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公开(公告)号：US08263519B2
公开(公告)日：2012-09-11
申请号：US12316977
申请日：2008-12-18
申请人： Christine N. Elia , Mohan Kalyanaraman , Michel A. Daage , Stephen H. Brown , Lei Zhang , Robert A. Crane , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, Jr.
发明人： Christine N. Elia , Mohan Kalyanaraman , Michel A. Daage , Stephen H. Brown , Lei Zhang , Robert A. Crane , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, Jr.
IPC分类号： B01J29/06
CPC分类号： B01J29/703 , B01J21/06 , B01J21/063 , B01J29/7046 , B01J29/7461 , B01J29/7492 , B01J35/1014 , B01J37/0009 , B01J2229/20 , B01J2229/36 , B01J2229/42 , C10G45/64
摘要： Catalysts for dewaxing of hydrocarbon feeds, particularly feeds with elevated sulfur and nitrogen levels, are provided. The dewaxing catalysts include a zeolite with a low silica to alumina ratio combined with a low surface binder, or alternatively the formulated catalyst has a high ratio of zeolite surface area to external surface area.
摘要翻译： 提供用于烃进料脱蜡的催化剂，特别是具有升高的硫和氮水平的进料。 脱蜡催化剂包括具有低二氧化硅与氧化铝比率与低表面粘合剂组合的沸石，或者配制的催化剂具有高比例的沸石表面积与外表面积。
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公开(公告)号：US20090176643A1
公开(公告)日：2009-07-09
申请号：US12316977
申请日：2008-12-18
申请人： Christine N. Elia , Mohan Kalyanaraman , Michel A. Daage , Stephen H. Brown , Lei Zhang , Robert A. Crane , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, JR.
发明人： Christine N. Elia , Mohan Kalyanaraman , Michel A. Daage , Stephen H. Brown , Lei Zhang , Robert A. Crane , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, JR.
IPC分类号： B01J29/44 , B01J29/06 , B01J29/40 , B01J29/068
CPC分类号： B01J29/703 , B01J21/06 , B01J21/063 , B01J29/7046 , B01J29/7461 , B01J29/7492 , B01J35/1014 , B01J37/0009 , B01J2229/20 , B01J2229/36 , B01J2229/42 , C10G45/64
摘要： Catalysts for dewaxing of hydrocarbon feeds, particularly feeds with elevated sulfur and nitrogen levels, are provided. The dewaxing catalysts include a zeolite with a low silica to alumina ratio combined with a low surface binder, or alternatively the formulated catalyst has a high ratio of zeolite surface area to external surface area.
摘要翻译： 提供用于烃进料脱蜡的催化剂，特别是具有升高的硫和氮水平的进料。 脱蜡催化剂包括具有低二氧化硅与氧化铝比率与低表面粘合剂组合的沸石，或者配制的催化剂具有高比例的沸石表面积与外表面积。
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公开(公告)号：US08030240B2
公开(公告)日：2011-10-04
申请号：US12316979
申请日：2008-12-18
申请人： Christine N. Elia , Mohan Kalyanaraman , Lei Zhang , Michel A. Daage , Darden Sinclair , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, Jr.
发明人： Christine N. Elia , Mohan Kalyanaraman , Lei Zhang , Michel A. Daage , Darden Sinclair , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, Jr.
IPC分类号： B01J29/06
CPC分类号： B01J29/80 , B01J29/18 , B01J29/22 , B01J29/405 , B01J29/44 , B01J29/70 , B01J29/74 , B01J37/0009 , B01J2229/12 , B01J2229/20 , B01J2229/32 , B01J2229/42 , C10G45/64
摘要： Catalysts for dewaxing of hydrocarbon feeds, particularly feeds with elevated sulfur and nitrogen levels, are provided. The dewaxing catalysts include at least two zeolites, including a zeolite with a low silica to alumina ratio. The catalysts may be combined with a low surface binder, or alternatively the catalysts as formulated may have a high ratio of zeolite surface area to external surface area.
