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公开(公告)号：US5744619A
公开(公告)日：1998-04-28
申请号：US818265
申请日：1997-03-17
IPC分类号： C07D301/03 , C07D301/12
CPC分类号： C07D301/12
摘要： Titanovanadosilicalites have been found to be very selective, active catalysts in the epoxidation of olefins by peroxides. Dilute hydrogen peroxide suffices to afford high yields of the epoxide. Vanadium incorporation at levels of Si:V in the range 100-2500 effectively changes the characteristics of the titanosilicalite into which it is incorporated to give near quantitative conversion of propylene at selectivities greater than 90%.
摘要翻译： 已经发现，在过氧化物对烯烃的环氧化中，非常有选择性的活性催化剂。 稀释过氧化氢足以提供高产率的环氧化物。 钒含量在100-2500范围内的Si：V水平有效地改变了其掺入其中的钛硅硅沸石的特性，使得选择性大于90％的丙烯接近定量转化。
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公开(公告)号：US6074624A
公开(公告)日：2000-06-13
申请号：US109854
申请日：1998-07-02
IPC分类号： C07D301/12 , C01B39/06
CPC分类号： C07D301/12 , Y10S423/22
摘要： A new family of crystalline titanostannosilicate molecular sieves have been synthesized. These molecular sieves have a microporous three-dimensional framework of TiO.sub.2, SnO.sub.2 and SiO.sub.2 tetrahedral oxide units and are represented by the empirical formula:(Ti.sub.x Sn.sub.y Si.sub.z)O.sub.2where "X", "y" and "z" are the mole fractions of Ti, Sn and Si respectively. These molecular sieves are active catalysts for the epoxidation of olefins by peroxides such as hydrogen peroxide.
摘要翻译： 已经合成了一种新的结晶钛酸铵分子筛系列。 这些分子筛具有TiO 2，SnO 2和SiO 2四面体氧化物单元的微孔三维框架，并且由经验式（TixSnySiz）O 2表示，其中“X”，“y”和“z”是Ti的摩尔分数， Sn和Si。 这些分子筛是用过氧化物如过氧化氢对烯烃进行环氧化的活性催化剂。
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公开(公告)号：US5780654A
公开(公告)日：1998-07-14
申请号：US840531
申请日：1997-04-22
IPC分类号： B01J29/04 , C01B39/04 , C07B41/04 , C07B61/00 , C07D301/12 , C07D303/04
CPC分类号： C07D301/12
摘要： Titanostannosilicalites molecular sieves as new compositions of matter have been found to be very selective, active catalysts in the epoxidation of olefins by peroxides. Dilute hydrogen peroxide suffices to afford high yields of the epoxide with good selectivity. The sieves described within have a unit empirical formula, on an anhydrous basis of (Ti.sub.x Sn.sub.y Si.sub.z)O.sub.2, where 0.0005
摘要翻译： 已经发现，作为物质的新组合物的Titanostannosilicalites分子筛是非常选择性的，通过过氧化物使烯烃环氧化的活性催化剂。 稀释的过氧化氢足以以良好的选择性提供高产率的环氧化物。 所述筛子具有单位经验公式，以（TixSnySiz）O 2的无水为基准，其中0.0005
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公开(公告)号：US20140005452A1
公开(公告)日：2014-01-02
申请号：US13537448
申请日：2012-06-29
CPC分类号： B01J23/06 , B01J23/02 , B01J23/75 , B01J29/83 , B01J29/84 , B01J29/85 , C07C1/20 , C07C2/66 , C07C2529/84 , C07C2529/85 , C10G3/49 , C10G29/205 , C10G35/095 , C10G45/00 , C10G45/12 , C10G45/54 , C10G47/16 , C10G50/00 , Y02P30/42 , C07C11/02 , C07C15/02
摘要： A new family of crystalline microporous metallophosphates designated AlPO-59 has been synthesized. These metallophosphates are represented by the empirical formula R+rMm2+EPxSiyOz where R is an organoammonium cation such as the ETMA+, M is a framework metal alkaline earth or transition metal of valence 2+, and E is a trivalent framework element such as aluminum or gallium. The AlPO-59 compositions are characterized by a new unique ABC-6 net structure and compositions and have catalytic properties for carrying out various hydrocarbon conversion processes, and separation properties for separating at least one component.
