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    POLYALKYL (METH)ACRYLATE COPOLYMERS HAVING OUTSTANDING PROPERTIES
    4.
    发明申请
    POLYALKYL (METH)ACRYLATE COPOLYMERS HAVING OUTSTANDING PROPERTIES 有权

    公开(公告)号：US20120046207A1

    公开(公告)日：2012-02-23

    申请号：US13213547

    申请日：2011-08-19

    申请人： Michael Müller ,  Torsten Stöhr ,  Boris Eisenberg

    发明人： Michael Müller ,  Torsten Stöhr ,  Boris Eisenberg

    IPC分类号： C10M145/14 ,  C08F220/26 ,  C08F220/36

    CPC分类号： C08F220/36 ,  C10M145/10 ,  C10M2209/08 ,  C10N2230/06

    摘要： The present invention relates to copolymers obtainable by polymerizing a monomer composition composed of a) 0% to 40% by weight of one or more ethylenically unsaturated ester compounds of the formula (I) in which R is hydrogen or methyl, R1 is a linear or branched alkyl radical having 1 to 5 carbon atoms, R2 and R3 independently are hydrogen or a group of the formula —COOR′, in which R1 is hydrogen or an alkyl group having 1 to 5 carbon atoms, b) 10% to 99.9% by weight of one or more ethylenically unsaturated ester compounds of the formula (II) in which R is hydrogen or methyl, R4 is a linear or branched alkyl radical having 6 to 15 carbon atoms, R5 and R6 independently are hydrogen or a group of the formula —COOR′, in which R′ is hydrogen or an alkyl group having 6 to 15 carbon atoms, c) 0% to 80% by weight of one or more ethylenically unsaturated ester compounds of the formula (III) in which R is hydrogen or methyl, R7 is a linear or branched alkyl radical having 16 to 30 carbon atoms, R8 and R9 independently are hydrogen or a group of the formula —COOR″, in which R″ is hydrogen or an alkyl group having 16 to 30 carbon atoms, d) 0.1% to 30% by weight of one or more ethylenically unsaturated, polar ester compounds of the formula (IV) in which R is hydrogen or methyl, X is oxygen, sulphur or an amino group of the formula —NH— or —NRa— in which Ra is an alkyl radical having 1 to 40 carbon atoms, R10 is a radical which encompasses 2 to 1000 carbon atoms and has at least 2 heteroatoms, R11 and R12 independently are hydrogen or a group of the formula —COX′R10′, in which X′ is oxygen or an amino group of the formula —NH— or —NRa—, in which Ra′ is an alkyl radical having 1 to 40 carbon atoms, and R10′ is a radical which encompasses 1 to 100 carbon atoms, and e) 0% to 50% by weight of comonomer, based in each case on the total weight of the ethylenically unsaturated monomers.

    Oil soluble comb polymers
    6.
    发明授权
    Oil soluble comb polymers 有权
    油溶性梳状聚合物

    公开(公告)号：US08067349B2

    公开(公告)日：2011-11-29

    申请号：US11909171

    申请日：2006-04-07

    申请人： Torsten Stoehr ,  Boris Eisenberg ,  Michael Mueller

    发明人： Torsten Stoehr ,  Boris Eisenberg ,  Michael Mueller

    IPC分类号： C10M145/14 ,  C10M149/04 ,  C10L1/18

    CPC分类号： C08F290/04 ,  C08F299/00 ,  C10M159/005 ,  C10M2203/1006 ,  C10M2203/1025 ,  C10M2205/028 ,  C10M2205/0285 ,  C10M2209/04 ,  C10M2209/062 ,  C10M2209/084 ,  C10M2209/086 ,  C10N2220/021 ,  C10N2220/028 ,  C10N2230/02 ,  C10N2230/04 ,  C10N2230/06 ,  C10N2230/68 ,  C10N2220/022

    摘要： The invention relates to comb polymers which comprise, in the main chain, repeating units which are derived from polyolefin-based macromonomers, and repeating units which are derived from low molecular monomers which are selected from the group consisting of styrene monomers having 8-17 carbon atoms, alkyl(meth)acrylates having 1-10 carbon atoms in the alcohol group, vinyl esters having 1-11 carbon atoms in the acyl group, vinyl ethers having 1-10 carbon atoms in the alcohol group, (Di)alkylfumarates having 1-10 carbon atoms in the alcohol group, (Di)alkylmaleates having 1-10 carbon atoms in the alcohol group and mixtures of said monomers. The molar branching degree lies in the region between 0.1-10 mol. % and the comb polymer represents the sum of at least 80 wt. %, in relation to the weight of the repeating units, on repeating units which are derived from polyolefin-based macromonomers, and repeating units which are selected from low molecular monomers which are selected from the group consisting of styrene monomers having 8-17 carbon atoms, alkyl(meth)acrylates having 1-10 carbon atoms in the alcohol group, vinyl esters having 1-11 carbon atoms in the acyl group, vinyl ethers having 1-10 carbon atoms in the alcohol group, (Di)alkylfumarates having 1-10 carbon atoms in the alcohol group, (Di)alkylmaleates having 1-10 carbon atoms in the alcohol group, and mixtures of said monomers.