摘要翻译： 提供用于烃进料脱蜡的催化剂，特别是具有升高的硫和氮水平的进料。 脱蜡催化剂包括至少两种沸石，包括具有低二氧化硅与氧化铝比的沸石。 催化剂可以与低表面粘合剂组合，或者配制的催化剂可以具有高比例的沸石表面积与外表面积。
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公开(公告)号：US20100075831A1
公开(公告)日：2010-03-25
申请号：US12316979
申请日：2008-12-18
申请人： Christine N. Elia , Mohan Kalyanaraman , Lei Zhang , Michel A. Daage , Darden Sinclair , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, JR.
发明人： Christine N. Elia , Mohan Kalyanaraman , Lei Zhang , Michel A. Daage , Darden Sinclair , Valery Sokolovskii , David M. Lowe , Jun Han , Nicholas Ohler , Daniel M. Giaquinta , Anthony F. Volpe, JR.
IPC分类号： B01J29/068 , B01J29/06
CPC分类号： B01J29/80 , B01J29/18 , B01J29/22 , B01J29/405 , B01J29/44 , B01J29/70 , B01J29/74 , B01J37/0009 , B01J2229/12 , B01J2229/20 , B01J2229/32 , B01J2229/42 , C10G45/64
摘要： Catalysts for dewaxing of hydrocarbon feeds, particularly feeds with elevated sulfur and nitrogen levels, are provided. The dewaxing catalysts include at least two zeolites, including a zeolite with a low silica to alumina ratio. The catalysts may be combined with a low surface binder, or alternatively the catalysts as formulated may have a high ratio of zeolite surface area to external surface area.
摘要翻译： 提供用于烃进料脱蜡的催化剂，特别是具有升高的硫和氮水平的进料。 脱蜡催化剂包括至少两种沸石，包括具有低二氧化硅与氧化铝比的沸石。 催化剂可以与低表面粘合剂组合，或者配制的催化剂可以具有高比例的沸石表面积与外表面积。
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公开(公告)号：US08263517B2
公开(公告)日：2012-09-11
申请号：US12316978
申请日：2008-12-18
申请人： Christine N. Elia , Mohan Kalyanaraman , Lei Zhang , Madhav Acharya , Michael A. Daage , Darden Sinclair , Jocelyn A. Kowalski , Jose G. Santiesteban , Ajit B. Dandekar
发明人： Christine N. Elia , Mohan Kalyanaraman , Lei Zhang , Madhav Acharya , Michael A. Daage , Darden Sinclair , Jocelyn A. Kowalski , Jose G. Santiesteban , Ajit B. Dandekar
IPC分类号： B01J29/06
CPC分类号： B01J37/0009 , B01J21/04 , B01J21/063 , B01J21/066 , B01J21/08 , B01J29/068 , B01J29/7261 , B01J29/7292 , B01J29/7461 , B01J29/7492 , B01J29/7861 , B01J29/7892 , B01J35/1014 , B01J2229/20 , B01J2229/42 , C10G45/64 , C10G47/20
摘要： Catalysts for dewaxing of hydrocarbon feeds, particularly feeds with elevated sulfur and nitrogen levels, are provided. The dewaxing catalysts include a zeolite with a low silica to alumina ratio combined with a low surface binder, or alternatively the formulated catalyst has a high ratio of zeolite surface area to external surface area.
摘要翻译： 提供用于烃进料脱蜡的催化剂，特别是具有升高的硫和氮水平的进料。 脱蜡催化剂包括具有低二氧化硅与氧化铝比率与低表面粘合剂组合的沸石，或者配制的催化剂具有高比例的沸石表面积与外表面积。
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公开(公告)号：US08366908B2
公开(公告)日：2013-02-05
申请号：US12655120
申请日：2009-12-23
申请人： Krista Marie Prentice , Gary Paul Schleicher , Lei Zhang , Timothy Lee Hilbert , Michel A. Daage , Sylvain Hantzer , Wenyih F. Lai , David Mentzer , William Francis Heaney , Christine Nicole Elia , Shifang Luo , Stephen J. McCarthy , Mohan Kalyanaraman
发明人： Krista Marie Prentice , Gary Paul Schleicher , Lei Zhang , Timothy Lee Hilbert , Michel A. Daage , Sylvain Hantzer , Wenyih F. Lai , David Mentzer , William Francis Heaney , Christine Nicole Elia , Shifang Luo , Stephen J. McCarthy , Mohan Kalyanaraman
CPC分类号： C10G45/62 , C10G2300/202 , C10G2300/207 , C10G2400/10
摘要： An integrated process for producing lubricant base oils from feedstocks under sour conditions is provided. The ability to process feedstocks under higher sulfur conditions allows for reduced cost processing and increases the flexibility in selecting a suitable feedstock. The sour feed can be delivered to a catalytic dewaxing step without any separation of sulfur and nitrogen contaminants, or a high pressure separation can be used to partially eliminate contaminants.
