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公开(公告)号：US06756030B1
公开(公告)日：2004-06-29
申请号：US10395466
申请日：2003-03-21
申请人： Lisa M. Rohde , Gregory J. Lewis , Mark A. Miller , Jaime G. Moscoso , Jana L. Gisselquist , R. Lyle Patton , Stephen T. Wilson , Deng Yang Jan
发明人： Lisa M. Rohde , Gregory J. Lewis , Mark A. Miller , Jaime G. Moscoso , Jana L. Gisselquist , R. Lyle Patton , Stephen T. Wilson , Deng Yang Jan
IPC分类号： C01B3948
CPC分类号： C10G45/62 , B01J29/70 , B01J29/74 , C01B39/06 , C01B39/065 , C01B39/48 , C10G45/10 , C10G45/12 , C10G45/64 , C10G47/14 , C10G47/20 , C10G49/06 , C10G49/08
摘要： Applicants have synthesized a family of microporous aluminosilicate zeolites and substituted versions thereof which are identified as UZM-8. These new compositions can be prepared using either only one or more organoammonium cations, such as diethyldimethylammonium or ethyltrimethylammonium cations and optionally an alkali and/or an alkaline earth cation as structure directing agents. The UZM-8 compositions are described by an empirical formula of Mmn+Rrp+Al1-xExSiyOz and have a unique x-ray diffraction pattern.
摘要翻译： 申请人已经合成了一系列微孔硅铝酸盐沸石及其取代形式，其被鉴定为UZM-8。 这些新的组合物可以使用仅一种或多种有机铵阳离子，如二乙基二甲基铵或乙基三甲基铵阳离子和任选的碱和/或碱土金属阳离子作为结构定向剂来制备。 UZM-8组合物由经验公式描述并具有独特的x射线衍射图。
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2.发明授权UZM-5, UZM-5P and UZM-6: crystalline aluminosilicate zeolites and processes using the same 有权UZM-5，UZM-5P和UZM-6：结晶硅铝酸盐沸石及其使用方法公开(公告)号：US06613302B1
公开(公告)日：2003-09-02
申请号：US09705860
申请日：2000-11-03
申请人： Jaime G. Moscoso , Gregory J. Lewis , Mark A. Miller , Deng-Yang Jan , R. Lyle Patton , Lisa M. Rohde
发明人： Jaime G. Moscoso , Gregory J. Lewis , Mark A. Miller , Deng-Yang Jan , R. Lyle Patton , Lisa M. Rohde
IPC分类号： C01B3948
CPC分类号： C07C5/2724 , B01J29/70 , B01J29/87 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , Y10S977/775 , Y10S977/776 , Y10S977/895 , Y10S977/896 , Y10S977/949 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A new family of crystalline alumino-silicate zeolites has been synthesized. These zeolites are represented by the empirical formula. Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl ammonium and E is a framework element such as gallium. They are also characterized by unique x-ray diffraction patterns and have catalytic properties for carrying out various hydrocarbon conversion processes.
摘要翻译： 已经合成了一系列新型的结晶铝硅酸盐沸石。 这些沸石由经验式表示，其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。 它们的特征还在于独特的X射线衍射图，并且具有用于进行各种烃转化过程的催化性能。
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公开(公告)号：US06890511B2
公开(公告)日：2005-05-10
申请号：US10395399
申请日：2003-03-21
申请人： Lisa M. Rohde , Gregory J. Lewis , Stephen T. Wilson , Deng-Yang Jan , R. Lyle Patton , Susan C. Koster , Jaime G. Moscoso , Mark A. Miller , Michael G. Gatter
发明人： Lisa M. Rohde , Gregory J. Lewis , Stephen T. Wilson , Deng-Yang Jan , R. Lyle Patton , Susan C. Koster , Jaime G. Moscoso , Mark A. Miller , Michael G. Gatter
CPC分类号： B01J29/87 , B01J29/70 , B01J2229/16 , B01J2229/32 , B01J2229/36 , B01J2229/37 , C01B39/026 , C01B39/082 , C01B39/48 , C01P2002/72 , C07C7/13
摘要： An aluminosilicate zeolite and substituted versions designated UZM-15 have been synthesized. These zeolites are prepared using an organoammonium cation as a template in which at least one organic group has at least 2 carbon atoms. An example of such a cation is diethyldimethylammonium cation. The template can optionally comprise other organoammonium cations, alkali metals and alkaline earth metals. These UZM-15 materials can be dealuminated by various processes to provide UZM-15HS compositions. Both the UZM-15 and UZM-15HS compositions are useful as catalysts or catalyst supports in various process such as the conversion of cyclic hydrocarbons to non-cyclic hydrocarbons and olefin oligomerization.
