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    Inducing turbulent flow in catalyst beds
    1.
    发明申请
    Inducing turbulent flow in catalyst beds 审中-公开
    诱导催化剂床中的湍流

    公开(公告)号：US20020198429A1

    公开(公告)日：2002-12-26

    申请号：US10150850

    申请日：2002-05-16

    Applicant: Conoco Inc.

    Inventor： Sriram Ramani ,  Joe D. Allison ,  Richard Delgado

    IPC: C07C005/367 ,  C07C005/333 ,  B01J035/02

    CPC classification number: C10G2/33 ,  B01F5/064 ,  B01F5/0646 ,  B01F5/0647 ,  B01F5/065 ,  B01J19/2485 ,  B01J35/04 ,  C10G2/341

    Abstract: A catalyst bed is made of a monolith having a plurality of pores extending through the monolith, the pores forming tortuous flow paths through the monolith. The tortuous flow paths are obtained by modifying the monolith channels with turbulence-inducing objects or means. Catalyst is disposed on the wall surfaces formed by the pores. Reactants are passed through the tortuous flow paths creating turbulent flow thereby increasing the contact of the reactants with the catalyst on the wall surfaces and the mixing across the reactant stream.

    Abstract translation: 催化剂床由具有延伸穿过整料的多个孔的整料制成，孔形成通过整料的曲折的流动路径。 曲折的流动路径是通过用湍流诱导物体或装置修改整体通道获得的。 催化剂设置在由孔形成的壁表面上。 反应物通过曲折的流动路径，产生湍流，从而增加反应物与壁上的催化剂的接触以及反应物流的混合。

    Oxidative dehydrogenation of hydrocarbons using catalysts with trace promoter metal loading
    2.
    发明申请
    Oxidative dehydrogenation of hydrocarbons using catalysts with trace promoter metal loading 审中-公开
    使用具有痕量促进剂金属负载的催化剂进行烃的氧化脱氢

    公开(公告)号：US20040068148A1

    公开(公告)日：2004-04-08

    申请号：US10266404

    申请日：2002-10-08

    Applicant: Conoco Inc.

    Inventor： Joe D. Allison ,  Sriram Ramani ,  Zhen Chen ,  Lisa M. Carmichael ,  Shang Y. Chen ,  Steve R. McDonald ,  Anne Gaffney

    IPC: C07C005/333 ,  C07C005/327 ,  C07C005/373

    CPC classification number: B01J23/56 ,  B01J23/42 ,  B01J23/44 ,  C07C5/48 ,  C07C2523/26 ,  C07C2523/42 ,  C07C2523/44 ,  C07C2523/745 ,  C07C11/02

    Abstract: Catalysts and methods useful for the production of olefins from alkanes via oxidative dehydrogenation (ODH) are disclosed. The ODH catalysts are comprised of a Group VIII promoter metal present at trace levels. The Group VIII promoter metal is preferably platinum, palladium or a combination thereof and is preferably present at a promoter metal loading of between about 0.005 and about 0.1 weight percent. Optionally, the ODH catalysts include a base metal, metal oxide, or combination thereof. The optional base metal is selected from the group consisting of Group IB-IIB metals, Group IVB-VIIB metals, Group IIA-VA metals, scandium, yttrium, actinium, iron, cobalt, nickel, their oxides, and combinations thereof. The base metal is more preferably selected from the group consisting copper, tin, chromium, gold, manganese and their respective oxides and any combinations thereof. The base metal loading is preferably between about 0.5 and about 10 weight percent. Optionally, the promoter metal can be supported on a refractory material. The refractory support is preferably comprised of a material selected from group consisting of zirconia, stabilized zirconias, alumina, stabilized aluminas, and combinations thereof.

    Abstract translation: 公开了可用于通过氧化脱氢（ODH）从烷烃生产烯烃的催化剂和方法。 ODH催化剂由痕量存在的VIII族助催化剂金属组成。 VIII族助催化剂金属优选为铂，钯或其组合，优选以约0.005至约0.1重量％的助催化剂金属负载存在。 任选地，ODH催化剂包括贱金属，金属氧化物或其组合。 可选择的贱金属选自IB-IIB族金属，IVB-VIIB族金属，IIA-VA族金属，钪，钇，锕，铁，钴，镍，它们的氧化物及其组合。 贱金属更优选选自铜，锡，铬，金，锰及其各自的氧化物及其任何组合。 贱金属负载量优选为约0.5至约10重量％。 任选地，促进剂金属可以负载在耐火材料上。 耐火载体优选由选自氧化锆，稳定化氧化锆，氧化铝，稳定化氧化铝及其组合的材料组成。

    MCrAlY supported catalysts for oxidative dehydrogenation of alkanes
    5.
    发明申请
    MCrAlY supported catalysts for oxidative dehydrogenation of alkanes 失效
    MCrAlY负载催化剂用于烷烃的氧化脱氢

    公开(公告)号：US20040072685A1

    公开(公告)日：2004-04-15

    申请号：US10269174

    申请日：2002-10-11

    Applicant: Conoco Inc.

