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公开(公告)号：US20090139900A1
公开(公告)日：2009-06-04
申请号：US12322485
申请日：2009-02-03
IPC分类号： C10G11/02
摘要： This invention relates to a FCC process using a mesoporous catalytic cracking catalyst. The mesoporous fluidized catalytic cracking catalyst is selective for minimizing the production of coke and light gas. The catalyst comprises at least one amorphous, porous matrix, each matrix having pores ranging in diameter from about 1 Å to about 10 Å and pores ranging in diameter from about 40 Å to about 500 Å, wherein in the pore range from 50 Å to 250 Å, there is a single maximum in differential pore volume distribution over the 50 Å to 250 Å range.
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公开(公告)号：US07504021B2
公开(公告)日：2009-03-17
申请号：US11106289
申请日：2005-04-14
IPC分类号： C10G11/05
摘要： This invention relates to a FCC process using a mesoporous catalytic cracking catalyst. The mesoporous fluidized catalytic cracking catalyst is selective for minimizing the production of coke and light gas. The catalyst comprises at least one amorphous, porous matrix, each matrix having pores ranging in diameter from about 1 Å to about 10 Å and pores ranging in diameter from about 40 Å to about 500 Å, wherein in the pore range from 50 Å to 250 Å, there is a single maximum in differential pore volume distribution over the 50 Å to 250 Å range.
摘要翻译： 本发明涉及使用中孔催化裂化催化剂的FCC方法。 中孔流化催化裂化催化剂是选择性地使焦炭和轻质气体的生产最小化。 催化剂包含至少一种无定形多孔基质，每个基质的孔直径约为约至约10埃，孔径范围为约40至约500，其中孔径范围为50埃至250埃 Å，在50Å至250Å范围内，微分孔体积分布有单一最大值。
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3.发明授权Hydrocarbon conversion process with alkaline earth metal ion exchanged selectivated zeolite catalyst 失效碳氢转化过程用碱土金属离子交换选择沸石催化剂
公开(公告)号：US5849968A
公开(公告)日：1998-12-15
申请号：US901822
申请日：1997-07-28
申请人： Jeffrey S. Beck , David L. Stern
发明人： Jeffrey S. Beck , David L. Stern
IPC分类号： B01J29/40 , B01J31/02 , C07C2/12 , C07C2/66 , C07C5/27 , C07C5/41 , C07C6/12 , C10G35/095 , C07C5/22
CPC分类号： C07C6/123 , B01J29/40 , C07C2/12 , C07C2/66 , C07C5/2708 , C07C5/41 , B01J2229/12 , B01J2229/42 , C07C2521/08 , C07C2529/06 , C07C2529/40
摘要： There is provided a zeolite catalyst, which is first selectivated with a siliceous material and then treated with an aqueous solution comprising alkaline earth metal ions under ion exchange conditions.
摘要翻译： 提供沸石催化剂，其首先用硅质材料选择，然后在离子交换条件下用包含碱土金属离子的水溶液处理。
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公开(公告)号：US5773679A
公开(公告)日：1998-06-30
申请号：US578346
申请日：1995-12-26
申请人： Jeffrey S. Beck , David L. Stern
发明人： Jeffrey S. Beck , David L. Stern
CPC分类号： C07C6/123 , B01J2229/12 , B01J2229/32 , C07C2529/40
摘要： A process for shape-selective hydrocarbon conversion that involves initially contacting a feed stream which includes an alkylaromatic compound and a co-feed of water, under conversion conditions with a catalytic molecular sieve. Preferably, the catalytic molecular sieve has been modified by being ex situ selectivated with a silicon compound. After an effective amount of time, the water co-feed is omitted from the feed stream and the hydrocarbon conversion process is continued. Optionally, the catalytic molecular sieve can also be in situ trim-selectivated.
摘要翻译： 一种用于形状选择性烃转化的方法，其包括在转化条件下与催化分子筛接触包括烷基芳族化合物和水的共同进料的进料流。 优选地，通过用硅化合物进行异地选择来改变催化分子筛。 在有效量的时间之后，从进料流中省去水共同进料，继续进行烃转化过程。 任选地，催化分子筛也可以原位修剪选择。
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公开(公告)号：US5602066A
公开(公告)日：1997-02-11
申请号：US441106
申请日：1995-06-29
申请人： Jeffrey S. Beck , David L. Stern
发明人： Jeffrey S. Beck , David L. Stern
CPC分类号： B01J37/086 , B01J29/40 , B01J37/06 , B01J2229/26 , B01J2229/42
摘要： There is provided a zeolite catalyst, which is first selectivated with a siliceous material and then washed with a liquid. The washing step may comprise slurrying the catalyst in water and recovering the washed catalyst by filtration.
摘要翻译： 提供沸石催化剂，其首先用硅质材料选择，然后用液体洗涤。 洗涤步骤可以包括将催化剂浆化成水，并通过过滤回收洗涤过的催化剂。
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公开(公告)号：US20080237129A1
公开(公告)日：2008-10-02
申请号：US10579175
申请日：2004-12-01
IPC分类号： B01D61/16
CPC分类号： C10G21/28 , C10G17/10 , C10G2300/202 , C10G2300/4081
摘要： This invention relates to a process for recycling acid used to remove nitrogen contaminants from hydrocarbons using polymeric membranes to separate spent acid from the acid extraction of hydrocarbons into acid for recycle and acid for regeneration.
