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1.发明授权Multimetal zeolites based catalyst for transalkylation of heavy reformate to produce xylenes and petrochemical feedstocks 有权用于重质油重链烷基转移以制备二甲苯和石化原料的多金属沸石基催化剂公开(公告)号：US09221037B2
公开(公告)日：2015-12-29
申请号：US13796383
申请日：2013-03-12
发明人： Cemal Ercan , Yuguo Wang , Mohammed Ashraf Ali , Sulaiman Saleh Al-Khattaf , Syed Ahmed Ali , Abdullah Mohammed Aitani
IPC分类号： B01J29/80 , C07C6/12 , B01J37/04 , B01J29/00 , B01J29/06 , B01J29/068 , B01J29/072 , B01J29/076 , B01J29/40 , B01J29/42 , B01J29/44 , B01J29/46 , B01J29/48 , B01J29/70 , B01J29/72 , B01J29/74 , B01J29/76 , B01J29/78 , B01J29/84 , B01J29/85 , B01J37/02 , C10G45/64 , C10G29/20
CPC分类号： B01J29/80 , B01J29/005 , B01J29/061 , B01J29/068 , B01J29/072 , B01J29/076 , B01J29/40 , B01J29/405 , B01J29/42 , B01J29/44 , B01J29/46 , B01J29/48 , B01J29/7007 , B01J29/7049 , B01J29/7057 , B01J29/72 , B01J29/7215 , B01J29/74 , B01J29/7415 , B01J29/76 , B01J29/7615 , B01J29/78 , B01J29/7815 , B01J29/84 , B01J29/85 , B01J37/0201 , B01J37/04 , B01J2029/062 , B01J2229/18 , B01J2229/183 , B01J2229/186 , B01J2229/20 , B01J2229/42 , C07C6/123 , C07C6/126 , C07C2529/40 , C07C2529/70 , C07C2529/80 , C07C2529/85 , C10G29/205 , C10G45/64 , Y02P20/52 , C07C15/08
摘要： A transalkylation catalyst for the transalkylation of a heavy reformate is provided. The catalyst includes two solid acid zeolites having different physical and chemical properties, and at least three metals selected from the group 4 lanthanthides, and the elements found in groups 6 and 10 of the periodic table.
摘要翻译： 提供了用于重质化合物的烷基转移的烷基转移催化剂。 该催化剂包括具有不同物理和化学性质的两种固体酸沸石，以及选自4-元素的至少三种金属和元素周期表第6和10族中找到的元素。
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公开(公告)号：US20200254428A1
公开(公告)日：2020-08-13
申请号：US16849038
申请日：2020-04-15
发明人： Balasamy Rabindran Jermy , Syed Ahmed Ali , Raed Hasan Abudawoud , Abdullah Mohammed Aitani , Sulaiman Saleh Al-Khattaf
IPC分类号： B01J29/80 , C07C6/06 , B01J37/08 , B01J37/04 , B01J37/02 , B01J37/00 , B01J35/10 , B01J29/70 , C07C6/12 , B01J29/72 , C01B39/02
摘要： Embodiments of zeolite composite catalysts and methods of producing the zeolite composite catalysts are provided, where the methods comprise dissolving in an alkaline solution a catalyst precursor comprising at least one mesoporous zeolite while heating, stirring, or both to yield a dissolved zeolite solution, where the mesoporous zeolite has a molar ratio of SiO2/Al2O3 of at least 30, where the mesoporous zeolite comprises zeolite beta, adjusting the pH of the dissolved zeolite solution, aging the pH adjusted dissolved zeolite solution to yield solid zeolite composite from the dissolved zeolite solution, and calcining the solid zeolite composite to produce the zeolite composite catalyst, where the zeolite composite catalyst has a mesostructure comprising at least one disordered mesophase and at least one ordered mesophase, and where the zeolite composite catalyst has a surface area defined by the Brunauer-Emmett-Teller (BET) analysis of at least 600 m2/g.