    摘要翻译： 本发明涉及在主链中包含衍生自聚烯烃基大分子单体的重复单元和衍生自低分子单体的重复单元的梳状聚合物，所述低分子单体选自具有8-17个碳原子的苯乙烯单体 原子，醇基中具有1-10个碳原子的（甲基）丙烯酸烷基酯，酰基中具有1-11个碳原子的乙烯基酯，醇基中具有1-10个碳原子的乙烯基醚，具有1个碳原子的（Di）烷基富马酸盐 -10个碳原子，醇基中具有1-10个碳原子的（Di）烷基马来酸酯和所述单体的混合物。 摩尔分支度位于0.1-10mol之间的区域。 ％，梳状聚合物代表至少80wt。 相对于重复单元的重量，衍生自聚烯烃基大分子单体的重复单元的重复单元和选自具有8-17个碳原子的苯乙烯单体的低分子单体的重复单元 ，醇基中具有1-10个碳原子的（甲基）丙烯酸烷基酯，酰基中具有1-11个碳原子的乙烯基酯，醇基中具有1-10个碳原子的乙烯基醚，具有1- 醇基中的10个碳原子，醇基中具有1-10个碳原子的（Di）烷基马来酸化物，以及所述单体的混合物。

    Oil Soluble Comb Polymers
    9.
    发明申请
    Oil Soluble Comb Polymers 有权
    油溶性梳子聚合物

    公开(公告)号：US20080194443A1

    公开(公告)日：2008-08-14

    申请号：US11909171

    申请日：2006-04-07

    申请人： Torsten Stohr ,  Boris Eisenberg ,  Michael Muller

    发明人： Torsten Stohr ,  Boris Eisenberg ,  Michael Muller

    IPC分类号： C08F120/00 ,  C08F112/08 ,  C08F136/00 ,  C10M169/04

    CPC分类号： C08F290/04 ,  C08F299/00 ,  C10M159/005 ,  C10M2203/1006 ,  C10M2203/1025 ,  C10M2205/028 ,  C10M2205/0285 ,  C10M2209/04 ,  C10M2209/062 ,  C10M2209/084 ,  C10M2209/086 ,  C10N2220/021 ,  C10N2220/028 ,  C10N2230/02 ,  C10N2230/04 ,  C10N2230/06 ,  C10N2230/68 ,  C10N2220/022

    摘要： The invention relates to comb polymers which comprise, in the main chain, repeating units which are derived from polyolefin-based macromonomers, and repeating units which are derived from low molecular monomers which are selected from the group consisting of styrene monomers having 8-17 carbon atoms, alkyl(meth)acrylates having 1-10 carbon atoms in the alcohol group, vinyl esters having 1-11 carbon atoms in the acyl group, vinyl ethers having 1-10 carbon atoms in the alcohol group, (Di)alkylfumarates having 1-10 carbon atoms in the alcohol group, (Di)alkylmaleates having 1-10 carbon atoms in the alcohol group and mixtures of said monomers. The molar branching degree lies in the region between 0.1-10 mol. % and the comb polymer represents the sum of at least 80 wt. %, in relation to the weight of the repeating units, on repeating units which are derived from polyolefin-based macromonomers, and repeating units which are selected from low molecular monomers which are selected from the group consisting of styrene monomers having 8-17 carbon atoms, alkyl(meth)acrylates having 1-10 carbon atoms in the alcohol group, vinyl esters having 1-11 carbon atoms in the acyl group, vinyl ethers having 1-10 carbon atoms in the alcohol group, (Di)alkylfumarates having 1-10 carbon atoms in the alcohol group, (Di)alkylmaleates having 1-10 carbon atoms in the alcohol group, and mixtures of said monomers.

