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    Manufacture of improved catalyst
    5.
    发明授权
    Manufacture of improved catalyst 失效
    改良催化剂的制造

    公开(公告)号：US5472922A

    公开(公告)日：1995-12-05

    申请号：US140936

    申请日：1993-10-25

    申请人： Thomas F. Degnan ,  Terry E. Helton ,  Grant H. Yokomizo

    发明人： Thomas F. Degnan ,  Terry E. Helton ,  Grant H. Yokomizo

    IPC分类号： B01J29/70 ,  B01J29/04

    CPC分类号： B01J29/7007 ,  B01J2229/26 ,  B01J2229/36 ,  B01J2229/42

    摘要： Methods for preparing phosphorus containing catalysts comprising a large-pore zeolite, e.g., zeolite Beta, zeolite ZSM-12, or zeolite ZSM-20, and a matrix which have improved attrition resistance. The present invention includes the catalyst compositions produced by the above methods. Also included in the present invention are methods for the use of catalysts prepared by the present method in hydrocarbon cracking processes. It is desired to develop cracking catalysts for organic compound conversion that have improved cracking yields and have good attrition resistance. This invention involves the use of large pore siliceous zeolites and a highly siliceous matrix to produce a cracking catalyst with improved cracking yields and good attrition resistance. The invention further involves the use of phosphorus and the use of selected sequences for combining the compounds in the manufacture of the catalyst to enhance the attrition resistance of the catalyst.

    摘要翻译： 制备含有大孔沸石的含磷催化剂的方法，例如β沸石沸石，沸石ZSM-12或沸石ZSM-20，以及具有改善耐磨性的基体。 本发明包括通过上述方法制备的催化剂组合物。 本发明还包括使用本方法制备的催化剂在烃裂解方法中的方法。 需要开发有机化合物转化的裂化催化剂，其具有改善的裂化产率并具有良好的耐磨性。 本发明涉及使用大孔硅质沸石和高度硅质基质来生产具有改进的裂化产率和良好耐磨性的裂化催化剂。 本发明进一步涉及磷的使用和选择的序列用于在催化剂制造中组合化合物以提高催化剂耐磨耗性的用途。

    Process for isomerization dewaxing of hydrocarbon streams
    8.
    发明授权
    Process for isomerization dewaxing of hydrocarbon streams 有权
    烃流异构化脱蜡方法

    公开(公告)号：US06652735B2

    公开(公告)日：2003-11-25

    申请号：US09843125

    申请日：2001-04-26

    申请人： Thomas F. Degnan ,  Philip J. Angevine

    发明人： Thomas F. Degnan ,  Philip J. Angevine

    IPC分类号： C10G7338

    CPC分类号： C10G45/62 ,  B01J29/74 ,  B01J29/7415 ,  B01J29/80 ,  B01J2229/20 ,  B01J2229/42 ,  C10G45/64 ,  C10G65/043

    摘要： A process for isomerization dewaxing of a hydrocarbon feed which includes contacting the hydrocarbon feed with a large pore size, small crystal size, crystalline molecular sieve and an intermediate pore size, small crystal size, crystalline molecular sieve to produce a dewaxed product with a reduced pour point and a reduced cloud point. In a preferred embodiment, the feed is contacted with the molecular sieves sequentially, first with the large pore sieve followed by the intermediate pore sieve.

    摘要翻译： 烃原料异构化脱蜡的方法，其包括使烃进料与大孔径，小结晶尺寸，结晶分子筛和中等孔径，小晶体尺寸，结晶分子筛接触以产生具有降低的倾倒的脱蜡产物 点和减少的浊点。 在一个优选的实施方案中，进料与分子筛依次接触，首先用大孔筛，然后是中间孔筛。

    Aromatic alkylation process
    9.
    发明授权
    Aromatic alkylation process 有权
    芳香烷基化工艺

    公开(公告)号：US06313362B1

    公开(公告)日：2001-11-06

    申请号：US09213798

    申请日：1998-12-17

    申请人： John R. Green ,  Thomas F. Degnan ,  Yun-Yang Huang ,  Chaya R. Venkat ,  Ronald A. Weiss

