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公开(公告)号：US10532346B2
公开(公告)日：2020-01-14
申请号：US15239210
申请日：2016-08-17
IPC分类号： B01J21/02 , B01J23/44 , B01J23/63 , B01J23/755 , B01J23/80 , B01J23/84 , B01J23/86 , B01J23/89 , B01J25/00 , B01J25/02 , B01J32/00 , B01J35/00 , B01J35/06 , B01J35/10 , B01J37/02 , B01J37/06 , B01J37/08 , B01J37/14 , B01J37/18 , C01B3/40 , C07C5/03 , B01J23/847 , C10G2/00 , C10G3/00
摘要： The present invention relates to methods for producing metal-supported thin layer skeletal catalyst structures, to methods for producing catalyst support structures without separately applying an intermediate washcoat layer, and to novel catalyst compositions produced by these methods. Catalyst precursors may be interdiffused with the underlying metal support then activated to create catalytically active skeletal alloy surfaces. The resulting metal-anchored skeletal layers provide increased conversion per geometric area compared to conversions from other types of supported alloy catalysts of similar bulk compositions, and provide resistance to activity loss when used under severe on-stream conditions. Particular compositions of the metal-supported skeletal catalyst alloy structures can be used for conventional steam methane reforming to produce syngas from natural gas and steam, for hydrodeoxygenation of pyrolysis bio-oils, and for other metal-catalyzed reactions inter alia.
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2.发明授权公开(公告)号：US09446386B2
公开(公告)日：2016-09-20
申请号：US13649622
申请日：2012-10-11
IPC分类号： B01J23/755 , B01J21/02 , B01J32/00 , B01J23/89 , B01J37/02 , B01J37/06 , B01J37/18 , B01J23/847 , B01J23/44 , B01J23/63 , B01J23/80 , B01J23/86 , B01J25/02 , B01J35/10 , C01B3/40
CPC分类号： B01J23/894 , B01J21/02 , B01J23/44 , B01J23/63 , B01J23/755 , B01J23/80 , B01J23/8472 , B01J23/8476 , B01J23/866 , B01J23/8906 , B01J25/02 , B01J32/00 , B01J35/06 , B01J35/1019 , B01J37/0225 , B01J37/0228 , B01J37/06 , B01J37/14 , B01J37/18 , C01B3/40 , C01B2203/0233 , C01B2203/1041 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1076 , C01B2203/1082 , C01B2203/1235 , C01B2203/1241 , C07C5/03 , C07C2521/02 , C07C2521/06 , C07C2523/44 , C07C2523/63 , C07C2523/755 , C07C2523/89 , C10G2/332 , C10G2/333 , C10G3/45 , C10G3/47 , Y02P20/52 , Y02P30/20
摘要： The present invention relates to methods for producing metal-supported thin layer skeletal catalyst structures, to methods for producing catalyst support structures without separately applying an intermediate washcoat layer, and to novel catalyst compositions produced by these methods. Catalyst precursors may be interdiffused with the underlying metal support then activated to create catalytically active skeletal alloy surfaces. The resulting metal-anchored skeletal layers provide increased conversion per geometric area compared to conversions from other types of supported alloy catalysts of similar bulk compositions, and provide resistance to activity loss when used under severe on-stream conditions. Particular compositions of the metal-supported skeletal catalyst alloy structures can be used for conventional steam methane reforming to produce syngas from natural gas and steam, for hydrodeoxygenation of pyrolysis bio-oils, and for other metal-catalyzed reactions inter alia.
摘要翻译： 本发明涉及金属负载型薄层骨架催化剂结构体的制造方法，以及不分别涂布中间涂层的催化剂载体结构体的制造方法，以及由这些方法制造的新型催化剂组合物。 催化剂前体可以与下面的金属载体相互扩散，然后被活化以产生催化活性的骨架合金表面。 与来自其他类型的类似体积组合物的支撑合金催化剂的转化相比，所得到的金属锚定骨架层提供每几何面积的增加的转化率，并且当在严格的流动条件下使用时提供对活性损失的抵抗力。 金属支撑的骨架催化剂合金结构的特定组成可用于常规蒸汽甲烷重整，以从天然气和蒸汽产生合成气，用于热解生物油的加氢脱氧，以及其它金属催化反应。
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3.发明申请公开(公告)号：US20160354767A1
公开(公告)日：2016-12-08
申请号：US15239210
申请日：2016-08-17
IPC分类号： B01J23/89 , C10G2/00 , C07C5/03 , B01J23/755 , C01B3/40 , B01J23/63 , B01J35/06 , B01J37/02 , B01J37/14 , C10G3/00 , B01J23/44
CPC分类号： B01J23/894 , B01J21/02 , B01J23/44 , B01J23/63 , B01J23/755 , B01J23/80 , B01J23/8472 , B01J23/8476 , B01J23/866 , B01J23/8906 , B01J25/00 , B01J25/02 , B01J32/00 , B01J35/002 , B01J35/06 , B01J35/1019 , B01J37/0217 , B01J37/0225 , B01J37/0228 , B01J37/06 , B01J37/08 , B01J37/14 , B01J37/18 , C01B3/40 , C01B2203/0233 , C01B2203/1041 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1076 , C01B2203/1082 , C01B2203/1235 , C01B2203/1241 , C07C5/03 , C07C2521/02 , C07C2521/06 , C07C2523/44 , C07C2523/63 , C07C2523/755 , C07C2523/89 , C10G2/331 , C10G2/332 , C10G2/333 , C10G3/44 , C10G3/45 , C10G3/47 , C10G3/48 , C10G45/36 , C10G45/38 , C10G49/04 , Y02P20/52 , Y02P30/20
摘要： The present invention relates to methods for producing metal-supported thin layer skeletal catalyst structures, to methods for producing catalyst support structures without separately applying an intermediate washcoat layer, and to novel catalyst compositions produced by these methods. Catalyst precursors may be interdiffused with the underlying metal support then activated to create catalytically active skeletal alloy surfaces. The resulting metal-anchored skeletal layers provide increased conversion per geometric area compared to conversions from other types of supported alloy catalysts of similar bulk compositions, and provide resistance to activity loss when used under severe on-stream conditions. Particular compositions of the metal-supported skeletal catalyst alloy structures can be used for conventional steam methane reforming to produce syngas from natural gas and steam, for hydrodeoxygenation of pyrolysis bio-oils, and for other metal-catalyzed reactions inter alia.
摘要翻译： 本发明涉及金属负载型薄层骨架催化剂结构体的制造方法，以及不分别涂布中间涂层的催化剂载体结构体的制造方法，以及由这些方法制造的新型催化剂组合物。 催化剂前体可以与下面的金属载体相互扩散，然后被活化以产生催化活性的骨架合金表面。 与来自其他类型的类似体积组合物的支撑合金催化剂的转化相比，所得到的金属锚定骨架层提供每几何面积的增加的转化率，并且当在严格的流动条件下使用时提供对活性损失的抵抗力。 金属支撑的骨架催化剂合金结构的特定组成可用于常规蒸汽甲烷重整，以从天然气和蒸汽产生合成气，用于热解生物油的加氢脱氧，以及其它金属催化反应。
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