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公开(公告)号：US07935734B2
公开(公告)日：2011-05-03
申请号：US11480348
申请日：2006-06-30
Applicant: Anna Lee Tonkovich , Kai Tod Paul Jarosch , Timothy J. Sullivan , Terry Mazanec , Sean Patrick Fitzgerald , Maddalena Fanelli
Inventor： Anna Lee Tonkovich , Kai Tod Paul Jarosch , Timothy J. Sullivan , Terry Mazanec , Sean Patrick Fitzgerald , Maddalena Fanelli
IPC: C07C27/00
CPC classification number: B01J23/8896 , B01J19/0093 , B01J35/023 , B01J2219/00783 , B01J2219/00788 , B01J2219/00835 , B01J2219/00873 , B01J2219/00889 , B01J2219/00984 , C10G2/32 , C10G2/33 , C10G29/205 , C10G45/02 , C10G47/02 , C10G50/00 , C10G2300/301 , C10G2300/302 , C10G2300/4018 , C10G2300/4025 , C10G2300/802 , C10G2300/805 , C10G2300/807 , C10G2400/04 , C10G2400/10 , C10L1/08
Abstract: The disclosed technology relates to a process for conducting a chemical reaction between at least one liquid reactant and at least one gaseous reactant in a process microchannel containing at least one catalyst, the catalyst comprising a solid phase catalyst or a homogeneous catalyst immobilized on a solid. In one embodiment, the process microchannel comprises a processing zone containing one or more structures for disrupting fluid flow and a reaction zone containing one or more structures for contacting and/or supporting the catalyst, the one or more structures for contacting and/or supporting the catalyst containing openings to permit the reactants to flow through the one or more structures and contact the catalyst.
Abstract translation: 所公开的技术涉及在含有至少一种催化剂的工艺微通道中的至少一种液体反应物与至少一种气体反应物之间进行化学反应的方法，所述催化剂包含固相催化剂或固相在固体上的均相催化剂。 在一个实施方案中，工艺微通道包括含有用于破坏流体流动的一种或多种结构的处理区和含有用于接触和/或支撑催化剂的一种或多种结构的反应区，用于接触和/或支撑催化剂的一种或多种结构 催化剂含有开口以允许反应物流过一个或多个结构并与催化剂接触。
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42.发明申请公开(公告)号：US20110009653A1
公开(公告)日：2011-01-13
申请号：US12501505
申请日：2009-07-13
Applicant: Terry Mazanec , Soumitra Desmukh , Laura J. Silva , Torsten Maurer , Radwan Abdallah , Frank Rasowski
Inventor： Terry Mazanec , Soumitra Desmukh , Laura J. Silva , Torsten Maurer , Radwan Abdallah , Frank Rasowski
IPC: C07D301/03
CPC classification number: C07D301/08
Abstract: This invention relates to a process comprising reacting ethylene and oxygen or a source of oxygen in a process microchannel in the presence of a catalyst to form a product comprising ethylene oxide.
Abstract translation: 本发明涉及一种方法，其包括在催化剂存在下在工艺微通道中使乙烯和氧气或氧源反应，形成包含环氧乙烷的产物。
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43.发明申请FISCHER-TROPSCH SYNTHESIS USING MICROCHANNEL TECHNOLOGY AND NOVEL CATALYST AND MICROCHANNEL REACOTR 有权使用微通道技术和新型催化剂和微通道反应器进行FISCHER-TROPSCH合成公开(公告)号：US20100160463A1
公开(公告)日：2010-06-24
申请号：US12718356
申请日：2010-03-05
Applicant: Yong Wang , Anna Lee Tonkovich , Terry Mazanec , Francis P. Daly , Dave VanderWiel , Jianli Hu , Chunshe Cao , Charles Kibby , Xiaohong Shari Li , Michael D. Briscoe , Nathan Gano , Ya-Huei Chin
Inventor： Yong Wang , Anna Lee Tonkovich , Terry Mazanec , Francis P. Daly , Dave VanderWiel , Jianli Hu , Chunshe Cao , Charles Kibby , Xiaohong Shari Li , Michael D. Briscoe , Nathan Gano , Ya-Huei Chin
CPC classification number: C10G2/332 , B01J19/0093 , B01J21/04 , B01J23/75 , B01J23/8896 , B01J23/8913 , B01J35/0066 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J37/0205 , B01J2219/00783 , B01J2219/00822 , B01J2219/00824 , B01J2219/00826 , B01J2219/00831 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , C10G2/341 , C10G2300/301 , C10G2300/4018 , C10G2300/4025 , C10G2300/70 , C10G2400/04 , C10G2400/10 , Y02P20/582
Abstract: The disclosed invention relates to a process for converting a reactant composition comprising H2 and CO to a product comprising at least one aliphatic hydrocarbon having at least about 5 carbon atoms, the process comprising: flowing the reactant composition through a microchannel reactor in contact with a Fischer-Tropsch catalyst to convert the reactant composition to the product, the microchannel reactor comprising a plurality of process microchannels containing the catalyst; transferring heat from the process microchannels to a heat exchanger; and removing the product from the microchannel reactor; the process producing at least about 0.5 gram of aliphatic hydrocarbon having at least about 5 carbon atoms per gram of catalyst per hour; the selectivity to methane in the product being less than about 25%. The disclosed invention also relates to a supported catalyst comprising Co, and a microchannel reactor comprising at least one process microchannel and at least one adjacent heat exchange zone.
