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公开(公告)号：US08226896B2
公开(公告)日：2012-07-24
申请号：US12525678
申请日：2008-01-28
申请人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
发明人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
IPC分类号： B01D50/00
CPC分类号： F01N3/0814 , B01D53/9418 , B01D53/944 , B01D53/9468 , B01D2255/1021 , B01D2255/1023 , B01D2255/20738 , B01D2255/20761 , B01D2255/502 , B01D2255/9022 , B01D2258/012 , B01J23/40 , B01J23/63 , B01J29/106 , B01J29/24 , B01J29/46 , B01J29/7615 , B01J35/0006 , B01J37/0244 , F01N3/035 , F01N3/0821 , F01N3/0828 , F01N3/0842 , F01N3/2066 , F01N2240/25 , F01N2570/18 , F01N2610/02 , Y02T10/22 , Y02T10/24
摘要： A catalytically active diesel particulate filter with ammonia trap action is presented, which, in addition to an oxidation-active coating (2), comprises a coating (1) which is catalytically active in the SCR reaction. By means of this inventive diesel particulate filter, it is possible to make exhaust gas aftertreatment systems for removing nitrogen oxides and particulates from the exhaust gas of lean engines considerably simpler and less expensive.
摘要翻译： 提出了具有氨捕集作用的催化活性柴油微粒过滤器，除了氧化活性涂层（2）外，还包括在SCR反应中具有催化活性的涂层（1）。 通过本发明的柴油微粒过滤器，可以制备用于从贫燃机的废气中除去氮氧化物和颗粒物的废气后处理系统更简单且更便宜。
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公开(公告)号：US20100058746A1
公开(公告)日：2010-03-11
申请号：US12525678
申请日：2008-01-28
申请人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
发明人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
CPC分类号： F01N3/0814 , B01D53/9418 , B01D53/944 , B01D53/9468 , B01D2255/1021 , B01D2255/1023 , B01D2255/20738 , B01D2255/20761 , B01D2255/502 , B01D2255/9022 , B01D2258/012 , B01J23/40 , B01J23/63 , B01J29/106 , B01J29/24 , B01J29/46 , B01J29/7615 , B01J35/0006 , B01J37/0244 , F01N3/035 , F01N3/0821 , F01N3/0828 , F01N3/0842 , F01N3/2066 , F01N2240/25 , F01N2570/18 , F01N2610/02 , Y02T10/22 , Y02T10/24
摘要： A catalytically active diesel particulate filter with ammonia trap action is presented, which, in addition to an oxidation-active coating (2), comprises a coating (1) which is catalytically active in the SCR reaction. By means of this inventive diesel particulate filter, it is possible to make exhaust gas aftertreatment systems for removing nitrogen oxides and particulates from the exhaust gas of lean engines considerably simpler and less expensive.
摘要翻译： 提出了具有氨捕集作用的催化活性柴油微粒过滤器，除了氧化活性涂层（2）外，还包括在SCR反应中具有催化活性的涂层（1）。 通过本发明的柴油微粒过滤器，可以制备用于从贫燃机的废气中除去氮氧化物和颗粒物的废气后处理系统更简单且更便宜。
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3.发明申请EXHAUST GAS PURIFICATION SYSTEM FOR THE TREATMENT OF ENGINE EXHAUST GASES BY MEANS OF SCR CATALYST 有权通过SCR催化剂处理发动机排气的排气净化系统公开(公告)号：US20110146237A1
公开(公告)日：2011-06-23
申请号：US12937089
申请日：2009-03-18
申请人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
发明人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
CPC分类号： B01D53/9418 , B01D53/9477 , B01D2255/20761 , B01D2255/20776 , B01D2255/407 , B01D2255/50 , B01D2258/012 , B01J23/002 , B01J23/30 , B01J29/072 , B01J29/7615 , B01J35/0006 , B01J37/0201 , B01J37/0246 , B01J37/0248 , B01J2523/00 , F01N3/035 , F01N3/106 , F01N3/2066 , F01N13/0093 , F01N2510/0682 , F01N2570/18 , Y02T10/24 , B01J2523/3712 , B01J2523/48
摘要： An exhaust gas purification system (method and device) for the treatment of diesel exhaust gases containing nitrogen oxides and hydrocarbons is disclosed, which comprises the addition of ammonia or of a compound decomposable to ammonia into the exhaust gas stream and the subsequent leading of the exhaust gas stream over two successively arranged SCR catalysts with different properties and compositions. Both SCR catalysts are free of vanadium compounds and only the downstream SCR catalyst contains zeolite compounds. The exhaust gas purification system according to the invention is characterized by good “kick-off” behavior at low temperatures and a simultaneously high conversion performance over a wide temperature range.