摘要翻译： 已经合成了一种硅铝酸盐沸石，并且被认为是UZM-15的取代物。 使用有机铵阳离子作为模板制备这些沸石，其中至少一个有机基团具有至少2个碳原子。 这种阳离子的实例是二乙基二甲基铵阳离子。 模板可任选地包含其它有机铵阳离子，碱金属和碱土金属。 这些UZM-15材料可以通过各种工艺脱铝以提供UZM-15HS组合物。 UZM-15和UZM-15HS组合物可用作各种方法中的催化剂或催化剂载体，例如将环烃转化为非环烃和烯烃低聚。
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公开(公告)号：US07713513B2
公开(公告)日：2010-05-11
申请号：US11340914
申请日：2006-01-27
申请人： Deng-Yang Jan , Jaime G. Moscoso , Susan C. Koster , Lisa M. Knight , Gregory J. Lewis , Mark A. Miller , R. Lyle Patton , Stephen T. Wilson
发明人： Deng-Yang Jan , Jaime G. Moscoso , Susan C. Koster , Lisa M. Knight , Gregory J. Lewis , Mark A. Miller , R. Lyle Patton , Stephen T. Wilson
CPC分类号： C01B39/026 , C01B39/48 , C01P2002/72 , C10G11/05 , C10G35/095 , C10G45/12 , C10G47/16
摘要： A family of crystalline aluminosilicate zeolites designated UZM-8HS and derived from UZM-8 have been synthesized. The aluminum content of the UZM-8HS is lower than that of the starting UZM-8 thus changing its ion exchange capacity and acidity. These UZM-8HS are represented by the empirical formula: M1an+Al(1−x)ExSiy′Oz″ and are prepared by treatments such as acid extraction and AFS treatments.
摘要翻译： 已经合成了一系列称为UZM-8HS并衍生自UZM-8的结晶硅铝酸盐沸石。 UZM-8HS的铝含量低于起始UZM-8的铝含量，从而改变其离子交换能力和酸度。 这些UZM-8HS由经验公式：M1an + Al（1-x）ExSiy'Oz表示，并且通过诸如酸提取和AFS处理的处理来制备。
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5.发明授权UZM-12 and UZM-12HS: crystalline aluminosilicate zeolitic compositions and processes for preparing and using the compositions 有权UZM-12和UZM-12HS：结晶硅铝酸盐沸石组合物和制备和使用组合物的方法公开(公告)号：US07344694B2
公开(公告)日：2008-03-18
申请号：US10959453
申请日：2004-10-06
IPC分类号： C01B39/30
CPC分类号： C01B39/48 , B01J29/50 , C01B39/305
摘要： A series of crystalline alumino-silicate zeolites identified as UZM-12 have been synthesized. These UZM-12 compositions have the ERI topology, a Si/Al>5.5 and can be prepared as nanocrystallites having an average particle size of about 15 to about 50 nanometers and a spheroidal morphology. The UZM-12 composition can be treated to remove at least a fraction of the framework aluminum atoms thereby providing zeolites with a Si/Al>5.75 and identified as UZM-12HS. Both the UZM-12 and UZM-12HS can catalyze various hydrocarbon conversion processes.
摘要翻译： 已经合成了一系列标准为UZM-12的结晶铝硅酸盐沸石。 这些UZM-12组合物具有ERI拓扑结构，Si / Al> 5.5，并且可以制备为具有约15至约50纳米的平均粒度和球形形态的纳米晶体。 可以处理UZM-12组合物以除去至少一部分骨架铝原子，从而提供具有Si / Al> 5.75的沸石并鉴定为UZM-12HS。 UZM-12和UZM-12HS都可以催化各种烃转化过程。
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公开(公告)号：US06776975B2
公开(公告)日：2004-08-17
申请号：US10142806
申请日：2002-05-09
IPC分类号： C01B3906
CPC分类号： C10G47/16 , B01J29/70 , B01J2229/36 , C01B39/026 , C01B39/48 , C10G2400/30
摘要： Applicants have synthesized a new crystalline aluminosilicate zeolite identified as UZM-4M. This new zeolite is obtained by treating a UZM-4 zeolite with a fluorosilicate salt to obtain a zeolite having the empirical formula: M1an+Al1-xExSiyOz where M1 is an alkali metal, alkaline earth metal, rare earth metal, hydronium ion or ammonium ion, E can be gallium, iron, boron, indium and mixtures thereof and has a Si/Al ratio of 1.5 to about 10.