Abstract translation: 所公开的发明涉及将包含H 2和CO的反应物组合物转化为包含至少一种具有至少约5个碳原子的脂族烃的产物的方法，该方法包括：使反应物组合物流过与Fischer接触的微通道反应器 - 催化剂将反应物组合物转化成产物，微通道反应器包含多个含有催化剂的工艺微通道; 将热量从工艺微通道传递到热交换器; 并从微通道反应器中除去产物; 该方法每小时产生至少约0.5克具有至少约5个碳原子的每克催化剂的脂族烃; 产品中甲烷的选择性小于约25％。 所公开的发明还涉及包含Co的载体催化剂和包含至少一个工艺微通道和至少一个相邻的热交换区的微通道反应器。
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公开(公告)号：US20090043141A1
公开(公告)日：2009-02-12
申请号：US12156461
申请日：2008-05-30
Applicant: Terry Mazanec , Wayne Simmons , John Brophy , Fred Pesa , Anna Lee Y. Tonkovich , Robert D. Litt , Dongming Qiu , Laura J. Silva , Micheal J. Lamont , Maddalena Fanelli
Inventor： Terry Mazanec , Wayne Simmons , John Brophy , Fred Pesa , Anna Lee Y. Tonkovich , Robert D. Litt , Dongming Qiu , Laura J. Silva , Micheal J. Lamont , Maddalena Fanelli
CPC classification number: B01J19/0093 , B01J2219/00783 , B01J2219/00835 , B01J2219/0086 , B01J2219/00867 , B01J2219/00873 , B01J2219/00889 , B01J2219/00891 , B01J2219/00905 , B01J2219/00907 , B01J2219/00918 , B01J2219/00921 , C07C2/84 , C10G50/00 , C10G2400/20 , Y02P30/40
Abstract: A microchannel apparatus comprising a conduit including a microchannel mixing section, a microchannel reaction section, a microchannel heat transfer section, and a separation section, where the microchannel mixing section includes direct injection inlets, where the microchannel mixing section is downstream from the reaction section, and where the separation section is downstream from the reaction section. Further exemplary embodiments are also disclosed.
Abstract translation: 一种微通道装置，包括微通道混合部分，微通道反应部分，微通道传热部分和分离部分的导管，其中微通道混合部分包括直接注射入口，其中微通道混合部分在反应部分的下游， 并且其中分离部分在反应部分的下游。 还公开了另外的示例性实施例。
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Patent Agency Ranking
45.发明授权Process and apparatus for improved methods for making vinyl acetate monomer (VAM) 有权制备乙酸乙烯酯单体（VAM）的改进方法的方法和设备公开(公告)号：US07468455B2
公开(公告)日：2008-12-23
申请号：US11256217
申请日：2005-10-20
Applicant: Terry Mazanec , Victor J. Johnston , Michael Huckman , Sean P. Fitzgerald , James A. Foster , Daniel Lindley , Anna Lee Tonkovich , Francis P. Daly , Leslie Wade , Tony Hammock , Thomas Yuschak , Bin Yang , Kai Jarosch
Inventor： Terry Mazanec , Victor J. Johnston , Michael Huckman , Sean P. Fitzgerald , James A. Foster , Daniel Lindley , Anna Lee Tonkovich , Francis P. Daly , Leslie Wade , Tony Hammock , Thomas Yuschak , Bin Yang , Kai Jarosch
CPC classification number: B01J19/0093 , B01J2219/00783 , B01J2219/00835 , B01J2219/0086 , B01J2219/00862 , B01J2219/00873 , B01J2219/00889 , C07C67/055 , C07C69/01 , C07C69/15
Abstract: The invention provides methods, apparatus and chemical systems for making vinyl acetate from ethylene, oxygen, and acetic acid.
