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公开(公告)号：US5723641A
公开(公告)日：1998-03-03
申请号：US721068
申请日：1996-09-26
IPC分类号： B01J31/28 , B01J31/18 , B01J31/26 , C07B61/00 , C07C253/10 , C07C255/02 , C07F9/02 , C07F15/04
CPC分类号： B01J31/185 , B01J31/26 , C07C253/10 , B01J2231/323 , B01J2531/0266 , B01J2531/847
摘要： Processes for hydrocyanation of nonconjugated acyclic aliphatic monoolefins, monoolefins conjugated to an ester group, or monoolefins conjugated to a nitrile group which utilize a catalyst precursor composition comprising a bidentate phosphite ligand and zero-valent nickel preferably in the presence of a Lewis acid promoter. Catalyst precursor compositions are also disclosed.
摘要翻译： 非共轭非环脂族单烯烃，与烯基相结合的单烯烃或与腈基缀合的单烯烃的方法，其使用包含二齿亚磷酸酯配体和零价镍的催化剂前体组合物，优选在路易斯酸促进剂存在下进行。 还公开了催化剂前体组合物。
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2.发明授权Bidentate phosphite and nickel catalyst compositions for hydrocyanation of monoolefins 失效用于单烯烃氢化的双齿亚磷酸酯和镍催化剂组合物公开(公告)号：US06646148B1
公开(公告)日：2003-11-11
申请号：US08564513
申请日：1995-11-29
申请人： Kristina Ann Kreutzer , Wilson Tam
发明人： Kristina Ann Kreutzer , Wilson Tam
IPC分类号： B01J3120
CPC分类号： C07C253/10 , B01J2231/323 , B01J2531/0266 , B01J2531/847 , C07C255/03
摘要： Processes for hydrocyanation of nonconjugated aliphatic monoolefins or monoolefins conjugated to an ester group utilizing a catalyst precursor composition comprising an unsymmetrical bidentate phosphite ligand and zero-valent nickel, preferably in the presence of a Lewis acid promoter, to produce a terminal organo-nitrile. Catalyst precursor compositions are also disclosed.
摘要翻译： 利用包含不对称二齿亚磷酸酯配体和零价镍的催化剂前体组合物，优选在路易斯酸促进剂的存在下，使非共轭脂族单烯烃或与酯基偶联的单烯烃氢化生成末端有机腈的方法。 还公开了催化剂前体组合物。
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公开(公告)号：US06515161B1
公开(公告)日：2003-02-04
申请号：US09650609
申请日：2000-08-30
IPC分类号： C06C25500
CPC分类号： C07F9/6552 , B01J31/1616 , B01J31/1658 , B01J31/185 , B01J2231/321 , B01J2531/0266 , B01J2531/80 , B01J2531/822 , C07C45/50 , C07C67/347 , C07C253/30 , C07F9/145 , C07F9/653 , C07F9/65515 , C07C69/716 , C07C47/02
摘要： A hydroformylation process is disclosed which employs multidentate phosphite ligands in a catalyst composition. In particular, the ligands have heteroatom-containing substituents on the carbon attached to the ortho position of the terminal phenol group.