摘要翻译： 公开了一种用于处理含有氮氧化物和烃的柴油废气的废气净化系统（方法和装置），其包括将氨或可分解成氨的化合物加入排气流中，随后引导排气 气流在两个连续排列的SCR催化剂上具有不同的性能和组成。 两种SCR催化剂都不含钒化合物，只有下游SCR催化剂含有沸石化合物。 根据本发明的废气净化系统的特征在于在低温下具有良好的“启动”行为，并且在宽的温度范围内具有同时高的转换性能。
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4.发明授权Exhaust gas purification system for the treatment of engine exhaust gases by means of SCR catalyst 有权用于通过SCR催化剂处理发动机废气的废气净化系统公开(公告)号：US08863507B2
公开(公告)日：2014-10-21
申请号：US12937089
申请日：2009-03-18
申请人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
发明人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
IPC分类号： F01N3/10 , B01J23/00 , B01J29/76 , F01N3/20 , B01J35/00 , F01N13/00 , B01J23/30 , B01D53/94 , F01N3/035 , B01J37/02 , B01J29/072
CPC分类号： B01D53/9418 , B01D53/9477 , B01D2255/20761 , B01D2255/20776 , B01D2255/407 , B01D2255/50 , B01D2258/012 , B01J23/002 , B01J23/30 , B01J29/072 , B01J29/7615 , B01J35/0006 , B01J37/0201 , B01J37/0246 , B01J37/0248 , B01J2523/00 , F01N3/035 , F01N3/106 , F01N3/2066 , F01N13/0093 , F01N2510/0682 , F01N2570/18 , Y02T10/24 , B01J2523/3712 , B01J2523/48
摘要： An exhaust gas purification system (method and device) for the treatment of diesel exhaust gases containing nitrogen oxides and hydrocarbons is disclosed, which comprises the addition of ammonia or of a compound decomposable to ammonia into the exhaust gas stream and the subsequent leading of the exhaust gas stream over two successively arranged SCR catalysts with different properties and compositions. Both SCR catalysts are free of vanadium compounds and only the downstream SCR catalyst contains zeolite compounds. The exhaust gas purification system according to the invention is characterized by good “kick-off” behavior at low temperatures and a simultaneously high conversion performance over a wide temperature range.
