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公开(公告)号：US06548447B1
公开(公告)日：2003-04-15
申请号：US09253265
申请日：1999-02-19
IPC分类号： B01J2362
CPC分类号： B01J23/8926 , B01J23/626 , B01J35/04 , C07C5/48 , C07C2521/04 , C07C2521/06 , C07C2523/14 , C07C2523/42 , C07C2523/62 , C07C2523/72 , C07C2523/89 , C07C11/02
摘要： A process for the production of a mono-olefin from a gaseous paraffinic hydrocarbon having at least two carbon atoms or mixtures thereof comprising reacting the hydrocarbons and molecular oxygen in the presence of a platinum catalyst. The catalyst consists essentially of platinum modified with Sn or Cu and supported on a ceramic monolith.
摘要翻译： 一种从具有至少两个碳原子的气态链烷烃或其混合物生产单烯烃的方法，包括在铂催化剂存在下使烃和分子氧反应。 催化剂基本上由用Sn或Cu改性并负载在陶瓷整料上的铂组成。
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2.发明授权On-line synthesis and regeneration of a catalyst used in autothermal oxidation 有权用于自热氧化的催化剂的在线合成和再生公开(公告)号：US06624116B1
公开(公告)日：2003-09-23
申请号：US09706464
申请日：2000-11-03
IPC分类号： B01J2396
CPC分类号： C07C5/48 , B01J21/04 , B01J21/10 , B01J23/40 , B01J23/54 , B01J23/56 , B01J23/626 , B01J23/6445 , B01J23/70 , B01J23/76 , B01J23/8926 , B01J23/8966 , B01J23/96 , B01J35/04 , B01J35/06 , B01J37/0201 , B01J37/0207 , B01J37/0238 , B01J37/18 , C07C2521/02 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2521/12 , C07C2521/14 , C07C2523/04 , C07C2523/08 , C07C2523/14 , C07C2523/18 , C07C2523/42 , C07C2523/44 , C07C2523/50 , C07C2523/72 , C07C2527/224 , C10G2400/20 , Y02P20/52 , Y02P20/584 , Y10S502/514 , C07C11/04 , C07C11/02
摘要： An on-line method of synthesizing or regenerating catalysts for autothermal oxidation processes, specifically, the oxidation of paraffinic hydrocarbons, for example, ethane, propane, and naphtha, to olefins, for example, ethylene and propylene. The catalyst comprises a Group 8B metal, for example, a platinum group metal and, optionally, a promoter, such as tin, antimony, or copper, on a support, preferably a monolith support. On-line synthesis or regeneration involves co-feeding a volatile Group 8B metal compound and/or a volatile promoter compound with the paraffinic hydrocarbon and oxygen into the oxidation reactor under ignition or autothermal conditions.
摘要翻译： 合成或再生用于自热氧化方法的催化剂的在线方法，具体地，将链烷烃如乙烷，丙烷和石脑油氧化成烯烃，例如乙烯和丙烯。 催化剂在载体上，优选整料载体上包含8B族金属，例如铂族金属和任选的助催化剂，例如锡，锑或铜。 在线合成或再生包括在点燃或自热条件下将挥发性第8B族金属化合物和/或挥发性促进剂化合物与链烷烃和氧共同进料到氧化反应器中。
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公开(公告)号：US06566573B1
公开(公告)日：2003-05-20
申请号：US09388219
申请日：1999-09-01
申请人： Sameer S. Bharadwaj , Joseph J. Maj , Jonathan H. Siddall , Mark D. Bearden , Craig B. Murchison , Gerald E. Lazaruk
发明人： Sameer S. Bharadwaj , Joseph J. Maj , Jonathan H. Siddall , Mark D. Bearden , Craig B. Murchison , Gerald E. Lazaruk
IPC分类号： C07C5333
CPC分类号： C07C5/48 , B01J21/04 , B01J21/10 , B01J23/40 , B01J23/54 , B01J23/56 , B01J23/626 , B01J23/6445 , B01J23/70 , B01J23/76 , B01J23/8926 , B01J23/8966 , B01J23/96 , B01J35/04 , B01J35/06 , B01J37/0201 , B01J37/0207 , B01J37/0238 , B01J37/18 , C07C2521/02 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2521/12 , C07C2521/14 , C07C2523/04 , C07C2523/08 , C07C2523/14 , C07C2523/18 , C07C2523/42 , C07C2523/44 , C07C2523/50 , C07C2523/72 , C07C2527/224 , C10G2400/20 , Y02P20/52 , Y02P20/584 , Y10S502/514 , C07C11/04 , C07C11/02
摘要： A process and catalyst for the partial oxidation of paraffinic hydrocarbons, such as ethane, propane, naphtha, and natural gas condensates, to olefins, such as ethylene and propylene. The process involves contacting a paraffinic hydrocarbon with oxygen in the presence of hydrogen and a catalyst under autothermal process conditions. Preheating the feed decreases oxygen consumption and increases the net hydrogen balance. The catalyst comprises a Group 8B metal, preferably, a platinum group metal, and at least one promoter selected from Groups 1B, 6B, 3A, 4A, and 5A, optionally supported on a catalytic support, such as magnesia or alumina. In preferred embodiments, the support is pretreated with a support modifier selected from Groups 1A, 2A, 3B, 4B, 5B, 6B, 1B, 3A, 4A, 5A, the rare earth lanthanides, and the actinides. A modified fluidized bed reactor is disclosed for the process.