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公开(公告)号：US20180361365A1
公开(公告)日：2018-12-20
申请号：US15624090
申请日：2017-06-15
发明人： Balasamy Rabindran Jermy , Syed Ahmed Ali , Raed Hasan Abudawoud , Abdullah Mohammed Aitani , Sulaiman Saleh Al-Khattaf
CPC分类号： B01J29/80 , B01J29/7007 , B01J29/7215 , B01J29/74 , B01J29/7415 , B01J29/78 , B01J29/7815 , B01J35/1019 , B01J35/1023 , B01J35/1042 , B01J35/1047 , B01J35/1057 , B01J35/1061 , B01J37/0018 , B01J37/0201 , B01J37/04 , B01J37/08 , B01J2229/14 , B01J2229/186 , B01J2229/22 , B01J2229/34 , B01J2229/38 , B01J2229/42 , C01B39/026 , C07C6/06 , C07C6/126 , C07C2529/70 , C07C2529/72 , C07C2529/74 , C07C2529/78 , C07C2529/80 , C07C15/08
摘要： Embodiments of zeolite composite catalysts and methods of producing the zeolite composite catalysts are provided, where the methods comprise dissolving in an alkaline solution a catalyst precursor comprising at least one mesoporous zeolite while heating, stirring, or both to yield a dissolved zeolite solution, where the mesoporous zeolite has a molar ratio of SiO2/Al2O3 of at least 30, where the mesoporous zeolite comprises zeolite beta, adjusting the pH of the dissolved zeolite solution, aging the pH adjusted dissolved zeolite solution to yield solid zeolite composite from the dissolved zeolite solution, and calcining the solid zeolite composite to produce the zeolite composite catalyst, where the zeolite composite catalyst has a mesostructure comprising at least one disordered mesophase and at least one ordered mesophase, and where the zeolite composite catalyst has a surface area defined by the Brunauer—Emmett—Teller (BET) analysis of at least 600 m2/g.
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公开(公告)号：US10661260B2
公开(公告)日：2020-05-26
申请号：US15624090
申请日：2017-06-15
发明人： Balasamy Rabindran Jermy , Syed Ahmed Ali , Raed Hasan Abudawoud , Abdullah Mohammed Aitani , Sulaiman Saleh Al-Khattaf
IPC分类号： B01J29/80 , B01J29/72 , B01J35/10 , C01B39/02 , C07C6/12 , B01J29/70 , B01J37/00 , B01J37/02 , B01J37/04 , B01J37/08 , C07C6/06 , B01J29/74 , B01J29/78
摘要： Embodiments of zeolite composite catalysts and methods of producing the zeolite composite catalysts are provided, where the methods comprise dissolving in an alkaline solution a catalyst precursor comprising at least one mesoporous zeolite while heating, stirring, or both to yield a dissolved zeolite solution, where the mesoporous zeolite has a molar ratio of SiO2/Al2O3 of at least 30, where the mesoporous zeolite comprises zeolite beta, adjusting the pH of the dissolved zeolite solution, aging the pH adjusted dissolved zeolite solution to yield solid zeolite composite from the dissolved zeolite solution, and calcining the solid zeolite composite to produce the zeolite composite catalyst, where the zeolite composite catalyst has a mesostructure comprising at least one disordered mesophase and at least one ordered mesophase, and where the zeolite composite catalyst has a surface area defined by the Brunauer-Emmett-Teller (BET) analysis of at least 600 m2/g.
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公开(公告)号：US11351527B2
公开(公告)日：2022-06-07
申请号：US16849038
申请日：2020-04-15
发明人： Balasamy Rabindran Jermy , Syed Ahmed Ali , Raed Hasan Abudawoud , Abdullah Mohammed Aitani , Sulaiman Saleh Al-Khattaf
IPC分类号： B01J29/80 , B01J35/10 , C01B39/02 , B01J29/72 , C07C6/12 , B01J29/70 , B01J37/00 , B01J37/02 , B01J37/04 , B01J37/08 , C07C6/06 , B01J29/74 , B01J29/78
摘要： Embodiments of zeolite composite catalysts and methods of producing the zeolite composite catalysts are provided, where the methods comprise dissolving in an alkaline solution a catalyst precursor comprising at least one mesoporous zeolite while heating, stirring, or both to yield a dissolved zeolite solution, where the mesoporous zeolite has a molar ratio of SiO2/Al2O3 of at least 30, where the mesoporous zeolite comprises zeolite beta, adjusting the pH of the dissolved zeolite solution, aging the pH adjusted dissolved zeolite solution to yield solid zeolite composite from the dissolved zeolite solution, and calcining the solid zeolite composite to produce the zeolite composite catalyst, where the zeolite composite catalyst has a mesostructure comprising at least one disordered mesophase and at least one ordered mesophase, and where the zeolite composite catalyst has a surface area defined by the Brunauer-Emmett-Teller (BET) analysis of at least 600 m2/g.
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公开(公告)号：US10173204B2
公开(公告)日：2019-01-08
申请号：US15975114
申请日：2018-05-09
摘要： A method of preparing a metal-doped zeolite catalyst with a modified topology (e.g. a pillared zeolite or a delaminated zeolite), and a method of using thereof in a process for converting an alkyl-aromatic hydrocarbon stream to BTX (benzene/toluene/xylene), wherein an enhanced pore topology in the metal-doped zeolite catalyst determines a selectivity to transalkylation of trimethylbenzene to xylene, which in turn leads to a higher xylene yield. Various embodiments of the method of preparing the metal-doped zeolite catalyst, and the process for converting the alkyl-aromatic hydrocarbon stream to BTX are also provided.
