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公开(公告)号：US06756030B1
公开(公告)日：2004-06-29
申请号：US10395466
申请日：2003-03-21
申请人： Lisa M. Rohde , Gregory J. Lewis , Mark A. Miller , Jaime G. Moscoso , Jana L. Gisselquist , R. Lyle Patton , Stephen T. Wilson , Deng Yang Jan
发明人： Lisa M. Rohde , Gregory J. Lewis , Mark A. Miller , Jaime G. Moscoso , Jana L. Gisselquist , R. Lyle Patton , Stephen T. Wilson , Deng Yang Jan
IPC分类号： C01B3948
CPC分类号： C10G45/62 , B01J29/70 , B01J29/74 , C01B39/06 , C01B39/065 , C01B39/48 , C10G45/10 , C10G45/12 , C10G45/64 , C10G47/14 , C10G47/20 , C10G49/06 , C10G49/08
摘要： Applicants have synthesized a family of microporous aluminosilicate zeolites and substituted versions thereof which are identified as UZM-8. These new compositions can be prepared using either only one or more organoammonium cations, such as diethyldimethylammonium or ethyltrimethylammonium cations and optionally an alkali and/or an alkaline earth cation as structure directing agents. The UZM-8 compositions are described by an empirical formula of Mmn+Rrp+Al1-xExSiyOz and have a unique x-ray diffraction pattern.
摘要翻译： 申请人已经合成了一系列微孔硅铝酸盐沸石及其取代形式，其被鉴定为UZM-8。 这些新的组合物可以使用仅一种或多种有机铵阳离子，如二乙基二甲基铵或乙基三甲基铵阳离子和任选的碱和/或碱土金属阳离子作为结构定向剂来制备。 UZM-8组合物由经验公式描述并具有独特的x射线衍射图。
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2.发明授权UZM-5, UZM-5P and UZM-6: crystalline aluminosilicate zeolites and processes using the same 有权UZM-5，UZM-5P和UZM-6：结晶硅铝酸盐沸石及其使用方法公开(公告)号：US06613302B1
公开(公告)日：2003-09-02
申请号：US09705860
申请日：2000-11-03
申请人： Jaime G. Moscoso , Gregory J. Lewis , Mark A. Miller , Deng-Yang Jan , R. Lyle Patton , Lisa M. Rohde
发明人： Jaime G. Moscoso , Gregory J. Lewis , Mark A. Miller , Deng-Yang Jan , R. Lyle Patton , Lisa M. Rohde
IPC分类号： C01B3948
CPC分类号： C07C5/2724 , B01J29/70 , B01J29/87 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , Y10S977/775 , Y10S977/776 , Y10S977/895 , Y10S977/896 , Y10S977/949 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A new family of crystalline alumino-silicate zeolites has been synthesized. These zeolites are represented by the empirical formula. Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl ammonium and E is a framework element such as gallium. They are also characterized by unique x-ray diffraction patterns and have catalytic properties for carrying out various hydrocarbon conversion processes.
摘要翻译： 已经合成了一系列新型的结晶铝硅酸盐沸石。 这些沸石由经验式表示，其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。 它们的特征还在于独特的X射线衍射图，并且具有用于进行各种烃转化过程的催化性能。
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公开(公告)号：US06890511B2
公开(公告)日：2005-05-10
申请号：US10395399
申请日：2003-03-21
申请人： Lisa M. Rohde , Gregory J. Lewis , Stephen T. Wilson , Deng-Yang Jan , R. Lyle Patton , Susan C. Koster , Jaime G. Moscoso , Mark A. Miller , Michael G. Gatter
发明人： Lisa M. Rohde , Gregory J. Lewis , Stephen T. Wilson , Deng-Yang Jan , R. Lyle Patton , Susan C. Koster , Jaime G. Moscoso , Mark A. Miller , Michael G. Gatter
CPC分类号： B01J29/87 , B01J29/70 , B01J2229/16 , B01J2229/32 , B01J2229/36 , B01J2229/37 , C01B39/026 , C01B39/082 , C01B39/48 , C01P2002/72 , C07C7/13
摘要： An aluminosilicate zeolite and substituted versions designated UZM-15 have been synthesized. These zeolites are prepared using an organoammonium cation as a template in which at least one organic group has at least 2 carbon atoms. An example of such a cation is diethyldimethylammonium cation. The template can optionally comprise other organoammonium cations, alkali metals and alkaline earth metals. These UZM-15 materials can be dealuminated by various processes to provide UZM-15HS compositions. Both the UZM-15 and UZM-15HS compositions are useful as catalysts or catalyst supports in various process such as the conversion of cyclic hydrocarbons to non-cyclic hydrocarbons and olefin oligomerization.
