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    In situ moisture generation and use of polyfunctional alcohols for crosslinking of silane-functionalized resins
    2.
    发明授权
    In situ moisture generation and use of polyfunctional alcohols for crosslinking of silane-functionalized resins 有权
    用于交联硅烷官能化树脂的多官能醇的原位水分产生和使用

    公开(公告)号：US08460770B2

    公开(公告)日：2013-06-11

    申请号：US12740838

    申请日：2008-10-13

    申请人： Bharat I. Chaudhary ,  Jeffrey M. Cogen ,  Saurav S. Sengupta

    发明人： Bharat I. Chaudhary ,  Jeffrey M. Cogen ,  Saurav S. Sengupta

    IPC分类号： B32B1/02 ,  B32B1/08 ,  C08F8/00 ,  C08F273/00 ,  C08F130/08 ,  C08G77/442

    CPC分类号： C08K5/05 ,  C08K5/42 ,  Y10T428/1352 ,  Y10T428/139 ,  C08L43/04

    摘要： Polymer compositions comprise a (i) silane-functionalized polymer, e.g., a polyethylene grafted with vinyl triethoxy silane, (H) polyfunctional alcohol e.g., α,α,α′,α′˜tetramethyl-I,3-benzenediethanol and, optionally, (iii) acid, e.g., an alkylated aryl disulfonic acid. The use of polyfunctional alcohols in the absence of a strong acid yields a light-crosslinking of the silane-functionalized polymer and this, in turn, provides a polymer melt with improved extensional properties such as elongational viscosity and melt strength. The use of a polyfunctional alcohol in combination with a blocked strong acid provides a slow rate of crosslinking during melt processing and a high degree of ultimate crosslinking after the polymer composition has been shaped or molded.

    摘要翻译： 聚合物组合物包含（i）硅烷官能化聚合物，例如用乙烯基三乙氧基硅烷接枝的聚乙烯，（H）多官能醇，例如α，α，α'，α'-四甲基-1,3-苯二甲醇， （iii）酸，例如烷基化芳基二磺酸。 在不存在强酸的情况下使用多官能醇产生硅烷官能化聚合物的轻交联，这又提供具有改进的拉伸性能如伸长粘度和熔体强度的聚合物熔体。 使用多官能醇与封闭的强酸组合提供了在熔融加工过程中缓慢的交联速率，以及在聚合物组合物成型或模制之后的高度极限交联。

    In Situ Moisture Generation and Use of Polyfunctional Alcohols for Crosslinking of Silane-Functionalized Resins
    3.
    发明申请
    In Situ Moisture Generation and Use of Polyfunctional Alcohols for Crosslinking of Silane-Functionalized Resins 有权
    多官能醇的原位水分产生和使用用于硅烷官能化树脂的交联

    公开(公告)号：US20100297374A1

    公开(公告)日：2010-11-25

    申请号：US12740838

    申请日：2008-10-13

    申请人： Bharat I. Chaudhary ,  Jeffrey M. Cogen ,  Saurav S. Sengupta

    发明人： Bharat I. Chaudhary ,  Jeffrey M. Cogen ,  Saurav S. Sengupta

    IPC分类号： B32B1/08 ,  C08G77/00 ,  C08F30/08 ,  B05D5/12 ,  H01B3/00

    CPC分类号： C08K5/05 ,  C08K5/42 ,  Y10T428/1352 ,  Y10T428/139 ,  C08L43/04

    摘要： Polymer compositions comprise a (i) silane-functionalized polymer, e.g., a polyethylene grafted with vinyl triethoxy silane, (H) polyfunctional alcohol e.g., α,α,α′,α′˜tetramethyl-I,3-benzenediethanol and, optionally, (iii) acid, e.g., an alkylated aryl disulfonic acid. The use of polyfunctional alcohols in the absence of a strong acid yields a light-crosslinking of the silane-functionalized polymer and this, in turn, provides a polymer melt with improved extensional properties such as elongational viscosity and melt strength. The use of a polyfunctional alcohol in combination with a blocked strong acid provides a slow rate of crosslinking during melt processing and a high degree of ultimate crosslinking after the polymer composition has been shaped or molded.