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公开(公告)号：US10023813B2
公开(公告)日：2018-07-17
申请号：US15190435
申请日：2016-06-23
申请人： KING FAHD UNIVERSITY OF PETROLEUM AND MINERALS , COMMISSARIAT A L'ENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES
发明人： Zain Hassan Yamani , Nouar Tabet , Syed Ahmed Ali , Yann Leconte , Frederic Schuster , Axelle Quinsac
IPC分类号： B01J27/047 , B01J37/20 , C10G45/08 , B01J27/051 , B01J35/00 , B01J35/02 , B01J37/08 , C10G45/04 , B01J37/34 , C10G45/00
摘要： A process for producing an unsupported molybdenum sulfide nanocatalyst comprising atomizing a molybdenum oxide solution to form a molybdenum oxide aerosol, pyrolyzing the molybdenum oxide aerosol with a laser beam to form the unsupported molybdenum-based nanocatalyst, and pre-sulfiding at least a portion of the unsupported molybdenum-based nanocatalyst to form an unsupported molybdenum sulfide nanocatalyst, wherein the unsupported molybdenum-based nanocatalyst, the unsupported molybdenum sulfide catalyst or both are in the form of nanoparticles with a diameter of 1-10 nm and in a distorted rutile crystalline structure. A method of selective deep hydrodesulfurization whereby a hydrocarbon feedstock having at least one sulfur-containing component and at least one hydrocarbon is contacted with the unsupported molybdenum sulfide nanocatalyst.
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公开(公告)号：US20180257064A1
公开(公告)日：2018-09-13
申请号：US15975114
申请日：2018-05-09
CPC分类号： B01J29/7876 , B01J29/78 , C07C4/06 , C07C5/222 , C07C6/06 , C07C2529/74 , C07C2529/78 , Y02P20/52 , C07C15/08 , C07C15/04 , C07C15/06 , C07C15/073 , C07C15/02
摘要： A method of preparing a metal-doped zeolite catalyst with a modified topology (e.g. a pillared zeolite or a delaminated zeolite), and a method of using thereof in a process for converting an alkyl-aromatic hydrocarbon stream to BTX (benzene/toluene/xylene), wherein an enhanced pore topology in the metal-doped zeolite catalyst determines a selectivity to transalkylation of trimethylbenzene to xylene, which in turn leads to a higher xylene yield. Various embodiments of the method of preparing the metal-doped zeolite catalyst, and the process for converting the alkyl-aromatic hydrocarbon stream to BTX are also provided.
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公开(公告)号：US12098112B1
公开(公告)日：2024-09-24
申请号：US18617660
申请日：2024-03-27
发明人： Aniz Chennampilly Ummer , Galal Atef Ahmed Nasser , Syed Ahmed Ali , Mohammed Ahmed Yahya Sanhoob , Akolade Idris Bakare
CPC分类号： C07C1/12 , B01J6/001 , B01J21/16 , B01J35/612 , B01J35/613 , B01J35/615 , B01J35/633 , B01J37/0009 , B01J37/0201 , B01J37/0203 , B01J37/0236 , C07C2521/16
摘要： A method for chemically reducing carbon dioxide (CO2) with a red mud catalyst composition is provided includes introducing a gaseous mixture of CO2 and H2 into a reactor containing particles of the red mud catalyst composition. The method further includes reacting at least a portion of the CO2 and H2 in the gaseous mixture in the presence of the red mud catalyst composition at a temperature of 200 to 800° C., and under a pressure ranging from 5 to 100 bar to form a gaseous product including a chemical reduction product of the CO2. A volume ratio of the CO2 to the H2 in the gaseous mixture is in a range of 1:10 to 10:1.
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公开(公告)号：US12098113B1
公开(公告)日：2024-09-24
申请号：US18617661
申请日：2024-03-27
发明人： Aniz Chennampilly Ummer , Galal Atef Ahmed Nasser , Syed Ahmed Ali , Mohammed Ahmed Yahya Sanhoob , Akolade Idris Bakare
CPC分类号： C07C1/12 , B01J6/001 , B01J21/16 , B01J35/612 , B01J35/613 , B01J35/615 , B01J35/633 , B01J37/0009 , B01J37/0201 , B01J37/0203 , B01J37/0236 , C07C2521/16
摘要： A method for chemically reducing carbon dioxide (CO2) with a red mud catalyst composition is provided includes introducing a gaseous mixture of CO2 and H2 into a reactor containing particles of the red mud catalyst composition. The method further includes reacting at least a portion of the CO2 and H2 in the gaseous mixture in the presence of the red mud catalyst composition at a temperature of 200 to 800° C., and under a pressure ranging from 5 to 100 bar to form a gaseous product including a chemical reduction product of the CO2. A volume ratio of the CO2 to the H2 in the gaseous mixture is in a range of 1:10 to 10:1.
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