摘要翻译： 已经合成了一系列名为AlPO-59的结晶微孔金属磷酸盐系列。 这些金属磷酸盐由经验式R + rMm2 + EPxSiyOz表示，其中R是有机铵阳离子，例如ETMA +，M是骨架金属碱土金属或价态2+的过渡金属，E是三价骨架元素如铝或 镓。 AlPO-59组合物的特征在于新的独特的ABC-6网结构和组合物，并且具有用于进行各种烃转化方法的催化性能，以及用于分离至少一种组分的分离性质。
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公开(公告)号：US20140004024A1
公开(公告)日：2014-01-02
申请号：US13537337
申请日：2012-06-29
IPC分类号： B01J29/85 , C10G47/18 , C10G11/02 , B01D53/00 , B01D15/36 , C07C1/20 , C07C2/58 , C07C2/86 , B01D15/26 , C10G47/20 , C07C2/66
CPC分类号： C07C2/66 , B01J29/83 , B01J29/85 , C01B37/065 , C01B37/08 , C01B39/54 , C07C1/20 , C07C2/58 , C07C2529/83 , C07C2529/84 , C07C2529/85 , C07C2531/02 , Y02P30/42 , C07C11/02 , C07C9/00
摘要： A new family of crystalline microporous metallophosphates designated AlPO-57 has been synthesized. These metallophosphates are represented by the empirical formula R+rMmn+EPxSiyOz where R is an organoammonium cation such as the DEDMA+, M is a divalent framework metal such as an alkaline earth or transition metal, and E is a framework element such as aluminum or gallium. The microporous AlPO-57 compositions are characterized by a new unique ABC-6 net structure and have catalytic properties for carrying out various hydrocarbon conversion processes and separation properties for separating at least one component.
摘要翻译： 已经合成了一系列名为AlPO-57的结晶微孔金属磷酸盐系列。 这些金属磷酸盐由经验式R + rMmn + EPxSiyOz表示，其中R是有机铵阳离子，例如DEDMA +，M是二价骨架金属如碱土金属或过渡金属，E是骨架元素如铝或镓 。 微孔AlPO-57组合物的特征在于新的独特的ABC-6网状结构，并且具有用于进行各种烃转化方法和用于分离至少一种组分的分离性能的催化性质。
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6.发明申请Hydrocarbon Conversion Processes Using UZM-26 and UZM-26X Crystalline Microporous Zeolitic Compositions 有权使用UZM-26和UZM-26X结晶微孔沸石组合物的烃转化方法公开(公告)号：US20100152510A1
公开(公告)日：2010-06-17
申请号：US12335648
申请日：2008-12-16
申请人： Mark A Miller , Gregory J. Lewis
发明人： Mark A Miller , Gregory J. Lewis
摘要： This invention relates to hydrocarbon conversion processes using crystalline zeolitic compositions designated the UZM-26 and UZM-26X. UZM-26 is a microporous three-dimensional zeolitic composition that is derived from UZM-26P (an as synthesized layered composition) by calcination. UZM-26X is a microporous three-dimensional zeolitic composition that is derived from UZM-26PX by calcination, where UZM-26PX is an ion-exchanged form of UZM-26P.
摘要翻译： 本发明涉及使用称为UZM-26和UZM-26X的结晶沸石组合物的烃转化方法。 UZM-26是通过煅烧从UZM-26P（作为合成层状组合物）衍生的微孔三维沸石组合物。 UZM-26X是通过煅烧从UZM-26PX衍生的微孔三维沸石组合物，其中UZM-26PX是离子交换形式的UZM-26P。
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7.发明申请公开(公告)号：US20100152023A1
公开(公告)日：2010-06-17
申请号：US12335657
申请日：2008-12-16
申请人： Mark A. Miller , Gregory J. Lewis
发明人： Mark A. Miller , Gregory J. Lewis
IPC分类号： C01B39/04 , B01J29/072 , B01J29/06
摘要： This invention relates to a new family of crystalline aluminosilicate compositions designated the UZM-26 family. These include the species UZM-26P, UZM-26PX, UZM-26 and UZM-26X, which have unique structures. UZM-26P is an as synthesized layered composition, while UZM-26 is a calcined form of UZM-26P which has a three-dimensional structure. UZM-26PX is an ion-exchanged form of UZM-26P while UZM-26X is a calcined form of UZM-26PX which has a three-dimensional structure.