摘要翻译： 公开了一种用于处理含有氮氧化物和烃的柴油废气的废气净化系统（方法和装置），其包括将氨或可分解成氨的化合物加入排气流中，随后引导排气 气流在两个连续排列的SCR催化剂上具有不同的性能和组成。 两种SCR催化剂都不含钒化合物，只有下游SCR催化剂含有沸石化合物。 根据本发明的废气净化系统的特征在于在低温下具有良好的“启动”行为，并且在宽的温度范围内具有同时高的转换性能。
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5.发明授权Vanadium-free catalyst for selective catalytic reduction and process for it's preparation 有权用于选择性催化还原的无钒催化剂及其制备方法公开(公告)号：US08569199B2
公开(公告)日：2013-10-29
申请号：US12444312
申请日：2007-09-17
申请人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
发明人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
CPC分类号： B01J23/002 , B01D53/9418 , B01D2251/2062 , B01D2255/2063 , B01D2255/20769 , B01D2255/20776 , B01D2255/20784 , B01D2255/407 , B01D2255/9155 , B01J23/10 , B01J23/24 , B01J23/30 , B01J23/888 , B01J27/04 , B01J37/0201 , B01J37/0248 , B01J2523/00 , B01J2523/3706 , B01J2523/3712 , B01J2523/48 , Y02A50/2325 , Y02T10/24 , B01J2523/69 , B01J2523/842
摘要： Selective catalytic reduction with ammonia or a compound that decomposes to ammonia is a known method for the removal of nitrogen oxides from the exhaust gas of primarily lean-burn internal combustion engines. The vanadium-containing SCR catalysts that have long been generally used for this are characterized by a good conversion profile. However, the volatility of vanadium oxide can, at higher exhaust gas temperatures, lead to the emission of toxic vanadium compounds. Zeolite-based SCR catalysts, which are used in particular in discontinuous SCR systems, constitute a very cost-intensive solution for the problem.A method is proposed by which a homogeneous cerium-zirconium mixed oxide is activated for the SCR reaction in a defined manner by the introduction of sulphur and/or transition metal. Using this method, a highly active, ageing-resistant SCR catalyst is provided, which represents a vanadium-free, cost-effective and high-performance alternative to the existing SCR catalysts and is suitable in particular for use in motor vehicles.
摘要翻译： 用氨或分解成氨的化合物进行选择性催化还原是从主要贫燃内燃机的废气中除去氮氧化物的已知方法。 长期以来一般使用的含钒SCR催化剂的特征在于良好的转化率。 然而，在更高的废气温度下，氧化钒的挥发性会导致有毒的钒化合物的排放。 特别是在不连续SCR系统中使用的基于沸石的SCR催化剂构成了该问题的非常成本高的解决方案。 提出了一种通过引入硫和/或过渡金属以规定的方式使均相铈锆混合氧化物活化用于SCR反应的方法。 使用这种方法，提供了高活性，耐老化的SCR催化剂，其代表了现有SCR催化剂的无钒，成本效益和高性能替代物，并且特别适用于机动车辆。
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6.发明申请VANADIUM-FREE CATALYST FOR SELECTIVE CATALYTIC REDUCTION AND PROCESS FOR IT'S PREPARATION 有权用于选择性催化还原的无钒催化剂及其制备方法公开(公告)号：US20100034717A1
公开(公告)日：2010-02-11
申请号：US12444312
申请日：2007-09-17
申请人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
发明人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
IPC分类号： B01D53/94 , B01J23/10 , B01J27/02 , B01J27/051 , B01J27/047 , B01J27/045 , B01J27/043 , B01D53/56
CPC分类号： B01J23/002 , B01D53/9418 , B01D2251/2062 , B01D2255/2063 , B01D2255/20769 , B01D2255/20776 , B01D2255/20784 , B01D2255/407 , B01D2255/9155 , B01J23/10 , B01J23/24 , B01J23/30 , B01J23/888 , B01J27/04 , B01J37/0201 , B01J37/0248 , B01J2523/00 , B01J2523/3706 , B01J2523/3712 , B01J2523/48 , Y02A50/2325 , Y02T10/24 , B01J2523/69 , B01J2523/842
摘要： Selective catalytic reduction with ammonia or a compound that decomposes to ammonia is a known method for the removal of nitrogen oxides from the exhaust gas of primarily lean-burn internal combustion engines. The vanadium-containing SCR catalysts that have long been generally used for this are characterized by a good conversion profile. However, the volatility of vanadium oxide can, at higher exhaust gas temperatures, lead to the emission of toxic vanadium compounds. Zeolite-based SCR catalysts, which are used in particular in discontinuous SCR systems, constitute a very cost-intensive solution for the problem.A method is proposed by which a homogeneous cerium-zirconium mixed oxide is activated for the SCR reaction in a defined manner by the introduction of sulphur and/or transition metal. Using this method, a highly active, ageing-resistant SCR catalyst is provided, which represents a vanadium-free, cost-effective and high-performance alternative to the existing SCR catalysts and is suitable in particular for use in motor vehicles.