Abstract translation: 本发明提供从乙烯，氧和乙酸制备乙酸乙烯酯的方法，装置和化学体系。
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公开(公告)号：US20080214884A1
公开(公告)日：2008-09-04
申请号：US11549625
申请日：2006-10-13
Applicant: Francis P. Daly , Richard Long , Junko Ida , Rachid Taha , Terry Mazanec , Barry L. Yang
Inventor： Francis P. Daly , Richard Long , Junko Ida , Rachid Taha , Terry Mazanec , Barry L. Yang
CPC classification number: B01J19/0053 , B01J19/0093 , B01J21/066 , B01J23/42 , B01J23/464 , B01J23/628 , B01J23/892 , B01J23/8926 , B01J35/002 , B01J35/006 , B01J37/0225 , B01J37/0226 , B01J37/0244 , B01J37/14 , B01J37/16 , B01J37/18 , B01J2219/00783 , B01J2219/00822 , B01J2219/00824 , B01J2219/00831 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00891 , C01B3/384 , C01B3/40 , C01B32/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0244 , C01B2203/0261 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/1047 , C01B2203/107 , C01B2203/1241 , C07C5/48 , C07C2523/42 , C07C2523/46 , C23C18/1216 , C23C18/1644 , C23C18/1803 , C23C18/1817 , C23C18/44 , Y02E60/364 , Y02P20/128 , Y02P20/142 , Y02P20/52 , Y02T50/67 , C07C11/04
Abstract: Novel methods of electroless plating are described. Catalyst coatings can be applied within microchannel apparatus. Various reactions, including combustion and steam reforming, can be conducted over electroless catalyst coatings.
Abstract translation: 描述了无电镀的新方法。 催化剂涂层可以应用于微通道设备内。 可以通过无电催化剂涂层进行各种反应，包括燃烧和蒸汽重整。
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47.发明授权Process for conducting an equilibrium limited chemical reaction in a single stage process channel 有权在单级过程通道中进行平衡有限化学反应的方法公开(公告)号：US06969505B2
公开(公告)日：2005-11-29
申请号：US10219956
申请日：2002-08-15
Applicant: Anna Lee Tonkovich , Wayne W. Simmons , Kai Tod Paul Jarosch , Terry Mazanec , Eric Daymo , Ying Peng , Jennifer Lynne Marco
Inventor： Anna Lee Tonkovich , Wayne W. Simmons , Kai Tod Paul Jarosch , Terry Mazanec , Eric Daymo , Ying Peng , Jennifer Lynne Marco
CPC classification number: B01J19/0093 , B01J23/80 , B01J2219/00783 , B01J2219/00835 , B01J2219/0086 , B01J2219/00873 , C01B3/16 , C01B2203/0283 , C01B2203/1041 , Y02P20/52
Abstract: This invention relates to a process for conducting an equilibrium limited chemical reaction in a single stage process channel. A process for conducting a water shift reaction is disclosed. A multichannel reactor with cross flow heat exchange is disclosed.
Abstract translation: 本发明涉及在单级工艺通道中进行平衡有限化学反应的方法。 公开了进行水位变换反应的方法。 公开了一种具有横流热交换的多通道反应器。
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公开(公告)号：US20050244304A1
公开(公告)日：2005-11-03
申请号：US11089440
申请日：2005-03-23
Applicant: Anna Tonkovich , Barry Yang , Terry Mazanec , Francis Daly , Sean Fitzgerald , Ravi Arora , Dongming Qiu , Bin Yang , Steven Perry , Kai Jarosh , Paul Neagle , David Hesse , Rachid Taha , Richard Long , Jeff Marco , Thomas Yuschak , Jeffrey Ramler , Mike Marchiando
Inventor： Anna Tonkovich , Barry Yang , Terry Mazanec , Francis Daly , Sean Fitzgerald , Ravi Arora , Dongming Qiu , Bin Yang , Steven Perry , Kai Jarosh , Paul Neagle , David Hesse , Rachid Taha , Richard Long , Jeff Marco , Thomas Yuschak , Jeffrey Ramler , Mike Marchiando
CPC classification number: B01J37/0226 , B01J19/0093 , B01J35/04 , B01J37/0215 , B01J37/0238 , B01J2219/00783 , B01J2219/00822 , B01J2219/00824 , B01J2219/00835 , B01J2219/00837 , B01J2219/00873 , B01J2219/00891 , B01J2219/00905 , B01J2219/00995 , B01L3/502707 , B01L3/502746 , B01L2200/12 , B01L2300/16 , B01L2400/0406 , B01L2400/086 , B01L2400/088
Abstract: Interior microchannels within microchannel apparatus are uniformly coated. Remarkably, these uniform coatings are formed from materials that are applied to the interior microchannels after an apparatus has been assembled or manufactured. Coatings can be made uniform along the length of a microchannel, in the corner of a microchannel, and/or throughout numerous microchannels in an array of microchannels. Techniques for tailoring the application of washcoats onto microchannels is also described.