摘要翻译： 本发明涉及一种使用聚合物膜从碳氢化合物中除去氮污染物的方法，以将废酸从碳酸的酸萃取中分离出来，再循环酸和用于再生。
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7.发明授权High temperature calcination of selectivated molecular sieve catalysts for activity and diffusional modification 失效用于活性和扩散修饰的选择性分子筛催化剂的高温煅烧公开(公告)号：US07238636B2
公开(公告)日：2007-07-03
申请号：US10625322
申请日：2003-07-23
IPC分类号： B01J20/04
CPC分类号： C10G11/05 , B01J29/04 , B01J29/06 , B01J29/40 , B01J29/44 , B01J37/08 , B01J2229/12 , B01J2229/32 , B01J2229/40 , C07C5/2708 , C07C6/123 , C07C2529/40 , C07C2529/44 , C10G2300/1044 , C10G2300/1096 , C10G2400/30 , Y02P20/52 , C07C15/08
摘要： A method is disclosed for modifying a catalytic molecular sieve for shape-selective hydrocarbon conversions comprises: a) selectivating said catalytic molecular sieve by contacting with a silicon-containing selectivating agent; and b) calcining the selectivated catalytic molecular sieve at high temperature calcination conditions comprising temperatures greater than 700° C., which conditions are sufficient to reduce acid activity as measured by alpha value and increase diffusion barrier of said catalytic molecular sieve as measured by the rate of 2,3-dimethylbutane uptake, as compared to the selectivated catalyst. Catalytic molecular sieves thus prepared, such as silica-bound ZSM-5, and their use in hydrocarbon conversion processes such as aromatics isomerization, e.g., xylene isomerization, ethylbenzene conversion and aromatics disproportionation, e.g., toluene disproportionation are also disclosed.
摘要翻译： 公开了一种修饰用于形状选择性烃转化的催化分子筛的方法，包括：a）通过与含硅选择性剂接触来选择所述催化分子筛; 和b）在包括温度大于700℃的高温煅烧条件下煅烧所选择的催化分子筛，该条件足以降低由α值测量的酸活性，并增加所述催化分子筛的扩散阻挡，通过速率 与选择的催化剂相比，2,3-二甲基丁烷的吸收。 由此制备的催化分子筛，例如二氧化硅结合的ZSM-5，以及它们在烃转化方法中的用途，例如芳族化合物异构化，例如二甲苯异构化，乙苯转化和芳烃歧化，例如甲苯歧化。
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公开(公告)号：US06576582B1
公开(公告)日：2003-06-10
申请号：US08558309
申请日：1995-11-15
IPC分类号： B01J2906
CPC分类号： C07C6/123 , B01J29/40 , B01J37/086 , B01J2229/12 , B01J2229/32 , B01J2229/42 , C07C2/66 , C07C2/864 , C07C2529/06 , C07C2529/40 , C07C2529/65 , C07C2529/70 , Y02P20/52 , C07C15/02 , C07C15/00
摘要： There is provided a substantially binder-free catalytic molecular sieve which has been modified by being ex situ selectivated with a silicon compound. The ex situ selectivation involves exposing the molecular sieve to at least two silicon impregnation sequences, each sequence comprising an impregnation with a silicon compound followed by calcination. The catalyst may be used in a hydrocarbon conversion process, such as toluene disproportionation.
摘要翻译： 提供了基本上不含粘合剂的催化分子筛，其通过用硅化合物进行异地选择而被改性。 异位选择包括将分子筛暴露于至少两个硅浸渍序列，每个序列包含用硅化合物浸渍，随后煅烧。 催化剂可用于烃转化过程中，例如甲苯歧化。
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公开(公告)号：US06504075B2
公开(公告)日：2003-01-07
申请号：US09767183
申请日：2001-01-22
IPC分类号： C07C552
CPC分类号： C01B39/38 , B01J29/04 , B01J29/40 , C01B39/40 , C07C5/2702 , C07C6/123 , C07C2529/40 , C07C15/067
摘要： A synthetic porous crystalline material has the structure of ZSM-5 and a composition involving the molar relationship: X2O3:(n)YO2, wherein X is a trivalent element; Y is a tetravalent element; and n is less than 25, and wherein the slope of the nitrogen sorption isotherm of the material at a partial pressure of nitrogen of 0.4 to 0.7 and a temperature 77° K is greater than 30. The material has a mesoporous surface area (MSA) greater than 45 m2/g and is useful as a catalyst in the liquid phase isomerization of xylene.
摘要翻译： 合成多孔结晶材料具有ZSM-5的结构和涉及摩尔关系的组成：其中X是三价元素; Y是四价元素; 并且n小于25，并且其中在氮分压为0.4至0.7且温度为77°K的材料的氮吸附等温线的斜率大于30.该材料具有介孔表面积（MSA） 大于45m 2 / g，可用作二甲苯液相异构化中的催化剂。
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公开(公告)号：US06180550B2
公开(公告)日：2001-01-30
申请号：US09218191
申请日：1998-12-22
IPC分类号： B01J2900
CPC分类号： C01B39/38 , B01J29/04 , B01J29/40 , C01B39/40 , C07C5/2702 , C07C6/123 , C07C2529/40 , C07C15/067
摘要： A synthetic porous crystalline material has the structure of ZSM-5 and a composition involving the molar relationship: X2O3:(n)YO2, wherein X is a trivalent element; Y is a tetravalent element; and n is less than 25, and wherein the slope of the nitrogen sorption isotherm of the material at a partial pressure of nitrogen of 0.4 to 0.7 and a temperature 77° K is greater than 30. The material has a mesoporous surface area (MSA) greater than 45 m2/g and is useful as a catalyst in the liquid phase isomerization of xylene.
摘要翻译： 合成多孔结晶材料具有ZSM-5的结构和涉及摩尔关系的组成：其中X是三价元素; Y是四价元素; 并且n小于25，并且其中在氮分压为0.4至0.7且温度为77°K的材料的氮吸附等温线的斜率大于30.该材料具有介孔表面积（MSA） 大于45m 2 / g，可用作二甲苯液相异构化中的催化剂。
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