摘要翻译： 公开了在催化剂组合物中使用多齿亚磷酸酯配体的加氢甲酰化方法。 特别地，配体在连接到末端苯酚基团的邻位的碳上具有含杂原子的取代基。
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公开(公告)号：US06310163B1
公开(公告)日：2001-10-30
申请号：US08899002
申请日：1997-07-10
申请人： Maurice S. Brookhart , Lynda Kaye Johnson , Christopher Moore Killian , Samuel David Arthur , Jerald Feldman , Elizabeth Forrester McCord , Stephan James McLain , Kristina Ann Kreutzer , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Steven Dale Ittel , Anju Parthasarathy , Daniel Joseph Tempel
发明人： Maurice S. Brookhart , Lynda Kaye Johnson , Christopher Moore Killian , Samuel David Arthur , Jerald Feldman , Elizabeth Forrester McCord , Stephan James McLain , Kristina Ann Kreutzer , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Steven Dale Ittel , Anju Parthasarathy , Daniel Joseph Tempel
IPC分类号： C08F22010
CPC分类号： C08F110/02 , C08F10/00 , C08F10/02 , C08F10/06 , C08F110/06 , C08F110/14 , C08F210/02 , C08F210/14 , C08F210/16 , C08F232/00 , C08L23/02 , Y10S430/165 , Y10T428/1352 , Y10T428/1386 , Y10T428/139 , Y10T428/24942 , Y10T428/2878 , Y10T428/31692 , Y10T428/31855 , Y10T428/31895 , Y10T428/31938 , Y10T442/20 , Y10T442/60 , Y10T442/626
摘要： Disclosed herein are processes for polymerizing ethylene, acyclic olefins, and/or selected cyclic olefins, and optionally selected olefinic esters or carboxylic acids, and other monomers. The polymerizations are catalyzed by selected transition metal compounds, and sometimes other co-catalysts. Since some of the polymerizations exhibit some characteristics of living polymerizations, block copolymers can be readily made. Many of the polymers produced are often novel, particularly in regard to their microstructure which gives some of them unusual properties. Numerous novel catalysts are disclosed, as well as some novel processes for making them. The polymers made are useful as elastomers, molding resins, in adhesives, etc. Also described herein is the synthesis of linear &agr;-olefins by the oligomerization of ethylene using as a catalyst system a combination a nickel compound having a selected &agr;-diimine ligand and a selected Lewis or Bronsted acid, or by contacting selected &agr;-diimine nickel complexes with ethylene.
摘要翻译： 本文公开了聚合乙烯，无环烯烃和/或选择的环烯烃，和任选选择的烯属酯或羧酸和其它单体的方法。 聚合由选择的过渡金属化合物，有时是其他助催化剂催化。 由于一些聚合表现出活性聚合的某些特性，因此可以容易地制备嵌段共聚物。 所生产的许多聚合物通常是新颖的，特别是关于它们的微观结构，这给出了其中一些不寻常的性质。 公开了许多新颖的催化剂，以及一些制备它们的新方法。 制备的聚合物可用作弹性体，模塑树脂，粘合剂等。本文还描述了通过使用作为催化剂体系的乙烯低聚法合成线性α-烯烃，将具有选定的α-二亚胺配体的镍化合物和 选择的Lewis或布朗斯台德酸，或通过使选择的α-二亚胺镍络合物与乙烯接触。
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5.发明授权Multidentate phosphite ligands, catalytic compositions containing such ligands, and catalytic processes utilizing such catalytic compositions 失效多齿亚磷酸酯配体，含有这些配体的催化组合物，以及利用这种催化组合物的催化方法公开(公告)号：US06812352B2
公开(公告)日：2004-11-02
申请号：US10118551
申请日：2002-04-09
IPC分类号： C07C25310
CPC分类号： C07F9/6552 , B01J31/1658 , B01J31/185 , B01J31/26 , B01J2231/323 , B01J2231/52 , B01J2531/0266 , B01J2531/80 , B01J2531/821 , B01J2531/822 , B01J2531/824 , B01J2531/827 , B01J2531/845 , B01J2531/847 , C07C253/10 , C07F9/145 , C07F9/653 , C07F9/65515 , C07C255/04 , C07C255/07
摘要： Multidentate phosphite ligands are disclosed for use in reactions such as hydrocyanation and isomerization. The catalyst compositions made therefrom and the various catalytic processes which employ such multidentate phosphite ligands are also disclosed. In particular, the ligands have heteroatom-containing substituents on the carbon attached to the ortho position of the terminal phenol group.
