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    Process for alcohol production by selective ether decomposition
    61.
    发明申请
    Process for alcohol production by selective ether decomposition 失效
    通过选择性醚分解生产酒精的方法

    公开(公告)号：US20060281954A1

    公开(公告)日：2006-12-14

    申请号：US11147919

    申请日：2005-06-08

    Applicant: Charles Yarbrough ,  Brian Roberts ,  Dennis Davoren ,  Kenneth Buturla ,  Carl Katzenstein ,  Doron Levin ,  Hans Korsten ,  Vijay Swarup

    Inventor： Charles Yarbrough ,  Brian Roberts ,  Dennis Davoren ,  Kenneth Buturla ,  Carl Katzenstein ,  Doron Levin ,  Hans Korsten ,  Vijay Swarup

    IPC: C07C29/03

    CPC classification number: B01J23/24 ,  B01J21/06 ,  B01J21/066 ,  B01J23/10 ,  C07C29/04 ,  C07C29/10 ,  C07C31/10 ,  C07C31/12

    Abstract: This invention relates to a process for the production of an alcohol, the process comprising (a) reacting an olefin and water in the presence of a catalyst under conditions sufficient to form a crude alcohol stream comprising alcohol, and a dialkyl ether; (b) separating at least a portion of the crude alcohol stream into an alcohol-containing stream and a dialkyl ether stream; (c) contacting at least a portion of the dialkyl ether stream with an ether decomposition catalyst, the ether decomposition catalyst comprising a mixed metal oxide having the following composition XmYnZpOq where X is at least one metal selected from Group 4 of the Periodic Table of Elements, Y is at least one metal selected from Group 3 (including the Lanthanides and Actinides) and Group 6 of the Periodic Table of Elements and Z is at least one metal selected from Groups 7, 8, and 11 of the Periodic Table of Elements; m, n, p, and q are the atomic ratios of their respective components and, when m is 1, n is from about 0.01 to about 0.75, p is from 0 to about 0.1, and q is the number of oxygen atoms necessary to satisfy the valence of the other components, to form a crude dialkyl ether decomposition stream comprising alcohol and olefin; (d) recovering at least a portion of the olefin from the crude dialkyl ether decomposition stream; and (e) recycling at least a portion of the olefin recovered in step (d) to step (a).

    Abstract translation: 本发明涉及一种生产醇的方法，该方法包括（a）在足以形成包含醇和二烷基醚的粗醇物流的条件下，在催化剂存在下使烯烃和水反应; （b）将至少一部分粗醇流分离成含醇流和二烷基醚流; （c）使至少一部分二烷基醚料流与醚分解催化剂接触，所述醚分解催化剂包含具有以下组成的混合金属氧化物： 其中X是选自元素周期表第4族的至少一种金属，Y是选自第3族（包括镧系元素）中的至少一种金属 和锕系元素）和元素周期表第6族，Z是选自元素周期表第7,8和11族中的至少一种金属; m，n，p和q是它们各自成分的原子比，当m为1时，n为约0.01至约0.75，p为0至约0.1，q为必需的氧原子数 满足其他组分的化合价，形成包含醇和烯烃的粗二烷基醚分解物流; （d）从粗二烷基醚分解流中回收至少一部分烯烃; 和（e）将步骤（d）中回收的烯烃的至少一部分再循环到步骤（a）。

    High silica chabazite, its synthesis and its use in the conversion of oxygenates to olefins
    62.
    发明授权
    High silica chabazite, its synthesis and its use in the conversion of oxygenates to olefins 有权
    高二氧化硅菱沸石，其合成及其在含氧化合物转化为烯烃的应用

    公开(公告)号：US07148172B2

    公开(公告)日：2006-12-12

    申请号：US10370923

    申请日：2003-02-20

    Applicant: Karl G. Strohmaier ,  Sebastian C. Reyes ,  Doron Levin

    Inventor： Karl G. Strohmaier ,  Sebastian C. Reyes ,  Doron Levin

    IPC: B01J29/06

    CPC classification number: B01J29/7015 ,  C01B39/46 ,  C01B39/48 ,  C07C1/20 ,  Y02P30/42 ,  C07C11/02

    Abstract: A porous crystalline material is described having the chabazite framework type and having a composition involving the molar relationship: X2O3:(n)YO2, wherein X is a trivalent element, such as aluminum, boron, iron, indium, and/or gallium; Y is a tetravalent element such as silicon, tin, titanium and/or germanium; and n is greater than 100 and typically greater than 200, such as about 300 to about 4000, for example from about 400 to about 1200. The material is synthesized in a fluoride medium and exhibits activity and selectivity in the conversion of methanol to lower olefins, especially ethylene and propylene.

    Abstract translation: 描述了具有菱沸石骨架类型并且具有摩尔关系的组成的多孔结晶材料：<？in-line-formula description =“In-line Formulas”end =“lead”？> X 2 >○3（n）YO 2，<？in-line-formula description =“In-line Formulas”end =“tail”？>其中X是 三价元素，例如铝，硼，铁，铟和/或镓; Y是四价元素，例如硅，锡，钛和/或锗; 并且n大于100，通常大于200，例如约300至约4000，例如约400至约1200.该物质在氟化物介质中合成，并且在甲醇转化为低级烯烃中表现出活性和选择性 ，特别是乙烯和丙烯。

    Conversion of oxygenates to olefins
    67.
    发明申请
    Conversion of oxygenates to olefins 有权
    含氧化合物转化为烯烃

    公开(公告)号：US20060025645A1

    公开(公告)日：2006-02-02

    申请号：US10909012

    申请日：2004-07-30

    Applicant: Shun Fung ,  Doron Levin ,  Jose Santiesteban ,  Nicolas Coute

    Inventor： Shun Fung ,  Doron Levin ,  Jose Santiesteban ,  Nicolas Coute

    IPC: C07C1/00

    CPC classification number: C07C1/20 ,  C07C2521/04 ,  C07C2521/06 ,  C07C2521/10 ,  C07C2521/16 ,  C07C2523/02 ,  C07C2523/10 ,  C07C2529/70 ,  C07C2529/85 ,  Y02P20/584 ,  C07C11/02

    Abstract: A process is described for converting an oxygenate-containing feedstock into one or more olefins in a reactor system including a plurality of fixed bed reactors each containing a catalyst composition comprising a molecular sieve and at least one metal oxide having an uptake of carbon dioxide at 100° C. of at least 0.03 mg/m2 of the metal oxide. Each reactor is sequentially rotated between at least one operating mode, wherein the catalyst composition in the reactor is contacted with the oxygenate-containing feedstock, and a regeneration mode, wherein the catalyst composition in the reactor is contacted with a regeneration medium.

    Abstract translation: 描述了一种在含有含氧化合物的原料转化为一种或多种烯烃的方法，该反应器系统包括多个固定床反应器，每个反应器均含有包含分子筛和至少一种二氧化碳吸收量的至少一种金属氧化物， 至少为0.03mg / m 2的金属氧化物。 每个反应器在至少一个操作模式之间依次旋转，其中反应器中的催化剂组合物与含氧化合物的原料接触，再生模式，其中反应器中的催化剂组合物与再生介质接触。

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