯含量以及使用氯化铝 - 有机硝基化合物催化剂制备化合物的方法。
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9.发明授权Oxidation process for the manufacture of aromatic acids from alkylaromatic compounds 失效从烷基芳族化合物制造芳香酸的氧化工艺
公开(公告)号：US4786753A
公开(公告)日：1988-11-22
申请号：US50860
申请日：1987-05-18
IPC分类号： C07C51/265
CPC分类号： C07C51/265 , B01J23/8892 , B01J27/128 , B01J31/0231 , B01J31/04 , B01J2231/76
摘要： A novel method of oxidizing di- and trimethylbenzenes with molecular oxygen to the corresponding di- or tricarboxylic acid under liquid-phase conditions is disclosed. The process is conducted at a temperature of about 100.degree. C. to 260.degree. C. This process comprises conducting the oxidation in the presence of a catalyst system comprising a source of bromine with nickel, manganese and zirconium. The benzene di- and tricarboxylic acids have wide industrial application, including the manufacture of polyesters, polyamides, and fibers and films.
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公开(公告)号：US20120041246A1
公开(公告)日：2012-02-16
申请号：US13115082
申请日：2011-05-24
申请人： Erik C. Scher , Fabio R. Zurcher , Joel M. Cizeron , Wayne P. Schammel , Alex Tkachenko , Joel Gamoras , Dmitry Karshtedt , Greg Nyce
发明人： Erik C. Scher , Fabio R. Zurcher , Joel M. Cizeron , Wayne P. Schammel , Alex Tkachenko , Joel Gamoras , Dmitry Karshtedt , Greg Nyce
IPC分类号： C07C2/76 , B01J23/10 , B01J21/06 , B01J23/34 , B01J21/08 , B01J23/22 , B01J21/04 , B01J31/26 , B01J31/38 , B01J31/34 , B01J31/32 , B01J31/36 , B01J21/12 , B01J21/10 , B82Y30/00 , B82Y40/00
CPC分类号： B01J35/06 , B01J21/066 , B01J21/10 , B01J23/10 , B01J23/22 , B01J23/34 , B01J35/0013 , B01J37/0018 , B01J37/031 , B01J37/08 , B01J37/10 , B82Y30/00 , C01F5/02 , C01F5/14 , C01F7/02 , C01F11/02 , C01F17/0043 , C01G25/00 , C01G31/02 , C01G41/02 , C01G45/00 , C01G45/006 , C01G45/02 , C01P2002/52 , C01P2002/72 , C01P2004/04 , C01P2004/16 , C01P2004/54 , C01P2004/84 , C01P2006/12 , C07C2/84 , C07C5/48 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/10 , C07C2523/30 , C07C2523/34 , C07C2523/75 , C10G2/33 , C10G9/00 , C10G2300/1025 , C10G2300/70 , C10G2400/02 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/40 , C07C11/04 , C07C11/06
摘要： Nanowires useful as heterogeneous catalysts are provided. The nanowire catalysts are useful in a variety of catalytic reactions, for example, the oxidative coupling of methane to ethylene. Related methods for use and manufacture of the same are also disclosed.
摘要翻译： 提供用作非均相催化剂的纳米线。 纳米线催化剂可用于各种催化反应，例如甲烷与乙烯的氧化偶联。 还公开了相关的使用和制造方法。
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