    摘要翻译： 本发明涉及在主链中包含衍生自聚烯烃基大分子单体的重复单元和衍生自低分子单体的重复单元的梳状聚合物，所述低分子单体选自具有8-17个碳原子的苯乙烯单体 原子，醇基中具有1-10个碳原子的（甲基）丙烯酸烷基酯，酰基中具有1-11个碳原子的乙烯基酯，醇基中具有1-10个碳原子的乙烯基醚，具有1个碳原子的（Di）烷基富马酸盐 -10个碳原子，醇基中具有1-10个碳原子的（Di）烷基马来酸酯和所述单体的混合物。 摩尔分支度位于0.1-10mol之间的区域。 ％，梳状聚合物代表至少80wt。 相对于重复单元的重量，衍生自聚烯烃基大分子单体的重复单元的重复单元和选自具有8-17个碳原子的苯乙烯单体的低分子单体的重复单元 ，醇基中具有1-10个碳原子的（甲基）丙烯酸烷基酯，酰基中具有1-11个碳原子的乙烯基酯，醇基中具有1-10个碳原子的乙烯基醚，具有1- 醇基中的10个碳原子，醇基中具有1-10个碳原子的（Di）烷基马来酸化物，以及所述单体的混合物。

    USE OF GRAFT POLYMERS
    10.
    发明申请
    USE OF GRAFT POLYMERS 有权
    聚合物的使用

    公开(公告)号：US20070213237A1

    公开(公告)日：2007-09-13

    申请号：US11572181

    申请日：2005-06-23

    申请人： Markus Scherer ,  Klaus Hedrich ,  Alexander Dardin ,  Michael Muller ,  Thorsten Stoehr ,  Boris Eisenberg

    发明人： Markus Scherer ,  Klaus Hedrich ,  Alexander Dardin ,  Michael Muller ,  Thorsten Stoehr ,  Boris Eisenberg

    IPC分类号： C10M145/14

    CPC分类号： C10M149/10 ,  C08L51/06 ,  C10M149/02 ,  C10M161/00 ,  C10M2209/084 ,  C10M2217/02 ,  C10M2217/028 ,  C10N2220/021 ,  C10N2220/022 ,  C10N2230/02 ,  C10N2230/04 ,  C10N2230/06 ,  C10N2230/43 ,  C10N2240/04 ,  C10N2240/08 ,  C10N2240/10

    摘要： The invention relates to the use of graft polymers obtained by polymerization in two stages. In a first stage, at least one graft basis is produced by radically polymerizing a monomer composition A) containing 0 to 40 percent by weight of one or several ethylenically unsaturated ester compounds of formula (I), wherein R represents hydrogen or methyl, R1 represents a linear or branched alkyl radical comprising 1 to 5 carbon atoms, R2 and R3 independently represent hydrogen or a group of formula —COOR′, wherein R′ represents hydrogen or an alkyl group comprising 1 to 5 carbon atoms, 60 to 100 percent by weight of one or several ethylenically unsaturated ester compounds of formula (II), wherein R represents hydrogen or methyl, R4 represents a linear or branched alkyl radical comprising 6 to 40 carbon atoms, R5 and R6 independently represent hydrogen or a group of formula —COOR′, wherein R′ represents hydrogen or an alkyl group comprising 6 to 40 carbon atoms, and 0 to 40 percent by weight of comonomers, the percentages being relative to the weight of monomer composition A). In a second stage, a monomer composition B) containing 20 to 100 percent by weight of at least one monomer that comprises at least one nitrogen-containing group is grafted onto the graft basis in order to reduce wear in lubricant oil compositions. Said graft polymer comprises a maximum of 200 ppm of sulfur while the weight ratio between monomer composition A) and monomer composition B) ranges between 99.7:0.3 and 80:20.

    摘要翻译： 本发明涉及通过两步聚合获得的接枝聚合物的用途。 在第一阶段中，通过自由基聚合含有0至40重量％的一种或几种式（I）的烯键式不饱和酯化合物，其中R表示氢或甲基， SUP> 1表示包含1至5个碳原子的直链或支链烷基，R 2和R 3独立地表示氢或式-COOR基团 '，其中R'表示氢或包含1至5个碳原子的烷基，60至100重量％的一种或几种式（II）的烯属不饱和酯化合物，其中R表示氢或甲基，R 4 代表含有6至40个碳原子的直链或支链烷基，R 5和R 6独立代表氢或式-COOR'基团，其中 R'表示氢或含有6〜40个碳原子的烷基，0〜40重量％的共聚单体，百分比 年龄相对于单体组合物A）的重量。 在第二阶段中，将包含20至100重量％的至少一种包含至少一个含氮基团的单体的单体组合物B）接枝到接枝基上以减少润滑油组合物中的磨损。 所述接枝聚合物包含最多200ppm的硫，而单体组合物A）和单体组合物B）之间的重量比在99.7:0.3和80:20之间。