摘要翻译： 已经合成了一种硅铝酸盐沸石，并且被认为是UZM-15的取代物。 使用有机铵阳离子作为模板制备这些沸石，其中至少一个有机基团具有至少2个碳原子。 这种阳离子的实例是二乙基二甲基铵阳离子。 模板可任选地包含其它有机铵阳离子，碱金属和碱土金属。 这些UZM-15材料可以通过各种工艺脱铝以提供UZM-15HS组合物。 UZM-15和UZM-15HS组合物可用作各种方法中的催化剂或催化剂载体，例如将环烃转化为非环烃和烯烃低聚。
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公开(公告)号：US07713513B2
公开(公告)日：2010-05-11
申请号：US11340914
申请日：2006-01-27
申请人： Deng-Yang Jan , Jaime G. Moscoso , Susan C. Koster , Lisa M. Knight , Gregory J. Lewis , Mark A. Miller , R. Lyle Patton , Stephen T. Wilson
发明人： Deng-Yang Jan , Jaime G. Moscoso , Susan C. Koster , Lisa M. Knight , Gregory J. Lewis , Mark A. Miller , R. Lyle Patton , Stephen T. Wilson
CPC分类号： C01B39/026 , C01B39/48 , C01P2002/72 , C10G11/05 , C10G35/095 , C10G45/12 , C10G47/16
摘要： A family of crystalline aluminosilicate zeolites designated UZM-8HS and derived from UZM-8 have been synthesized. The aluminum content of the UZM-8HS is lower than that of the starting UZM-8 thus changing its ion exchange capacity and acidity. These UZM-8HS are represented by the empirical formula: M1an+Al(1−x)ExSiy′Oz″ and are prepared by treatments such as acid extraction and AFS treatments.
摘要翻译： 已经合成了一系列称为UZM-8HS并衍生自UZM-8的结晶硅铝酸盐沸石。 UZM-8HS的铝含量低于起始UZM-8的铝含量，从而改变其离子交换能力和酸度。 这些UZM-8HS由经验公式：M1an + Al（1-x）ExSiy'Oz表示，并且通过诸如酸提取和AFS处理的处理来制备。
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5.发明授权UZM-12 and UZM-12HS: crystalline aluminosilicate zeolitic compositions and processes for preparing and using the compositions 有权UZM-12和UZM-12HS：结晶硅铝酸盐沸石组合物和制备和使用组合物的方法公开(公告)号：US07344694B2
公开(公告)日：2008-03-18
申请号：US10959453
申请日：2004-10-06
IPC分类号： C01B39/30
CPC分类号： C01B39/48 , B01J29/50 , C01B39/305
摘要： A series of crystalline alumino-silicate zeolites identified as UZM-12 have been synthesized. These UZM-12 compositions have the ERI topology, a Si/Al>5.5 and can be prepared as nanocrystallites having an average particle size of about 15 to about 50 nanometers and a spheroidal morphology. The UZM-12 composition can be treated to remove at least a fraction of the framework aluminum atoms thereby providing zeolites with a Si/Al>5.75 and identified as UZM-12HS. Both the UZM-12 and UZM-12HS can catalyze various hydrocarbon conversion processes.
摘要翻译： 已经合成了一系列标准为UZM-12的结晶铝硅酸盐沸石。 这些UZM-12组合物具有ERI拓扑结构，Si / Al> 5.5，并且可以制备为具有约15至约50纳米的平均粒度和球形形态的纳米晶体。 可以处理UZM-12组合物以除去至少一部分骨架铝原子，从而提供具有Si / Al> 5.75的沸石并鉴定为UZM-12HS。 UZM-12和UZM-12HS都可以催化各种烃转化过程。
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6.发明授权公开(公告)号：US06500998B1
公开(公告)日：2002-12-31
申请号：US10062691
申请日：2002-01-31
IPC分类号： C07C424
CPC分类号： C07C5/2724 , B01J29/04 , B01J29/70 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A process for transalkylating a polyalkylated aromatic compound with a non-alkylated aromatic compound using a new family of related crystalline aluminosilicate zeolites has been developed. These zeolites are represented by the empirical formula: Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl-ammonium and E is a framework element such as gallium.