摘要翻译： 公开了用于反应如氢化氰化和异构化的多齿亚磷酸酯配体。 还公开了由其制备的催化剂组合物和使用这种多齿亚磷酸酯配体的各种催化方法。 特别地，配体在连接到末端苯酚基团的邻位的碳上具有含杂原子的取代基。
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公开(公告)号：US6034259A
公开(公告)日：2000-03-07
申请号：US891398
申请日：1997-07-10
申请人： Maurice S. Brookhart , Lynda Kaye Johnson , Christopher Moore Killian , Samuel David Arthur , Jerald Feldman , Stephan James McLain , Kristina Ann Kreutzer , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Steven Dale Ittel , Anju Parthasarathy , Daniel Joseph Tempel
发明人： Maurice S. Brookhart , Lynda Kaye Johnson , Christopher Moore Killian , Samuel David Arthur , Jerald Feldman , Stephan James McLain , Kristina Ann Kreutzer , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Steven Dale Ittel , Anju Parthasarathy , Daniel Joseph Tempel
IPC分类号： B01J31/00 , B01J37/00 , C07C2/32 , C07C69/52 , C07C251/08 , C07F7/00 , C07F15/00 , C07F19/00 , C08F4/02 , C08F4/06 , C08F4/60 , C08F4/70 , C08F4/80 , C08F10/00 , C08F10/02 , C08F10/06 , C08F10/08 , C08F12/30 , C08F20/06 , C08F110/02 , C08F110/06 , C08F110/14 , C08F132/04 , C08F210/02 , C08F210/14 , C08F210/16 , C08F220/10 , C08F232/00 , C08F232/04 , C08F255/00 , C08L23/02
CPC分类号： C08F110/02 , C08F110/06 , C08F210/02 , C08F210/14 , C08F210/16 , C08L23/02 , C08F10/00 , C08F10/02 , C08F10/06 , C08F110/14 , C08F232/00 , Y10S430/165 , Y10T428/1352 , Y10T428/1386 , Y10T428/139 , Y10T428/24942 , Y10T428/2878 , Y10T428/31692 , Y10T428/31855 , Y10T428/31895 , Y10T428/31938 , Y10T442/20 , Y10T442/60 , Y10T442/626
摘要： Disclosed herein are processes for polymerizing ethylene, acyclic olefins, and/or selected cyclic olefins, and optionally selected olefinic esters or carboxylic acids, and other monomers. The polymerizations are catalyzed by selected transition metal compounds, and sometimes other co-catalysts. Since some of the polymerizations exhibit some characteristics of living polymerizations, block copolymers can be readily made. Many of the polymers produced are often novel, particularly in regard to their microstructure, which gives some of them unusual properties. Numerous novel catalysts are disclosed, as well as some novel processes for making them. The polymers made are useful as elastomers, molding resins, in adhesives, etc. Also described herein is the synthesis of linear .alpha.-olefins by the oligomerization of ethylene using as a catalyst system a combination a nickel compound having a selected .alpha.-diimine ligand and a selected Lewis or Bronsted acid, or by contacting selected .alpha.-diimine nickel complexes with ethylene.