摘要翻译： 本发明涉及一种名为UZM-26族的新型结晶硅铝酸盐组合物。 这些包括具有独特结构的物种UZM-26P，UZM-26PX，UZM-26和UZM-26X。 UZM-26P是一种合成的层状组合物，而UZM-26是具有三维结构的UZM-26P的煅烧形式。 UZM-26PX是UZM-26P的离子交换形式，而UZM-26X是具有三维结构的UZM-26PX的煅烧形式。
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8.发明授权Hydrocarbon conversion processes using a catalyst comprising a UZM-8HS composition 有权使用包含UZM-8HS组合物的催化剂的烃转化方法公开(公告)号：US07638667B2
公开(公告)日：2009-12-29
申请号：US11457184
申请日：2006-07-13
申请人： Deng-Yang Jan , Raelynn M. Miller , Mathias P. Koljack , John E. Bauer , Paula L. Bogdan , Gregory J. Lewis , Gregory J. Gajda , Susan C. Koster , Michael G. Gatter , Jaime G. Moscoso
发明人： Deng-Yang Jan , Raelynn M. Miller , Mathias P. Koljack , John E. Bauer , Paula L. Bogdan , Gregory J. Lewis , Gregory J. Gajda , Susan C. Koster , Michael G. Gatter , Jaime G. Moscoso
IPC分类号： C07C2/66
CPC分类号： B01J29/06 , B01J29/70 , B01J29/7007 , B01J29/74 , B01J2229/42 , C01B39/026 , C01B39/06 , C01B39/065 , C01B39/48 , C01P2002/72 , C07C2/66 , C07C5/2708 , C07C6/126 , C07C2529/70 , C10G29/205 , C10G45/10 , C10G45/12 , C10G45/62 , C10G45/64 , C10G47/14 , C10G47/20 , C10G49/06 , C10G49/08 , Y02P20/52 , C07C15/073 , C07C15/085 , C07C15/08
摘要： Hydrocarbon conversion processes using a new family of zeolites identified as UZM-8HS are described. The UZM-8HS zeolite are derived from UZM-8 zeolites by treating the UZM-8 with a fluoro-silicate salt, an acid, etc. The UZM-8HS zeolites have unique x-ray diffraction patterns. These zeolites can be used in alkylation of aromatics, transalkylation of aromatics, isomerization of aromatics and alkylation of isoparaffins.
摘要翻译： 描述了使用识别为UZM-8HS的新家族沸石的烃转化方法。 UZM-8HS沸石通过用氟硅酸盐，酸等处理UZM-8而衍生自UZM-8沸石.UZM-8HS沸石具有独特的x射线衍射图。 这些沸石可用于芳族化合物的烷基化，芳烃的烷基转移，芳族化合物的异构化和异构烷烃的烷基化。
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9.发明授权Process for preparing crystalline aluminosilicate compositions using charge density matching 有权使用电荷密度匹配制备结晶硅铝酸盐组合物的方法公开(公告)号：US07578993B2
公开(公告)日：2009-08-25
申请号：US10978001
申请日：2004-10-29
IPC分类号： B01J29/70
摘要： A process for preparing crystalline alumino-silicate compositions has been developed. The process involves preparing a charge density mismatch reaction mixture comprising sources of aluminum, silicon, optionally an E metal and at least one charge density mismatch (CDM) template. The CDM template is an organic nitrogen containing template, in the hydroxide form, e.g. tetraethylammonium hydroxide and is characterized in that it is incapable of inducing crystallization. To this mixture there is added a solution comprising a second templating agent termed a crystallization template (CT). The CT can be an organic template different from the CDM template, an alkali metal, an alkaline earth metal and mixtures thereof.
摘要翻译： 已经开发了制备结晶铝硅酸盐组合物的方法。 该方法包括制备电荷密度不匹配反应混合物，其包含铝，硅，任选的E金属和至少一种电荷密度不匹配（CDM）模板的来源。 CDM模板是含有有机氮的模板，以氢氧化物形式，例如， 四乙基氢氧化铵，其特征在于它不能诱导结晶。 向该混合物中加入包含称为结晶模板（CT）的第二模板剂的溶液。 CT可以是与CDM模板，碱金属，碱土金属及其混合物不同的有机模板。
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10.发明授权Oxidation of hydrocarbons using crystalline manganese (II/III) phosphate compositions 失效使用结晶锰（II / III）磷酸盐组合物对碳氢化合物进行氧化公开(公告)号：US06512144B1
公开(公告)日：2003-01-28
申请号：US09728536
申请日：2000-12-01
申请人： Gregory J. Lewis , Paula L. Bogdan , Feng Xu , Joseph A. Kocal
发明人： Gregory J. Lewis , Paula L. Bogdan , Feng Xu , Joseph A. Kocal
IPC分类号： C07C4500
CPC分类号： B01J27/187 , B01J29/82 , C01B25/377 , C07C45/33 , C07C315/02
摘要： Processes for oxidizing hydrocarbons using a new family of crystalline manganese phosphate compositions have been developed. These compositions have an extended network which network can be a one-, two-, or three-dimensional network. The composition has an empirical formula of: (Aa+)v(Mnb+)(Mc+)xPyOz where A is a structure directing agent such as an alkali metal, M is a metal such as Al, Fe3+ and “b” is the average manganese oxidation state and varies from greater than 2.0 to a maximum of 3.0. Specific oxidation processes are oxidative dehydrodimerization and oxidative dehydrogenation.
摘要翻译： 已经开发了使用新的结晶磷酸锰组合物来氧化烃的方法。 这些组合物具有扩展网络，其网络可以是一维，二维或三维网络。 该组合物具有以下经验式：其中A是结构导向剂如碱金属，M是金属如Al，Fe 3+，“b”是平均锰氧化态，并且从大于2.0变化到最大值 3.0。 具体的氧化过程是氧化脱氢二聚化和氧化脱氢。
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