摘要翻译： 提供了一种在酸性条件下从原料生产润滑剂基础油的综合方法。 在较高硫条件下处理原料的能力允许降低成本处理并增加选择合适原料的灵活性。 可以将酸性进料输送到催化脱蜡步骤，而不会分离硫和氮污染物，或者可以使用高压分离来部分地消除污染物。
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公开(公告)号：US20100187156A1
公开(公告)日：2010-07-29
申请号：US12655120
申请日：2009-12-23
申请人： Krista Marie Prentice , Gary Paul Schleicher , Lei Zhang , Timothy Lee Hilbert , Michel A. Daage , Sylvain Hantzer , Wenyih F. Lai , David Mentzer , William Francis Heaney , Christine Nicole Elia , Shifang Luo , Stephen J. McCarthy , Mohan Kalyanaraman
发明人： Krista Marie Prentice , Gary Paul Schleicher , Lei Zhang , Timothy Lee Hilbert , Michel A. Daage , Sylvain Hantzer , Wenyih F. Lai , David Mentzer , William Francis Heaney , Christine Nicole Elia , Shifang Luo , Stephen J. McCarthy , Mohan Kalyanaraman
IPC分类号： C10G69/02
CPC分类号： C10G45/62 , C10G2300/202 , C10G2300/207 , C10G2400/10
摘要： An integrated process for producing lubricant base oils from feedstocks under sour conditions is provided. The ability to process feedstocks under higher sulfur conditions allows for reduced cost processing and increases the flexibility in selecting a suitable feedstock. The sour feed can be delivered to a catalytic dewaxing step without any separation of sulfur and nitrogen contaminants, or a high pressure separation can be used to partially eliminate contaminants.
摘要翻译： 提供了一种在酸性条件下从原料生产润滑剂基础油的综合方法。 在较高硫条件下处理原料的能力允许降低成本处理并增加选择合适原料的灵活性。 可以将酸性进料输送到催化脱蜡步骤，而不会分离硫和氮污染物，或者可以使用高压分离来部分地消除污染物。
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8.发明授权Catalyst composition, the method of manufacturing, and the process of use thereof in aromatics alkylation 有权催化剂组合物，制备方法及其在芳烃烷基化中的应用方法公开(公告)号：US08022261B2
公开(公告)日：2011-09-20
申请号：US12906393
申请日：2010-10-18
IPC分类号： C07C2/66
CPC分类号： B01J29/7038 , B01J29/70 , B01J29/7007 , B01J29/80 , B01J35/10 , B01J37/0009 , B01J2229/42 , C07C2/66 , C07C2529/08 , C07C2529/18 , C07C2529/40 , C07C2529/65 , C07C2529/70 , C07C2529/80 , Y02P20/52 , C07C15/085
摘要： A catalyst composition comprises a crystalline MCM-22 family molecular sieve and a binder, wherein the catalyst composition is characterized by an extra-molecular sieve porosity greater than or equal to 0.122 ml/g for pores having a pore diameter ranging from about 2 nm to about 8 nm, wherein the porosity is measured by N2 porosimetry. The catalyst composition may be used for the process of alkylation or transalkylation of an alkylatable aromatic compound with an alkylating agent. The molecular sieve may have a Constraint Index of less than 12, e.g., less than 2. Examples of molecular sieve useful for this disclosure are a MCM-22 family molecular sieve, zeolite Y, and zeolite Beta.