摘要翻译： 本文公开了聚合乙烯，无环烯烃和/或选择的环烯烃，和任选选择的烯属酯或羧酸和其它单体的方法。 聚合由选择的过渡金属化合物，有时是其他助催化剂催化。 由于一些聚合表现出活性聚合的某些特性，因此可以容易地制备嵌段共聚物。 所生产的许多聚合物通常是新颖的，特别是在它们的微结构方面，这给出了其中一些不寻常的性质。 公开了许多新颖的催化剂，以及一些制备它们的新方法。 制备的聚合物可用作弹性体，模塑树脂，粘合剂等。本文还描述了通过使用作为催化剂体系的乙烯低聚来合成线性α-烯烃，将具有选定的α-二亚胺配体的镍化合物和 选择的Lewis或布朗斯台德酸，或通过使选择的α-二亚胺镍络合物与乙烯接触。
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公开(公告)号：US5714556A
公开(公告)日：1998-02-03
申请号：US671392
申请日：1996-06-27
申请人： Lynda Kaye Johnson , Jerald Feldman , Kristina Ann Kreutzer , Stephan James McLain , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Dennis Scott Donald , Lissa Taka Jennings Nelson , Anju Parthasarathy , Xing Shen , Wilson Tam , Yueli Wang
发明人： Lynda Kaye Johnson , Jerald Feldman , Kristina Ann Kreutzer , Stephan James McLain , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Dennis Scott Donald , Lissa Taka Jennings Nelson , Anju Parthasarathy , Xing Shen , Wilson Tam , Yueli Wang
IPC分类号： C07F15/04 , C08F4/06 , C08F4/70 , C08F10/00 , C08F10/02 , C08F12/00 , C08F12/04 , C08F12/08 , C08F32/08 , C08F36/00 , C08F36/20 , C08F110/02 , C08F210/02
CPC分类号： C08F32/08 , C07F15/04 , C08F10/00 , C08F10/02 , C08F12/08 , C08F110/02 , C08F210/02
摘要： Disclosed herein is a process for the polymerization of ethylene, norbornenes and styrenes, by contacting in solution a selected nickel compound and a selected compound which is or can coordinated to the nickel with the olefin(s). The polymers produced are useful for films and molding resins.
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公开(公告)号：US5688986A
公开(公告)日：1997-11-18
申请号：US424351
申请日：1995-04-26
IPC分类号： B01J31/28 , B01J31/18 , B01J31/26 , C07B61/00 , C07C253/10 , C07C255/02 , C07C253/30
CPC分类号： B01J31/185 , B01J31/26 , C07C253/10 , B01J2231/323 , B01J2531/0266 , B01J2531/847
摘要： Processes for hydrocyanation of nonconjugated acyclic aliphatic monoolefins, monoolefins conjugated to an ester group, or monoolefins conjugated to a nitrile group which utilize a catalyst precursor composition comprising a bidentate phosphite ligand and zero-valent nickel preferably in the presence of a Lewis acid prompter. Catalyst precursor compositions are also disclosed.
摘要翻译： PCT No.PCT / US94 / 12794 Sec。 371日期1995年04月26日 102（e）日期1995年4月26日PCT 1994年11月7日PCT PCT。 公开号WO95 / 14659 日期1995年6月1日非共轭非环脂族单烯烃，与酯基共轭的单烯烃或与腈基缀合的单烯烃的氢化氰化处理，其利用包含二齿亚磷酸酯配体和零价镍的催化剂前体组合物，优选在 路易斯酸提取物。 还公开了催化剂前体组合物。
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公开(公告)号：US6103920A
公开(公告)日：2000-08-15
申请号：US899032
申请日：1997-07-23
申请人： Lynda Kaye Johnson , Jerald Feldman , Kristina Ann Kreutzer , Stephan James Mclain , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Dennis Scott Donald , Lissa Taka Jennings Nelson , Anju Parthasarathy , Xing Shen , Wilson Tam , Yueli Wang
发明人： Lynda Kaye Johnson , Jerald Feldman , Kristina Ann Kreutzer , Stephan James Mclain , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Dennis Scott Donald , Lissa Taka Jennings Nelson , Anju Parthasarathy , Xing Shen , Wilson Tam , Yueli Wang
IPC分类号： C07F15/04 , C08F4/06 , C08F4/70 , C08F10/00 , C08F10/02 , C08F12/00 , C08F12/04 , C08F12/08 , C08F32/08 , C08F36/00 , C08F36/20 , C08F110/02 , C08F210/02
CPC分类号： C08F32/08 , C07F15/04 , C08F10/00 , C08F10/02 , C08F12/08 , C08F110/02 , C08F210/02
摘要： Disclosed herein is a process for the polymerization of ethylene, norbornenes and styrenes, by contacting in solution a selected nickel compound and a selected compound which is or can coordinated to the nickel with the olefin(s). The polymers produced are useful for films and molding resins.
