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    LADDER-TYPE OLIGO-P-PHENYLENE-CONTAINING COPOLYMERS WITH HIGH OPEN-CIRCUIT VOLTAGES AND AMBIENT PHOTOVOLTAIC ACTIVITY
    5.
    发明申请
    LADDER-TYPE OLIGO-P-PHENYLENE-CONTAINING COPOLYMERS WITH HIGH OPEN-CIRCUIT VOLTAGES AND AMBIENT PHOTOVOLTAIC ACTIVITY 审中-公开
    具有高开路电压和环境光伏活性的梯度型含OLYO-对苯乙烯共聚物

    公开(公告)号：US20120232238A1

    公开(公告)日：2012-09-13

    申请号：US13388855

    申请日：2010-08-03

    Applicant: Howard Edan Katz ,  Qingdong Zheng ,  Byung Jun Jung

    Inventor： Howard Edan Katz ,  Qingdong Zheng ,  Byung Jun Jung

    IPC: C08G75/06 ,  B82Y30/00

    CPC classification number: H01L51/0036 ,  C08G61/126 ,  C08G2261/1336 ,  C08G2261/164 ,  C08G2261/3142 ,  C08G2261/3223 ,  C08G2261/91 ,  H01L51/0043 ,  H01L51/0044 ,  H01L51/0056 ,  H01L51/0068 ,  Y02E10/549

    Abstract: Ladder-type oligo-p-phenylene containing donor-acceptor copolymers are disclosed. The ladder-type oligo-p-phenylene can be used as an electron donor unit in the disclosed copolymers to provide a deeper highest occupied molecular orbital (HOMO) level for obtaining polymeric solar cells having a higher open-circuit voltage. Particular electron-accepting units, e.g., a divalent fused-ring heterocyclic moiety selected from the group consisting of a substituted or unsubstituted benzothiadiazole, a substituted or unsubstituted quinoxaline, a substituted or unsubstituted benzobisthiazole, and a substituted or unsubstituted naphthothiadiazole, can be used to tune the electronic band gaps of the polymers for a better light harvesting ability. The disclosed copolymers exhibit field-effect mobilities as high as 0.011 cm2/(V s). Compared to fluorene-containing copolymers with the same acceptor unit, the disclosed ladder-type oligo-p-phenylene containing copolymers have enhanced and bathochromically shifted absorption bands and much better solubility in organic solvents.

    Abstract translation: 公开了含梯度型低聚对苯二烯的供体 - 受体共聚物。 在所公开的共聚物中，梯型低聚对亚苯基可用作电子给体单元，以提供更高的最高占据分子轨道（HOMO）水平，以获得具有较高开路电压的聚合物太阳能电池。 可以使用特定的电子接受单元，例如选自取代或未取代的苯并噻二唑，取代或未取代的喹喔啉，取代或未取代的苯并二噻唑和取代或未取代的萘并噻二唑的二价稠环杂环部分， 调整聚合物的电子带隙以获得更好的光捕获能力。 所公开的共聚物表现出高达0.011cm2 /（Vs）的场效应迁移率。 与具有相同受体单元的含芴共聚物相比，所公开的梯型低聚对亚苯基共聚物具有增强的和红移的吸收带和在有机溶剂中更好的溶解度。

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