摘要翻译： 用于将链烷烃（例如乙烷，丙烷，石脑油和天然气）部分氧化的方法和催化剂冷凝成烯烃，例如乙烯和丙烯。 该方法包括在自热过程条件下在氢气和催化剂存在下使链烷烃与氧接触。 饲料预热会减少氧气消耗，并增加净氢平衡。 该催化剂包含8B族金属，优选铂族金属和至少一种选自1B，6B，3A，4A和5A族的助催化剂，任选负载在催化载体如氧化镁或氧化铝上。 在优选的实施方案中，载体用选自组1A，2A，3B，4B，5B，6B，1B，3A，4A，5A，稀土镧系元素和锕系元素的载体改性剂预处理。 公开了改进的流化床反应器。
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4.发明授权On-line synthesis and regenerating of a catalyst used in autothermal oxidation 有权用于自热氧化的催化剂的在线合成和再生
公开(公告)号：US6166283A
公开(公告)日：2000-12-26
申请号：US388220
申请日：1999-09-01
IPC分类号： B01J21/04 , B01J21/10 , B01J23/40 , B01J23/54 , B01J23/56 , B01J23/62 , B01J23/644 , B01J23/70 , B01J23/755 , B01J23/76 , B01J23/89 , B01J23/96 , B01J35/04 , B01J35/06 , B01J37/02 , B01J37/16 , B01J37/18 , C07B61/00 , C07C4/06 , C07C5/48 , C07C11/04 , C07C11/06 , C07C11/09 , C07C11/167 , C10G11/02 , C10G11/22 , C10G27/04 , C07C5/327 , C07C5/333 , C07C5/373
CPC分类号： C07C5/48 , B01J21/04 , B01J21/10 , B01J23/40 , B01J23/54 , B01J23/56 , B01J23/626 , B01J23/6445 , B01J23/70 , B01J23/76 , B01J23/8926 , B01J23/8966 , B01J23/96 , B01J35/04 , B01J35/06 , B01J37/0201 , B01J37/0207 , B01J37/0238 , B01J37/18 , C07C2521/02 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2521/12 , C07C2521/14 , C07C2523/04 , C07C2523/08 , C07C2523/14 , C07C2523/18 , C07C2523/42 , C07C2523/44 , C07C2523/50 , C07C2523/72 , C07C2527/224 , C10G2400/20 , Y02P20/52 , Y02P20/584 , Y10S502/514 , C07C11/04 , C07C11/02
摘要： An on-line method of synthesizing or regenerating catalysts for autothermal oxidation processes, specifically, the oxidation of paraffinic hydrocarbons, for example, ethane, propane, and naphtha, to olefins, for example, ethylene and propylene. The catalyst comprises a Group 8B metal, for example, a platinum group metal and, optionally, a promoter, such as tin, antimony, or copper, on a support, preferably a monolith support. On-line synthesis or regeneration involves co-feeding a volatile Group 8B metal compound and/or a volatile promoter compound with the paraffinic hydrocarbon and oxygen into the oxidation reactor under ignition or autothermal conditions.