摘要翻译： 申请人已经合成了一种新的结晶硅铝酸盐沸石，被认定为UZM-4M。 这种新的沸石是通过用氟硅酸盐处理UZM-4沸石得到具有以下经验式的沸石得到的：其中M1是碱金属，碱土金属，稀土金属，水合氢离子或铵离子，E可以是镓 ，铁，硼，铟及其混合物，Si / Al比为1.5至约10。
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公开(公告)号：US07585489B2
公开(公告)日：2009-09-08
申请号：US12198911
申请日：2008-08-27
申请人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
发明人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
CPC分类号： C07C4/06 , B01J29/18 , B01J29/65 , B01J29/70 , B01J29/7007 , B01J29/7011 , B01J29/7023 , B01J29/7042 , B01J29/7046 , B01J29/80 , B01J29/90 , B01J35/002 , B01J2229/12 , B01J2229/16 , B01J2229/32 , B01J2229/42 , B01J2229/62 , C07C2529/65 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/06 , C07C11/04
摘要： A process is disclosed for enhancing the production of light olefins using a catalyst with small pores. The catalyst comprises a molecular sieve having 10 membered rings with channels of limited length. The molecular sieve has a high silica to alumina ratio and has pores sized to limit production of aromatics in the cracking process.
摘要翻译： 公开了一种使用具有小孔的催化剂增强轻质烯烃生产的方法。 该催化剂包括具有10个长度环通道的分子筛。 分子筛具有高的二氧化硅与氧化铝的比例，并具有孔径以限制裂化过程中芳族化合物的生产。
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公开(公告)号：US07446071B2
公开(公告)日：2008-11-04
申请号：US10990803
申请日：2004-11-17
申请人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
发明人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
IPC分类号： B01J29/80
CPC分类号： C07C4/06 , B01J29/18 , B01J29/65 , B01J29/70 , B01J29/7007 , B01J29/7011 , B01J29/7023 , B01J29/7042 , B01J29/7046 , B01J29/80 , B01J29/90 , B01J35/002 , B01J2229/12 , B01J2229/16 , B01J2229/32 , B01J2229/42 , B01J2229/62 , C07C2529/65 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/06 , C07C11/04
摘要： A process is disclosed for enhancing the production of light olefins using a catalyst with small pores. The catalyst comprises a layered zeolite material comprising an inner layer having pores of 8 or 10 membered rings and an outer layer having pores of 10 membered rings. The pores in the outer layer overlaying the pores in the inner layer. The zeolite has a silicon to aluminum atomic ratio of about 20 to about 200 and its surface acid sites external to the pores have been substantially neutralized.
摘要翻译： 公开了一种使用具有小孔的催化剂增强轻质烯烃生产的方法。 该催化剂包括层状沸石材料，其包括具有8或10元环孔的内层和具有10元环孔的外层。 外层中的孔覆盖内层中的孔。 沸石的硅铝原子比为约20至约200，并且其孔外部的表面酸性位点已被基本上中和。
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公开(公告)号：US06867341B1
公开(公告)日：2005-03-15
申请号：US10246801
申请日：2002-09-17
申请人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
发明人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
CPC分类号： C07C4/06 , B01J29/18 , B01J29/65 , B01J29/70 , B01J29/7007 , B01J29/7011 , B01J29/7023 , B01J29/7042 , B01J29/7046 , B01J29/80 , B01J29/90 , B01J35/002 , B01J2229/12 , B01J2229/16 , B01J2229/32 , B01J2229/42 , B01J2229/62 , C07C2529/65 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/06 , C07C11/04
摘要： A process is disclosed for enhancing the production of light olefins using a catalyst with small pores. The catalyst comprises a molecular sieve having 10 membered rings with channels of limited length. The molecular sieve has a high silica to alumina ratio and has pores sized to limit production of aromatics in the cracking process.
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公开(公告)号：US20080318764A1
公开(公告)日：2008-12-25
申请号：US12198911
申请日：2008-08-27
申请人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
发明人： Hayim Abrevaya , Suheil F. Abdo , R. Lyle Patton
CPC分类号： C07C4/06 , B01J29/18 , B01J29/65 , B01J29/70 , B01J29/7007 , B01J29/7011 , B01J29/7023 , B01J29/7042 , B01J29/7046 , B01J29/80 , B01J29/90 , B01J35/002 , B01J2229/12 , B01J2229/16 , B01J2229/32 , B01J2229/42 , B01J2229/62 , C07C2529/65 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/06 , C07C11/04
摘要： A process is disclosed for enhancing the production of light olefins using a catalyst with small pores. The catalyst comprises a molecular sieve having 10 membered rings with channels of limited length. The molecular sieve has a high silica to alumina ratio and has pores sized to limit production of aromatics in the cracking process.
摘要翻译： 公开了一种使用具有小孔的催化剂增强轻质烯烃生产的方法。 该催化剂包括具有10个长度环通道的分子筛。 分子筛具有高的二氧化硅与氧化铝的比例，并具有孔径以限制裂化过程中芳族化合物的生产。
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