摘要翻译： 用氨或分解成氨的化合物进行选择性催化还原是从主要贫燃内燃机的废气中除去氮氧化物的已知方法。 长期以来一般使用的含钒SCR催化剂的特征在于良好的转化率。 然而，在更高的废气温度下，氧化钒的挥发性会导致有毒的钒化合物的排放。 特别是在不连续SCR系统中使用的基于沸石的SCR催化剂构成了该问题的非常成本高的解决方案。 提出了一种通过引入硫和/或过渡金属以规定的方式使均相铈锆混合氧化物活化用于SCR反应的方法。 使用这种方法，提供了高活性，耐老化的SCR催化剂，其代表了现有SCR催化剂的无钒，成本效益和高性能替代物，并且特别适用于机动车辆。
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7.发明授权Catalytically coated diesel particle filter, process for producing it and its use 有权催化涂层柴油颗粒过滤器，生产过程及其应用公开(公告)号：US07922987B2
公开(公告)日：2011-04-12
申请号：US12377753
申请日：2007-08-17
申请人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
发明人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
CPC分类号： F01N3/035 , B01D53/944 , B01D2255/102 , B01D2255/206 , B01D2255/20738 , B01D2255/20761 , B01D2255/50 , B01D2255/912 , B01D2255/9155 , B01J23/44 , B01J29/126 , B01J29/7415 , B01J29/80 , B01J35/0006 , B01J37/0244 , B01J37/0246 , B01J37/0248 , F01N3/0222 , F01N3/0821 , F01N3/0835 , F01N2370/02 , F01N2370/04 , F01N2510/063 , F01N2510/0682 , Y02A50/2341 , Y10S502/514
摘要： A diesel particulate filter with an oxidation catalyst comprising platinum and palladium deposited thereon is described. Addition of HC storage components to the oxidation catalyst allows the conversion of hydrocarbons and carbon monoxide to be improved significantly.
摘要翻译： 描述了具有沉积在其上的铂和钯的氧化催化剂的柴油微粒过滤器。 将HC储存组分添加到氧化催化剂允许烃和一氧化碳的转化显着改善。
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8.发明申请CATALYTICALLY COATED DIESEL PARTICLE FILTER, PROCESS FOR PRODUCING IT AND ITS USE 有权催化涂层柴油颗粒过滤器，生产工艺及其使用过程公开(公告)号：US20100092358A1
公开(公告)日：2010-04-15
申请号：US12377753
申请日：2007-08-17
申请人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
发明人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
CPC分类号： F01N3/035 , B01D53/944 , B01D2255/102 , B01D2255/206 , B01D2255/20738 , B01D2255/20761 , B01D2255/50 , B01D2255/912 , B01D2255/9155 , B01J23/44 , B01J29/126 , B01J29/7415 , B01J29/80 , B01J35/0006 , B01J37/0244 , B01J37/0246 , B01J37/0248 , F01N3/0222 , F01N3/0821 , F01N3/0835 , F01N2370/02 , F01N2370/04 , F01N2510/063 , F01N2510/0682 , Y02A50/2341 , Y10S502/514
摘要： A diesel particulate filter with an oxidation catalyst comprising platinum and palladium deposited thereon is described. Addition of HC storage components to the oxidation catalyst allows the conversion of hydrocarbons and carbon monoxide to be improved significantly.