摘要翻译： 已经开发了使用新的相关结晶硅铝酸盐沸石系列将多烷基化芳族化合物与非烷基化芳族化合物烷基化的方法。 这些沸石由经验式表示：其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。
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公开(公告)号：US06713041B1
公开(公告)日：2004-03-30
申请号：US10074612
申请日：2002-02-12
IPC分类号： C01B3914
CPC分类号： C01B39/145 , B01J29/70 , B01J29/7003 , B01J2229/32 , C10G11/05 , C10G45/64 , C10G47/16 , Y10S423/24
摘要： Applicants have synthesized a new aluminosilicate zeolite identified as UZM-9. This new zeolite has the LTA topology and has an empirical formula of: Mmn+Rrp+Al1-xExSiyOz where M is an alkali or alkaline earth metal ion, R is at least two organic ions, at least one of which has an organic group with at least two carbon atoms and E can be gallium, iron, boron and mixtures thereof. The Si/Al ratio can range from greater than 3.5 to about 6.0.
摘要翻译： 申请人合成了一种被认定为UZM-9的新型硅铝酸盐沸石。 这种新沸石具有LTA拓扑结构，并且具有以下经验式：其中M是碱金属或碱土金属离子，R是至少两个有机离子，其中至少一个具有至少两个碳原子的有机基团，E 可以是镓，铁，硼及其混合物。 Si / Al比可以在大于3.5至约6.0的范围内。
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8.发明授权公开(公告)号：US06388157B1
公开(公告)日：2002-05-14
申请号：US09706285
申请日：2000-11-03
IPC分类号： C07C268
CPC分类号： C07C5/2724 , B01J29/04 , B01J29/70 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A process for alkylation of aromatic compounds using a new family of related crystalline aluminosilicate zeolites has been developed. These zeolites are represented by the empirical formula: Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl-ammonium and E is a framework element such as gallium.
摘要翻译： 已经开发了使用新的相关结晶硅铝酸盐沸石族烷基化芳族化合物的方法。 这些沸石由经验式表示：其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。
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公开(公告)号：US06388159B1
公开(公告)日：2002-05-14
申请号：US09705839
申请日：2000-11-03
IPC分类号： C07C522
CPC分类号： C07C5/2724 , B01J29/04 , B01J29/70 , B01J2229/26 , B01J2229/42 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A process for isomerising xylene using a new family of related crystalline aluminosilicate zeolites has been developed. These zeolites are represented by the empirical formula: Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl-ammonium and E is a framework element such as gallium.
摘要翻译： 已经开发了使用新的相关结晶硅铝酸盐沸石族异构化二甲苯的方法。 这些沸石由经验式表示：其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。
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公开(公告)号：US06752980B1
公开(公告)日：2004-06-22
申请号：US10395639
申请日：2003-03-21
IPC分类号： C01B3948
CPC分类号： C10G11/05 , B01J29/50 , B01J29/70 , B01J2229/16 , B01J2229/32 , B01J2229/36 , B01J2229/37 , C01B39/026 , C01B39/06 , C01B39/065 , C01B39/48
摘要： An aluminosilicate zeolite and substituted version designated UZM-16 have been synthesized. These zeolites are prepared using benzyltrimethyl-ammonium (BzTMA) cation or a combination of BzTMA and at least one other quaternary ammonium cation These zeolites have a structure that is related to offretite, but shows structurally different and distinct features. The UZM-16 zeolites can be dealuminated to form UZM-16HS zeolites which have different acidity, porosity and ion-exchange properties. Both UZM-16 and UZM-16HS are useful in various hydrocarbon conversion processes.
摘要翻译： 已经合成了一种硅铝酸盐沸石，并且被认定为UZM-16的取代物。 这些沸石使用苄基三甲基铵（BzTMA）阳离子或BzTMA和至少一种其他季铵阳离子的组合制备。这些沸石具有与白云母相关的结构，但显示出结构上不同和明显的特征。 UZM-16沸石可以脱铝以形成具有不同酸度，孔隙率和离子交换性能的UZM-16HS沸石。 UZM-16和UZM-16HS都可用于各种烃转化过程。
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