    发明人： John R. Green ,  Thomas F. Degnan ,  Yun-Yang Huang ,  Chaya R. Venkat ,  Ronald A. Weiss

    IPC分类号： C07C264

    CPC分类号： C07C15/085 ,  C07C15/073

    摘要： Akylation product is contacted with a purification medium in a liquid phase pre-reaction step to remove impurities and form a purified stream. The purified stream may then be further processed by liquid phase transalkylation to convert the polyalkylated aromatic compound to a monoalkylated aromatic compound. The process may use a large pore molecular sieve catalyst such as MCM-22 as the purification medium in the pre-reaction step because of its high reactivity for alkylation, strong retention of catalyst poisons and low reactivity for oligomerization under the pre-reactor conditions. Olefins, diolefins, styrene, oxygenated organic compounds, sulfur containing compounds, nitrogen containing compounds and oligomeric compounds are removed.

    摘要翻译： 将Akylation产物在液相预反应步骤中与净化介质接触以除去杂质并形成纯化的物流。 然后可以通过液相烷基转移进一步处理纯化的物流，以将多烷基化芳族化合物转化为单烷基化芳族化合物。 在预反应步骤中，该方法可以使用大孔分子筛催化剂例如MCM-22作为纯化介质，因为其在烷基化反应活性高，催化剂毒物强烈的保留和在反应器前条件下的低聚反应低。 除去烯烃，二烯烃，苯乙烯，含氧有机化合物，含硫化合物，含氮化合物和低聚物。

    Hydrocarbon coversion using improved zeolite Beta catalyst
    10.
    发明授权
    Hydrocarbon coversion using improved zeolite Beta catalyst 失效
    使用改进的沸石β催化剂进行烃转化

    公开(公告)号：US5658454A

    公开(公告)日：1997-08-19

    申请号：US461484

    申请日：1995-06-05

    申请人： Robert P. L. Absil ,  Thomas F. Degnan ,  George H. Hatzikos ,  Jocelyn A. Kowalski ,  Thomas Mebrahtu ,  Grant H. Yokomizo

    发明人： Robert P. L. Absil ,  Thomas F. Degnan ,  George H. Hatzikos ,  Jocelyn A. Kowalski ,  Thomas Mebrahtu ,  Grant H. Yokomizo

    IPC分类号： B01J29/40 ,  B01J29/70 ,  B01J37/00 ,  C10G11/05 ,  C07C4/06 ,  C10G47/04

    CPC分类号： C10G11/05 ,  B01J29/7007 ,  B01J37/0009 ,  B01J2229/26 ,  B01J2229/36 ,  B01J2229/42 ,  B01J29/40 ,  B01J29/7034 ,  B01J29/7042

    摘要： A catalyst composition which comprises a crystalline metallosilicate having the structure of zeolite Beta, phosphor and a matrix that is substantially free of crystalline aluminum phosphate which has improved resistance to steam deactivation which has higher cracking activity than analogous catalysts prepared without phosphorus. The crystalline metallosilicate be used in the as-synthesized form or in the calcined form. included is the method to produce the catalyst composition and methods for the use of catalysts prepared by the present method in organic conversion processes. Specific embodiments of the invention involve various techniques for preparation of catalyst containing phosphorus and crystalline metallosilicates having the structure of zeolite Beta. Catalysts prepared according to the method of this invention are useful for organic compound, e.g., hydrocarbon compound, conversion processes. Organic compound conversion processes include cracking, hydrocracking, and transalkylation, among others.

    摘要翻译： 一种催化剂组合物，其包含具有沸石β，磷光体和基本上不含结晶磷酸铝的结构的结晶金属硅酸盐，其具有改善的对蒸汽失活的抗性，其具有比不用磷制备的类似催化剂更高的裂化活性。 结晶金属硅酸盐以合成形式或煅烧形式使用。 包括制备催化剂组合物的方法和通过本发明方法在有机转化方法中制备的催化剂的使用方法。 本发明的具体实施方案涉及用于制备含有β沸石结构的磷的磷和结晶金属硅酸盐的各种技术。 根据本发明方法制备的催化剂可用于有机化合物，例如烃化合物，转化方法。 有机化合物转化方法包括裂化，加氢裂化和烷基转移等。