摘要翻译： 描述了具有沉积在其上的铂和钯的氧化催化剂的柴油微粒过滤器。 将HC储存组分添加到氧化催化剂允许烃和一氧化碳的转化显着改善。
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公开(公告)号：US20080026141A1
公开(公告)日：2008-01-31
申请号：US11628657
申请日：2005-06-04
申请人： Marcus Pfeifer , Rainer Domesle , Nicola Soeger , Christian Kuehn , Roger Staab , Thomas Kreuzer
发明人： Marcus Pfeifer , Rainer Domesle , Nicola Soeger , Christian Kuehn , Roger Staab , Thomas Kreuzer
CPC分类号： B01D53/944
摘要： The invention relates to particle filters having an open pore structure for separating particles from fluids, which, for modification of their properties or for treatment of the fluid to be filtered, are provided with additional metal oxides or mixed metal oxides and optionally with further catalytically active components. In particular, the invention relates to particle filters treated with a catalytically active material, which is used for the treatment of the waste gases from combustion processes, in particular for the treatment of the exhaust gases of internal combustion engines. By impregnation of the filter bodies in a solution of a metal oxide sol or a mixed metal oxide sol, the preformed sol particles are deposited on the pore surfaces. Consequently, catalytic activations of the filter with good temperature stability in combination with a moderate increase in the exhaust gas back-pressure are possible.
摘要翻译： 本发明涉及具有用于从流体中分离颗粒的开孔结构的颗粒过滤器，为了改变其性能或处理待过滤的流体，提供另外的金属氧化物或混合金属氧化物，并且任选具有进一步的催化活性 组件。 特别地，本发明涉及用催化活性材料处理的颗粒过滤器，其用于处理来自燃烧过程的废气，特别是用于处理内燃机的废气。 通过在金属氧化物溶胶或混合金属氧化物溶胶的溶液中浸渍过滤体，预先形成的溶胶颗粒沉积在孔表面上。 因此，具有良好的温度稳定性的过滤器的催化活化与废气背压的适度增加相结合是可能的。
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10.发明申请公开(公告)号：US20070110650A1
公开(公告)日：2007-05-17
申请号：US10567204
申请日：2004-07-29
申请人： Marcus Pfeifer , Nicola Soeger , Yvonne Demel , Tobias Kuhl , Paul Spurk , Jurgen Gieshoff , Egbert Lox , Thomas Kreuzer
发明人： Marcus Pfeifer , Nicola Soeger , Yvonne Demel , Tobias Kuhl , Paul Spurk , Jurgen Gieshoff , Egbert Lox , Thomas Kreuzer
CPC分类号： B01D53/945 , B01D53/9418 , B01D53/9422 , B01D53/9431 , B01D53/9454 , B01D2251/208 , B01D2255/1021 , B01D2255/204 , B01D2255/2042 , B01D2255/2065 , B01D2255/20707 , B01D2255/2073 , B01D2255/20738 , B01D2255/20761 , B01D2255/2092 , B01D2255/407 , B01D2255/504 , B01D2255/9155 , F01N3/035 , F01N3/0814 , F01N3/0821 , F01N3/0842 , F01N3/2066 , F01N3/2828 , F01N2250/12 , F01N2510/06 , Y02T10/22 , Y02T10/24
摘要： The invention relates to a catalyst arrangement for purifying the exhaust gases of internal combustion engines operated under lean conditions. It is proposed that a thinwalled, porous carrier be coated on one side with a nitrogen oxide storage catalyst and on the other side with an SCR catalyst. When the exhaust gas is passed through the catalytic coatings and the support material, a significant improvement in the nitrogen oxide conversion is achieved compared to a series arrangement of the catalysts on separate carriers. Wall flow filters have been found to be useful as thin-walled carriers.
摘要翻译： 本发明涉及一种用于净化在稀薄条件下运行的内燃机废气的催化剂装置。 建议在一侧用氮氧化物储存催化剂涂覆薄壁多孔载体，另一侧用SCR催化剂涂覆。 当排气通过催化涂层和载体材料时，与单独的载体上的催化剂的串联排列相比，实现了氮氧化物转化率的显着改善。 已经发现壁流式过滤器可用作薄壁载体。
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