    摘要翻译： 聚合物组合物包含（i）硅烷官能化聚合物，例如用乙烯基三乙氧基硅烷接枝的聚乙烯，（H）多官能醇，例如α，α，α'，α'-四甲基-1,3-苯二甲醇， （iii）酸，例如烷基化芳基二磺酸。 在不存在强酸的情况下使用多官能醇产生硅烷官能化聚合物的轻交联，这又提供具有改进的拉伸性能如伸长粘度和熔体强度的聚合物熔体。 使用多官能醇与封闭的强酸组合提供了在熔融加工过程中缓慢的交联速率，以及在聚合物组合物成型或模制之后的高度极限交联。

    Catalyst System for Moisture Cure of Ethylene-Vinylsilane Copolymers
    4.
    发明申请
    Catalyst System for Moisture Cure of Ethylene-Vinylsilane Copolymers 审中-公开
    乙烯 - 乙烯基硅烷共聚物水分固化催化剂体系

    公开(公告)号：US20100160471A1

    公开(公告)日：2010-06-24

    申请号：US12630915

    申请日：2009-12-04

    申请人： Saurav S. Sengupta ,  Abhijit Ghosh-Dastidar ,  Bharat I. Chaudhary

    发明人： Saurav S. Sengupta ,  Abhijit Ghosh-Dastidar ,  Bharat I. Chaudhary

    IPC分类号： C08F8/00 ,  C08L43/04 ,  C08F30/08

    CPC分类号： C08K5/42 ,  C08K5/56 ,  C08L43/04

    摘要： Ethylene-vinylsilane copolymers are moisture-cured under ambient conditions using a synergistic combination of at least one Lewis acid and at least one Brønsted acid or at least one Lewis base and at least one Brønsted base. Preferably the catalyst system comprises a Lewis acid, e.g., dibutyltin dilaurate, in combination with a Brønsted acid, e.g., sulfonic acid. The Lewis acid or base and the Brønsted acid or base is present in the catalyst system at a molar ratio of Lewis acid/base to Brønsted acid/base of 1:10 to 10:1.

    摘要翻译： 乙烯 - 乙烯基硅烷共聚物在环境条件下使用至少一种路易斯酸和至少一种布朗斯台德酸或至少一种路易斯碱和至少一种布朗斯台德碱的协同组合进行湿固化。 优选地，催化剂体系包含与布朗斯台德酸例如磺酸组合的路易斯酸，例如二月桂酸二丁基锡。 路易斯酸或碱和布朗斯台德酸或碱以路易斯酸/碱与布朗斯台德酸/碱的摩尔比1:10至10:1存在于催化剂体系中。

    Tap-mediated, rheology-modified polymers and preparation methods
    5.
    发明申请
    Tap-mediated, rheology-modified polymers and preparation methods 审中-公开
    水分子介导的流变改性聚合物及其制备方法

    公开(公告)号：US20080188623A1

    公开(公告)日：2008-08-07

    申请号：US11592524

    申请日：2006-11-03

    申请人： Bharat I. Chaudhary ,  Malcolm F. Finlayson ,  Stephen F. Hahn ,  Stephane Costeux ,  John Scott Parent ,  Saurav S. Sengupta

    发明人： Bharat I. Chaudhary ,  Malcolm F. Finlayson ,  Stephen F. Hahn ,  Stephane Costeux ,  John Scott Parent ,  Saurav S. Sengupta

    IPC分类号： C08F8/40

    CPC分类号： C08F8/40

    摘要： The present invention yields a triallyl phosphate (TAP)-mediated, rheology-modified polymer being prepared in a reaction from a reaction mixture made from or containing (a) a free-radical, chain-scissionable organic polymer and (b) TAP, wherein the TAP-mediated, rheology-modified polymer has extensional viscosity at Hencky strains above one greater than that of the free-radical, chain-scissionable organic polymer and/or a Relaxation Spectra Index (RSI) greater than that of the free-radical, chain-scissionable organic polymer.

    摘要翻译： 本发明产生了一种由烯丙基（TAP）介导的流变学改性的聚合物，它是在由（a）自由基，可断开的有机聚合物和（b）TAP制成的反应混合物的反应中制备的，其中 TAP介导的流变改性聚合物在Hencky菌株具有比自由基，可断开链段的有机聚合物和/或大于自由基的松弛光谱指数（RSI）大一倍以上的拉伸粘度， 可断链的有机聚合物。