Abstract translation: 微通道设备内部的微通道均匀涂覆。 值得注意的是，这些均匀的涂层由在装置组装或制造之后施加到内部微通道的材料形成。 涂层可以沿着微通道的长度，微通道的角部和/或整个微通道阵列中的许多微通道而均匀。 还描述了将洗衣布应用于微通道的技术。
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49.发明申请Fischer-Tropsch synthesis using microchannel technology and novel catalyst and microchannel reactor 有权使用微通道技术的费 - 托合成和新型催化剂和微通道反应器公开(公告)号：US20050165121A1
公开(公告)日：2005-07-28
申请号：US10766297
申请日：2004-01-28
Applicant: Yong Wang , Anna Tonkovich , Terry Mazanec , Francis Daly , Dave VanderWiel , Jianli Hu , Chunshe Cao , Charles Kibby , Xiaohong Li , Michael Briscoe , Nathan Gano , Ya-Huei Chin
Inventor： Yong Wang , Anna Tonkovich , Terry Mazanec , Francis Daly , Dave VanderWiel , Jianli Hu , Chunshe Cao , Charles Kibby , Xiaohong Li , Michael Briscoe , Nathan Gano , Ya-Huei Chin
IPC: B01J19/00 , B01J19/24 , B01J21/04 , B01J23/75 , B01J23/889 , B01J23/89 , B01J35/10 , B01J37/02 , C10G2/00 , C07C27/26
CPC classification number: C10G2/332 , B01J19/0093 , B01J21/04 , B01J23/75 , B01J23/8896 , B01J23/8913 , B01J35/0066 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J37/0205 , B01J2219/00783 , B01J2219/00822 , B01J2219/00824 , B01J2219/00826 , B01J2219/00831 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , C10G2/341 , C10G2300/301 , C10G2300/4018 , C10G2300/4025 , C10G2300/70 , C10G2400/04 , C10G2400/10 , Y02P20/582
Abstract: The disclosed invention relates to a process for converting a reactant composition comprising H2 and CO to a product comprising at least one aliphatic hydrocarbon having at least about 5 carbon atoms, the process comprising: flowing the reactant composition through a microchannel reactor in contact with a Fischer-Tropsch catalyst to convert the reactant composition to the product, the microchannel reactor comprising a plurality of process microchannels containing the catalyst; transferring heat from the process microchannels to a heat exchanger; and removing the product from the microchannel reactor; the process producing at least about 0.5 gram of aliphatic hydrocarbon having at least about 5 carbon atoms per gram of catalyst per hour; the selectivity to methane in the product being less than about 25%. The disclosed invention also relates to a supported catalyst comprising Co, and a microchannel reactor comprising at least one process microchannel and at least one adjacent heat exchange zone.
Abstract translation: 所公开的发明涉及将包含H 2 CO和CO的反应物组合物转化成包含至少一种具有至少约5个碳原子的脂族烃的产物的方法，该方法包括：使反应物组合物通过 与费 - 托催化剂接触以将反应物组合物转化成产物的微通道反应器，该微通道反应器包含多个含有该催化剂的工艺微通道; 将热量从工艺微通道传递到热交换器; 并从微通道反应器中除去产物; 该方法每小时产生至少约0.5克具有至少约5个碳原子的每克催化剂的脂族烃; 产品中甲烷的选择性小于约25％。 所公开的发明还涉及包含Co的载体催化剂和包含至少一个工艺微通道和至少一个相邻的热交换区的微通道反应器。
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