摘要翻译： 一种催化剂组合物包括结晶MCM-22族分子筛和粘合剂，其中该催化剂组合物的特征在于具有大于或等于0.122ml / g的分子量以上孔隙，孔隙范围为约2nm至 约8nm，其中通过N 2孔隙率法测量孔隙度。 催化剂组合物可用于烷基化芳族化合物与烷基化剂的烷基化或烷基转移过程。 分子筛可以具有小于12，例如小于2的约束指数。可用于本公开的分子筛的实例是MCM-22族分子筛，沸石Y和沸石β。
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9.发明授权公开(公告)号：US07960304B2
公开(公告)日：2011-06-14
申请号：US12767559
申请日：2010-04-26
IPC分类号： B01J29/06
CPC分类号： B01J29/7038 , B01J29/7007 , B01J29/80 , B01J37/0009 , B01J37/0036 , B01J2229/42 , C07C2/66 , C07C6/126 , C07C2529/70 , Y02P20/52 , C07C15/085 , C07C15/073
摘要： A catalyst composition comprises (a) a MCM-22 family molecular sieve; and (b) a binder, wherein the MCM-22 family molecular sieve is characterized by an average crystal agglomerate size of less than or equal to 16 microns. The catalyst composition may further have a second molecular sieve having a Constraint Index of less than 12, e.g., less than 2. Examples of molecular sieve useful for this disclosure are a MCM-22 family molecular sieve, zeolite Y, and zeolite Beta. The catalyst composition may be used for the process of alkylation or transalkylation of an alkylatable aromatic compound with an alkylating agent.
摘要翻译： 催化剂组合物包含（a）MCM-22族分子筛; 和（b）粘合剂，其中MCM-22族分子筛的特征在于平均晶体聚集体尺寸小于或等于16微米。 催化剂组合物还可以具有约束指数小于12，例如小于2的第二分子筛。可用于本发明的分子筛的实例是MCM-22族分子筛，Y沸石和β沸石。 催化剂组合物可用于烷基化芳族化合物与烷基化剂的烷基化或烷基转移过程。
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公开(公告)号：US20100036184A1
公开(公告)日：2010-02-11
申请号：US12520608
申请日：2007-12-20
CPC分类号： B01J29/7088 , B01J21/063 , B01J29/08 , B01J29/40 , B01J29/70 , B01J29/7007 , B01J29/7038 , B01J29/7057 , B01J29/80 , B01J37/0009 , B01J2229/42 , C07C2/66 , C07C6/126 , C07C2521/04 , C07C2521/06 , C07C2529/70
摘要： This disclosure relates to a catalyst composition comprising (a) a crystalline MCM-49 molecular sieve; and (b) a binder comprising at least 1 wt. % of a titanium compound. In one aspect of this disclosure, the titanium compound comprises at least one of titanium oxide, titanium hydroxide, titanium sulfate, titanium phosphate, or any combination thereof. In another aspect of this disclosure, the catalyst composition further comprises a crystalline MCM-22 family molecular sieve comprising at least one of MCM-22, MCM-36, MCM-49, MCM-56, ITQ-1, ITQ-2, ITQ-30, PSH-3, ERB-1, SSZ-25, or any combination thereof. In other embodiments, this disclosure relates to a process for preparing the catalyst composition of this disclosure, the process comprises (a) providing the crystalline MCM-49 molecular sieve and the binder comprising at least 1 wt. % of a titanium compound to form a mixture; and (b) forming the mixture into the catalyst composition. In a preferred embodiment, the forming step comprises extruding. In yet other embodiments, this disclosure discloses a process for alkylating an aromatic hydrocarbon with an alkylating agent to produce an alkylated aromatic product by contacting the aromatic hydrocarbon and the alkylating agent with the catalyst composition.
摘要翻译： 本公开涉及一种催化剂组合物，其包含（a）结晶MCM-49分子筛; 和（b）包含至少1重量％ ％的钛化合物。 在本公开的一个方面，钛化合物包括氧化钛，氢氧化钛，硫酸钛，磷酸钛或其任何组合中的至少一种。 在本公开的另一方面，催化剂组合物还包含结晶MCM-22族分子筛，其包含MCM-22，MCM-36，MCM-49，MCM-56，ITQ-1，ITQ-2，ITQ -30，PSH-3，ERB-1，SSZ-25或其任何组合。 在其它实施方案中，本公开涉及制备本发明的催化剂组合物的方法，该方法包括（a）提供结晶MCM-49分子筛和包含至少1wt。 ％的钛化合物以形成混合物; 和（b）将该混合物形成到催化剂组合物中。 在优选实施例中，成形步骤包括挤出。 在其它实施方案中，本公开公开了一种使用烷基化剂烷基化芳族烃以通过使芳族烃和烷基化剂与催化剂组合物接触而产生烷基化芳族化合物的方法。
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