摘要翻译： 本文公开了通过使溶液中的选定的镍化合物和选择的与镍与烯烃配位的化合物接触来聚合乙烯，降冰片烯和苯乙烯的方法。 所生产的聚合物可用于膜和模制树脂。
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公开(公告)号：US5886224A
公开(公告)日：1999-03-23
申请号：US891403
申请日：1997-07-10
申请人： Maurice S. Brookhart , Lynda Kaye Johnson , Samuel David Arthur , Jerald Feldman , Kristina Ann Kreutzer , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Steven Dale Ittel , Anju Parthasarathy , Daniel Joseph Tempel
发明人： Maurice S. Brookhart , Lynda Kaye Johnson , Samuel David Arthur , Jerald Feldman , Kristina Ann Kreutzer , Alison Margaret Anne Bennett , Edward Bryan Coughlin , Steven Dale Ittel , Anju Parthasarathy , Daniel Joseph Tempel
IPC分类号： B01J31/00 , B01J37/00 , C07C2/32 , C07C69/52 , C07C251/08 , C07F7/00 , C07F15/00 , C07F19/00 , C08F4/02 , C08F4/06 , C08F4/60 , C08F4/70 , C08F4/80 , C08F10/00 , C08F10/02 , C08F10/06 , C08F10/08 , C08F12/30 , C08F20/06 , C08F110/02 , C08F110/06 , C08F110/14 , C08F132/04 , C08F210/02 , C08F210/14 , C08F210/16 , C08F220/10 , C08F232/00 , C08F232/04 , C08F255/00 , C08L23/02
CPC分类号： C08F110/02 , C08F110/06 , C08F210/02 , C08F210/14 , C08F210/16 , C08L23/02 , C08F10/00 , C08F10/02 , C08F10/06 , C08F110/14 , C08F232/00 , Y10S430/165 , Y10T428/1352 , Y10T428/1386 , Y10T428/139 , Y10T428/24942 , Y10T428/2878 , Y10T428/31692 , Y10T428/31855 , Y10T428/31895 , Y10T428/31938 , Y10T442/20 , Y10T442/60 , Y10T442/626
摘要： Disclosed herein are processes for polymerizing ethylene, acyclic olefins, and/or selected cyclic olefins, and optionally selected olefinic esters or carboxylic acids, and other monomers. The polymerizations are catalyzed by selected transition metal compounds, and sometimes other co-catalysts. Since some of the polymerizations exhibit some characteristics of living polymerizations, block copolymers can be readily made. Many of the polymers produced are often novel, particularly in regard to their microstructure, which gives some of them unusual properties. Numerous novel catalysts are disclosed, as well as some novel processes for making them. The polymers made are useful as elastomers, molding resins, in adhesives, etc. Also described herein is the synthesis of linear .alpha.-olefins by the oligomerization of ethylene using as a catalyst system a combination a nickel compound having a selected .alpha.-diimine ligand and a selected Lewis or Bronsted acid, or by contacting selected .alpha.-diimine nickel complexes with ethylene.
摘要翻译： 本文公开了聚合乙烯，无环烯烃和/或选择的环烯烃，和任选选择的烯属酯或羧酸和其它单体的方法。 聚合由选择的过渡金属化合物，有时是其他助催化剂催化。 由于一些聚合表现出活性聚合的某些特性，因此可以容易地制备嵌段共聚物。 所生产的许多聚合物通常是新颖的，特别是在它们的微结构方面，这给出了其中一些不寻常的性质。 公开了许多新颖的催化剂，以及一些制备它们的新方法。 制备的聚合物可用作弹性体，模塑树脂，粘合剂等。本文还描述了通过使用作为催化剂体系的乙烯低聚来合成线性α-烯烃，将具有选定的α-二亚胺配体的镍化合物和 选择的Lewis或布朗斯台德酸，或通过使选择的α-二亚胺镍络合物与乙烯接触。
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