摘要翻译： 合成或再生用于自热氧化方法的催化剂的在线方法，具体地，将链烷烃如乙烷，丙烷和石脑油氧化成烯烃，例如乙烯和丙烯。 催化剂在载体上，优选整料载体上包含8B族金属，例如铂族金属和任选的助催化剂，例如锡，锑或铜。 在线合成或再生包括在点燃或自热条件下将挥发性第8B族金属化合物和/或挥发性促进剂化合物与链烷烃和氧共同进料到氧化反应器中。
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公开(公告)号：US5905180A
公开(公告)日：1999-05-18
申请号：US720562
申请日：1996-09-30
IPC分类号： B01J23/62 , B01J23/89 , B01J35/04 , C07B61/00 , C07C5/327 , C07C5/48 , C07C11/02 , C07C5/333
CPC分类号： B01J23/8926 , B01J23/626 , C07C5/48 , B01J35/04 , C07C2521/04 , C07C2521/06 , C07C2523/14 , C07C2523/42 , C07C2523/62 , C07C2523/72 , C07C2523/89
摘要： A process for the production of a mono-olefin from a gaseous paraffinic hydrocarbon having at least two carbon atoms or mixtures thereof comprising reacting said hydrocarbons and molecular oxygen in the presence of a platinum catalyst. The catalyst consists essentially of platinum modified with Sn or Cu and supported on a ceramic monolith.
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公开(公告)号：US5639929A
公开(公告)日：1997-06-17
申请号：US422787
申请日：1995-04-17
CPC分类号： C07C5/48 , C07C2521/04 , C07C2521/06 , C07C2523/42 , C07C2523/46 , C07C2523/52 , C07C2523/755
摘要： A process for the oxidative dehydrogenation of hydrocarbons is disclosed in which C.sub.2 -C.sub.6 alkanes are contacted with an oxygen containing gas in a fluidized catalyst bed of platinum, rhodium, nickel or platinum-gold supported on .alpha.-alumina or zirconia. Ethane is dehydrogenated to ethylene and higher alkanes are dehydrogenated to ethylene, propylene and iso-butylene.
摘要翻译： 公开了一种烃的氧化脱氢方法，其中在负载在α-氧化铝或氧化锆上的铂，铑，镍或铂金的流化催化剂床中，C2-C6烷烃与含氧气体接触。 乙烷脱氢为乙烯，高级烷烃脱氢为乙烯，丙烯和异丁烯。
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公开(公告)号：US06846773B1
公开(公告)日：2005-01-25
申请号：US08821384
申请日：1997-03-20
IPC分类号： B01J23/62 , B01J23/89 , B01J35/04 , C07B61/00 , C07C5/327 , C07C5/48 , C07C11/02 , B01J23/42
CPC分类号： B01J23/8926 , B01J23/626 , B01J35/04 , C07C5/48 , C07C2521/04 , C07C2521/06 , C07C2523/14 , C07C2523/42 , C07C2523/62 , C07C2523/72 , C07C2523/89 , C07C11/02
摘要： A process for the production of a mono-olefin from a gaseous paraffinic hydrocarbon having at least two carbon atoms or mixtures thereof comprising reacting said hydrocarbons and molecular oxygen in the presence of a platinum catalyst. The catalyst consists essentially of platinum modified with Sn or Cu and supported on a ceramic monolith.
摘要翻译： 一种由具有至少两个碳原子的气态链烷烃或其混合物生产单烯烃的方法，包括在铂催化剂存在下使所述烃和分子氧反应。 催化剂基本上由用Sn或Cu改性并负载在陶瓷整料上的铂组成。
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公开(公告)号：US6072097A
公开(公告)日：2000-06-06
申请号：US146409
申请日：1998-09-03
CPC分类号： B01J23/8926 , B01J23/626 , C07C5/48 , B01J35/04 , C07C2521/04 , C07C2521/06 , C07C2523/14 , C07C2523/42 , C07C2523/62 , C07C2523/72 , C07C2523/89
摘要： A process for the production of a mono-olefin from a gaseous paraffinic hydrocarbon having at least two carbon atoms or mixtures thereof comprising reacting said hydrocarbons and molecular oxygen in the presence of a platinum catalyst. The catalyst consists essentially of platinum modified with Sn or Cu and supported on a ceramic monolith.
摘要翻译： 一种由具有至少两个碳原子的气态链烷烃或其混合物生产单烯烃的方法，包括在铂催化剂存在下使所述烃和分子氧反应。 催化剂基本上由用Sn或Cu改性并负载在陶瓷整料上的铂组成。
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