    Inventor： Zhen Y. Chen ,  Sriram Ramani ,  Lisa M. Carmichael ,  Joe D. Allison

    IPC: C07C005/333 ,  C07C005/327

    CPC classification number: C07C5/48 ,  C07C2523/76 ,  C07C2523/89 ,  C07C11/02

    Abstract: A catalyst useful for the production of olefins from alkanes via oxidative dehydrogenation (ODH) is disclosed. In accordance with a preferred embodiment of the present invention, a catalyst for use in ODH processes includes a MCrAlY support. M is preferably a base metal, or combination of base metals. A base metal is herein defined as a non-Group VIII metal, with the exception of iron, cobalt and nickel. Suitable base metals include Group IB-VIIB metals, Group IIIA-VA metals, Lanthanide metals, iron, cobalt and nickel. In a preferred embodiment, M is iron. Additionally, the catalyst may optionally include a Group VIII promoter. Suitable Group VIII promoters include Ru, Rh, Pd, Os, Ir, and Pt. In another preferred embodiment, M is a combination of a Lanthanide metal and iron with a front-loaded Group VIII promoter.

    Abstract translation: 公开了一种可用于通过氧化脱氢（ODH）从烷烃生产烯烃的催化剂。 根据本发明的优选实施方案，用于ODH方法的催化剂包括MCrAlY载体。 M优选为贱金属或贱金属的组合。 本文将贱金属定义为非Ⅷ族金属，铁，钴和镍除外。 合适的贱金属包括IB-VIIB族金属，IIIA-VA族金属，镧系金属，铁，钴和镍。 在优选的实施方案中，M是铁。 另外，催化剂可任选地包括VIII族促进剂。 合适的VIII族促进剂包括Ru，Rh，Pd，Os，Ir和Pt。 在另一个优选的实施方案中，M是镧系金属和铁与前负载的VIII族促进剂的组合。

    Process for converting alkanes to carbon filaments
    9.
    发明申请
    Process for converting alkanes to carbon filaments 有权
    将烷烃转化为碳丝的方法

    公开(公告)号：US20040062704A1

    公开(公告)日：2004-04-01

    申请号：US10263315

    申请日：2002-10-01

    Applicant: Conoco Inc.

    Inventor： Joe D. Allison ,  Sriram Ramani ,  Priya Rangarajan ,  Kenneth M. York ,  Troy L. Amundson ,  Gary E. Welch

    IPC: D01F009/12

    CPC classification number: B82Y30/00 ,  D01F9/1271

    Abstract: The present invention includes a process for producing carbon filaments and synthesis gas from a mixture of alkanes, preferably natural gas, comprising converting a first portion of the alkanes, preferably C2null hydrocarbons, directly to carbon filaments and converting a second portion of the alkanes, preferably methane, to syngas. The natural gas may be separated into a first feed stream comprising ethane, propane, and butane and a second feed stream comprising methane. The first feed stream is fed to a carbon filament CF reactor to produce carbon filaments and hydrogen. The second feed stream is fed to a syngas production reactor to produce syngas. Alternatively, the natural gas is fed to at least one carbon filament reactor that is maintained at an effective temperature to convert C2null hydrocarbons in the natural gas to carbon filaments and hydrogen, thereby filtering methane from the natural gas.

    Abstract translation: 本发明包括从烷烃（优选天然气）的混合物中生产碳丝和合成气的方法，包括将第一部分烷烃，优选C2 +碳直接转化成碳丝，并将第二部分的 烷烃，优选甲烷，合成气。 天然气可以分离成包含乙烷，丙烷和丁烷的第一进料流和包含甲烷的第二进料流。 将第一进料流送入碳丝CF反应器以产生碳丝和氢。 将第二进料流送入合成气生产反应器以产生合成气。 或者，将天然气进料至至少一个碳丝反应器，其保持在有效温度以将天然气中的C2 +转化为碳丝和氢，从而从天然气中过滤甲烷。

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